arXiv subjects

M. Motokawa

Publications and source records attributed to M. Motokawa.

14 recordsLinked to original sources

arXiv2004

The Competition between Staggered Field and Antiferromagnetic Interactions in Cugeo3:Fe

The EPR spectra along different crystallographic axes for single crystals of CuGeO3 containing 1% of Fe impurity have been studied in the frequency range 60-360 GHz at temperatures 0.5-30 K. The analysis based on the Oshikawa-Affleck (OA) theory suggests that the temperature dependences of the line width and g-factor are formed as a result of the competition between interchain antiferromagnetic interactions and staggered Zeeman energy. It is found that staggered magnetic moments in CuGeO3:Fe are located predominantly along b axis.

cond-mat.str-el↗

arXiv2004

Quantum Critiality and Collective Effects in Low Dimensional Magnet CuGeO3 Probed by High Frequency EPR

For the CuGeO3 single crystals doped with 1% of Fe the quantum critical behavior in a wide temperature range 1-40 K is reported. The critical exponents for susceptibility along different crystallographic axes are determined: a=0.34 (B //a and B //c) and a=0.31 (B //b). The description of the temperature dependences of the line width and g-factor could be obtained in the OA theory assuming that staggered component of the magnetic moment is located predominantly along b axis. Possible arguments favoring the competition between effects of the staggered field and antiferromagnetic ordering are provided.

cond-mat.str-el↗

arXiv2004

Disorder driven quantum critical behavior in CuGeO3 doped with magnetic impurity

For the CuGeO3 doped with 1% of Fe the quantum critical behavior in a wide temperature range 1-40 K is reported. The critical exponents for susceptibility along different crystallographic axes are determined: a=0.34 (B//a and B//c) and a=0.31 (B//b). New effect of the frequency dependence of the critical exponent is discussed.

cond-mat.str-el↗

arXiv2003

ESR study on the excited state energy spectrum of SrCu$_2$(BO$_3$)$_2$ -a central role of multiple-triplet bound states

The excited state energy spectrum of a two-dimensional dimer system SrCu$_2$(BO$_3$)$_2$ has been investigated by high field ESR. Various types of multiple-triplet bound states-excited singlet, triplet and quintet states are identified, besides two non-degenerated one-triplet excitations. Extremely strong intensity is found for these higher order bound states, which is an important consequence of the strong suppression of the one-triplet process due to the orthogonality of dimers. A new bound singlet state is found slightly below the energy gap of the one-triplet state, indicating the proximity to a quantum critical point. A band of two-triplet bound state splits into at least eight sharp and discrete levels, which indicates the contribution of distant neighbor interactions. A bound quintet state is observed, which is the direct evidence of two-triplet object made up of four $S=1/2$ spins. The energy of the lowest quintet becomes lower than that of the one-triplet excitation before the closing of the lowest spin gap. It indicates that the two-triplet bound state touches to the ground singlet state before the one-triplet state does. The present investigation exhibits an essential role of various multiple-triplet bound states in the magnetic excitation spectrum of SrCu$_2$(BO$_3$)$_2$.

cond-mat.str-el↗

arXiv2002

Fermi Surface Study of Quasi-Two-Dimensional Organic Conductors by Magnetooptical Measurements

Magnetooptical measurements of several quasi-two-dimensional (q2D) organic conductors, which have simple Fermi surface structure, have been performed by using a cavity perturbation technique. Despite of the simple Fermi surface structure, magnetooptical resonance results show a dramatic difference for each sample. Cyclotron resonances (CR) were observed for q-(BEDT-TTF)2I3 and (BEDT-TTF)3Br(pBIB), while periodic orbit resonances (POR) were observed for (BEDT-TTF)2Br(DIA) and (BEDT-TTF)3Cl(DFBIB). The selection of the resonance seems to correspond with the skin depth for each sample. The effective mass of POR seems to have a mass enhancement due to the many-body effect, while effective mass of CR is independent of the strength of the electron-electron interaction. The scattering time deduced from each resonance's linewidth will be also presented.

