arXiv subjects

M. L. Wall

Publications and source records attributed to M. L. Wall.

At least 19 recordsLinked to original sources

arXiv2018

Quantum dynamics of disordered spin chains with power-law interactions

We use extensive numerical simulations based on matrix product state methods to study the quantum dynamics of spin chains with strong on-site disorder and power-law decaying ($1/r^α$) interactions. We focus on two spin-$1/2$ Hamiltonians featuring power-law interactions: Heisenberg and XY and characterize their corresponding long-time dynamics using three distinct diagnostics: decay of a staggered magnetization pattern $I(t)$, growth of entanglement entropy $S(t)$, and growth of quantum Fisher information $F_Q(t).$ For sufficiently rapidly decaying interactions $α>α_c$ we find a many-body localized phase, in which $I(t)$ saturates to a non-zero value, entanglement entropy grows as $S(t)\propto t^{1/α}$, and Fisher information grows logarithmically. Importantly, entanglement entropy and Fisher information do not scale the same way (unlike short range interacting models). The critical power $α_c$ is smaller for the XY model than for the Heisenberg model.

cond-mat.dis-nn↗

arXiv2017

Dynamics of interacting fermions under spin-orbit coupling in an optical lattice clock

Quantum statistics and symmetrization dictate that identical fermions do not interact via s-wave collisions. However, in the presence of spin-orbit coupling (SOC), fermions prepared in identical internal states with distinct momenta become distinguishable. The resulting strongly interacting system can exhibit exotic topological and pairing behaviors, many of which are yet to be observed in condensed matter systems. Ultracold atomic gases offer a promising pathway for simulating these rich phenomena. Two recent experiments reported the observation of single atom SOC in optical lattice clocks (OLCs) based on alkaline-earth atoms. In these works encoding the effective spin degree of freedom in the long-lived electronic clock states significantly reduced the detrimental effects of spontaneous emission and heating that have thus far hindered the study of interacting SOC with alkali atoms. Beyond first studies of interacting SOC with alkali atoms in a bulk gas and with two particles in a lattice, here we enter a new regime of many-body interacting SOC in an OLC. Using clock spectroscopy, we observe the precession of the collective magnetization and the emergence of spin locking effects arising from an interplay between p-wave and SOC-induced exchange interactions. The many-body dynamics are well captured by a collective XXZ spin model, which describes a broad class of condensed matter systems ranging from superconductors to quantum magnets. Furthermore, our work will aid in the design of next-generation OLCs by offering a route for avoiding the observed large density shifts caused by SOC-induced exchange interactions.

physics.atom-ph↗

arXiv2017

Abdominal aortic aneurysms and endovascular sealing: deformation and dynamic response

Endovascular sealing is a new technique for the repair of abdominal aortic aneurysms. Commercially available in Europe since~2013, it takes a revolutionary approach to aneurysm repair through minimally invasive techniques. Although aneurysm sealing may be thought as more stable than conventional endovascular stent graft repairs, post-implantation movement of the endoprosthesis has been described, potentially leading to late complications. The paper presents for the first time a model, which explains the nature of forces, in static and dynamic regimes, acting on sealed abdominal aortic aneurysms, with references to real case studies. It is shown that elastic deformation of the aorta and of the endoprosthesis induced by static forces and vibrations during daily activities can potentially promote undesired movements of the endovascular sealing structure.

physics.med-ph↗

arXiv2017

Exploring many body localization and thermalization using semiclassical method

The Discrete Truncated Wigner Approximation (DTWA) is a semi-classical phase space method useful for the exploration of Many-body quantum dynamics. In this work we investigate Many-Body Localization (MBL) and thermalization using DTWA and compare its performance to exact numerical solutions. By taking as a benchmark case a 1D random field Heisenberg spin chain with short range interactions, and by comparing to numerically exact techniques, we show that DTWA is able to reproduce dynamical signatures that characterize both the thermal and the MBL phases. It exhibits the best quantitative agreement at short times deep in each of the phases and larger mismatches close to the phase transition. The DTWA captures the logarithmic growth of entanglement in the MBL phase, even though a pure classical mean-field analysis would lead to no dynamics at all. Our results suggest the DTWA can become a useful method to investigate MBL and thermalization in experimentally relevant settings intractable with exact numerical techniques, such as systems with long range interactions and/or systems in higher dimensions.

