arXiv subjects

M. Okawa

Publications and source records attributed to M. Okawa.

At least 19 recordsLinked to original sources

arXiv2023

Linear dichroic x-ray absorption response of Ti-Ti dimers along the $c$ axis in Ti$_2$O$_3$ upon Mg substitution

Corundum oxide Ti$_2$O$_3$ shows the metal-insulator transition around 400-600 K accompanying the nearest Ti$^{3+}$-Ti$^{3+}$ bond ($a_{1g}a_{1g}$ singlet state) formation along the $c$ axis. In order to clarify the hole-doping effect for the $a_{1g}a_{1g}$ singlet bond in Ti$_2$O$_3$, we investigated Ti $3d$ orbital anisotropy between corundum-type Ti$_2$O$_3$ and ilmenite-type MgTiO$_3$ using linear dichroism of soft x-ray absorption spectroscopy of the Ti $L_{2,3}$ edge. From the linear dichroic spectral weight in Mg$_y$Ti$_{2-y}$O$_3$, we confirmed that the $a_{1g}a_{1g}$ state is dominant not only in $y=0.01$ (almost Ti$_2$O$_3$), but also in $y = 0.29$, indicating that the Ti-Ti bond survives against a certain level of hole doping. In $y=0.63$ corresponding to 46% hole doping per Ti, the $3d$ orbital symmetry changes from $a_{1g}$ to $e_g^π$.

cond-mat.str-el↗

arXiv2021

Scale setting for $\mathcal{N} = 1$ SUSY Yang-Mills at large-$N$ through volume-reduced twisted matrix model

$\mathcal{N}=1$ SUSY Yang-Mills theory is an appealing theoretical framework that has been studied in the literature using different methods, including standard lattice simulations. Among these, the volume-reduced twisted Eguchi-Kawai model, endowed with one adjoint Majorana fermion, could play an important role in studying its large-$N$ limit via the Curci-Veneziano prescription. In this talk, we present our results on the analysis of the scale of the theory, performed via different methods based on purely gluonic observables as well as (quenched) fundamental mesons in the chiral limit. These lattice results will be used as a scale setting for the analysis of the spectrum of the theory.

hep-lat↗

arXiv2015

Hybridization gap formation in the Kondo insulator YbB$_{12}$ observed using time-resolved photoemission spectroscopy

A detailed low-energy electronic structure of a Kondo insulator YbB$_{12}$ was revealed by a synergetic combination of ultrahigh-resolution laser photoemission spectroscopy (PES) and time-resolved PES. The former confirmed a 25-meV pseudogap corresponding to the Kondo temperature of this material, and more importantly, it revealed that a 15-meV gap and a Kondo-peak feature developed below a crossover temperature $T^\ast \sim 110$ K. In harmony with this, the latter discovered a very long recombination time exceeding 100 ps below $\sim$$T^\ast$. This is a clear manifestation of photoexcited carriers due to the bottleneck in the recovery dynamics, which is interpreted as a developing hybridization gap of a hard gap.

cond-mat.str-el↗

arXiv2015

Emergent photovoltage on SmB6 surface upon bulk-gap evolution revealed by pump-and-probe photoemission spectroscopy

Recent studies suggest that an exemplary Kondo insulator SmB6 belongs to a new class of topological insulators (TIs), in which non-trivial spin-polarized metallic states emerge on surface upon the formation of Kondo hybridization gap in the bulk. Remarkably, the bulk resistivity reaches more than 20 Ohm cm at 4 K, making SmB6 a candidate for a so-called bulk-insulating TI. We here investigate optical-pulse responses of SmB6 by pump-and-probe photoemission spectroscopy. Surface photovoltage effect is observed below ~90 K. This indicates that an optically-active band bending region develops beneath the novel metallic surface upon the bulk-gap evolution. The photovoltaic effect persists for >200 microsec, which is long enough to be detected by electronics devices, and could be utilized for optical gating of the novel metallic surface.

cond-mat.str-el↗

arXiv2013

Empirical relationship between x-ray photoemission spectra and electrical conductivity in a colossal magnetoresistive manganite La_{1-x}Sr_{x}MnO_{3}

By using laboratory x-ray photoemission spectroscopy (XPS) and hard x-ray photoemission spectroscopy (HX-PES) at a synchrotron facility, we report an empirical semi-quantitative relationship between the valence/core-level x-ray photoemission spectral weight and electrical conductivity in La_{1-x}Sr_{x}MnO_{3} as a function of x. In the Mn 2p_{3/2} HX-PES spectra, we observed the shoulder structure due to the Mn^{3+} well-screened state. However, the intensity at x=0.8 was too small to explain its higher electrical conductivity than x=0.0, which confirms our recent analysis on the Mn 2p_{3/2} XPS spectra. The near-Fermi level XPS spectral weight was found to be a measure of the variation of electrical conductivity with x in spite of a far lower energy resolution compared with the energy scale of the quasiparticle (coherent) peak because of the concurrent change of the coherent and incoherent spectral weight.

