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M. Niikura

Publications and source records attributed to M. Niikura.

36 records · Page 2Linked to original sources

Persistence of the ${Z=28}$ shell gap in ${A=75}$ isobars: Identification of a possible ${(1/2^-)}$ $μ$s isomer in ${^{75}}$Co and $β$ decay to ${^{75}}$Ni

Background: The evolution of shell structure around doubly magic exotic nuclei is of great interest in nuclear physics and astrophysics. In the `southwest' region of $^{78}$Ni, the development of deformation might trigger a major shift in our understanding of explosive nucleosynthesis. To this end, new spectroscopic information on key close-lying nuclei is very valuable. Purpose: We intend to measure the isomeric and $β$ decay of $^{75}$Co, with one-proton and two-neutron holes relative to $^{78}$Ni, to access new nuclear structure information in $^{75}$Co and its $β$-decay daughters $^{75}$Ni and $^{74}$Ni. Methods: The nucleus $^{75}$Co is produced in relativistic in-flight fission reactions of $^{238}$U at the Radioactive Ion Beam Factory in the RIKEN Nishina Center. Its isomeric and $β$ decay are studied exploiting the BigRIPS and EURICA setups. Results: We obtain partial $β$-decay spectra for $^{75}$Ni and $^{74}$Ni, and report a new isomeric transition in $^{75}$Co. The energy [$E_γ=1914(2)$ keV] and half-life [$t_{1/2}=13(6)$ $μ$s] of the delayed $γ$ ray lend support for the existence of a $J^π=(1/2^-)$ isomeric state at 1914(2) keV. A comparison with PFSDG-U shell-model calculations provides a good account for the observed states in $^{75}$Ni, but the first calculated $1/2^-$ level in $^{75}$Co, a prolate $K=1/2$ state, is predicted about 1 MeV below the observed $(1/2^-)$ level. Conclusions: The spherical-like structure of the lowest-lying excited states in $^{75}$Ni is proved. In the case of $^{75}$Co, the results suggest that the dominance of the spherical configurations over the deformed ones might be stronger than expected below $^{78}$Ni. Further experimental efforts to discern the nature of the $J^π=(1/2^-)$ isomer are necessary.

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Shape changes in the mirror nuclei $^{70}$Kr and $^{70}$Se

We studied the proton-rich $T_z=-1$ nucleus $^{70}$Kr through inelastic scattering at intermediate energies in order to extract the reduced transition probability, $B(E2;\;0^+ \rightarrow 2^+)$. Comparison with the other members of the $A=70$ isospin triplet, $^{70}$Br and $^{70}$Se, studied in the same experiment, shows a $3σ$ deviation from the expected linearity of the electromagnetic matrix elements as a function of $T_z$. At present, no established nuclear structure theory can describe this observed deviation quantitatively. This is the first violation of isospin symmetry at this level observed in the transition matrix elements. A heuristic approach may explain the anomaly by a shape change between the mirror nuclei $^{70}$Kr and $^{70}$Se contrary to the model predictions.

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Probing nuclear forces beyond the nuclear drip line: The cases of $^{16}$F and $^{15}$F

The unbound proton-rich nuclei $^{16}$F and $^{15}$F are investigated experimentally and theoretically. Several experiments using the resonant elastic scattering method were performed at GANIL with radioactive beams to determine the properties of the low lying states of these nuclei. Strong asymmetry between $^{16}$F-$^{16}$N and $^{15}$F-$^{15}$C mirror nuclei is observed. The strength of the $nucleon-nucleon$ effective interaction involving the loosely bound proton in the $s_{1/2}$ orbit is significantly modified with respect to their mirror nuclei $^{16}$N and $^{15}$C. The reduction of the effective interaction is estimated by calculating the interaction energies with a schematic zero-range force. It is found that, after correcting for the effects due to changes in the radial distribution of the single-particle wave functions, the mirror symmetry of the $n-p$ interaction is preserved between $^{16}$F and $^{16}$N, while a difference of 63\% is measured between the $p-p$ versus $n-n$ interactions in the second excited state of $^{15}$F and $^{15}$C nuclei. Several explanations are proposed.