quant-ph↗

arXiv2017

Nonequilibrium dynamics of spin-boson models from phase space methods

An accurate description of the nonequilibrium dynamics of systems with coupled spin and bosonic degrees of freedom remains theoretically challenging, especially for large system sizes and in higher than one dimension. Phase space methods such as the Truncated Wigner Approximation (TWA) have the advantage of being easily scalable and applicable to arbitrary dimensions. In this work we adapt the TWA to generic spin-boson models by making use of recently developed algorithms for discrete phase spaces [Schachenmayer, PRX 5, 011022 (2015)]. Furthermore we go beyond the standard TWA approximation by applying a scheme based on the Bogoliubov-Born-Green-Kirkwood-Yvon (BBGKY) hierarchy of equations [Pucci, PRB 93, 174302 (2016)] to our coupled spin-boson model. This allows in principle to study how systematically adding higher order corrections improves the convergence of the method. To test various levels of approximation we study an exactly solvable spin-boson model which is particularly relevant for trapped-ion arrays. Using TWA and its BBGKY extension we accurately reproduce the time evolution of a number of one- and two-point correlation functions in several dimensions and for arbitrary number of bosonic modes.

cond-mat.quant-gas↗

arXiv2016

Spin-orbit coupled fermions in an optical lattice clock

Engineered spin-orbit coupling (SOC) in cold atom systems can aid in the study of novel synthetic materials and complex condensed matter phenomena. Despite great advances, alkali atom SOC systems are hindered by heating from spontaneous emission, which limits the observation of many-body effects, motivating research into potential alternatives. Here we demonstrate that SOC can be engineered to occur naturally in a one-dimensional fermionic 87Sr optical lattice clock (OLC). In contrast to previous SOC experiments, in this work the SOC is both generated and probed using a direct ultra-narrow optical clock transition between two electronic orbital states. We use clock spectroscopy to prepare lattice band populations, internal electronic states, and quasimomenta, as well as to produce SOC dynamics. The exceptionally long lifetime of the excited clock state (160 s) eliminates decoherence and atom loss from spontaneous emission at all relevant experimental timescales, allowing subsequent momentum- and spin-resolved in situ probing of the SOC band structure and eigenstates. We utilize these capabilities to study Bloch oscillations, spin-momentum locking, and Van Hove singularities in the transition density of states. Our results lay the groundwork for the use of OLCs to probe novel SOC phases of matter.

cond-mat.quant-gas↗

arXiv2015

Entangling two transportable neutral atoms via local spin exchange

To advance quantum information science a constant pursuit is the search for physical systems that meet the stringent requirements for creating and preserving quantum entanglement. In atomic physics, robust two-qubit entanglement is typically achieved by strong, long-range interactions in the form of Coulomb interactions between ions or dipolar interactions between Rydberg atoms. While these interactions allow fast gates, atoms subject to these interactions must overcome the associated coupling to the environment and cross-talk among qubits. Local interactions, such as those requiring significant wavefunction overlap, can alleviate these detrimental effects yet present a new challenge: To distribute entanglement, qubits must be transported, merged for interaction, and then isolated for storage and subsequent operations. Here we show how, via a mobile optical tweezer, it is possible to prepare and locally entangle two ultracold neutral atoms, and then separate them while preserving their entanglement. While ground-state neutral atom experiments have measured dynamics consistent with spin entanglement, and detected entanglement with macroscopic observables, we are now able to demonstrate position-resolved two-particle coherence via application of a local gradient and parity measurements; this new entanglement-verification protocol could be applied to arbitrary spin-entangled states of spatially-separated atoms. The local entangling operation is achieved via ultracold spin-exchange interactions, and quantum tunneling is used to combine and separate atoms. Our toolset provides a framework for dynamically entangling remote qubits via local operations within a large-scale quantum register.

