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M. Moukaddam

Publications and source records attributed to M. Moukaddam.

At least 19 recordsLinked to original sources

Refining the deep sub-barrier 12C+12C excitation function with STELLA

Purpose: We have investigated the cross section around the lowest direct coincident gamma-particle measurements, where previously only limits could be established with the aim of obtaining a detailed description of the excitation function. We have furthermore analysed the ratio of extreme decay branching into the first excited state of daughter nuclei with alpha or proton emission at relative kinetic energies where previous measurements are in disagreement with each other. Conclusions: Our findings in the astrophysics RoI support reaction-rate models with a lower average S-factor trend, that deviates significantly from standard extrapolations between 2.2 MeV and 2.6 MeV, for stellar carbon burning simulations of up to 25 Msol stars. Based on our data, an overall increase of the S-factor at deep subbarrier energy cannot be confirmed. The extremely low ratio of the branching into the first excited state with proton over alpha emission of ~ 2% at 3.23 MeV might indicate the presence of alpha cluster compound states in 24Mg. This highly favours {\alpha} emission with fundamental consequences in possible stellar carbon burning sites.

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First application of Markov Chain Monte Carlo-based Bayesian data analysis to the Doppler-Shift Attenuation Method

Motivated primarily by the large uncertainties in the thermonuclear rate of the $^{30}$P$(p,γ)^{31}$S reaction that limit our understanding of classical novae, we carried out lifetime measurements of $^{31}$S excited states using the Doppler Shift Lifetimes (DSL) facility at the TRIUMF Isotope Separator and Accelerator (ISAC-II) facility. The $^{31}$S excited states were populated by the $^{3}$He$(^{32}$S$,α)^{31}$S reaction. The deexcitation $γ$ rays were detected by a clover-type high-purity germanium detector in coincidence with the $α$ particles detected by a silicon detector telescope. We have applied modern Markov chain Monte Carlo-based Bayesian methods to perform lineshape analyses of Doppler-shift attenuation method $γ$-ray data for the first time. We have determined the lifetimes of the two lowest-lying $^{31}$S excited states. First experimental upper limits on the lifetimes of four higher-lying states have been obtained. The experimental results were compared to shell-model calculations using five universal $sd$-shell Hamiltonians. Evidence for $γ$ rays originating from the astrophysically important $J^π=3/2^+$, 260-keV $^{30}$P$(p,γ)^{31}$S resonance has also been observed, although strong constraints on the lifetime will require better statistics.

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Single neutron transfer on 23Ne and its relevance forthepathway ofnucleosynthesis in astrophysical X-ray bursts

We present new experimental measurements of resonance strengths in the astrophysical 23Al(p, γ)24Si reaction, constraining the pathway of nucleosynthesis beyond 22Mg in X-ray burster scenarios. Specifically, we have performed the first measurement of the (d, p) reaction using a radioactive beam of 23Ne to explore levels in 24Ne, the mirror analog of 24Si. Four strong single-particle states were observed and corresponding neutron spectroscopic factors were extracted with a precision of {\sim}20{\%}. Using these spectroscopic factors, together with mirror state identifications, we have reduced uncertainties in the strength of the key {\ell} = 0 resonance at Er= 157 keV, in the astrophysical 23Al(p, γ) reaction, by a factor of 4. Our results show that the 22Mg(p, γ)23Al(p, γ) pathway dominates over the competing 22Mg(α, p) reaction in all but the most energetic X-ray burster events (T>0.85GK), significantly affecting energy production and the preservation of hydrogen fuel.

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Improved measurement of the $0_2^+\rightarrow0_1^+$ E0 transition strength for $^{72}$Se using the SPICE spectrometer

The selenium isotopes lie at the heart of a tumultuous region of the nuclear chart where shape coexistence effects grapple with neutron-proton pairing correlations, triaxiality, and the impending proton dripline. In this work a study of $^{72}$Se by internal conversion electron and $γ$-ray spectroscopy was undertaken with the SPICE and TIGRESS arrays. New measurements of the branching ratio and lifetime of the $0_2^+$ state were performed yielding a determination of $ρ^2(E0;0_2^+{\rightarrow}0_1^+)=29(3)$ milliunits. two state mixing calculations were performed that highlighted the importance of interpretation of such $E0$ strength values in the context of shape-coexistence.

