arXiv subjects

M. Nicklas

Publications and source records attributed to M. Nicklas.

At least 73 records · Page 4Linked to original sources

arXiv2010

Competition of local-moment ferromagnetism and superconductivity in Co-substituted EuFe2As2

In contrast to SrFe2As2, where only the iron possesses a magnetic moment, in EuFe2As2 an additional large, local magnetic moment is carried by Eu2+. Like SrFe2As2, EuFe2As2 exhibits a spin-density wave transition at high temperatures, but in addition the magnetic moments of the Eu2+ order at around 20 K. The interplay of pressure-induced superconductivity and the Eu2+ order leads to a behavior which is reminiscent of re-entrant superconductivity as it was observed, for example, in the ternary Chevrel phases or in the rare-earth nickel borocarbides. Here, we study the delicate interplay of the ordering of the Eu2+ moments and superconductivity in EuFe1.9Co0.1As2, where application of external pressure makes it possible to sensitively tune the ratio of the magnetic (T_C) and the superconducting (T_{c,onset}) critical temperatures. We find that superconductivity disappears once T_C > T_{c,onset}.

cond-mat.supr-con↗

arXiv2010

Effect of chemical substitution and pressure on YbRh2Si2

We carried out electrical resistivity experiments on (Yb,La)Rh2Si2 and on Yb(Rh,Ir)2Si2 under pressure and in magnetic fields. YbRh2Si2 exhibits a weak antiferromagnetic transition at atmospheric pressure with a Néel temperature of only T_N = 70 mK. By applying a small magnetic field T_N can be continuously suppressed to T=0 at B_c = 60 mT (B_|_c) driving the system to a quantum critical point (QCP). On applying external pressure the magnetic phase is stabilized and T_N(p) is increasing as usually observed in Yb-based heavy-fermion metals. Substituting Yb by La or Rh by Ir allows to create a negative chemical pressure, La (Ir) being smaller than Yb (Rh), and eventually to drive YbRh2Si2 to a pressure controlled QCP. In this paper we compare the effect of external hydrostatic pressure and chemical substitution on the ground-state properties of YbRh2Si2.

cond-mat.str-el↗

arXiv2010

Temperature - pressure phase diagram of the superconducting iron pnictide LiFeP

Electrical-resistivity and magnetic-susceptibility measurements under hydrostatic pressure up to p = 2.75 GPa have been performed on superconducting LiFeP. A broad superconducting (SC) region exists in the temperature - pressure (T-p) phase diagram. No indications for a spin-density-wave transition have been found, but an enhanced resistivity coefficient at low pressures hints at the presence of magnetic fluctuations. Our results show that the superconducting state in LiFeP is more robust than in the isostructural and isoelectronic LiFeAs. We suggest that this finding is related to the nearly regular [FeP_4] tetrahedron in LiFeP.

cond-mat.supr-con↗

arXiv2009

Pressure-induced change of the pairing symmetry in superconducting CeCu2Si2

Low-temperature (T) heat-capacity measurements under hydrostatic pressure of up to p=2.1 GPa have been performed on single-crystalline CeCu2Si2. A broad superconducting (SC) region exists in the T-p phase diagram. In the low-pressure region antiferromagnetic spin fluctuations and in the high-pressure region valence fluctuations had previously been proposed to mediate Cooper pairing. We could identify these two distinct SC regions. We found different thermodynamic properties of the SC phase in both regions, supporting the proposal that different mechanisms might be implied in the formation of superconductivity.

