arXiv subjects

M. Mostovoy

Publications and source records attributed to M. Mostovoy.

At least 19 recordsLinked to original sources

arXiv2026

Highly controllable switching pathways in multiferroic GdMn$_2$O$_5$

Controlling magnetic moments using electric fields remains a central challenge in spintronics. Multiferroics, where magnetic and electric orders coexist, may be a natural platform for such control, but progress has been limited because interactions between these orders are typically too weak to overcome the energy barriers between magnetic states. A recently demonstrated topologically protected switching circumvents this limitation by exploiting reduced barriers at a phase transition. Nevertheless, the conditions enabling this phenomenon remain elusive and electric field control is poorly understood. Here, we experimentally map the energy landscape by tracking transitions in GdMn$_2$O$_5$ under combined electric and magnetic fields. The experiments reveal that the switching pathways can be controlled by the electric field. A minimal theoretical model captures the observed behavior, identifies the parameter space where switching paths are sensitive to small perturbations and reveals design principles for implementing topological switching in other materials.

cond-mat.mtrl-sci↗

arXiv2025

Competition Between Multiferroic and Magnetic Soliton Lattice States in DyFeO$_3$

Simultaneous breaking of time reversal and inversion symmetries in multiferroics couples ferroelectricity to magnetism and is a source of unusual physical phenomena that can be used in next-generation electronic devices. A notable example is DyFeO$_3$, which under applied magnetic fields exhibits a giant linear magnetoelectric response and a large spontaneous electric polarization induced by coexisting orders of Fe and Dy spins. Here, we use high-resolution neutron diffraction to show that at zero field DyFeO$_3$ hosts an incommensurate magnetic soliton lattice formed by spatially ordered Dy domain walls with an average domain size of 231(8) \AA. The long-ranged interaction between the domain walls is mediated by magnons propagating through the Fe subsystem and is analogous to the Yukawa force in particle physics. An applied magnetic field destroys the long-ranged incommensurate order, unlocks the linear magnetoelectric response and stabilizes the ferroelectric state. The magnetic domain walls are electrically charged and the soliton array dimerizes when both electric and magnetic fields are applied. Numerical simulations with experimental parameters suggest, that the generic competition between the ferroelectric and incommensurate states can be effectively controlled by an applied electric field.

cond-mat.str-el↗

arXiv2024

Reentrant multiple-$\mathbf{q}$ magnetic order and a "spin-cholesteric" phase in Sr$_3$Fe$_2$O$_7$

Spin-nematic and spin-smectic phases have been reported in magnetic materials, which break rotational symmetry while preserving translational symmetry along certain directions. However, until now the analogy to liquid crystals remained incomplete because no magnetic analog of cholesteric order was known. Here we show that the bilayer perovskite Sr$_3$Fe$_2$O$_7$, previously believed to adopt a simple single-$\mathbf{q}$ spin-helical order, hosts two distinct types of multi-$\mathbf{q}$ spin textures and the first "spin-cholesteric". Its ground state represents a novel multi-$\mathbf{q}$ spin texture with unequally intense spin modulations at the two ordering vectors. This is followed in temperature by the new "spin-cholesteric" phase with spontaneously broken chiral symmetry, in which the translational symmetry is broken only along one of the crystal directions while the weaker orthogonal modulation melts, giving rise to intense short-range dynamical fluctuations. Shortly before the transition to the paramagnetic state, vortex-crystal order spanned by two equivalent $\mathbf{q}$ vectors emerges. The "spin-cholesteric" phase completes the spin analogy with liquid crystals and renders Sr$_3$Fe$_2$O$_7$ a touchstone for studying transitions among multiple-$\mathbf{q}$ spin textures in a centrosymmetric host.

cond-mat.str-el↗

arXiv2020

All-electrical detection of skyrmion lattice state and chiral surface twists

We study the high-temperature phase diagram of the chiral magnetic insulator Cu$_2$OSeO$_3$ by measuring the spin-Hall magnetoresistance (SMR) in a thin Pt electrode. We find distinct changes in the phase and amplitude of the SMR signal at critical lines separating different magnetic phases of bulk Cu$_2$OSeO$_3$. The skyrmion lattice state appears as a strong dip in the SMR phase. A strong enhancement of the SMR amplitude is observed in the conical spiral state, which we explain by an additional symmetry-allowed contribution to the SMR present in non-collinear magnets. We demonstrate that the SMR can be used as an all-electrical probe of chiral surface twists and skyrmions in magnetic insulators.