quant-ph↗

arXiv2015

Exact calculation of phonon effects on spin squeezing

Theoretical models of spins coupled to bosons provide a simple setting for studying a broad range of important phenomena in many-body physics, from virtually mediated interactions to decoherence and thermalization. In many atomic, molecular, and optical systems, such models also underlie the most successful attempts to engineer strong, long-ranged interactions for the purpose of entanglement generation. Especially when the coupling between the spins and bosons is strong---such that it cannot be treated perturbatively---the properties of such models are extremely challenging to calculate theoretically. Here, exact analytical expressions for nonequilibrium spin-spin correlation functions are derived for a specific model of spins coupled to bosons. The spatial structure of the coupling between spins and bosons is completely arbitrary, and thus the solution can be applied to systems in any number of dimensions. The explicit and nonperturbative inclusion of the bosons enables the study of entanglement generation (in the form of spin squeezing) even when the bosons are driven strongly and near-resonantly, and thus provides a quantitative view of the breakdown of adiabatic elimination that inevitably occurs as one pushes towards the fastest entanglement generation possible. The solution also helps elucidate the effect of finite temperature on spin squeezing. The model considered is relevant to a variety of atomic, molecular, and optical systems, such as atoms in cavities or trapped ions. As an explicit example, the results are used to quantify phonon effects in trapped ion quantum simulators, which are expected to become increasingly important as these experiments push towards larger numbers of ions.

cond-mat.quant-gas↗

arXiv2015

The Role of Interspecies Interactions in the Preparation of a Low-entropy Gas of Polar Molecules in a Lattice

The preparation of a quantum degenerate gas of heteronuclear molecules has been an outstanding challenge. We use path integral Quantum Monte Carlo simulations to understand the role of interactions and finite temperature effects in the protocol currently employed to adiabatically prepare a low-entropy gas of polar molecules in a lattice starting from an ultracold Bose-Fermi mixture. We find that interspecies interactions affect the final temperature of the mixture after the adiabatic loading procedure and detrimentally limit the molecular peak filling. Our conclusions are in agreement with recent experimental measurements [1] and therefore are of immediate relevance for the myriad experiments that aim to form molecules from dual-species atomic gases.

quant-ph↗

arXiv2014

Realizing unconventional quantum magnetism with symmetric top molecules

We demonstrate that ultracold symmetric top molecules loaded into an optical lattice can realize highly tunable and unconventional models of quantum magnetism, such as an XYZ Heisenberg spin model. We show that anisotropic dipole-dipole interactions between molecules can lead to effective spin-spin interactions which exchange spin and orbital angular momentum. This exchange produces effective spin models which do not conserve magnetization and feature tunable degrees of spatial and spin-coupling anisotropy. In addition to deriving pure spin models when molecules are pinned in a deep optical lattice, we show that models of itinerant magnetism are possible when molecules can tunnel through the lattice. Additionally, we demonstrate rich tunability of the effective models' parameters using only a single microwave frequency, in contrast to proposals with $^1Σ$ diatomic molecules, which often require many microwave frequencies. Our results are germane not only for experiments with polyatomic symmetric top molecules, such as methyl fluoride (CH$_3$F), but also diatomic molecules with an effective symmetric top structure, such as the hydroxyl radical OH.

cond-mat.quant-gas↗

arXiv2014

Quantum magnetism with ultracold molecules

This article gives an introduction to the realization of effective quantum magnetism with ultracold molecules in an optical lattice, reviews experimental and theoretical progress, and highlights future opportunities opened up by ongoing experiments. Ultracold molecules offer capabilities that are otherwise difficult or impossible to achieve in other effective spin systems, such as long-ranged spin-spin interactions with controllable degrees of spatial and spin anisotropy and favorable energy scales. Realizing quantum magnetism with ultracold molecules provides access to rich many-body behaviors, including many exotic phases of matter and interesting excitations and dynamics. Far-from-equilibrium dynamics plays a key role in our exposition, just as it did in recent ultracold molecule experiments realizing effective quantum magnetism. In particular, we show that dynamical probes allow the observation of correlated many-body spin physics, even in polar molecule gases that are not quantum degenerate. After describing how quantum magnetism arises in ultracold molecules and discussing recent observations of quantum magnetism with polar molecules, we survey prospects for the future, ranging from immediate goals to long-term visions.