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A new $^{12}$C + $^{12}$C nuclear reaction rate: impact on stellar evolution

This work presents new $^{12}$C + $^{12}$C reaction rates in the form of numerical tables with associated uncertainty estimation, as well as analytical formulae that can be directly implemented into stellar evolution codes. This article further describes the impact of these new rates on C-burning in stars. We determine reaction rates for two cross-section extrapolation models: one based on the fusion-hindrance phenomenon, and the other on fusion-hindrance plus a resonance, and compare our results to previous data. Using the GENEC stellar evolution code, we study how these new rates impact the C-burning phases in two sets of stellar models for stars with 12 M$_{\odot}$ and 25 M$_{\odot}$ initial masses chosen to be highly representative of the diversity of massive stars. The effective temperatures of C-burning in both sets of stellar models are entirely covered by the sensitivity of the present experimental data, and no extrapolation of the rates is required. Although, the rates may differ by more than an order of magnitude for temperatures typical of C-burning, the impacts on the stellar structures during that phase remain modest. This is a consequence of the readjustment of the stellar structure to a change of nuclear reaction rate for reactions important for energy production. For the hindrance case, the C-burning phase is found to occur at central temperatures 10\% higher than with the hindrance plus resonance rate. Its C-burning lifetime is reduced by a factor of two. This model, nevertheless, loses more entropy than the other one thus enters earlier into the degeneracy regime which will impact the last stages of the evolution at the pre-core collapse time. The hindrance model produces up to 60% more neon. The impact of the different rates on the s-process occurring during the C-burning phase is modest, changing final abundances of s-processed elements by at most 20% (cobalt).

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High-Precision Branching Ratio Measurement and Spin Assignment Implications for $^{62}$Ga Superallowed $β$ Decay

A high-precision branching ratio measurement for the superallowed Fermi $β^{+}$ emitter $^{62}$Ga was performed with the Gamma-Ray Infrastructure for Fundamental Investigations of Nuclei (GRIFFIN) spectrometer at the Isotope Separator and Accelerator (ISAC) radioactive ion beam facility at TRIUMF. The high efficiency of the GRIFFIN spectrometer allowed 63 $γ$-ray transitions, with intensities down to $\approx$1 part per million (ppm) per $^{62}$Ga $β^{+}$ decay, to be placed in the level scheme of the daughter nucleus $^{62}$Zn, establishing the superallowed $β$ branching ratio for $^{62}$Ga decay to be 99.8577$^{+0.0023}_{-0.0029}\%$, a factor of 4 more precise than the previous world average. For several cascades, $γ-γ$ angular correlation measurements were performed to assign spins and/or determine the mixing ratios of transitions. In particular, the spin of the 2.342 MeV excited state in the daughter nucleus $^{62}$Zn was definitively assigned as $J = 0$. This assignment resolves a discrepancy between previous measurements and has important implications for the isospin symmetry breaking correction, $δ_{C1}$, in $^{62}$Ga superallowed Fermi $β$ decay.

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Spectroscopic study of $^{47}$Ca from the $β^-$ decay of $^{47}$K

The $β^-$ decay of $^{47}$K to $^{47}$Ca is an appropriate mechanism for benchmarking interactions spanning the $sd$ and $pf$ shells, but current knowledge of the $β^-$-decay scheme is limited. We have performed a high-resolution, high-efficiency study of the $β^-$-decay of $^{47}$K with the GRIFFIN spectrometer at TRIUMF-ISAC. The study revealed 48 new transitions, a more precise value for the $^{47}$K half-life (17.38(3)~s), and new spin and parity assignments for eight excited states. Levels placed for the first time here raise the highest state observed in $β^-$ decay to within 568(3) keV of the $Q$-value and confirm the previously measured large $β^-$-decay branching ratios to the low-lying states. Previously unobserved $β^-$-feeding to 3/2$^+$ states between 4.5 and 6.1~MeV excitation energy was identified with a total $β^-$-feeding intensity of 1.29(2)\%. The sum of the $B(GT)$ values for these states indicates that the $1s_{1/2}$ proton hole strength near this excitation energy is comparable to the previously known $1s_{1/2}$ proton and neutron hole strengths near 2.6 MeV.