cond-mat.mes-hall↗

arXiv2020

Unusual magnetoelectric effect in paramagnetic rare-earth langasite

Violation of time reversal and spatial inversion symmetries has profound consequences for elementary particles and cosmology. Spontaneous breaking of these symmetries at phase transitions gives rise to unconventional physical phenomena in condensed matter systems, such as ferroelectricity induced by magnetic spirals, electromagnons, non-reciprocal propagation of light and spin waves, and the linear magnetoelectric (ME) effect - the electric polarization proportional to the applied magnetic field and the magnetization induced by the electric field. Here, we report the experimental study of the holmium-doped langasite, Ho$_{x}$La$_{3-x}$Ga$_5$SiO$_{14}$, showing a puzzling combination of linear and highly non-linear ME responses in the disordered paramagnetic state: its electric polarization grows linearly with the magnetic field but oscillates many times upon rotation of the magnetic field vector. We propose a simple phenomenological Hamiltonian describing this unusual behavior and derive it microscopically using the coupling of magnetic multipoles of the rare-earth ions to the electric field.

cond-mat.mtrl-sci↗

arXiv2020

The 2020 Skyrmionics Roadmap

The notion of non-trivial topological winding in condensed matter systems represents a major area of present-day theoretical and experimental research. Magnetic materials offer a versatile platform that is particularly amenable for the exploration of topological spin solitons in real space such as skyrmions. First identified in non-centrosymmetric bulk materials, the rapidly growing zoology of materials systems hosting skyrmions and related topological spin solitons includes bulk compounds, surfaces, thin films, heterostructures, nano-wires and nano-dots. This underscores an exceptional potential for major breakthroughs ranging from fundamental questions to applications as driven by an interdisciplinary exchange of ideas between areas in magnetism which traditionally have been pursued rather independently. The skyrmionics roadmap provides a review of the present state of the art and the wide range of research directions and strategies currently under way. These are, for instance, motivated by the identification of the fundamental structural properties of skyrmions and related textures, processes of nucleation and annihilation in the presence of non-trivial topological winding, an exceptionally efficient coupling to spin currents generating spin transfer torques at tiny current densities, as well as the capability to purpose-design broad-band spin dynamic and logic devices.

cond-mat.str-el↗

arXiv2020

Robust skyrmion-bubble textures in SrRuO$_3$ thin films stabilized by magnetic anisotropy

Topological spin textures in an itinerant ferromagnet, SrRuO$_3$ is studied combining Hall transport measurements and numerical simulations. We observe characteristic signatures of the Topological Hall Effect associated with skyrmions. A relatively large thickness of our films and absence of heavy metal layers make the interfacial Dzyaloshinskii-Moriya interaction an unlikely source of these topological spin textures. Additionally, the transport anomalies exhibit an unprecedented robustness to magnetic field tilting and temperature. Our numerical simulations suggest that this unconventional behavior results from magnetic bubbles with skyrmion topology stabilized by magnetodipolar interactions in an unexpected region of parameter space.

cond-mat.str-el↗

arXiv2018

Field-induced double spin spiral in a frustrated chiral magnet

We report the direct observation of a magnetic-feld induced long-wavelength spin spiral modulation in the chiral compound Ba3TaFe3Si2O14. This new spin texture emerges out of a chiral helical ground state, and is hallmarked by the onset of a unique contribution to the bulk electric polarization, the sign of which depends on the crystal chirality. The periodicity of the feld induced modulation, several hundreds of nm depending on the field value, is comparable to the length scales of mesoscopic topological defects such as skyrmions, merons and solitons. The phase transition and observed threshold behavior are consistent with a phenomenology based on the allowed Lifshitz invariants for the chiral symmetry of langasite, which intriguingly contain all the ingredients for the possible realization of topologically stable antiferromagnetic skyrmions.