cond-mat.quant-gas↗

arXiv2014

Hong-Ou-Mandel atom interferometry in tunnel-coupled optical tweezers

The quantum statistics of atoms is typically observed in the behavior of an ensemble via macroscopic observables. However, quantum statistics modifies the behavior of even two particles, inducing remarkable consequences that are at the heart of quantum science. Here we demonstrate near-complete control over all the internal and external degrees of freedom of two laser-cooled 87Rb atoms trapped in two optical tweezers. This full controllability allows us to implement a massive-particle analog of a Hong-Ou-Mandel interferometer where atom tunneling plays the role of a photon beamsplitter. We use the interferometer to probe the effect of quantum statistics on the two-atom dynamics under tunable initial conditions, chosen to adjust the degree of atomic indistinguishability. Our work thereby establishes laser-cooled atoms in optical tweezers as a new route to bottom-up engineering of scalable, low-entropy quantum systems.

cond-mat.quant-gas↗

arXiv2014

Realizing topological states with polyatomic symmetric top molecules

We demonstrate that ultracold polyatomic symmetric top molecules, such as methyl fluoride, loaded into an optical lattice and subject to DC electric and microwave field dressing, can display topological order via a self-consistent analog of a proximity effect in the internal state space of the molecule. The non-trivial topology arises from pairwise transitions between internal states induced by dipole-dipole interactions and made resonant by the field dressing. Topological order is explicitly demonstrated by matrix product state simulations on 1D chains. Additionally, we show that in the limit of pinned molecules our description maps onto a long-range and anisotropic XYZ spin model, where Majorana fermions are zero-energy edge excitations in the case of nearest-neighbor couplings.

cond-mat.quant-gas↗

arXiv2013

Dipole-dipole interactions in optical lattices do not follow an inverse cube power law

We study the effective dipole-dipole interactions in ultracold quantum gases on optical lattices as a function of asymmetry in confinement along the principal axes of the lattice. In particular, we study the matrix elements of the dipole-dipole interaction in the basis of lowest band Wannier functions which serve as a set of low-energy states for many-body physics on the lattice. We demonstrate that the effective interaction between dipoles in an optical lattice is non-algebraic in the inter-particle separation at short to medium distance on the lattice scale and has a long-range power-law tail, in contrast to the pure power-law behavior of the dipole-dipole interaction in free space. The modifications to the free-space interaction can be sizable; we identify differences of up to 36% from the free-space interaction at the nearest-neighbor distance in quasi-1D arrangements. The interaction difference depends essentially on asymmetry in confinement, due to the d-wave anisotropy of the dipole-dipole interaction. Our results do not depend on statistics, applying to both dipolar Bose-Einstein condensates and degenerate Fermi gases. Using matrix product state simulations, we demonstrate that use of the correct lattice dipolar interaction leads to significant deviations from many-body predictions using the free-space interaction. Our results are relevant to up and coming experiments with ultracold heteronuclear molecules, Rydberg atoms, and strongly magnetic atoms in optical lattices.

cond-mat.quant-gas↗

arXiv2013

Strongly interacting fermions in an optical lattice

We analyze a system of two-component fermions which interact via a Feshbach resonance in the presence of a three-dimensional lattice potential. By expressing a two-channel model of the resonance in the basis of Bloch states appropriate for the lattice, we derive an eigenvalue equation for the two-particle bound states which is nonlinear in the energy eigenvalue. Compact expressions for the interchannel matrix elements, numerical methods for the solution of the nonlinear eigenvalue problem, and a renormalization procedure to remove ultraviolet divergences are presented. From the structure of the two-body solutions we identify the relevant degrees of freedom which describe the resonance behavior in the lowest Bloch band. These degrees of freedom, which we call dressed molecules, form an effective closed channel in a many-body model of the resonance, the Fermi resonance Hamiltonian (FRH). It is shown how the properties of the FRH can be determined numerically by solving a projected lattice two-channel model at the two-particle level. As opposed to single-channel lattice models such as the Hubbard model, the FRH is valid for general s-wave scattering length and resonance width. Hence, the FRH provides an accurate description of the BEC-BCS crossover for ultracold fermions on an optical lattice.