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Single-particle structure in neutron-rich Sr isotopes approaching the N = 60 shape transition

Background: Neutron-rich nuclei around neutron number N = 60 show a dramatic shape transition from spherical ground states to prolate deformation in 98Sr and heavier nuclei. Purpose: The purpose of this study is to investigate the single-particle structure approaching the shape transitional region. Method: The level structures of neutron-rich 93,94,95Sr were studied via the d(94,95,96Sr,t) one-neutron stripping reactions at TRIUMF using a beam energy of 5.5 AMeV. γ-rays emitted from excited states and recoiling charged particles were detected by using the TIGRESS and SHARC arrays, respectively. States were identified by gating on the excitation energy and, if possible, the coincident γ radiation. Results: Triton angular distributions for the reactions populating states in ejectile nuclei 93,94,95Sr were compared with distorted wave Born approximation calculations to assign and revise spin and parity quantum numbers and extract spectroscopic factors. The results were compared with shell model calculations and the reverse (d,p) reactions and good agreement was obtained. Conclusions: The results for the d(94Sr,t)93Sr and d(95Sr,t)94Sr reactions are in good agreement with shell model calculations. A two level mixing analysis for the 0+ states in 94Sr suggest strong mixing of two shapes. For the d(96Sr,t)95Sr reaction the agreement with the shell model is less good. The configuration of the ground state of 96Sr is already more complex than predicted, and therefore indications for the shape transition can already be observed before N = 60.

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Decay Spectroscopy of $^{129}$Cd

Excited states of $^{129}$In populated following the $β$-decay of $^{129}$Cd were experimentally studied with the GRIFFIN spectrometer at the ISAC facility of TRIUMF, Canada. A 480-MeV proton beam was impinged on a uranium carbide target and $^{129}$Cd was extracted using the Ion Guide Laser Ion Source (IG-LIS). $β$- and $γ$-rays following the decay of $^{129}$Cd were detected with the GRIFFIN spectrometer comprising the plastic scintillator SCEPTAR and 16 high-purity germanium (HPGe) clover-type detectors. %, along with the $β$-particles were detected with SCEPTAR. From the $β$-$γ$-$γ$ coincidence analysis, 32 new transitions and 7 new excited states were established, expanding the previously known level scheme of $^{129}$In. The $\log ft$ values deduced from the $β$-feeding intensities suggest that some of the high-lying states were populated by the $ν0 g_{7/2} \rightarrow π0 g_{9/2}$ allowed Gamow-Teller (GT) transition, which indicates that the allowed GT transition is more dominant in the $^{129}$Cd decay than previously reported. Observation of fragmented Gamow-Teller strengths is consistent with theoretical calculations.

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Decay properties of $^{22}\mathrm{Ne} + α$ resonances and their impact on $s$-process nucleosynthesis

The astrophysical $s$-process is one of the two main processes forming elements heavier than iron. A key outstanding uncertainty surrounding $s$-process nucleosynthesis is the neutron flux generated by the ${}^{22}\mathrm{Ne}(α, n){}^{25}\mathrm{Mg}$ reaction during the He-core and C-shell burning phases of massive stars. This reaction, as well as the competing ${}^{22}\mathrm{Ne}(α, γ){}^{26}\mathrm{Mg}$ reaction, is not well constrained in the important temperature regime from ${\sim} 0.2$--$0.4$~GK, owing to uncertainties in the nuclear properties of resonances lying within the Gamow window. To address these uncertainties, we have performed a new measurement of the ${}^{22}\mathrm{Ne}({}^{6}\mathrm{Li}, d){}^{26}\mathrm{Mg}$ reaction in inverse kinematics, detecting the outgoing deuterons and ${}^{25,26}\mathrm{Mg}$ recoils in coincidence. We have established a new $n / γ$ decay branching ratio of $1.14(26)$ for the key $E_x = 11.32$ MeV resonance in $^{26}\mathrm{Mg}$, which results in a new $(α, n)$ strength for this resonance of $42(11)~μ$eV when combined with the well-established $(α, γ)$ strength of this resonance. We have also determined new upper limits on the $α$ partial widths of neutron-unbound resonances at $E_x = 11.112,$ $11.163$, $11.169$, and $11.171$ MeV. Monte-Carlo calculations of the stellar ${}^{22}\mathrm{Ne}(α, n){}^{25}\mathrm{Mg}$ and ${}^{22}\mathrm{Ne}(α, γ){}^{26}\mathrm{Mg}$ rates, which incorporate these results, indicate that both rates are substantially lower than previously thought in the temperature range from ${\sim} 0.2$--$0.4$~GK.

