arXiv subjects

M. M. Parish

Publications and source records attributed to M. M. Parish.

At least 19 recordsLinked to original sources

arXiv2024

Rydberg excitons and polaritons in monolayer transition metal dichalcogenides in a magnetic field

We develop a microscopic theory for excitons and cavity exciton polaritons in transition metal dichalcogenide (TMD) monolayers under a perpendicular static magnetic field. We obtain numerically exact solutions for the ground and excited states, accounting for the interplay between arbitrarily large magnetic fields and light-matter coupling strengths. This includes the very strong coupling regime, where light-induced modifications of the exciton wavefunction become essential and the approximate coupled oscillator description breaks down. Our results show excellent agreement with recent experimental measurements of the diamagnetic shift of the ground and excited exciton states in WS$_2$, MoS$_2$, MoSe$_2$, and MoTe$_2$ monolayers. For polaritons, we consider experimentally relevant system parameters and demonstrate that the diamagnetic shifts of both the ground and excited states at high magnetic fields exhibit clear signatures of the very strong coupling regime, highlighting the necessity of our microscopic and numerically exact treatment over perturbative approaches. Furthermore, our microscopic approach allows us to evaluate the exciton-exciton and polariton-polariton interaction strengths. Comparing results specific to TMD monolayers with those applicable to quantum wells, we find that variational approaches overestimate the TMD excitons' interaction strength. We also observe that magnetic fields weaken the interaction strength for both excitons and polaritons, with a less pronounced effect in TMDs than in quantum wells, and that light-induced modifications to the matter component in TMD polaritons can enhance interaction strengths beyond those of purely excitonic interactions.

cond-mat.mes-hall↗

arXiv2024

Multiple polaron quasiparticles with dipolar fermions in a bilayer geometry

We study the Fermi polaron problem with dipolar fermions in a bilayer geometry, where a single dipolar particle in one layer interacts with a Fermi sea of dipolar fermions in the other layer. By evaluating the polaron spectrum, we obtain the appearance of a series of attractive branches when the distance between the layers diminishes. We relate these to the appearance of a series of bound two-dipole states when the interlayer dipolar interaction strength increases. By inspecting the orbital angular momentum component of the polaron branches, we observe an interchange of orbital character when system parameters such as the gas density or the interlayer distance are varied. Further, we study the possibility that the lowest energy two-body bound state spontaneously acquires a finite center of mass momentum when the density of fermions exceeds a critical value, and we determine the dominating orbital angular momenta that characterize the pairing. Finally, we propose to use the tunneling rate from and into an auxiliary layer as an experimental probe of the impurity spectral function.

cond-mat.quant-gas↗

arXiv2022

Crossover from exciton polarons to trions in doped two-dimensional semiconductors at finite temperature

We study systematically the role of temperature in the optical response of doped two-dimensional semiconductors. By making use of a finite-temperature Fermi-polaron theory, we reveal a crossover from a quantum-degenerate regime with well-defined polaron quasiparticles to an incoherent regime at high temperature or low doping where the lowest energy "attractive" polaron quasiparticle is destroyed, becoming subsumed into a broad trion-hole continuum. We demonstrate that the crossover is accompanied by significant qualitative changes in both absorption and photoluminescence. In particular, with increasing temperature (or decreasing doping), the emission profile of the attractive branch evolves from a symmetric Lorentzian to an asymmetric peak with an exponential tail involving trions and recoil electrons at finite momentum. We discuss the effect of temperature on the coupling to light for structures embedded into a microcavity, and we show that there can exist well-defined polariton quasiparticles even when the exciton-polaron quasiparticle has been destroyed, where the transition from weak to strong light-matter coupling can be explained in terms of the polaron linewidths and spectral weights.

cond-mat.mes-hall↗

arXiv2022

Exact Quantum Virial Expansion for the Optical Response of Doped Two-Dimensional Semiconductors

We present a quantum virial expansion for the optical response of a doped two-dimensional semiconductor. As we show, this constitutes a perturbatively exact theory in the high-temperature or low-doping regime, where the electrons' thermal wavelength is smaller than their interparticle spacing. The virial expansion predicts new features of the photoluminescence, such as a non-trivial shape of the attractive branch related to universal low-energy exciton-electron scattering and an associated shift of the attractive peak from the trion energy. Our results are in excellent agreement with recent experiments on doped monolayer MoSe$_2$ [Zipfel et al., Phys. Rev. B 105, 075311 (2022)] and they imply that the trion binding energy is likely to have been overestimated in previous measurements. Our theory furthermore allows us to formally unify two distinct theoretical pictures that have been applied to this system, with the conventional trion picture results emerging as a high-temperature and weak-interaction limit of Fermi polaron theory.

