arXiv subjects

M. Macucci

Publications and source records attributed to M. Macucci.

15 recordsLinked to original sources

arXiv2017

Inkjet Printed 2D-Crystal Based Strain Gauges on Paper

We present an investigation of inkjet printed strain gauges based on two-dimensional (2D) materials. The technology leverages water-based and biocompatible inks to fabricate strain measurement devices on flexible substrates such as paper. We demonstrate that the device performance and sensitivity are strongly dependent on the printing parameter (i.e., drop- spacing, number of printing passes, etc.). We show that values of the Gauge Factor up to 125 can be obtained, with large sensitivity (>20%) even when small strains (0.3%) are applied. Furthermore, we provide preliminary examples of heterostructure-based strain sensors, enabled by the inkjet printing technology.

physics.app-ph↗

arXiv2017

Improvement of the 3$ω$ thermal conductivity measurement technique at nanoscale

The reduction of the thermal conductivity in nanostructures opens up the possibility of exploiting for thermoelectric purposes also materials such as silicon, which are cheap, available and sustainable but with a high thermal conductivity in their bulk form. The development of thermoelectric devices based on these innovative materials requires reliable techniques for the measurement of thermal conductivity on a nanometric scale. The approximations introduced by conventional techniques for thermal conductivity measurements can lead to unreliable results when applied to nanostructures, because heaters and temperature sensors needed for the measurement cannot have a negligible size, and therefore perturb the result. In this paper we focus on the 3$ω$ technique, applied to the thermal conductivity measurement of suspended silicon nanomembranes. To overcome the approximations introduced by conventional analytical models used for the interpretation of the 3$ω$ data, we propose to use a numerical solution, performed by means of finite element modeling, of the thermal and electrical transport equations. An excellent fit of the experimental data will be presented, discussed, and compared with an analytical model.

cond-mat.mes-hall↗

arXiv2017

Water-based and Biocompatible 2D Crystal Inks: from Ink Formulation to All- Inkjet Printed Heterostructures

Fully exploiting the properties of 2D crystals requires a mass production method able to produce heterostructures of arbitrary complexity on any substrate, including plastic. Solution processing of graphene allows simple and low-cost techniques such as inkjet printing to be used for device fabrication. However, available inkjet printable formulations are still far from ideal as they are either based on toxic solvents, have low concentration, or require time-consuming and expensive formulation processing. In addition, none of those formulations are suitable for thin-film heterostructure fabrication due to the re-mixing of different 2D crystals, giving rise to uncontrolled interfaces, which results in poor device performance and lack of reproducibility. In this work we show a general formulation engineering approach to achieve highly concentrated, and inkjet printable water-based 2D crystal formulations, which also provides optimal film formation for multi-stack fabrication. We show examples of all-inkjet printed heterostructures, such as large area arrays of photosensors on plastic and paper and programmable logic memory devices, fully exploiting the design flexibility of inkjet printing. Finally, dose-escalation cytotoxicity assays in vitro also confirm the inks biocompatible character, revealing the possibility of extending use of such 2D crystal formulations to drug delivery and biomedical applications.

cond-mat.mtrl-sci↗

arXiv2014

Direct Imaging of Coherent Quantum Transport in Graphene Heterojunctions

We fabricate a graphene p-n-p heterojunction and exploit the coherence of weakly-confined Dirac quasiparticles to resolve the underlying scattering potential using low temperature scanning gate microscopy. The tip-induced perturbation to the heterojunction modifies the condition for resonant scattering, enabling us to detect localized Fabry-Perot cavities from the focal point of halos in scanning gate images. In addition to halos over the bulk we also observe ones spatially registered to the physical edge of the graphene. Guided by quantum transport simulations we attribute these to modified resonant scattering at the edges within elongated cavities that form due to focusing of the electrostatic field.

cond-mat.mes-hall↗

arXiv2012

Unraveling quantum Hall breakdown in bilayer graphene with scanning gate microscopy

We use low-temperature scanning gate microscopy (SGM) to investigate the breakdown of the quantum Hall regime in an exfoliated bilayer graphene flake. SGM images captured during breakdown exhibit intricate patterns of "hotspots" where the conductance is strongly affected by the presence of the tip. Our results are well described by a model based on quantum percolation which relates the points of high responsivity to tip-induced scattering between localized Landau levels.

cond-mat.mes-hall↗

arXiv2009

Quantum analysis of shot noise suppression in a series of tunnel barriers

We report the results of an analysis, based on a straightforward quantum-mechanical model, of shot noise suppression in a structure containing cascaded tunneling barriers. Our results exhibit a behavior that is in sharp contrast with existing semiclassical models for this particular type of structure, which predict a limit of 1/3 for the Fano factor as the number of barriers is increased. The origin of this discrepancy is investigated and attributed to the presence of localization on the length scale of the mean free path, as a consequence of the strictly 1-dimensional nature of disorder, which does not create mode mixing, while no localization appears in common semiclassical models. We expect localization to be indeed present in practical situations with prevalent 1-D disorder, and the existing experimental evidence appears to be consistent with such a prediction.

cond-mat.mes-hall↗

arXiv2009

Symmetry causes a huge conductance peak in double quantum dots

We predict a huge interference effect contributing to the conductance through large ultra-clean quantum dots of chaotic shape. When a double-dot structure is made such that the dots are the mirror-image of each other, constructive interference can make a tunnel barrier located on the symmetry axis effectively transparent. We show (via theoretical analysis and numerical simulation) that this effect can be orders of magnitude larger than the well-known universal conductance fluctuations and weak-localization (both less than a conductance quantum). A small magnetic field destroys the effect, massively reducing the double-dot conductance; thus a magnetic field detector is obtained, with a similar sensitivity to a SQUID, but requiring no superconductors.