cond-mat.quant-gas↗

arXiv2013

The Molecular Hubbard Hamiltonian: Field Regimes and Molecular Species

The molecular Hubbard Hamiltonian (MHH) naturally arises for ultracold ground state polar alkali dimer molecules in optical lattices. We show that, unlike ultracold atoms, different molecules display different many-body phases due to intrinsic variances in molecular structure even when the molecular symmetry is the same. We also demonstrate a wide variety of experimental controls on $^1Σ$ molecules via external fields, including applied static electric and magnetic fields, an AC microwave field, and the polarization and strength of optical lattice beams. We provide explicit numerical calculations of the parameters of the MHH, including tunneling and direct and exchange dipole-dipole interaction energies, for the molecules {$^{6}$Li$^{133}$Cs}, $^{23}$Na$^{40}$K, $^{87}$Rb$^{133}$Cs, $^{40}$K$^{87}$Rb, and {$^{6}$Li$^{23}$Na} in weak and strong applied electric fields. As case studies of many-body physics, we use infinite-size matrix product state methods to explore the quantum phase transitions from the superfluid phase to half-filled and third-filled crystalline phases in one dimension.

cond-mat.quant-gas↗

arXiv2012

Microscopic model for Feshbach interacting fermions in an optical lattice with arbitrary scattering length and resonance width

We numerically study the problem of two fermions in a three dimensional optical lattice interacting via a zero-range Feshbach resonance, and display the dispersions of the bound states as a two-particle band structure with unique features compared to typical single-particle band structures. We show that the exact two-particle solutions of a projected Hamiltonian may be used to define an effective two-channel, few-band model for the low energy, low density physics of many fermions at arbitrary s-wave scattering length. Our method applies to resonances of any width, and can be adapted to multichannel situations or higher-$\ell$ pairing. In strong contrast to usual Hubbard physics, we find that pair hopping is significantly altered by strong interactions and the presence of the lattice, and the lattice induces multiple molecular bound states.

cond-mat.quant-gas↗

arXiv2012

Out of equilibrium dynamics with Matrix Product States

Theoretical understanding of strongly correlated systems in one spatial dimension (1D) has been greatly advanced by the density-matrix renormalization group (DMRG) algorithm, which is a variational approach using a class of entanglement-restricted states called Matrix Product States (MPSs). However, DRMG suffers from inherent accuracy restrictions when multiple states are involved due to multi-state targeting and also the approximate representation of the Hamiltonian and other operators. By formulating the variational approach of DMRG explicitly for MPSs one can avoid errors inherent in the multi-state targeting approach. Furthermore, by using the Matrix Product Operator (MPO) formalism, one can exactly represent the Hamiltonian and other operators. The MPO approach allows 1D Hamiltonians to be templated using a small set of finite state automaton rules without reference to the particular microscopic degrees of freedom. We present two algorithms which take advantage of these properties: eMPS to find excited states of 1D Hamiltonians and tMPS for the time evolution of a generic time-dependent 1D Hamiltonian. We properly account for time-ordering of the propagator such that the error does not depend on the rate of change of the Hamiltonian. Our algorithms use only the MPO form of the Hamiltonian, and so are applicable to microscopic degrees of freedom of any variety, and do not require Hamiltonian-specialized implementation. We benchmark our algorithms with a case study of the Ising model, where the critical point is located using entanglement measures. We then study the dynamics of this model under a time-dependent quench of the transverse field through the critical point. Finally, we present studies of a dipolar, or long-range Ising model, again using entanglement measures to find the critical point and study the dynamics of a time-dependent quench through the critical point.

cond-mat.stat-mech↗