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arXiv2009

Heavy fermion behavior in PrRh2B2C: Excitonic mass enhancement

We report magnetic and transport properties of a new quaternary borocarbide PrRh$_{2}$B$_{2}$C, based on magnetisation, resistivity and specific heat studies. This compound forms in LuNi$_{2}$B$_{2}$C-type tetragonal structure (space group {\it I4/mmm}) and does not exhibit magnetic ordering or superconductivity down to 0.5 K. The crystal field analysis of specific heat data suggests a singlet ground state in this compound. The high value of the Sommerfeld coefficient, $γ$ $\approx$ 250 mJ/mole K$^{2}$, together with a singlet ground state suggests that the heavy fermion behaviour in PrRh$_{2}$B$_{2}$C results from the interaction of the conduction electrons with the low lying crystal field excitations. No signature of magnetic ordering or superconductivity is observed in PrRh$_{2}$B$_{2}$C under the application of pressure up to 23 kbar.

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arXiv2009

Extreme vortex pinning in the non-centrosymmetric superconductor CePt$_{3}$Si

We report on the vortex dynamics of a single crystal of the non-centrosymmetric heavy-fermion superconductor CePt$_{3}$Si. Decays of the remnant magnetization display a clean logarithmic time dependence with rates that follow the temperature dependence expected from the Kim-Anderson theory. The creep rates are lower than observed in any other centrosymmetric superconductor and are not caused by high critical currents. On the contrary, the critical current in CePt$_{3}$Si is considerably lower than in other superconductors with strong vortex pinning indicating that an alternative impediment on the flux line motion might be at work in this superconductor.

cond-mat.supr-con↗

arXiv2009

Superfluid Density and Energy Gap-Function of Superconducting PrPt4Ge12

The filled skutterudite superconductor PrPt4Ge12 was studied in muon-spin rotation (muSR), specific heat, and electrical resistivity experiments. The continuous increase of the superfluid density with decreasing temperature and the dependence of the magnetic penetration depth λon the magnetic field obtained by means of muSR, as well as the observation of a T^3 dependence of the electronic specific heat establish the presence of point-like nodes in the superconducting energy gap. The energy gap was found to be well described by Δ=Δ_0| k_x - ik_y| or Δ= Δ_0(1 - k_y^4) functional forms, similar to that obtained for another skutterudite superconductor, PrOs4Sb12. The gap to T_c ratios were estimated to be Δ_0/k_BT_c = 2.68(5) and 2.29(5), respectively.

cond-mat.supr-con↗

arXiv2008

Unusual heavy-mass nearly ferromagnetic state with a surprisingly large Wilson ratio in the double layered ruthenates (Sr$_{1-x}$Ca$_{x}$)$_{3}$Ru$_{2}$O$_{7}$

We report an unusual nearly ferromagnetic, heavy-mass state with a surprisingly large Wilson ratio $R_{\textrm{w}}$ (e.g., $R_{\textrm{w}}\sim$ 700 for $x =$ 0.2) in double layered ruthenates (Sr$_{1-x}$Ca$_{x}$)$_{3}$Ru$_{2}$O$_{7}$ with 0.08 $< x <$ 0.4. This state does not evolve into a long-range ferromagnetically ordered state despite considerably strong ferromagnetic correlations, but freezes into a cluster-spin-glass at low temperatures. In addition, evidence of non-Fermi liquid behavior is observed as the spin freezing temperature of the cluster-spin-glass approaches zero near $x \approx$ 0.1. We discuss the origin of this unique magnetic state from the Fermi surface information probed by Hall effect measurements.

cond-mat.str-el↗

arXiv2008

Effect of pressure and Ir substitution in YbRh2Si2

In this article we present a study of the electrical resistivity of Yb(Rh-xIrx)2Si2, x=0.06, under high pressure and in magnetic field. Ir substitution is expanding the unit cell and leads to a suppression of the antiferromagnetic transition temperature to zero, where eventually a quantum critical point (QCP) exists. We applied hydrostatic pressure to reverse the effect of substitution. Our results indicate that Yb(Rh0.94Ir0.06)2Si2 is situated in the immediate proximity to a volume controlled QCP, but still on the magnetically ordered side of the phase diagram. The temperature - pressure phase diagram of Yb(Rh0.94Ir0.06)2Si2 resembles that of the pure compound. Substitution acts mainly as chemical pressure. Disorder introduced by substitution has only minor effects.