cond-mat.str-el↗

arXiv2018

New magnetic phase of the chiral skyrmion material Cu2OSeO3

The lack of inversion symmetry in the crystal lattice of magnetic materials gives rise to complex non-collinear spin orders through interactions of relativistic nature, resulting in interesting physical phenomena, such as emergent electromagnetism. Studies of cubic chiral magnets revealed a universal magnetic phase diagram, composed of helical spiral, conical spiral and skyrmion crystal phases. Here, we report a remarkable deviation from this universal behavior. By combining neutron diffraction with magnetization measurements we observe a new multi-domain state in Cu2OSeO3. Just below the upper critical field at which the conical spiral state disappears, the spiral wave vector rotates away from the magnetic field direction. This transition gives rise to large magnetic fluctuations. We clarify physical origin of the new state and discuss its multiferroic properties.

cond-mat.mtrl-sci↗

arXiv2017

Bound states of skyrmions and merons near the Lifshitz point

We study topological defects in anisotropic ferromagnets with competing interactions near the Lifshitz point. We show that skyrmions and bi-merons are stable in a large part of the phase diagram. We calculate skyrmion-skyrmion and meron-meron interactions and show that skyrmions attract each other and form ring-shaped bound states in a zero magnetic field. At the Lifshitz point merons carrying a fractional topological charge become deconfined. These results imply that unusual topological excitations may exist in weakly frustrated magnets with conventional crystal lattices.

cond-mat.str-el↗

arXiv2017

Magnetically induced Ferroelectricity in Bi$_2$CuO$_4$

The tetragonal copper oxide Bi$_2$CuO$_4$ has an unusual crystal structure with a three-dimensional network of well separated CuO$_4$ plaquettes. This material was recently predicted to host electronic excitations with an unconventional spectrum and the spin structure of its magnetically ordered state appearing at T$_N$ $\sim$43 K remains controversial. Here we present the results of detailed studies of specific heat, magnetic and dielectric properties of Bi$_2$CuO$_4$ single crystals grown by the floating zone technique, combined with the polarized neutron scattering and high-resolution X-ray measurements. Our polarized neutron scattering data show Cu spins are parallel to the $ab$ plane. Below the onset of the long range antiferromagnetic ordering we observe an electric polarization induced by an applied magnetic field, which indicates inversion symmetry breaking by the ordered state of Cu spins. For the magnetic field applied perpendicular to the tetragonal axis, the spin-induced ferroelectricity is explained in terms of the linear magnetoelectric effect that occurs in a metastable magnetic state. A relatively small electric polarization induced by the field parallel to the tetragonal axis may indicate a more complex magnetic ordering in Bi$_2$CuO$_4$.

cond-mat.str-el↗

arXiv2016

Electrical detection of spiral spin structures in Pt|Cu_2OSeO_3 heterostructures

The interaction between the itinerant spins in metals and localized spins in magnetic insulators thus far has only been explored in collinear spin systems, such as garnets. Here, we report the spin-Hall magnetoresistance (SMR) sensitive to the surface magnetization of the spin-spiral material, Cu_2OSeO_3. We experimentally demonstrate that the angular dependence of the SMR changes drastically at the transition between the helical spiral and the conical spiral phases. Furthermore, the sign and magnitude of the SMR in the conical spiral state are controlled by the cone angle. We show that this complex behaviour can be qualitatively explained within the SMR theory initially developed for collinear magnets. In addition, we studied the spin Seebeck effect (SSE), which is sensitive to the bulk magnetization. It originates from the conversion of thermally excited low-energy spin waves in the magnet, known as magnons, into the spin current in the adjacent metal contact (Pt). The SSE displays unconventional behavior where not only the magnitude but also the phase of the SSE vary with the applied magnetic field.

cond-mat.mtrl-sci↗

arXiv2016

Edge states and skyrmion dynamics in nanostripes of frustrated magnets

Magnetic skyrmions are particle-like topological excitations recently discovered in chiral magnets. Their small size, topological protection and the ease with which they can be manipulated by electric currents generated much interest in using skyrmions for information storage and processing. Recently, it was suggested that skyrmions with additional degrees of freedom can exist in magnetically frustrated materials. Here, we show that dynamics of skyrmions and antiskyrmions in nanostripes of frustrated magnets is strongly affected by complex spin states formed at the stripe edges. These states create multiple edge channels which guide the skyrmion motion. Non-trivial topology of edge states gives rise to complex current-induced dynamics, such as emission of skyrmion-antiskyrmion pairs. The edge state topology can be controlled with an electric current through the exchange of skyrmions and antiskyrmions between the edges of a magnetic nanostructure. These results can lead to conceptually new electronic devices.

