arXiv subjects
Publications and source records attributed to M. P. A. Jones.
Newly calculated multichannel quantum defect theory parameters and channel fractions are presented for the singlet and triplet S, P and D series and singlet F series of strontium. These results correct those reported in Vaillant C L, Jones M P A and Potvliege R M 2014 J. Phys. B: At. Mol. Opt. Phys. 47 155001.
We consider the potential use of optical traps for precision measurements in atomic hydrogen (H). Using an implicit summation method, we calculate the atomic polarisability, the rates of elastic/inelastic scattering and the ionisation rate in the wavelength range 395 to 1000 nm. We extend previous work to predict three new magic wavelengths for the 1S--2S transition. At the magic wavelengths, the 1S--2S transition is unavoidably and significantly broadened due to trap-induced ionisation associated with the high intensity required to trap the 1S state. However, we also find that this effect is partially mitigated by the low mass of H, which increases the trap frequency, enabling Lamb-Dicke confinement in shallow lattices. We find that a H optical lattice clock, free from the motional systematics which dominate in beam experiments, could operate with an intrinsic linewidth of O(1 kHz). Trap-induced losses are shown not to limit measurements of other transitions.
We demonstrate number-resolved detection of individual strontium atoms in a long working distance low numerical aperture (NA = 0.26) tweezer. Using a camera based on single-photon counting technology, we determine the presence of an atom in the tweezer with a fidelity of 0.989(6) (and loss of 0.13(5)) within a 200 $μ$s imaging time. Adding continuous narrow-line Sisyphus cooling yields similar fidelity, at the expense of much longer imaging times (30 ms). Under these conditions we determine whether the tweezer contains zero, one or two atoms, with a fidelity $>$0.8 in all cases with the high readout speed of the camera enabling real-time monitoring of the number of trapped atoms. Lastly we show that the fidelity can be further improved by using a pulsed cooling/imaging scheme that reduces the effect of camera dark noise.
We perform a comprehensive investigation of the coupling between a Rydberg-dressed atomic gas and an ultra-cold plasma. Using simultaneous time-resolved measurements of both neutral atoms and ions, we show that plasma formation occurs via a Coulomb anti-blockade mechanism, in which background ions DC Stark shift nearby atoms into resonance at specific distances. The result is a highly correlated growth of the Rydberg population that shares some similarities with that previously observed for van der Waals interactions. We show that a rate equation model that couples the laser-driven Rydberg gas to the ultra-cold plasma via a Coulomb anti-blockade mechanism accurately reproduces both the plasma formation and its subsequent decay. Using long-lived high angular momentum states as a probe, we also find evidence of a crossover from Coulomb anti-blockade to Coulomb blockade at high density. As well as shedding light on loss mechanisms in Rydberg-dressed gases, our results open new ways to create low-entropy states in ultra-cold plasmas.
We propose and demonstrate the laser cooling and trapping of Rydberg-dressed Sr atoms. By off-resonantly coupling the excited state of a narrow (7 kHz) cooling transition to a high-lying Rydberg state, we transfer Rydberg properties such as enhanced electric polarizability to a stable magneto-optical trap operating at $< 1 μK$. By increasing the density to $1 \times 10^{12} \rm{cm^{-3}}$, we show that it is possible to reach a regime where the long-range interaction between Rydberg-dressed atoms becomes comparable to the kinetic energy, opening a route to combining laser cooling with tunable long-range interactions.
Cold atomic gases resonantly excited to Rydberg states can exhibit strong optical nonlinearity at the single photon level. We observe that in such samples radiation trapping leads to an additional mechanism for Rydberg excitation. Conversely we demonstrate that Rydberg excitation provides a novel in situ probe of the spectral, statistical, temporal and spatial properties of the trapped re-scattered light. We also show that absorption can lead to an excitation saturation that mimics the Rydberg blockade effect. Collective effects due to multiple scattering may co-exist with co-operative effects due to long-range interactions between the Rydberg atoms, adding a new dimension to quantum optics experiments with cold Rydberg gases.
We investigate the effect of intercombination transitions in excitation hopping processes such as those found in Förster resonance energy transfer. Taking strontium Rydberg states as our model system, the breakdown of $LS$-coupling leads to weakly allowed transitions between Rydberg states of different spin quantum number. We show that the long-range interactions between two Rydberg atoms can be affected by these weakly allowed spin transitions, and the effect is greatest when there is a near-degeneracy between the initial state and a state with a different spin quantum number. We also consider a case of four atoms in a spin chain, and show that a spin impurity can resonantly hop along the chain. By engineering the many-body energy levels of the spin-chain, the breakdown of $LS$ coupling due to inter-electronic effects in individual atoms can be mapped onto a spatial separation of the total spin and the total orbital angular momentum along the spin chain.
A microwave field is used to control the interaction between pairs of optical photons stored in highly excited collective states (Rydberg polaritons). We show that strong dipole-dipole interactions induced by the microwave field destroy the coherence of polariton modes with more than one Rydberg excitation. Consequently single-polariton modes, which correspond to single stored photons, are preferentially retrieved from the sample. Measurements of the photon statistics of the retrieved light field also reveal non-trivial propagation dynamics of the interacting polaritons.