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Shell structure of $^{43}$S and collapse of the $N=28$ shell closure

The single-particle structure of the $N=27$ isotones provides insights into the shell evolution of neutron-rich nuclei from the doubly-magic $^{48}$Ca toward the drip line. $^{43}$S was studied employing the one-neutron knockout reaction from a radioactive $^{44}$S beam. Using a combination of prompt and delayed $γ$-ray spectroscopy the level structure of $^{43}$S was clarified. Momentum distributions were analyzed and allowed for spin and parity assignments. The deduced spectroscopic factors show that the $^{44}$S ground-state configuration has a strong intruder component. The results were confronted with shell model calculations using two effective interactions. General agreement was found between the calculations, but strong population of states originating from the removal of neutrons from the $2p_{3/2}$ orbital in the experiment indicates that the breakdown of the $N=28$ magic number is more rapid than the theoretical calculations suggest.

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Shape coexistence revealed in the $N=Z$ isotope $^{72}$Kr through inelastic scattering

The $N=Z=36$ nucleus $^{72}$Kr has been studied by inelastic scattering at intermediate energies. Two targets, $^{9}$Be and $^{197}$Au, were used to extract the nuclear deformation length, $δ_\text{N}$, and the reduced $E2$ transition probability, $B(E2)$. The previously unknown non-yrast $2^+$ and $4^+$ states as well as a new candidate for the octupole $3^-$ state have been observed in the scattering on the Be target and placed in the level scheme based on $γ-γ$ coincidences. The second $2^+$ state was also observed in the scattering on the Au target and the $B(E2;\;2^+_2 \rightarrow 0^+_1)$ value could be determined for the first time. Analyzing the results in terms of a two-band mixing model shows clear evidence for a oblate-prolate shape coexistence and can be explained by a shape change from an oblate ground state to prolate deformed yrast band from the first $2^+$ state. This interpretation is corroborated by beyond mean field calculations using the Gogny D1S interaction.

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$^{78}$Ni revealed as a doubly magic stronghold against nuclear deformation

Nuclear magic numbers, which emerge from the strong nuclear force based on quantum chromodynamics, correspond to fully occupied energy shells of protons, or neutrons inside atomic nuclei. Doubly magic nuclei, with magic numbers for both protons and neutrons, are spherical and extremely rare across the nuclear landscape. While the sequence of magic numbers is well established for stable nuclei, evidence reveals modifications for nuclei with a large proton-to-neutron asymmetry. Here, we provide the first spectroscopic study of the doubly magic nucleus $^{78}$Ni, fourteen neutrons beyond the last stable nickel isotope. We provide direct evidence for its doubly magic nature, which is also predicted by ab initio calculations based on chiral effective field theory interactions and the quasi-particle random-phase approximation. However, our results also provide the first indication of the breakdown of the neutron magic number 50 and proton magic number 28 beyond this stronghold, caused by a competing deformed structure. State-of-the-art phenomenological shell-model calculations reproduce this shape coexistence, predicting further a rapid transition from spherical to deformed ground states with $^{78}$Ni as turning point.

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Discovery of $^{68}$Br in secondary reactions of radioactive beams

The proton-rich isotope 68Br was discovered in secondary fragmentation reactions of fast radioactive beams. Proton-rich secondary beams of 70,71,72Kr and 70Br, produced at the RIKEN Nishina Center and identified by the BigRIPS fragment separator, impinged on a secondary 9Be target. Unambiguous particle identification behind the secondary target was achieved with the ZeroDegree spectrometer. Based on the expected direct production cross sections from neighboring isotopes, the lifetime of the ground or long-lived isomeric state of 68Br was estimated. The results suggest that secondary fragmentation reactions, where relatively few nucleons are removed from the projectile, offer an alternative way to search for new isotopes, as these reactions populate preferentially low-lying states.

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First spectroscopy of 61Ti and the transition to the Island of Inversion at N = 40

Isomeric states in 59,61Ti have been populated in the projectile fragmentation of a 345 AMeV 238U beam at the Radioactive Isotope Beam Factory. The decay lifetimes and delayed gamma-ray transitions were measured with the EURICA array. Besides the known isomeric state in 59Ti, two isomeric states in 61Ti are observed for the first time. Based on the measured lifetimes, transition multipolarities as well as tentative spins and parities are assigned. Large-scale shell model calculations based on the modified LNPS interaction show that both 59Ti and 61Ti belong to the Island of Inversion at N=40 with ground state configurations dominated by particle-hole excitations to the g_9/2 and d_5/2 orbits.