cond-mat.str-el↗

arXiv2013

Electronic structure of hole-doped delafossite oxides CuCr_{1-x}Mg_{x}O_{2}

We report the detailed electronic structure of a hole-doped delafossite oxide CuCr_{1-x}Mg_{x}O_{2} (0 <= x <= 0.03) studied by photoemission spectroscopy (PES), soft x-ray absorption spectroscopy (XAS), and band-structure calculations within the local-density approximation +U (LDA+U) scheme. Cr/Cu 3p-3d resonant PES reveals that the near-Fermi-level leading structure has primarily the Cr 3d character with a minor contribution from the Cu 3d through Cu 3d-O 2p-Cr 3d hybridization, having good agreement with the band-structure calculations. This indicates that a doped hole will have primarily the Cr 3d character. Cr 2p PES and L-edge XAS spectra exhibit typical Cr^{3+} features for all x, while the Cu L-edge XAS spectra exhibited a systematic change with x. This indicates now that the Cu valence is monovalent at x=0 and the doped hole should have Cu 3d character. Nevertheless, we surprisingly observed two types of charge-transfer satellites that should be attributed to Cu^{+} (3d^{10}) and Cu^{2+} (3d^{9}) like initial states in Cu 2p-3d resonant PES spectrum for at x=0, while Cu 2p PES spectra with no doubt shows the Cu^{+} character even for the lightly doped samples. We propose that these contradictory results can be understood by introducing no only the Cu 4s state, but also finite Cu 3d,4s-Cr 3d charge transfer via O 2p states in the ground-state electronic configuration.

cond-mat.str-el↗

arXiv2013

Charmed baryons at the physical point in 2+1 flavor lattice QCD

We investigate the charmed baryon mass spectrum using the relativistic heavy quark action on 2+1 flavor PACS-CS configurations previously generated on $32^3 \times 64$ lattice. The dynamical up-down and strange quark masses are tuned to their physical values, reweighted from those employed in the configuration generation. At the physical point, the inverse lattice spacing determined from the $Ω$ baryon mass gives $a^{-1}=2.194(10)$ GeV, and thus the spatial extent becomes $L = 32 a = 2.88(1)$ fm. Our results for the charmed baryon masses are consistent with experimental values, except for the mass of $Ξ_{cc}$, which has been measured by only one experimental group so far and has not been confirmed yet by others. In addition, we report values of other doubly and triply charmed baryon masses, which have never been measured experimentally.

hep-lat↗

arXiv2012

Coexisting pseudo-gap and superconducting gap in the high-Tc superconductor La2-xSrxCuO4

Relationship between the superconducting gap and the pseudogap has been the subject of controversies. In order to clarify this issue, we have studied the superconducting gap and pseudogap of the high-Tc superconductor La2-xSrxCuO4 (x=0.10, 0.14) by angle-resolved photoemission spectroscopy (ARPES). Through the analysis of the ARPES spectra above and below Tc, we have identified a superconducting coherence peak even in the anti-nodal region on top of the pseudogap of a larger energy scale. The superconducting peak energy nearly follows the pure d-wave form. The d-wave order parameter Δ_0 [defined by Δ(k)=Δ_0(cos(kxa)-cos(kya)) ] for x=0.10 and 0.14 are nearly the same, Δ_0 ~ 12-14 meV, leading to strong coupling 2Δ_0/kB Tc ~ 10. The present result indicates that the pseudogap and the superconducting gap are distinct phenomena and can be described by the "two-gap" scenario.

cond-mat.str-el↗

arXiv2012

1+1+1 flavor QCD + QED simulation at the physical point

We present the results of 1+1+1 flavor QCD+QED simulation at the physical point, in which the dynamical quark effects in QED and the up-down quark mass difference are incorporated by the reweighting technique. The physical quark masses together with the lattice spacing are determined with $m_{π^+}$, $m_{K^+}$, $m_{K^0}$ and $m_{Ω^-}$ as physical inputs. Calculations are carried out using a set of 2+1 flavor QCD configurations near the physical point generated by the non-perturbatively $O(a)$-improved Wilson quark action and the Iwasaki gauge action at $β=1.9$ on a $32^3\times 64$ lattice. We evaluate the values of the up, down and strange quark masses individually with non-perturbative QCD renormalization.