cond-mat.mes-hall↗

arXiv2021

Effect of fermion indistinguishability on optical absorption of doped two-dimensional semiconductors

We study the optical absorption spectrum of a doped two-dimensional semiconductor in the spin-valley polarized limit. In this configuration, the carriers in the Fermi sea are indistinguishable from one of the two carriers forming the exciton. Most notably, this indistinguishability requires the three-body trion state to have p-wave symmetry. To explore the consequences of this, we evaluate the system's optical properties within a polaron description, which can interpolate from the low density limit -- where the relevant excitations are few-body bound states -- to higher density many-body states. In the parameter regime where the trion is bound, we demonstrate that the spectrum is characterized by an attractive quasiparticle branch, a repulsive branch, and a many-body continuum, and we evaluate the doping dependence of the corresponding energies and spectral weights. In particular, at low doping we find that the oscillator strength of the attractive branch scales with the square of the Fermi energy as a result of the trion's p-wave symmetry. Upon increasing density, we find that both the repulsive and attractive branches blueshift, and that the orbital character of the states associated with these branches interchanges. We compare our results with previous investigations of the scenario where the Fermi sea involves carriers distinguishable from those in the exciton, for which the trion ground state is s-wave.

cond-mat.mes-hall↗

arXiv2020

Polariton interactions in microcavities with atomically thin semiconductor layers

We investigate the interactions between exciton-polaritons in N two-dimensional semiconductor layers embedded in a planar microcavity. In the limit of low-energy scattering, where we can ignore the composite nature of the excitons, we obtain exact analytical expressions for the spin-triplet and spin-singlet interaction strengths, which go beyond the Born approximation employed in previous calculations. Crucially, we find that the strong light-matter coupling enhances the strength of polariton-polariton interactions compared to that of the exciton-exciton interactions, due to the Rabi coupling and the small photon-exciton mass ratio. We furthermore obtain the dependence of the polariton interactions on the number of layers N, and we highlight the important role played by the optically dark states that exist in multiple layers. In particular, we predict that the singlet interaction strength is stronger than the triplet one for a wide range of parameters in most of the currently used transition metal dichalcogenides. This has consequences for the pursuit of polariton condensation and other interaction-driven phenomena in these materials.

cond-mat.mes-hall↗

arXiv2019

Extremely imbalanced two-dimensional electron-hole-photon systems

We investigate the phases of two-dimensional electron-hole systems strongly coupled to a microcavity photon field in the limit of extreme charge imbalance. Using variational wave functions, we examine the competition between different electron-hole paired states for the specific cases of semiconducting III-V single quantum wells, electron-hole bilayers, and transition metal dichalcogenide monolayers embedded in a planar microcavity. We show how the Fermi sea of excess charges modifies both the electron-hole bound state (exciton) properties and the dielectric constant of the cavity active medium, which in turn affects the photon component of the many-body polariton ground state. On the one hand, long-range Coulomb interactions and Pauli blocking of the Fermi sea promote electron-hole pairing with finite center-of-mass momentum, corresponding to an excitonic roton minimum. On the other hand, the strong coupling to the ultra-low-mass cavity photon mode favors zero-momentum pairs. We discuss the prospect of observing different types of electron-hole pairing in the photon spectrum.

cond-mat.mes-hall↗

arXiv2019

Frustrated orbital Feshbach resonances in a Fermi gas

The orbital Feshbach resonance (OFR) is a novel scheme for magnetically tuning the interactions in closed-shell fermionic atoms. Remarkably, unlike the Feshbach resonances in alkali atoms, the open and closed channels of the OFR are only very weakly detuned in energy. This leads to a unique effect whereby a medium in the closed channel can Pauli block, or frustrate, the two-body scattering processes. Here, we theoretically investigate the impact of frustration in the few- and many-body limits of the experimentally accessible three-dimensional $^{173}$Yb system. We find that by adding a closed-channel atom to the two-body problem, the binding energy of the ground state is significantly suppressed, and by introducing a closed-channel Fermi sea to the many-body problem, we can drive the system towards weaker fermion pairing. These results are potentially relevant to superconductivity in solid-state multiband materials, as well as to the current and continuing exploration of unconventional Fermi-gas superfluids near the OFR.