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Interplay between nuclear shell evolution and shape deformation revealed by magnetic moment of 75Cu

Exotic nuclei are characterized by a number of neutrons (or protons) in excess relative to stable nuclei. Their shell structure, which represents single-particle motion in a nucleus, may vary due to nuclear force and excess neutrons, in a phenomenon called shell evolution. This effect could be counterbalanced by collective modes causing deformations of the nuclear surface. Here, we study the interplay between shell evolution and shape deformation by focusing on the magnetic moment of an isomeric state of the neutron-rich nucleus 75Cu. We measure the magnetic moment using highly spin-controlled rare-isotope beams and achieving large spin alignment via a two-step reaction scheme that incorporates an angular-momentum-selecting nucleon removal. By combining our experiments with numerical simulations of many-fermion correlations, we find that the low-lying states in 75Cu are, to a large extent, of single-particle nature on top of a correlated 74Ni core. We elucidate the crucial role of shell evolution even in the presence of the collective mode, and within the same framework, we consider whether and how the double magicity of the 78Ni nucleus is restored, which is also of keen interest from the perspective of nucleosynthesis in explosive stellar processes.

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Shape coexistence and isospin symmetry in $A=70$ nuclei: Spectroscopy of the $T_z = -1$ nucleus $^{70}$Kr

Excited states in the $T_z=-1$ nucleus $^{70}$Kr have been populated using inelastic scattering of a radioactive $^{70}$Kr beam as well as one- and two-neutron removal reactions from $^{71,72}$Kr at intermediate beam energies. The level scheme of $^{70}$Kr was constructed from the observed $γ$-ray transitions and coincidences. Tentative spin and parity assignments were made based on comparison with the mirror nucleus $^{70}$Se. A second $2^+$ state and a candidate for the corresponding $4^+_2$ state suggest shape coexistence in $^{70}$Kr.

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Is Seniority a Partial Dynamic Symmetry in the First $νg_{9/2}$ Shell?

The low-lying structures of the midshell $νg_{9/2}$ Ni isotopes $^{72}$Ni and $^{74}$Ni have been investigated at the RIBF facility in RIKEN within the EURICA collaboration. Previously unobserved low-lying states were accessed for the first time following $β$ decay of the mother nuclei $^{72}$Co and $^{74}$Co. As a result, we provide a complete picture in terms of the seniority scheme up to the first $(8^+)$ levels for both nuclei. The experimental results are compared to shell-model calculations in order to define to what extent the seniority quantum number is preserved in the first neutron $g_{9/2}$ shell. We find that the disappearance of the seniority isomerism in the $(8^+_1)$ states can be explained by a lowering of the seniority-four $(6^+)$ levels as predicted years ago. For $^{74}$Ni, the internal de-excitation pattern of the newly observed $(6^+_2)$ state supports a restoration of the normal seniority ordering up to spin $J=4$. This property, unexplained by the shell-model calculations, is in agreement with a dominance of the single-particle spherical regime near $^{78}$Ni.

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Reinvestigation of the excited states in the proton emitter $^{151}$Lu: particle-hole excitations across the $N=Z=64$ subshell

The excited states of the proton emitter $^{151}$Lu were reinvestigated in a recoil-decay tagging experiment at the Accelerator Laboratory of the University of Jyväskylä (JYFL). The level scheme built on the ground state of $^{151}$Lu was updated with five new $γ$-ray transitions. Large-scale shell model calculations were carried out to interpret the experimental level scheme. It is found that the excitation energies of states above the $27/2^-$ and $23/2^+$ isomeric levels can be sensitive to excitations from $g_{7/2}$ and $d_{5/2}$ to single-particle orbitals above $N=Z=64$.

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Spectroscopic factor and proton formation probability for the d3/2 proton emitter 151mLu

The quenching of the experimental spectroscopic factor for proton emission from the short-lived $d_{3/2}$ isomeric state in $^{151m}$Lu was a long-standing problem. In the present work, proton emission from this isomer has been reinvestigated in an experiment at the Accelerator Laboratory of the University of Jyväskylä. The proton-decay energy and half-life of this isomer were measured to be 1295(5) keV and 15.4(8) $μ$s, respectively, in agreement with another recent study. These new experimental data can resolve the discrepancy in the spectroscopic factor calculated using the spherical WKB approximation. Using the R-matrix approach it is found that the proton formation probability indicates no significant hindrance for the proton decay of $^{151m}$Lu.