cond-mat.str-el↗

arXiv2002

Observation of High-Order Harmonic Resonances in Magnetooptical Measurements of (BEDT-TTF)2Br(DIA)

Magnetooptical measurements of a quasi-two-dimensional (q2D) organic conductor (BEDT-TTF)2Br(DIA) (DIA=diiodoacetylene) were performed using a cavity perturbation technique with a millimeter vector network analyzer (MVNA). Harmonic resonances were observed periodically as a function of the inverse field up to the 7th order. This is the first observation of higher-order harmonics up to the 7th order in an organic conductor. The observed resonance is assigned as a periodic orbit resonance (POR) which arises from a q2D elliptic Fermi surface (FS). The obtained effective mass (4.7me) is consistent with Shubnikov-de Haas measurements. Temperature dependence of the spectra observed in two different sample configurations will be presented.

cond-mat.str-el↗

arXiv2001

Susceptibility, Magnetization Process and ESR Studies on the Helical Spin System RbCuCl$_{3}$

The static and dynamic magnetic properties of an $S=1/2$ stacked triangular antiferromagnet RbCuCl$_{3}$ with a helical spin structure due to lattice distortion were investigated by susceptibility, high-field magnetization process and ESR measurements. The susceptibilities were analyzed by high-temperature expansion approximation in terms of ferromagnetic intrachain coupling and the antiferromagnetic interchain coupling. The magnetization saturates at $H_{\rm s}\approx 66.8$ T at 1.5 K, the value of which is twice that of CsCuCl$_3$. A small magnetization jump indicative of a phase transition was observed at $H_{\rm c}=21.2$ T $\approx (1/3)H_{\rm s}$ for $H{\perp}c$. ESR modes observed for $H\parallel c$ are well described by the calculation based on the helical spin structure. From the present measurements, the ferromagnetic intrachain and two kinds of antiferromagnetic interchain exchange interactions, and the planar anisotropy energy were determined as $J_0/k_{\rm B}=25.7$ K, $J_1/k_{\rm B}=-10.6$ K, $J_1'/k_{\rm B}=-17.4$ K, and $ΔJ_0/k_{\rm B}=-0.45$ K, respectively.

cond-mat.str-el↗

arXiv2000

High frequency ESR investigation on dynamical charge disproportionation and spin gap excitation in NaV_2O_5

A significant frequency dependence of the ESR line width is found in NaV_2O_5 between 34-100 K and the line width increases as the resonance frequency is increased from 95 GHz to 760 GHz. The observed frequency dependence is qualitatively explained in terms of the dynamical charge disproportionation. The present results show the essential role of the internal charge degree of freedom in a V-O-V bond. We have also proposed the existence of the Dzyaloshinsky-Moriya interaction in the low temperature charge ordered phase considering the breaking of the selection rule of ESR realized as the direct observation of the spin gap excitation.

cond-mat.str-el↗

arXiv1999

ESR investigation on the Breather mode and the Spinon-Breather dynamical crossover in Cu Benzoate

A new elementary-excitation, the so called "breather excitation", is observed directly by millimeter-submillimeter wave electron spin resonance (ESR) in the Heisenberg quantum spin-chain Cu benzoate, in which a field-induced gap is found recently by specific heat and neutron scattering measurements. Distinct anomalies were found in line width and in resonance field around the "dynamical crossover" regime between the gap-less spinon-regime and the gapped breather-regime. When the temperature becomes sufficiently lower than the energy gap, a new ESR-line with very narrow line-width is found, which is the manifestation of the breather excitation. The non-linear field dependence of the resonance field agrees well with the theoretical formula of the first breather-excitation proposed by Oshikawa and Affleck. The present work establishes experimentally for the first time that a sine-Gordon model is applicable to explain spin dynamics in a S=1/2 Heisenberg spin chain subjected to staggered field even in high fields.

cond-mat.str-el↗

arXiv1999

Magnetotransport properties of (Ga,Mn)As investigated at low temperature and high magnetic field