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$E0$ transition strength in stable Ni isotopes

Excited states in $^{58,60,62}$Ni were populated via inelastic proton scattering at the Australian National University as well as via inelastic neutron scattering at the University of Kentucky Accelerator Laboratory. The Super-e electron spectrometer and the CAESAR Compton-suppressed HPGe array were used in complementary experiments to measure conversion coefficients and $δ(E2/M1)$ mixing ratios, respectively, for a number of $2^+ \rightarrow 2^+$ transitions. The data obtained were combined with lifetimes and branching ratios to determine $E0$, $M1$, and $E2$ transition strengths between $2^+$ states. The $E0$ transition strengths between $0^+$ states were measured using internal conversion electron spectroscopy and compare well to previous results from internal pair formation spectroscopy. The $E0$ transition strengths between the lowest-lying $2^+$ states were found to be consistently large for the isotopes studied.

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Detailed spectroscopy of $^{46}$Ca: A study of the $β^-$ decay of $^{46}$K

We report on high-statistics data from the $β^-$ decay of the $^{46}$K $J^π$ = 2$^-$ ground state taken with the GRIFFIN spectrometer located at the TRIUMF-ISAC facility. In total, 199 $γ$ rays and 42 excited states were placed in the level scheme, and from the observed $β$ feeding and angular correlations of pairs of cascading $γ$ rays, it was possible to assign spins and parities to excited states and determine mixing ratios for selected $γ$ rays. The level structure of $^{46}$Ca is compared to theoretical predictions from a microscopic valence-space Hamiltonian derived from two- (NN) and three-nucleon (3N) forces. These calculations are in reasonable agreement with the experimental data and indicate that the protons in this region are not as inert as would be expected for semi-magic nuclei.

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Single-Particle Structure of Neutron-Rich Sr Isotopes Via d( 94,95,96 Sr, p) Reactions

The region around neutron number N = 60 in the neutron-rich Sr and Zr nuclei is one of the most dramatic examples of a ground state shape transition from (near) spherical below N = 60 to strongly deformed shapes in the heavier isotopes. The single-particle structure of 95-97Sr approaching the ground state shape transition at 98 Sr has been investigated via single-neutron transfer reactions using the (d, p) reaction in inverse kinematics. These reactions selectively populate states with a large overlap of the projectile ground state coupled to a neutron in a single-particle orbital. Radioactive 94,95,96Sr nuclei with energies of 5.5 AMeV were used to bombard a CD 2 target. Recoiling light charged particles and γ rays were detected using a quasi-4π silicon strip detector array and a 12 element Ge array. The excitation energy of states populated was reconstructed employing the missing mass method combined with γ-ray tagging and differential cross sections for final states were extracted. A reaction model analysis of the angular distributions allowed for firm spin assignments to be made for the low-lying 352, 556 and 681 keV excited states in 95Sr and a constraint has been placed on the spin of the higher-lying 1666 keV state. Angular distributions have been extracted for 10 states populated in the d(95Sr,p)96Sr reaction, and constraints have been provided for the spins and parities of several final states. Results are compared to shell model calculations in several model spaces and the structure of low-lying states in 94Sr and 95Sr is well-described. The spectroscopic strength of the 0+ and 2 states in 96Sr is significantly more fragmented than predicted.

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Shell evolution approaching the N=20 island of inversion: Structure of 29Mg

The "Island of Inversion" for neutron-rich nuclei in the vicinity of N=20 has become the testing ground par excellence for our understanding and modelling of shell evolution with isospin. In this context, the structure of the transitional nucleus 29Mg is critical. The first quantitative measurements of the single particle structure of 29Mg are reported, using data from the d(28Mg,p gamma)29Mg reaction. Two key states carrying significant ell=3 (f-wave) strength were identified at 2.40 +/- 0.10 (Jpi = 5/2-) and 4.28 +/- 0.04 MeV (7/2-). New state-of-the-art shell model calculations have been performed and the predictions are compared in detail with the experimental results. Whilst the two lowest 7/2- levels are well described, the sharing of single-particle strength disagrees with experiment for both the 3/2- and 5/2- levels and there appear to be general problems with configurations involving the p3/2 neutron orbital and core-excited components. These conclusions are supported by an analysis of the neutron occupancies in the shell model calculations.