hep-lat↗

arXiv2011

$ρ$ Meson Decay in 2+1 Flavor Lattice QCD

We perform a lattice QCD study of the $ρ$ meson decay from the $N_f=2+1$ full QCD configurations generated with a renormalization group improved gauge action and a non-perturbatively $O(a)$-improved Wilson fermion action. The resonance parameters, the effective $ρ\toππ$ coupling constant and the resonance mass, are estimated from the $P$-wave scattering phase shift for the isospin I=1 two-pion system. The finite size formulas are employed to calculate the phase shift from the energy on the lattice. Our calculations are carried out at two quark masses, $m_π=410\,{\rm MeV}$ ($m_π/m_ρ=0.46$) and $m_π=300\,{\rm MeV}$ ($m_π/m_ρ=0.35$), on a $32^3\times 64$ ($La=2.9\,{\rm fm}$) lattice at the lattice spacing $a=0.091\,{\rm fm}$. We compare our results at these two quark masses with those given in the previous works using $N_f=2$ full QCD configurations and the experiment.

hep-lat↗

arXiv2011

Common Origin of the Circular-dichroism Pattern in ARPES of SrTiO3 and CuxBi2Se3

Circular dichroism in the angular distribution (CDAD) of photoelectrons from SrTiO3:Nb and CuxBi2Se3 is investigated by 7-eV laser ARPES. In addition to the well-known node that occurs in CDAD when the incidence plane matches the mirror plane of the crystal, we show that another type of node occurs when the mirror plane of the crystal is vertical to the incidence plane and the electronic state is two dimensional. The flower-shaped CDAD's occurring around the Fermi level of SrTiO3:Nb and around the Dirac point of CuxBi2Se3 are explained on equal footings. We point out that the penetration depth of the topological states of CuxBi2Se3 depends on momentum.

cond-mat.mtrl-sci↗

arXiv2011

Charm quark system at the physical point of 2+1 flavor lattice QCD

We investigate the charm quark system using the relativistic heavy quark action on 2+1 flavor PACS-CS configurations previously generated on $32^3 \times 64$ lattice. The dynamical up-down and strange quark masses are set to the physical values by using the technique of reweighting to shift the quark hopping parameters from the values employed in the configuration generation. At the physical point, the lattice spacing equals $a^{-1}=2.194(10)$ GeV and the spatial extent $L=2.88(1)$ fm. The charm quark mass is determined by the spin-averaged mass of the 1S charmonium state, from which we obtain $m_{\rm charm}^{\msbar}(μ= m_{\rm charm}^{\msbar}) = 1.260(1)(6)(35)$ GeV, where the errors are due to our statistics, scale determination and renormalization factor. An additional systematic error from the heavy quark is of order $α_s^2 f(m_Q a)(a Λ_{QCD})$, which is estimated to be a percent level if the factor $f(m_Q a)$ analytic in $m_Q a$ is of order unity. Our results for the charmed and charmed-strange meson decay constants are $f_D=226(6)(1)(5)$ MeV, $f_{D_s}=257(2)(1)(5)$ MeV, again up to the heavy quark errors of order $α_s^2 f(m_Q a)(a Λ_{QCD})$. Combined with the CLEO values for the leptonic decay widths, these values yield $|V_{cd}| = 0.205(6)(1)(5)(9)$, $|V_{cs}| = 1.00(1)(1)(3)(3)$, where the last error is on account of the experimental uncertainty of the decay widths.

hep-lat↗

arXiv2010

Electronic structure of an antiferromagnetic metal: CaCrO3

We report on the electronic structure of the perovskite oxide CaCrO3 using valence-band, core-level, and Cr 2p - 3d resonant photoemission spectroscopy (PES). Despite its antiferromagnetic order, a clear Fermi edge characteristic of a metal with dominant Cr 3d character is observed in the valence band spectrum. The Cr 3d single particle density of states are spread over 2 eV, with the photoemission spectral weight distributed in two peaks centered at ~ 1.2 eV and 0.2 eV below EF, suggestive of the coherent and incoherent states resulting from strong electron-electron correlations. Resonant PES across the Cr 2p - 3d threshold identifies a 'two-hole' correlation satellite and yields an on-site Coulomb energy U ~4.8 eV. The metallic DOS at EF is also reflected through the presence of a well-screened feature at low binding energy side of the Cr 2p core-level spectrum. X-ray absorption spectroscopy (XAS) at Cr L3,2 and O K edges exhibit small temperature dependent changes that point towards a small change in Cr-O hybridization. The multiplet splitting in Cr 2p core level spectrum as well as the spectral shape of the Cr XAS can be reproduced using cluster model calculations which favour a negative value for charge transfer energy between the Cr 3d and O 2p states. The overall results indicate that CaCrO3 is a strongly hybridized antiferromagnetic metal, lying in the regime intermediate to Mott-Hubbard and charge-transfer systems.

