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M. P. Adams

Publications and source records attributed to M. P. Adams.

4 recordsLinked to original sources

Reduced vortex descriptors linking polycrystallinity in magnetic nanoparticles with polarized magnetic small-angle neutron scattering

Analytical vortex models reduce polarized magnetic small-angle neutron scattering (SANS) from nanoparticle ensembles to a small set of texture descriptors. In this work, we apply this reduction to micromagnetic simulations of polycrystalline iron oxide nanoflowers at a fixed particle size and examine how a controlled parametrization of multigrain disorder is reflected in the remanent descriptors. The particles are represented by explicit Voronoi microstructures, and intraparticle disorder is varied through the intergrain exchange coupling and anisotropy-axis coherence. Fitting each remanent magnetization state to a hyperbolic vortex model reveals a predominantly two-channel organization: the intergrain exchange coupling is associated mainly with the radial vortex profile, whereas the anisotropy-axis coherence is associated mainly with the orientational moment of the vortex-axis distribution. The normalized spin-flip SANS cross sections are accurately represented by independent fits of the analytical linear-vortex SANS expression obtained from the first-order expansion of the hyperbolic profile. The fitted orientational descriptor agrees closely with its independent real-space estimate, whereas the corresponding radial descriptors exhibit a strong global nonlinear relation. This separation identifies which information from the micromagnetic vortex textures is robustly retained by the reduced analytical representation.

cond-mat.mes-hall

Spin-disorder-induced angular anisotropy in polarized magnetic neutron scattering

We experimentally report a hitherto unseen angular anisotropy in the polarized small-angle neutron scattering (SANS) cross section of a magnetically strongly inhomogeneous material. Based on an analytical prediction using micromagnetic theory, the difference between the spin-up and spin-down SANS cross sections is expected to show a spin-disorder-induced anisotropy. The effect is particularly pronounced in inhomogeneous magnetic materials, such as nanoporous ferromagnets, magnetic nanocomposites, or steels, which exhibit large nanoscale jumps in the saturation magnetization at internal pore-matrix or particle-matrix interfaces. Analysis of the experimental neutron data constitutes a method for determining the exchange-stiffness constant. Our results are generic to the nuclear-magnetic interference terms contained in the polarized magnetic neutron scattering cross section and might also be of relevance to other neutron techniques.

cond-mat.mes-hall

Low-frequency signature of magnetization nutation in nanomagnets

In this work, we show that surface anisotropy in nanomagnets induces a nutational motion of their magnetization at various frequencies, the lowest of which can be described by the macrospin model whose dynamics is governed by an effective energy potential. We derive analytical expressions for the precession and nutation frequencies and amplitudes as functions of the size of the nanomagnet and its atomistic parameters, such as the exchange coupling and the onsite anisotropy. Our analytical model predicts a reduction of the precession frequency with increased surface anisotropy. We also simulate the dynamics of the corresponding atomistic many-spin system and compare the results with the effective model. We thereby show that the first nutation mode induced by the finite size and surface anisotropy occurs at a frequency that is four times larger than the precession frequency, thus lending itself to a relatively easy detection by standard experiments of magnetic resonance.

cond-mat.mes-hall

Spatial magnetization profile in spherical nanomagnets with surface anisotropy: Green's function approach

We consider a single spherical nanomagnet and investigate the spatial magnetization profile $\mathbf{m}\left(\mathbf{r}\right)$ in the continuum approach, using the Green's function formalism. The energy of the (many-spin) nanomagnet comprises an isotropic exchange interaction, a uniaxial anisotropy in the core and Néel's surface anisotropy, and an external magnetic field. We derive a semi-analytical expression for the magnetization vector field $\mathbf{m}\left(\mathbf{r}\right)$ for an arbitrary position $\mathbf{r}$ within and on the boundary of the nanomagnet, as a solution of a homogeneous Helmholtz equation with inhomogeneous Neumann boundary conditions. ... For a more plausible comparison with experiments, e.g. using the technique of small-angle magnetic neutron scattering, we have averaged over the direction solid angle and derived the spatial profile in terms of the distance $r$. We believe that the predictions of the present study could help to characterize and understand the effects of size and surface anisotropy on the magnetization configurations in nanomagnet assemblies such as arrays of well-spaced platelets.

cond-mat.mes-hall