arXiv subjects

M. L. Rosinberg

Publications and source records attributed to M. L. Rosinberg.

33 records · Page 2Linked to original sources

arXiv2008

The T=0 random-field Ising model on a Bethe lattice with large coordination number: hysteresis and metastable states

In order to elucidate the relationship between rate-independent hysteresis and metastability in disordered systems driven by an external field, we study the Gaussian RFIM at T=0 on regular random graphs (Bethe lattice) of finite connectivity z and compute to O(1/z) (i.e. beyond mean-field) the quenched complexity associated with the one-spin-flip stable states with magnetization m as a function of the magnetic field H. When the saturation hysteresis loop is smooth in the thermodynamic limit, we find that it coincides with the envelope of the typical metastable states (the quenched complexity vanishes exactly along the loop and is positive everywhere inside). On the other hand, the occurence of a jump discontinuity in the loop (associated with an infinite avalanche) can be traced back to the existence of a gap in the magnetization of the metastable states for a range of applied field, and the envelope of the typical metastable states is then reentrant. These findings confirm and complete earlier analytical and numerical studies.

cond-mat.dis-nn↗

arXiv2008

Stable, metastable and unstable states in the mean-field RFIM at T=0

We compute the probability of finding metastable states at a given field in the mean-field random field Ising model at T=0. Remarkably, this probability is finite in the thermodynamic limit, even on the so-called ``unstable'' branch of the magnetization curve. This implies that the branch is reachable when the magnetization is controlled instead of the magnetic field, in contrast with the situation in the pure system.

cond-mat.dis-nn↗

arXiv2007

Numerical study of metastable states in the T=0 RFIM

We study numerically the number of single-spin-flip stable states in the T=0 Random Field Ising Model (RFIM) on random regular graphs of connectivity $z=2$ and $z=4$ and on the cubic lattice. The annealed and quenched complexities (i.e. the entropy densities) of the metastable states with given magnetization are calculated as a function of the external magnetic field. The results show that the appearance of a (disorder-induced) out-of-equilibrium phase transition in the magnetization hysteresis loop at low disorder can be ascribed to a change in the distribution of the metastable states in the field-magnetization plane.

cond-mat.dis-nn↗

arXiv2005

Gas adsorption/desorption in silica aerogels: a theoretical study of scattering properties

We present a numerical study of the structural correlations associated to gas adsorption/desorption in silica aerogels in order to provide a theoretical interpretation of scattering experiments. Following our earlier work, we use a coarse-grained lattice-gas description and determine the nonequilibrium behavior of the adsorbed gas within a local mean-field analysis. We focus on the differences between the adsorption and desorption mechanisms and their signature in the fluid-fluid and gel-fluid structure factors as a function of temperature. At low temperature, but still in the regime where the isotherms are continuous, we find that the adsorbed fluid density, during both filling and draining, is correlated over distances that may be much larger than the gel correlation length. In particular, extended fractal correlations may occur during desorption, indicating the existence of a ramified cluster of vapor filled cavities. This also induces an important increase of the scattering intensity at small wave vectors. The similarity and differences with the scattering of fluids in other porous solids such as Vycor are discussed.

cond-mat.dis-nn↗

arXiv2005

Helium condensation in aerogel: avalanches and disorder-induced phase transition

We present a detailed numerical study of the elementary condensation events (avalanches) associated to the adsorption of $^4$He in silica aerogels. We use a coarse-grained lattice-gas description and determine the nonequilibrium behavior of the adsorbed gas within a local mean-field analysis, neglecting thermal fluctuations and activated processes. We investigate the statistical properties of the avalanches, such as their number, size and shape along the adsorption isotherms as a function of gel porosity, temperature, and chemical potential. Our calculations predict the existence of a line of critical points in the temperature-porosity diagram where the avalanche size distribution displays a power-law behavior and the adsorption isotherms have a universal scaling form. The estimated critical exponents seem compatible with those of the field-driven Random Field Ising Model at zero temperature.

cond-mat.dis-nn↗

arXiv2005

Metastable states and T=0 hysteresis in the random-field Ising model on random graphs

We study the ferromagnetic random-field Ising model on random graphs of fixed connectivity z (Bethe lattice) in the presence of an external magnetic field $H$. We compute the number of single-spin-flip stable configurations with a given magnetization m and study the connection between the distribution of these metastable states in the H-m plane (focusing on the region where the number is exponentially large) and the shape of the saturation hysteresis loop obtained by cycling the field between $-\infty$ and $+\infty$ at T=0. The annealed complexity $Σ_A(m,H)$ is calculated for z=2,3,4 and the quenched complexity $Σ_Q(m,H)$ for z=2. We prove explicitly for z=2 that the contour $Σ_Q(m,H)=0$ coincides with the saturation loop. On the other hand, we show that $Σ_A(m,H)$ is irrelevant for describing, even qualitatively, the observable hysteresis properties of the system.

cond-mat.dis-nn↗

arXiv2003

Local mean-field study of capillary condensation in silica aerogels

We apply local mean-field (i.e. density functional) theory to a lattice model of a fluid in contact with a dilute, disordered gel network. The gel structure is described by a diffusion-limited cluster aggregation model. We focus on the influence of porosity on both the hysteretic and the equilibrium behavior of the fluid as one varies the chemical potential at low temperature. We show that the shape of the hysteresis loop changes from smooth to rectangular as the porosity increases and that this change is associated to disorder-induced out-of-equilibrium phase transitions that differ on adsorption and on desorption. Our results provide insight in the behavior of $^4$He in silica aerogels.