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Nuclear structure of 140Te with N = 88: Structural symmetry and asymmetry in Te isotopes with respect to the double-shell closure Z = 50 and N = 82

We study for the first time the internal structure of 140Te through the beta-delayed gamma-ray spectroscopy of 140Sb. The very neutron-rich 140Sb, Z = 51 and N = 89, ions were produced by the in-flight fission of 238U beam on a 9Be target at 345 MeV per nucleon at the Radioactive Ion Beam Factory, RIKEN. The half-life and spin-parity of 140Sb are reported as 124(30) ms and (4-), respectively. In addition to the excited states of 140Te produced by the beta-decay branch, the beta-delayed one-neutron and two-neutron emission branches were also established. By identifying the first 2+ and 4+ excited states of 140Te, we found that Te isotopes persist their vibrator character with E(4+)/E(2+) = 2. We discuss the distinctive features manifest in this region, such as valence neutron symmetry and asymmetry, revealed in pairs of isotopes with the same neutron holes and particles with respect to N = 82.

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First direct lifetime measurement of the 2+1 state in 72,74Zn: new evidence for shape transition between N = 40 and N = 42 close to Z = 28

We report here the first direct lifetime measurement of the 2+1 state in 72,74Zn. The neutron-rich beam was produced by in-flight fragmentation of 76Ge at the Grand Accélérateur National d'Ions Lourds and separated with the LISE spectrometer. The 2+1 state was excited by inelastic scattering and knock-out reaction on a CD2 target and its lifetime was measured by the recoil-distance Dopplershift method with the Köln plunger device combined with the EXOGAM detectors. The lifetimes of the 2+1 states in 72,74Zn were determined to be 17.9(18) and 27.0(24) ps, which correspond to reduced transition probabilities B(E2; 2+1 \rightarrow 0+) = 385(39) and 370(33) e2fm4, respectively. These values support the idea of a systematic maximum of collectivity at N = 42 for Zn, Ge and Se nuclei. In addition, the available systematics in the neighboring nuclei point towards a transition from a spherical oscillator at N = 40 to complete γ-softness at N = 42.

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Low-lying non-normal parity states in 8B measured by proton elastic scattering on 7Be

A new measurement of proton resonance scattering on 7Be was performed up to the center-of-mass energy of 6.7 MeV using the low-energy RI beam facility CRIB (CNS Radioactive Ion Beam separator) at the Center for Nuclear Study of the University of Tokyo. The excitation function of 7Be+p elastic scattering above 3.5 MeV was measured successfully for the first time, providing important information about the resonance structure of the 8B nucleus. The resonances are related to the reaction rate of 7Be(p, gamma)8B, which is the key reaction in solar 8B neutrino production. Evidence for the presence of two negative parity states is presented. One of them is a 2- state observed as a broad s-wave resonance, the existence of which had been questionable. Its possible effects on the determination of the astrophysical S-factor of 7Be(p, gamma)8B at solar energy are discussed. The other state had not been observed in previous measurements, and its spin and parity were determined as 1-.

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Fragmentation cross-sections and binding energies of neutron-rich nuclei

An exponential dependence of the fragmentation cross-section on the average binding energy is observed and reproduced with a statistical model. The observed functional dependence is robust and allows the extraction of binding energies from measured cross-sections. From the systematics of 75,77,78,79Cu isotope cross-sections have been extracted. They are 636.94 +/- 0.40 MeV, 647.1 +/- 0.4 MeV, 651.6 +/- 0.4 MeV and 657.8 +/- 0.5 MeV, respectively. Specifically, the uncertainty of the binding energy of 75Cu is reduced from 980 keV (listed value in the 2003 mass table of Audi and Wapstra) to 400 keV. The predicted cross-sections of two near drip-line nuclei, 39Na and 40Mg, from the fragmentation of 48Ca are discussed.

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Projectile Fragmentation of $^{86}$Kr at 64 MeV/nucleon

We measured fragmentation cross sections produced using the primary beam of $^{86}$Kr at 64 MeV/nucleon on $^9$Be and $^{181}$Ta targets. The cross sections were obtained by integrating the momentum distributions of isotopes with 25<Z<36 measured using the RIPS fragment separator at RIKEN. The cross-section ratios obtained with the $^{181}$Ta and $^{9}$Be targets depend on the fragment masses, contrary to the simple geometrical models. We compared the extracted cross sections to EPAX; an empirical parameterization of fragmentation cross sections. Predictions from current EPAX parameterization severely overestimate the production cross sections of very neutron-rich isotopes. Attempts to obtain another set of EPAX parameters specific to the reaction studied here, to extrapolate the neutron-rich nuclei more accurately have not been very successful, suggesting that accurate predictions of production cross sections of nuclei far from the valley of stability require information of nuclear properties which are not present in EPAX.

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