cond-mat.str-el↗

arXiv2008

Effect of pressure on the magnetostructural transition in SrFe2As2

We present a systematic pressure study of poly- and single crystalline SrFe2As2 by electrical resistivity and X-ray diffraction measurements. SrFe2As2 exhibits a structural phase transition from a tetragonal to an orthorhombic phase at T0=205 K. The structural phase transition is intimately linked to a spin-density-wave transition taking place at the same temperature. Our pressure experiments show that T0 shifts to lower temperatures with increasing pressure. We can estimate a critical pressure of 4 to 5 GPa for the suppression of T0 to zero temperature. At pressures above 2.5 GPa the resistivity decreases significantly below Tx=40 K hinting at the emergence of superconductivity but no zero-resistance state is observed up to 3 GPa.

cond-mat.supr-con↗

arXiv2008

Analysis of the normal state magnetotransport in CeIrIn${_5}$

We present an analysis of the normal state magnetotransport in the heavy fermion superconductor CeIrIn${_5}$. The Hall effect and the transverse magnetoresistance in this material do not appear to be uniquely correlated, as inferred from the field dependence of the current ratio ($R_σ = σ_{xy} / σ_{xx}^2 H$). The Hall coefficient is seen to satisfy a scaling equation of the form $R_H = f [H / (a + b T^c)]$. These results are compared to those observed earlier in CeCoIn$_5$, and are discussed in terms of the contrasting phase diagram which the CeIrIn$_5$ system exhibits in relation to its Co counterpart.

cond-mat.str-el↗

arXiv2008

Magnetotransport in the CeIrIn${_5}$ system: The influence of antiferromagnetic fluctuations

We present an overview of magnetotransport measurements on the heavy-fermion superconductor CeIrIn$_5$. Sensitive measurements of the Hall effect and magnetoresistance (MR) are used to elucidate the low temperature phase diagram of this system. The normal-state magnetotransport is highly anomalous, and experimental signatures of a pseudogap-like precursor state to superconductivity as well as evidence for two distinct scattering times governing the Hall effect and the MR are observed. Our observations point out the influence of antiferromagnetic fluctuations on the magnetotransport in this class of materials. The implications of these findings, both in the context of unconventional superconductivity in heavy-fermion systems as well as in relation to the high temperature superconducting cuprates are discussed.

cond-mat.str-el↗

arXiv2008

The precursor state to superconductivity in CeIrIn${_5}$: Unusual scaling of magnetotransport

We present an analysis of the normal-state Hall effect and magnetoresistance in the heavy fermion superconductor CeIrIn${_5}$. It is demonstrated that the modified Kohler's scaling--which relates the magnetoresistance to the Hall angle--breaks down prior to the onset of superconductivity due to the presence of a precursor state to superconductivity in this system. A model-independent, single-parameter scaling of the Hall angle governed solely by this precursor state is observed. Neither the Hall coefficient nor the resistivity exhibit this scaling implying that this precursor state preferentially influences the Hall channel.

cond-mat.str-el↗

arXiv2008

Possible re-entrant superconductivity in EuFe2As2 under pressure

We studied the temperature-pressure phase diagram of EuFe2As2 by measurements of the electrical resistivity. The antiferromagnetic spin-density-wave transition at T_0 associated with the FeAs-layers is continuously suppressed with increasing pressure, while the antiferromagnetic ordering temperature of the Eu 2+ moments seems to be nearly pressure independent up to 2.6 GPa. Above 2 GPa a sharp drop of the resistivity, ρ(T), indicates the onset of superconductivity at T_c \approx 29.5 K. Surprisingly, on further reducing the temperature ρ(T) is increasing again and exhibiting a maximum caused by the ordering of the Eu 2+ moments, a behavior which is reminiscent of re-entrant superconductivity as it is observed in the ternary Chevrel phases or in the rare-earth nickel borocarbides.