cond-mat.dis-nn↗

arXiv2002

Percolation, depinning, and avalanches in capillary condensation of gases in disordered porous solids

We propose a comprehensive theoretical description of hysteresis in capillary condensation of gases in mesoporous disordered materials. Applying mean-field density functional theory to a coarse-grained lattice-gas model, we show that the morphology of the hysteresis loops is influenced by out-of-equilibrium transitions that are different on filling and on draining. In particular, desorption may be associated to a depinning process and be percolation-like without explicit pore-blocking effects.

cond-mat.dis-nn↗

arXiv2002

Adsorption hysteresis and capillary condensation in disordered porous solids: a density functional study

We present a theoretical study of capillary condensation of fluids adsorbed in mesoporous disordered media. Combining mean-field density functional theory with a coarse-grained description in terms of a lattice-gas model allows us to investigate both the out-of-equilibrium (hysteresis) and the equilibrium behavior. We show that the main features of capillary condensation in disordered solids result from the appearance of a complex free-energy landscape with a large number of metastable states. We detail the numerical procedures for finding these states, and the presence or absence of transitions in the thermodynamic limit is determined by careful finite-size studies.

cond-mat.dis-nn↗

arXiv2001

Capillary condensation in disordered porous materials: hysteresis versus equilibrium behavior

We study the interplay between hysteresis and equilibrium behavior in capillary condensation of fluids in mesoporous disordered materials via a mean-field density functional theory of a disordered lattice-gas model. The approach reproduces all major features observed experimentally. We show that the simple van der Waals picture of metastability fails due to the appearance of a complex free-energy landscape with a large number of metastable states. In particular, hysteresis can occur both with and without an underlying equilibrium transition, thermodynamic consistency is not satisfied along the hysteresis loop, and out-of-equilibrium phase transitions are possible.

cond-mat.dis-nn↗

arXiv2000

The ferromagnetic q-state Potts model on three-dimensional lattices: a study for real values of q

We study the phase diagram of the ferromagnetic $q$-state Potts model on the various three-dimensional lattices for integer and non-integer values of $q>1$. Our approach is based on a thermodynamically self-consistent Ornstein-Zernike approximation for the two-point correlation functions. We calculate the transition temperatures and, when the transition is first order, the jump discontinuities in the magnetization and the internal energy, as well as the coordinates of the critical endpoint in external field. Our predictions are in very good agreement with best available estimates. From the numerical study of the region of weak first-order transition, we estimate the critical value $q_c$ for which the transition changes from second to first-order. The $q->1$ limit that describes the bond-percolation problem is also investigated.

cond-mat.stat-mech↗

arXiv2000

A thermodynamically self-consistent theory for the Blume-Capel model

We use a self-consistent Ornstein-Zernike approximation to study the Blume-Capel ferromagnet on three-dimensional lattices. The correlation functions and the thermodynamics are obtained from the solution of two coupled partial differential equations. The theory provides a comprehensive and accurate description of the phase diagram in all regions, including the wing boundaries in non-zero magnetic field. In particular, the coordinates of the tricritical point are in very good agreement with the best estimates from simulation or series expansion. Numerical and analytical analysis strongly suggest that the theory predicts a universal Ising-like critical behavior along the $λ$-line and the wing critical lines, and a tricritical behavior governed by mean-field exponents.

cond-mat.stat-mech↗

arXiv1999

A self-consistent Ornstein-Zernike approximation for the Edwards-Anderson spin glass model

We propose a self-consistent Ornstein-Zernike approximation for studying the Edwards-Anderson spin glass model. By performing two Legendre transforms in replica space, we introduce a Gibbs free energy depending on both the magnetizations and the overlap order parameters. The correlation functions and the thermodynamics are then obtained from the solution of a set of coupled partial differential equations. The approximation becomes exact in the limit of infinite dimension and it provides a potential route for studying the stability of the high-temperature phase against replica-symmetry breaking fluctuations in finite dimensions. As a first step, we present the numerical predictions for the freezing temperature and the zero-field thermodynamic properties above freezing as a function of dimensionality.

cond-mat.dis-nn↗

arXiv1998

A self-consistent Ornstein-Zernike approximation for the Random Field Ising model

We extend the self-consistent Ornstein-Zernike approximation (SCOZA), first formulated in the context of liquid-state theory, to the study of the random field Ising model. Within the replica formalism, we treat the quenched random field as an annealed spin variable, thereby avoiding the usual average over the random field distribution. This allows to study the influence of the distribution on the phase diagram in finite dimensions. The thermodynamics and the correlation functions are obtained as solutions of a set a coupled partial differential equations with magnetization, temperature and disorder strength as independent variables. A preliminary analysis based on high-temperature and 1/d series expansions shows that the theory can predict accurately the dependence of the critical temperature on disorder strength for dimensions d>4. For the bimodal distribution, we find a tricritical point which moves to weaker fields as the dimension is reduced. For the Gaussian distribution, a tricritical point may appear for d slightly above 4.

cond-mat.dis-nn↗

arXiv1995

Critical behavior of a fluid in a disordered porous matrix: An Ornstein-Zernike approach

Using a liquid-state approach based on Ornstein-Zernike equations, we study the behavior of a fluid inside a porous disordered matrix near the liquid-gas critical point.The results obtained within various standard approximation schemes such as lowest-order $γ$-ordering and the mean-spherical approximation suggest that the critical behavior is closely related to that of the random-field Ising model (RFIM).

cond-mat↗