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M. Millot

Publications and source records attributed to M. Millot.

3 recordsLinked to original sources

Ionization and temperature measurements in warm dense copper using x-ray absorption spectroscopy

We detail experimental results inferring ionization and temperature for warm dense copper plasmas at several times solid density (15 to 25 g/cm$^3$) and temperatures of 10 to 21 eV. Experiments performed at the OMEGA Laser Facility generate uniform warm dense matter conditions via symmetric shock compression of a buried copper layer. The plasma is probed with a laser-generated x-ray source to collect the K-shell x-ray absorption spectrum. Fitting bound-bound absorption contributions from constituent charge states of copper provides an estimated $\overline{Z}$ of approximately 4 to 7 for these warm dense copper plasmas. We find that these partially ionized plasmas have K-edge shifts of 12 to 30 eV and bound-bound resonance 1s$\rightarrow$3p absorption shifts of 4 to 26 eV with respect to the cold K-edge. This study provides necessary experimental data to improve ionization and opacity models in the warm dense matter regime.

hep-ex

Multi-Messenger Measurements of the Static Structure of Shock-Compressed Liquid Silicon at 100 GPa

Ionic structure of high pressure, high temperature fluids is a challenging theoretical problem with applications to planetary interiors and fusion capsules. Here we report a multi-messenger platform using velocimetry and \textit{in situ} angularly and spectrally resolved X-ray scattering to measure the thermodynamic conditions and ion structure factor of materials at extreme pressures. We document the pressure, density, and temperature of shocked silicon near 100 GPa with uncertainties of 6%, 2%, and 20%, respectively. The measurements are sufficient to distinguish between and rule out some ion screening models.

hep-ex

Weak ferrimagnetism and multiple magnetization reversal in α-Cr3(PO4)2

The chromium(II) orthophosphate α-Cr3(PO4)2 is a weak ferrimagnet with the Curie temperature TC = 29 K confirmed by a λ-type peak in specific heat. Dominant antiferromagnetic interactions in this system are characterized by the Weiss temperature Θ = - 96 K, indicating an intermediate frustration ratio |Θ|/TC ~ 3. In its magnetically ordered states α-Cr3(PO4)2 exhibits a remarkable sequence of temperature-induced magnetization reversals sensitive to the protocol of measurements, i.e. either field-cooled or zero-field-cooled regimes. The reduction of the effective magnetic moment 4.5 μB/Cr2+, as compared to the spin-only moment 4.9 μB/Cr2+, cannot be ascribed to the occurence of the low-spin state in any crystallographic site of the Jahn-Teller active 3d4 Cr2+ ions. X-ray absorption spectra at the K-edge indicate divalent chromium and unravel the high-spin state of these ions at the L2,3-edges. Weak ferrimagnetism and multiple magnetization reversal phenomena seen in this compound could be ascribed to incomplete cancellation and distortion of partial spontaneous magnetization functions of Cr2+ in its six crystallographically inequivalent positions.

cond-mat.mtrl-sci