cond-mat.quant-gas↗

arXiv2019

Direct measurement of polariton-polariton interaction strength in the Thomas-Fermi regime of exciton-polariton condensation

Bosonic condensates of exciton polaritons (light-matter quasiparticles in a semiconductor) provide a solid-state platform for studies of non-equilibrium quantum systems with a spontaneous macroscopic coherence. These driven, dissipative condensates typically coexist and interact with an incoherent reservoir, which undermines measurements of key parameters of the condensate. Here, we overcome this limitation by creating a high-density exciton-polariton condensate in an optically-induced "box" trap. In this so-called Thomas-Fermi regime, the condensate is fully separated from the reservoir and its behaviour is dominated by interparticle interactions. We use this regime to directly measure the polariton-polariton interaction strength, and reduce the existing uncertainty in its value from four orders of magnitude to within three times the theoretical prediction. The Thomas-Fermi regime has previously been demonstrated only in ultracold atomic gases in thermal equilibrium. In a non-equilibrium exciton-polariton system, this regime offers a novel opportunity to study interaction-driven effects unmasked by an incoherent reservoir.

cond-mat.quant-gas↗

arXiv2018

Early-time dynamics of Bose gases quenched into the strongly interacting regime

We study the early-time dynamics of a degenerate Bose gas after a sudden quench of the interaction strength, starting from a weakly interacting gas. By making use of a time-dependent generalization of the Nozières-Saint-James variational formalism, we describe the crossover of the early-time dynamics from shallow to deep interaction quenches. We analyze the coherent oscillations that characterize both the density of excited states and the Tan's contact as a function of the final scattering length. For shallow quenches, the oscillatory behaviour is negligible and the dynamics is universally governed by the healing length and the mean-field interaction energy. By increasing the final scattering length to intermediate values, we reveal a universal regime where the period of the coherent atom-molecule oscillations is set by the molecule binding energy. For the largest scattering lengths we can numerically simulate in the unitary regime, we find a universal scaling behaviour of the typical growth time of the momentum distribution in agreement with recent experimental observations [C. Eigen et al., Nature 563, 221 (2018)].

cond-mat.quant-gas↗

arXiv2018

SU(N) Fermions in a One-Dimensional Harmonic Trap

We conduct a theoretical study of SU(N) fermions confined by a one-dimensional harmonic potential. Firstly, we introduce a new numerical approach for solving the trapped interacting few-body problem, by which one may obtain accurate energy spectra across the full range of interaction strengths. In the strong-coupling limit, we map the SU(N) Hamiltonian to a spin-chain model. We then show that an existing, extremely accurate ansatz - derived for a Heisenberg SU(2) spin chain - is extendable to these N-component systems. Lastly, we consider balanced SU(N) Fermi gases that have an equal number of particles in each spin state for N=2, 3, 4. In the weak- and strong-coupling regimes, we find that the ground-state energies rapidly converge to their expected values in the thermodynamic limit with increasing atom number. This suggests that the many-body energetics of N-component fermions may be accurately inferred from the corresponding few-body systems of N distinguishable particles.

cond-mat.quant-gas↗

arXiv2016

Ultrafast many-body interferometry of impurities coupled to a Fermi sea

The fastest possible collective response of a quantum many-body system is related to its excitations at the highest possible energy. In condensed-matter systems, the corresponding timescale is typically set by the Fermi energy. Taking advantage of fast and precise control of interactions between ultracold atoms, we report on the observation of ultrafast dynamics of impurities coupled to an atomic Fermi sea. Our interferometric measurements track the non-perturbative quantum evolution of a fermionic many-body system, revealing in real time the formation dynamics of quasiparticles and the quantum interference between attractive and repulsive states throughout the full depth of the Fermi sea. Ultrafast time-domain methods to manipulate and investigate strongly interacting quantum gases open up new windows on the dynamics of quantum matter under extreme non-equilibrium conditions.