cond-mat.mes-hall↗

arXiv2006

Analysis of shot noise suppression in mesoscopic cavities in a magnetic field

We present a numerical investigation of shot noise suppression in mesoscopic cavities and an intuitive semiclassical explanation of the behavior observed in the presence of an orthogonal magnetic field. In particular, we conclude that the decrease of shot noise for increasing magnetic field is the result of the interplay between the diameter of classical cyclotron orbits and the width of the apertures defining the cavity. Good agreement with published experimental results is obtained, without the need of introducing fitting parameters.

cond-mat.mes-hall↗

arXiv1999

Thermal behavior of Quantum Cellular Automaton wires

We investigate the effect of a finite temperature on the behavior of logic circuits based on the principle of Quantum Cellular Automata (QCA) and of ground state computation. In particular, we focus on the error probability for a wire of QCA cells that propagates a logic state. A numerical model and an analytical, more approximate, model are presented for the evaluation of the partition function of such a system and, consequently, of the desired probabilities. We compare the results of the two models, assessing the limits of validity of the analytical approach, and provide estimates for the maximum operating temperature.

cond-mat↗

arXiv1999

Operation of Quantum Cellular Automaton cells with more than two electrons

We present evidence that operation of QCA (Quantum Cellular Automaton) cells with four dots is possible with an occupancy of 4N+2 electrons per cell (N being an integer). We show that interaction between cells can be described in terms of a revised formula for cell polarization, which is based only on the difference between diagonal occupancies. We validate our conjectures with full quantum simulations of QCA cells for a number of electrons varying from 2 to 6, using the Configuration-Interaction method.

cond-mat.mes-hall↗

arXiv1998

Modeling and manufacturability assessment of bistable quantum-dot cells

We have investigated the behavior of bistable cells made up of four quantum dots and occupied by two electrons, in the presence of realistic confinement potentials produced by depletion gates on top of a GaAs/AlGaAs heterostructure. Such a cell represents the basic building block for logic architectures based on the concept of Quantum Cellular Automata (QCA) and of ground state computation, which have been proposed as an alternative to traditional transistor-based logic circuits. We have focused on the robustness of the operation of such cells with respect to asymmetries deriving from fabrication tolerances. We have developed a 2-D model for the calculation of the electron density in a driven cell in response to the polarization state of a driver cell. Our method is based on the one-shot Configuration-Interaction technique, adapted from molecular chemistry. From the results of our simulations, we conclude that an implementation of QCA logic based on simple ``hole-arrays'' is not feasible, because of the extreme sensitivity to fabrication tolerances. As an alternative, we propose cells defined by multiple gates, where geometrical asymmetries can be compensated for by adjusting the bias voltages. Even though not immediately applicable to the implementation of logic gates and not suitable for large scale integration, the proposed cell layout should allow an experimental demonstration of a chain of QCA cells.

cond-mat↗

arXiv1998

Simulation of a non-invasive charge detector for quantum cellular automata

Information in a Quantum Cellular Automata architecture is encoded in the polarizazion state of a cell, i.e., in the occupation numbers of the quantum dots of which the cell is made up. Non-invasive charge detectors of single electrons in a quantum dot are therefore needed, and recent experiments have shown that a quantum constriction electrostatically coupled to the quantum dot may be a viable solution. We have performed a numerical simulation of a system made of a quantum dot and a nearby quantum point contact defined, by means of depleting metal gates, in a two-dimensional electron gas at a GaAs/AlGaAs heterointerface. We have computed the occupancy of each dot and the resistance of the quantum wire as a function of the voltage applied to the plunger gate, and have derived design criteria for achieving optimal sensitivity.

cond-mat↗

arXiv1997

Enhanced shot noise in resonant tunneling: theory and experiment

We show that shot noise in a resonant tunneling diode biased in the negative differential resistance regions of the I-V characteristic is enhanced with respect to ``full'' shot noise. We provide experimental results showing a Fano factor up to 6.6, and show that it is a dramatic effect caused by electron-electron interaction through Coulomb force, enhanced by the particular shape of the density of states in the well. We also present numerical results from the proposed theory, which are in agreement with the experiment, demonstrating that the model accounts for the relevant physics involved in the phenomenon.

cond-mat.str-el↗

arXiv1997

Theory of conductance and noise additivity in parallel mesoscopic conductors

We present a theory of conductance and noise in generic mesoscopic conductors connected in parallel, and we demonstrate that the additivity of conductance and of shot noise arises as a sole property of the junctions connecting the two (or more) conductors in parallel. Consequences on the functionality of devices based on the Aharonov-Bohm effect are also drawn.

cond-mat.mes-hall↗

arXiv1996

Shot noise in resonant tunneling structures

We propose a quantum mechanical approach to noise in resonant tunneling structures, that can be applied in the whole range of transport regimes, from completely coherent to completely incoherent. In both limiting cases, well known results which have appeared in the literature are recovered. Shot noise reduction due to both Pauli exclusion and Coulomb repulsion, and their combined effect, are studied as a function of the rate of incoherent processes in the well (which are taken into account by means of a phenomenological relaxation time), and of temperature. Our approach allows the study of noise in a variety of operating conditions (i.e., equilibrium, sub-peak voltages, second resonance voltages), and as a function of temperature, explaining experimental results and predicting interesting new results.

cond-mat↗