Squeezed many-body states of atoms are a valuable resource for high precision frequency metrology and could tremendously boost the performance of atomic lattice clocks. Here, we theoretically demonstrate a viable approach to spin squeezing in lattice clocks via optical dressing of one clock state to a highly excited Rydberg state, generating switchable atomic interactions. For realistic experimental parameters, this is shown to generate over 10 dB of squeezing in a few microseconds interaction time without affecting the subsequent clock interrogation.
We use a microwave field to control the quantum state of optical photons stored in a cold atomic cloud. The photons are stored in highly excited collective states (Rydberg polaritons) enabling both fast qubit rotations and control of photon-photon interactions. Through the collective read-out of these pseudo-spin rotations it is shown that the microwave field modifies the long-range interactions between polaritons. This technique provides a powerful interface between the microwave and optical domains, with applications in quantum simulations of spin liquids, quantum metrology and quantum networks.
We report on a scanning microscopy technique for atom-number-resolved imaging of excited-state atoms. A tightly focused laser beam leads to local autoionization, and the resulting ions are counted electronically. Scanning the beam across the cloud builds up an image of the density distribution of excited atoms, with access to the full counting statistics at each spatial sampling point and an overall detection efficiency of 21 %. We apply this technique to the measurement of a spatially inhomogeneous electric field with a spatial resolution of 50 ?m and a sensitivity to electric field gradients of 0.04 V cm$^{-2}$.
Long-range dipole-dipole and quadrupole-quadrupole interactions between pairs of Rydberg atoms are calculated perturbatively for calcium, strontium and ytterbium within the Coulomb approximation. Quantum defects, obtained by fitting existing laser spectroscopic data, are provided for all $S$, $P$, $D$ and $F$ series of strontium and for the $^3P_2$ series of calcium. The results show qualitative differences with the alkali metal atoms, including isotropically attractive interactions of the strontium $^1S_0$ states and a greater rarity of Förster resonances. Only two such resonances are identified, both in triplet series of strontium. The angular dependence of the long range interaction is briefly discussed.
We explore the prospects for confining alkaline-earth Rydberg atoms in an optical lattice via optical dressing of the secondary core valence electron. Focussing on the particular case of strontium, we identify experimentally accessible magic wavelengths for simultaneous trapping of ground and Rydberg states. A detailed analysis of relevant loss mechanisms shows that the overall lifetime of such a system is limited only by the spontaneous decay of the Rydberg state, and is not significantly affected by photoionization or autoionization. The van der Waals C_6 coefficients for the 5sns series are calculated, and we find that the interactions are attractive. Finally we show that the combination of magic-wavelength lattices and attractive interactions could be exploited to generate many-body Greenberger-Horne-Zeilinger (GHZ) states.
We present a study of a cold strontium Rydberg gas. The narrowband laser excitation of Rydberg states in the range n=20-80 from a 6~mK cloud of strontium atoms is detected using the spontaneous ionization of the Rydberg atoms. Using a high-resolution step-scanning technique, we perform detailed measurements of the Stark maps of selected Rydberg states. We find excellent agreement between the measured Stark maps and a numerical calculation based on an independent-electron model. Finally we show that excitation of the second valence electron can be used to probe the dynamics of the Rydberg gas with nanosecond temporal resolution via autoionization.
We report the creation of an interacting cold Rydberg gas of strontium atoms. We show that the excitation spectrum of the inner valence electron is sensitive to the interactions in the Rydberg gas, even though they are mediated by the outer Rydberg electron. By studying the evolution of this spectrum we observe density-dependent population transfer to a state of higher angular momentum l. We determine the fraction of Rydberg atoms transferred, and identify the dominant transfer mechanism to be l-changing electron-Rydberg collisions associated with the formation of a cold plasma.
We consider a two-component Bose-Einstein condensate (BEC) in a ring trap in a rotating frame, and show how to determine the response of such a configuration to being in a rotating frame, via accumulation of a Sagnac phase. This may be accomplished either through population oscillations, or the motion of spatial density fringes. We explicitly include the effect of interactions via a mean-field description, and study the fidelity of the dynamics relative to an ideal configuration.
We demonstrate a cooperative optical non-linearity caused by dipolar interactions between Rydberg atoms in an ultra-cold atomic ensemble. By coupling a probe transition to the Rydberg state we map the strong dipole-dipole interactions between Rydberg pairs onto the optical field. We characterize the non-linearity as a function of electric field and density, and demonstrate the enhancement of the optical non-linearity due to cooperativity.
We have performed polarization spectroscopy and sub-Doppler DAVLL on the (5s5s) 1^S_0 -> (5s5p) 1^P_1 transition of atomic strontium. Both techniques generated a dispersion-type lineshape suitable for laser stabilization, without the need for frequency modulation. In both cases the signal is generated primarily by saturation effects, rather than optical pumping. The dependence of the amplitude and gradient on intensity and magnetic field were also investigated.