Magnetotransport properties of ferromagnetic semiconductor (Ga,Mn)As have been investigated. Measurements at low temperature (50 mK) and high magnetic field (<= 27 T) have been employed in order to determine the hole concentration p = 3.5x10^20 cm ^-3 of a metallic (Ga0.947Mn0.053)As layer. The analysis of the temperature and magnetic field dependencies of the resistivity in the paramagnetic region was performed with the use of the above value of p, which gave the magnitude of p-d exchange energy |N0beta | ~ 1.5 eV.

cond-mat.mtrl-sci↗

arXiv1999

Two ferromagnetic phases in La1-xSrxMnO3(x ~1/8)

It was discovered in La1-xSrxMnO3(x~1/8) that a field induced phase transition occurs from a ferromagnetic metal(FM) phase to a ferromagnetic insulator (FI) phase. The magnetization shows a sharp jump at the transition field accompanying with a remarkable increase of magnetoresistance. Striction measurements clarified that this transition is associated with the structural change from a Jahn-Teller(JT) distorted orthorhombic phase to a pseudo cubic phase. These results evidently show that the FI phase with a pseudo cubic symmetry is more stable in high fields than the FM phase due to the double exchange interaction. The driving force of this transition is explained by the enhancement of the ferromagnetic superexchange interaction induced by an antiferromagnetic type orbital ordering in the pseudo cubic phase, which was recently found in the anomalous X-ray scattering experiments.

cond-mat.str-el↗

arXiv1999

Direct observation of the multiple spin gap excitations in two-dimensional dimer system SrCu2(BO3)2

Various spin gap excitations have been observed in the two-dimensional dimer system SrCu_2(BO_3)_2 by means of submillimeter wave ESR. The zero-field energy gap of the lowest spin gap excitation shows a splitting into two triplet modes and the energy splitting clearly depends on the magnetic field orientation when a field is rotated in the {\mib {ac}}-plane. A zero-field splitting is also found between the S(_z)=+1 and S(_z)=-1 branches of each triplet. These behaviors are qualitatively explained by considering the anisotropic exchange coupling of inter-dimer and intra-dimer, respectively. The averaged value of the lowest spin gap energy is determined to be 722 \pm 2 GHz(34.7 K). We have also found the second spin gap excitation at 1140 GHz(54.7 K), which indicates that the inter-dimer coupling is significantly strong. Besides these modes, a number of gapped ESR absorption are found and we propose that these multiple magnetic excitations are caused by the localized nature of the excited state in the present system.

cond-mat.str-el↗

arXiv1999

Submillimeter Wave ESR Study of Spin Gap Excitations in CuGeO3

Transitions between the ground singlet state to the excited triplet state has been observed in CuGeO3 by means of submillimeter wave electron spin resonance. The strong absorption intensity shows the break down of the selection rule. The energy gap at zero field is evaluated to be 570 GHz(2.36 meV) and this value is nearly identical to the gap at the zone center observed by inelastic neutron scattering. The absorption intensity shows strong field orientation dependence but shows no significant dependence on magnetic field intensity. These features have been explained by considering the existence of Dzyaloshinsky-Moriya (DM) antisymmetric exchange interaction. The doping effect on this singlet-triplet excitation has been also studied. A drastic broadening of the absorption line is observed by the doping of only 0.5 % of Si.

cond-mat.str-el↗

arXiv1998

Field Induced Transition from Metal to Insulator in the CMR Manganites

The gigantic reduction of the electric resistivity under the applied magnetic field, CMR effect, is now widely accepted to appear in the vicinity of the insulator to metal transition of the perovskite manganites. Recently, we have discovered the first order transition from ferromagnetic metal to insulator in $\rm La_{0.88}Sr_{0.12}MnO_3$ of the CMR manganite. This phase transition induces the tremendous increase of the resistivity under the external magnetic field just near above the phase transition temperature. We report here fairly detailed results from the systematic experiments including neutron and synchrotron X-ray scattering studies.

cond-mat.str-el↗