cond-mat.str-el↗

arXiv2010

Calculation of $ρ$ meson decay width from the PACS-CS configurations

We present preliminary results on the $ρ$ meson decay width from $N_f=2+1$ full QCD configurations generated by PACS-CS Collaboration. The decay width is estimated from the $P$-wave scattering phase shift for the isospin $I=1$ two-pion system. The finite size formula presented by Lüscher in the center of mass frame and its extension to non-zero total momentum frame by Rummukainen and Gottlieb are employed for the calculations of the phase shift. Our calculations are carried out at $m_π=410\ {\rm MeV}$ ($m_π/m_ρ=0.46$) and $a=0.091\ {\rm fm}$ on a $32^3\times 64$ ($La=2.9 {\rm fm}$) lattice.

hep-lat↗

arXiv2010

Strong valence fluctuation in the quantum critical heavy fermion superconductor beta-YbAlB4: A hard x-ray photoemission study

Electronic structures of the quantum critical superconductor beta-YbAlB4 and its polymorph alpha-YbAlB4 are investigated by using bulk-sensitive hard x-ray photoemission spectroscopy. From the Yb 3d core level spectra, the values of the Yb valence are estimated to be ~2.73 and ~2.75 for alpha- and beta-YbAlB4, respectively, thus providing clear evidence for valence fluctuations. The valence band spectra of these compounds also show Yb2+ peaks at the Fermi level. These observations establish an unambiguous case of a strong mixed valence at quantum criticality for the first time among heavy fermion systems, calling for a novel scheme for a quantum critical model beyond the conventional Doniach picture in beta-YbAlB4.

cond-mat.str-el↗

arXiv2010

Non-perturbative renormalization of quark mass in Nf=2+1 QCD with the Schroedinger functional scheme

We present an evaluation of the quark mass renormalization factor for Nf=2+1 QCD. The Schroedinger functional scheme is employed as the intermediate scheme to carry out non-perturbative running from the low energy region, where renormalization of bare mass is performed on the lattice, to deep in the high energy perturbative region, where the conversion to the renormalization group invariant mass or the MS-bar scheme is safely carried out. For numerical simulations we adopted the Iwasaki gauge action and non-perturbatively improved Wilson fermion action with the clover term. Seven renormalization scales are used to cover from low to high energy regions and three lattice spacings to take the continuum limit at each scale. The regularization independent step scaling function of the quark mass for the Nf=2+1 QCD is obtained in the continuum limit. Renormalization factors for the pseudo scalar density and the axial vector current are also evaluated for the same action and the bare couplings as two recent large scale Nf=2+1 simulations; previous work of the CP-PACS/JLQCD collaboration, which covered the up-down quark mass range heavier than $m_π\sim 500$ MeV and that of PACS-CS collaboration for much lighter quark masses down to $m_π=155$ MeV. The quark mass renormalization factor is used to renormalize bare PCAC masses in these simulations.

hep-lat↗

arXiv2010

Physical Point Simulation in 2+1 Flavor Lattice QCD

We present the results of the physical point simulation in 2+1 flavor lattice QCD with the nonperturbatively $O(a)$-improved Wilson quark action and the Iwasaki gauge action at $β=1.9$ on a $32^3 \times 64$ lattice. The physical quark masses together with the lattice spacing is determined with $m_π$, $m_K$ and $m_Ω$ as physical inputs. There are two key algorithmic ingredients to make possible the direct simulation at the physical point: One is the mass-preconditioned domain-decomposed HMC algorithm to reduce the computational cost. The other is the reweighting technique to adjust the hopping parameters exactly to the physical point. The physics results include the hadron spectrum, the quark masses and the pseudoscalar meson decay constants. The renormalization factors are nonperturbatively evaluated with the Schr{ö}dinger functional method. The results are compared with the previous ones obtained by the chiral extrapolation method.

hep-lat↗

arXiv2010

Orbital-dependent modifications of electronic structure across magneto-structural transition in BaFe2As2

Laser angle-resolved photoemission spectroscopy (ARPES) is employed to investigate the temperature (T) dependence of the electronic structure in BaFe2As2 across the magneto-structural transition at TN ~ 140 K. A drastic transformation in Fermi surface (FS) shape across TN is observed, as expected by first-principles band calculations. Polarization-dependent ARPES and band calculations consistently indicate that the observed FSs at kz ~ pi in the low-T antiferromagnetic (AF) state are dominated by the Fe3dzx orbital, leading to the two-fold electronic structure. These results indicate that magneto-structural transition in BaFe2As2 accompanies orbital-dependent modifications in the electronic structure.

cond-mat.supr-con↗