cond-mat.supr-con↗

arXiv2007

A precursor state to unconventional superconductivity in CeIrIn${_5}$

We present sensitive measurements of the Hall effect and magnetoresistance in CeIrIn${_5}$ down to temperatures of 50 mK and magnetic fields up to 15 T. The presence of a low temperature coherent Kondo state is established. Deviations from Kohler's rule and a quadratic temperature dependence of the cotangent of the Hall angle are reminiscent of properties observed in the high temperature superconducting cuprates. The most striking observation pertains to the presence of a \textit{precursor} state--characterized by a change in the Hall mobility--that appears to precede the superconductivity in this material, in similarity to the pseudogap in the cuprate high $T_c$ superconductors.

cond-mat.str-el↗

arXiv2007

Antiferromagnetic fluctuations and the Fulde-Ferrell-Larkin-Ovchinnikov state in CeCoIn5

The heavy-fermion superconductor CeCoIn5 is the first material, where different experimental probes show strong evidence pointing to the realization of the Fulde-Ferrell-Larkin-Ovchinnikov (FFLO) state. The inhomogeneous superconducting FFLO state with a periodically modulated order parameter was predicted to appear in Pauli-limited, sufficiently clean type-II superconductors already more than 40 years ago. On the other hand, CeCoIn5 is supposed to be close to a magnetic quantum critical point (QCP) showing strong antiferromagnetic (AFM) spin fluctuations (SF) at atmospheric pressure. We studied the evolution of the FFLO phase away from the influence of the strong AFM-SF by heat capacity experiments under pressure (0 GPa <= P <= 1.5 GPa, 0 T <= mu_0 H <= 14 T, and 100 mK <= T <= 4 K). Our results prove the stability of the the FFLO phase under pressure. It even expands, while the Pauli-limiting becomes weaker and the AFM-SF are suppressed. This shows the intriguing influence of the AFM-SF on the FFLO state.

cond-mat.str-el↗

arXiv2007

Superconductivity in the New Platinum Germanides MPt4Ge12 (M = Rare-earth and Alkaline-earth Metals) with Filled Skutterudite Structure

New germanium-platinum compounds with the filled-skutterudite crystal structure were synthesized. The structure and composition were investigated by X-ray diffraction and microprobe analysis. Magnetic susceptibility, specific heat, and electrical resistivity measurements evidence superconductivity in LaPt4Ge12 and PrPt4Ge12 below 8.3K. The parameters of the normal and superconducting states were established. Strong coupling and a crystal electric field singlet groundstate is found for the Pr compound. Electronic structure calculations show a large density of states at the Fermi level. Similar behavior with lower T_c was observed for SrPt4Ge12 and BaPt4Ge12.

cond-mat.supr-con↗

arXiv2007

CeRuPO: A rare example of a Ferromagnetic Kondo lattice

We have determined the physical ground state properties of the compounds CeRuPO and CeOsPO by means of magnetic susceptibility chi(T), specific heat C(T), electrical resistivity rho(T), and thermopower S(T) measurements. chi(T) reveals a trivalent 4f1 cerium state in both compounds. For CeRuPO a pronounced decrease of rho(T) below 50K indicates the onset of coherent Kondo scattering which is confirmed by enhanced S(T). The temperature and magnetic field dependence of chi(T) and C(T) evidence ferromagnetic (FM) order at TC=15K. Thus, CeRuPO seems to be one of the rare example of a FM Kondo lattice. In contrast, CeOsPO shows antiferromagnetic order at TN=4.4K despite only minor changes in lattice parameters and electronic configuration. Additional 31P NMR results support these scenarios. LSDA+U calculations evidence a quasi two dimensional electronic band structure, reflecting a strong covalent bonding within the CeO and RuP layers and a weak ionic like bonding between the layers.

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