cond-mat.mes-hall↗

arXiv2015

Thermally Driven Ratchet Motion of Skyrmion Microcrystal and Topological Magnon Hall Effect

Spontaneously emergent chirality is an issue of fundamental importance across the natural sciences. It has been argued that a unidirectional (chiral) rotation of a mechanical ratchet is forbidden in thermal equilibrium, but becomes possible in systems out of equilibrium. Here we report our finding that a topologically nontrivial spin texture known as a skyrmion - a particle-like object in which spins point in all directions to wrap a sphere - constitutes such a ratchet. By means of Lorentz transmission electron microscopy we show that micron-sized crystals of skyrmions in thin films of Cu2OSeO3 and MnSi display a unidirectional rotation motion. Our numerical simulations based on a stochastic Landau-Lifshitz-Gilbert equation suggest that this rotation is driven solely by thermal fluctuations in the presence of a temperature gradient, whereas in thermal equilibrium it is forbidden by the Bohr-van Leeuwen theorem. We show that the rotational flow of magnons driven by the effective magnetic field of skyrmions gives rise to the skyrmion rotation, therefore suggesting that magnons can be used to control the motion of these spin textures.

cond-mat.str-el↗

arXiv2015

Multiply periodic states and isolated skyrmions in an anisotropic frustrated magnet

Multiply periodic states appear in a wide variety of physical contexts, such as the Rayleigh-Benard convection, Faraday waves, liquid crystals, domain patterns in ferromagnetic films and skyrmion crystals recently observed in chiral magnets. Here we study a simple model of an anisotropic frustrated magnet and show that its zero-temperature phase diagram contains numerous multi-q states including the skyrmion crystal. We clarify the mechanism for stabilization of these states, discuss their multiferroic properties and formulate rules for finding new skyrmion materials. In addition to skyrmion crystal, we find stable isolated skyrmions with topological charge 1 and 2. Physics of isolated skyrmions in frustrated magnets is very rich. Their statical and dynamical properties are strongly affected by the new zero mode - skyrmion helicity.

cond-mat.mes-hall↗

arXiv2013

Target-skyrmions and skyrmion clusters in nanowires of chiral magnets

In bulk non-centrosymmetric magnets the chiral Dzyaloshinskii-Moriya exchange stabilizes tubular skyrmions with a reversed magnetization in their centers. While the double-twist is favorable in the center of a skyrmion, it gives rise to an excess of the energy density at the outskirt. Therefore, magnetic anisotropies are required to make skyrmions more favorable than the conical spiral state in bulk materials. Using Monte Carlo simulations, we show that in magnetic nanowires unusual skyrmions with a doubly twisted core and a number of concentric helicoidal undulations (target-skyrmions) are thermodynamically stable even in absence of single-ion anisotropies. Such skyrmions are free of magnetic charges and, since the angle describing the direction of magnetization at the surface depends on the radius of the nanowire and an applied magnetic field, they carry a non-integer skyrmion charge s > 1. This state competes with clusters of spatially separated s=1 skyrmions. For very small radii, the target-skyrmion transforms into a skyrmion with s < 1, that resembles the vortex-like state stabilized by surface-induced anisotropies.

cond-mat.mes-hall↗

arXiv2013

Negative magnetostrictive magnetoelectric coupling of BiFeO3

How the magnetoelectric coupling actually occurs on a microscopic level in multiferroic BiFeO3 is not well known. By using the high-resolution single crystal neutron diffraction techniques, we have determined the electric polarization of each individual elements of BiFeO3, and concluded that the magnetostrictive coupling suppresses the electric polarization at the Fe site below TN. This negative magnetoelectric coupling appears to outweigh the spin current contributions arising from the cycloid spin structure, which should produce a positive magnetoelectric coupling.

cond-mat.str-el↗

arXiv2011

Magnetic excitations in the low-temperature ferroelectric phase of multiferroic YMn2O5 using inelastic neutron scattering

We studied magnetic excitations in a low-temperature ferroelectric phase of the multiferroic YMn2O5 using inelastic neutron scattering (INS). We identify low-energy magnon modes and establish a correspondence between the magnon peaks observed by INS and electromagnon peaks observed in optical absorption [1]. Furthermore, we explain the microscopic mechanism, which results in the lowest-energy electromagnon peak, by comparing the inelastic neutron spectral weight with the polarization in the commensurate ferroelectric phase.

cond-mat.str-el↗