cond-mat.quant-gas↗

arXiv2016

Dipolar fermions in a multilayer geometry

We investigate the behavior of identical dipolar fermions with aligned dipole moments in two-dimensional multilayers at zero temperature. We consider density instabilities that are driven by the attractive part of the dipolar interaction and, for the case of bilayers, we elucidate the properties of the stripe phase recently predicted to exist in this interaction regime. When the number of layers is increased, we find that this "attractive" stripe phase exists for an increasingly larger range of dipole angles, and if the interlayer distance is sufficiently small, the stripe phase eventually spans the full range of angles, including the situation where the dipole moments are aligned perpendicular to the planes. In the limit of an infinite number of layers, we derive an analytic expression for the interlayer effects in the density-density response function and, using this result, we find that the stripe phase is replaced by a collapse of the dipolar system.

cond-mat.quant-gas↗

arXiv2016

Observation of an orbital interaction-induced Feshbach resonance in 173-Yb

We report on the experimental observation of a novel inter-orbital Feshbach resonance in ultracold 173-Yb atoms, which opens the possibility of tuning the interactions between the 1S0 and 3P0 metastable state, both possessing vanishing total electronic angular momentum. The resonance is observed at experimentally accessible magnetic field strengths and occurs universally for all hyperfine state combinations. We characterize the resonance in the bulk via inter-orbital cross-thermalization as well as in a three-dimensional lattice using high-resolution clock-line spectroscopy.

cond-mat.quant-gas↗

arXiv2013

Optical recombination of biexcitons in semiconductors

We calculate the photoluminescence spectrum and lifetime of a biexciton in a semiconductor using Fermi's golden rule. Our biexciton wavefunction is obtained using a Quantum Monte Carlo calculation. We consider a recombination process where one of the excitons within the biexciton annihilates. For hole masses greater than or equal to the electron mass, we find that the surviving exciton is most likely to populate the ground state. We also investigate how the confinement of excitons in a quantum dot would modify the lifetime in the limit of a large quantum dot where confinement principally affects the centre of mass wavefunction. The lifetimes we obtain are in reasonable agreement with experimental values. Our calculation can be used as a benchmark for comparison with approximate methods.

cond-mat.str-el↗

arXiv2012

Density-wave phases of dipolar fermions in a bilayer

We investigate the phase diagram of dipolar fermions with aligned dipole moments in a two-dimensional (2D) bilayer. Using a version of the Singwi-Tosi-Land-Sjolander scheme recently adapted to dipolar fermions in a single layer [M. M. Parish and F. M. Marchetti, Phys. Rev. Lett. 108, 145304 (2012)], we determine the density-wave instabilities of the bilayer system within linear response theory. We find that the bilayer geometry can stabilize the collapse of the 2D dipolar Fermi gas with intralayer attraction to form a new density wave phase that has an orientation perpendicular to the density wave expected for strong intralayer repulsion. We thus obtain a quantum phase transition between stripe phases that is driven by the interplay between strong correlations and the architecture of the low dimensional system.

cond-mat.quant-gas↗

arXiv2009

Stability and pairing in quasi-one-dimensional Bose-Fermi mixtures

We consider a mixture of single-component bosonic and fermionic atoms in an array of coupled one-dimensional "tubes". For an attractive Bose-Fermi interaction, we show that the system exhibits phase separation instead of the usual collapse. Moreover, above a critical inter-tube hopping, all first-order instabilities disappear in both attractive and repulsive mixtures. The possibility of suppressing instabilities in this system suggests a route towards the realization of paired phases, including a superfluid of p-wave pairs unique to the coupled-tube system, and quantum critical phenomena.

cond-mat.other↗

arXiv2008

Phase separation and collapse in Bose-Fermi mixtures with a Feshbach resonance

We consider a mixture of single-component bosonic and fermionic atoms with an interspecies interaction that is varied using a Feshbach resonance. By performing a mean-field analysis of a two-channel model, which describes both narrow and broad Feshbach resonances, we find an unexpectedly rich phase diagram at zero temperature: Bose-condensed and non-Bose-condensed phases form a variety of phase-separated states that are accompanied by both critical and tricritical points. We discuss the implications of our results for the experimentally observed collapse of Bose-Fermi mixtures on the attractive side of the Feshbach resonance, and we make predictions for future experiments on Bose-Fermi mixtures close to a Feshbach resonance.

cond-mat.other↗