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Observation of excited states in $^{20}$Mg sheds light on nuclear forces and shell evolution

The exotic Borromean nucleus $^{20}$Mg with $N$ = 8, located at the proton drip-line provides a unique testing ground for nuclear forces and the evolution of shell structure in the neutron-deficient region. We report on the first observation of proton unbound resonances together with bound states in $^{20}$Mg from the $^{20}$Mg($d$,$d'$) reaction performed at TRIUMF. Phenomenological shell-model calculations offer a reasonable description. However, our experimental results present a challenge for current first-principles nuclear structure approaches and point to the need for improved chiral forces and {\it ab initio} calculations. Furthermore, the differential cross section of the first excited state is compared with distorted-wave Born approximation calculations to deduce a neutron quadrupole deformation parameter of $β_n$=0.46$\pm$0.21. This provides the first indication of a possible weakening of the $N$ = 8 shell closure at the proton drip-line.

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The GRIFFIN Facility for Decay-Spectroscopy Studies at TRIUMF-ISAC

Gamma-Ray Infrastructure For Fundamental Investigations of Nuclei, GRIFFIN, is a new high-efficiency $γ$-ray spectrometer designed for use in decay spectroscopy experiments with low-energy radioactive ion beams provided by TRIUMF's Isotope Separator and Accelerator (ISAC-I) facility. GRIFFIN is composed of sixteen Compton-suppressed large-volume clover-type high-purity germanium (HPGe) $γ$-ray detectors combined with a suite of ancillary detection systems and coupled to a custom digital data acquisition system. The infrastructure and detectors of the spectrometer as well as the performance characteristics and the analysis techniques applied to the experimental data are described.

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Half-Lives of Neutron Rich $^{130}$Cd and $^{131}$In

The half-lives of isotopes around the $N=82$ shell closure are an important ingredient in astrophysical simulations and strongly influence the magnitude of the second $r$-process abundance peak in the $A\sim130$ region. The most neutron-rich $N=82$ nuclei are not accessible to the current generation of radioactive beam facilities and $r$-process simulations must therefore rely on calculations of the half-lives of the isotopes involved. Half-life measurements of the experimentally accessible nuclei in this region are important in order to benchmark these calculations. The half-life of $^{130}$Cd is particularly important as it is used to tune the Gamow-Teller quenching in shell-model calculations for the $β$ decay of other nuclei in this region. In this work, the GRIFFIN $γ$-ray spectrometer at the TRIUMF-ISAC facility was used to measure the half-life of $^{130}_{~48}$Cd$_{82}$ to be $T_{1/2}= 126(4)$ ms. In addition, the half-lives of the three $β$ decaying states of $^{131}_{~49}$In$_{82}$ were measured to be $T_{1/2}(1/2^-)=328(15)$ ms, $T_{1/2}(9/2^+)=265(8)$ ms, and $T_{1/2}(21/2^+)=323(50)$ ms, respectively, providing an important benchmark for half-life calculations in this region.

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Shape Coexistence and Mixing of Low-Lying $0^+$ States in $^{96}$Sr

The low energy excited $0_{2,3}^+$ states in $^{96}$Sr are amongst the most prominent examples of shape coexistence across the nuclear landscape. In this work, the neutron $[2s_{1/2}]^2$ content of the $0_{1,2,3}^+$ states in $^{96}$Sr was determined by means of the d($^{95}$Sr,p) transfer reaction at the TRIUMF-ISAC2 facility using the SHARC and TIGRESS arrays. Spectroscopic factors of 0.19(3) and 0.22(3) were extracted for the $^{96}$Sr ground and 1229~keV $0^+$ states, respectively, by fitting the experimental angular distributions to DWBA reaction model calculations. A detailed analysis of the $γ$-decay of the isomeric $0_3^+$ state was used to determine a spectroscopic factor of 0.33(13). The experimental results are compared to shell model calculations, which predict negligible spectroscopic strength for the excited $0^+$ states in $^{96}$Sr. The strengths of the excited $0_{2,3}^+$ states were also analyzed within a two-level mixing model and are consistent with a mixing strength of $a^2$=0.40(14) and a difference in intrinsic deformations of $|Δβ|=0.31(3)$. These results suggest coexistence of three different configurations in $^{96}$Sr and strong shape mixing of the two excited $0^+$ states.

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