arXiv subjects

M. Passoni

Publications and source records attributed to M. Passoni.

14 recordsLinked to original sources

arXiv2025

Tungsten erosion and scrape-off layer transport modelling in L-mode helium plasma discharges in ASDEX Upgrade

Due to its unavoidable presence in thermonuclear DT plasmas and to its peculiar effects on materials, investigating the role of helium (He) in plasma-wall interaction (PWI) in current tokamaks is fundamental. In this work, PWI in L-mode He plasma discharges in ASDEX Upgrade (AUG) is modelled by exploiting simplified analytical approaches and two state-of-the-art codes. SOLPS-ITER is employed both to provide a suitable background plasma for erosion simulations and to interpret diagnostics measurements in terms of He+/2+ fraction. In particular, a 50-50% concentration of the two He ions is found in the proximity of the strike-points, while He2+ represents the dominant population farther in the scrape-off layer (SOL). The role of He ion fraction on AUG tungsten divertor erosion is first estimated by means of a simple analytical model and, afterwards, by exploiting ERO2.0, showing the major impact of He2+ in common AUG plasma temperatures. ERO2.0 findings are also compared with experimental erosion data in the strike-point region, showing the possible impact of extrinsic impurities on divertor erosion. Finally, the multi-fluid and kinetic approaches employed in this work to simulate W erosion and migration are compared, including W also in SOLPS-ITER modelling. The impact of target boundary conditions on the W source in SOLPS-ITER is investigated, in order to find a good agreement with ERO2.0 estimation. Then, W migration in the two codes is compared, showing a stronger W transport towards the X-point in ERO2.0 compared to present SOLPS-ITER simulations with no drifts. Similar W influx in core could be achieved by reducing anomalous diffusivity in ERO2.0.

physics.plasm-ph↗

arXiv2024

Numerical simulation of a helium Plasma-Material Interaction experiment in GyM linear device through SOLPS-ITER and ERO2.0 codes

Learning how to safely handle Plasma-Material Interaction (PMI) is a key challenge towards the commercialisation of energy from nuclear fusion. In this respect, linear plasma devices are ideal experimental testbeds, and numerical codes play a crucial complementary role. In this paper, a numerical investigation of PMI-relevant helium plasma experimental discharges in GyM linear device is presented, in which SOLPS-ITER and ERO2.0 codes are coupled for plasma background generation and material erosion investigation respectively, with the aim to support the interpretation and complement the available experimental dataset. On the plasma side, simulated profiles are validated against experimental data to provide a realistic plasma background, and the role of He metastable states is assessed for the first time in SOLPS simulations. On the material side, the erosion and deposition effects due to the introduction of the sample-holder in the simulation volume are investigated, now considering also the real stainless steel composition as wall material.

physics.plasm-ph↗

arXiv2024

Modelling of power exhaust in TCV positive and negative triangularity L-mode plasmas

L-mode negative triangularity (NT) operation is a promising alternative to the positive triangularity (PT) H-mode as a high-confinement ELM-free operational regime. In this work, two TCV L-mode lower single null Ohmic discharges with opposite triangularity $\delta \simeq \pm 0.3$ are investigated using SOLPS-ITER modelling. The main focus is the exploration of the reasons behind the experimentally observed feature of NT plasmas being more difficult to detach than similar PT experiments. SOLPS-ITER simulations are performed assuming the same anomalous diffusivity for particles $D_n^{AN}$ and energy $\kappa_{e/i}^{AN}$ in PT and NT. Nonetheless, the results clearly show dissimilar transport and accumulation of neutral particles in the scrape-off layer (SOL) of the two configurations, which consequently gives rise to different ionization sources for the plasma and produces different poloidal and cross-field fluxes. Simulations also recover the experimental feature of the outer target being hotter in the NT scenario (with $T_{e, NT} \gtrsim 5 \, \mathrm{eV}$) than in the PT counterpart.

physics.plasm-ph↗

arXiv2020

Integrated quantitative PIXE analysis and EDX spectroscopy using a laser-driven particle source

Among the existing elemental characterization techniques, Particle Induced X-ray Emission (PIXE) and Energy Dispersive X-ray (EDX) spectroscopy are two of the most widely used in different scientific and technological fields. Here we present the first quantitative laser-driven PIXE and laser-driven EDX experimental investigation performed at the Centro de L\'aseres Pulsados in Salamanca. Thanks to their potential for compactness and portability, laser-driven particle sources are very appealing for materials science applications, especially for materials analysis techniques. We demonstrate the possibility to exploit the X-ray signal produced by the co-irradiation with both electrons and protons to identify the elements in the sample. We show that, using the proton beam only, we can successfully obtain quantitative information about the sample structure through laser-driven PIXE analysis. These results pave the way towards the development of a compact and multi-functional apparatus for the elemental analysis of materials based on a laser-driven particle source.

physics.plasm-ph↗

arXiv2018

Helium load on W-O coatings grown by pulsed laser deposition

W-O deposits with complex morphologies and significant He contents will growth on the surface of plasma facing components exposed to He discharges. To mimic the re/co-deposition process, W-O-He coatings were produced by implanting He+ ions on W films grown by pulsed laser deposition (PLD). The use of appropriate PLD experimental parameters such as Ar or He background atmospheres induces the deposition of porous or amorphous-like W-O structures, respectively. After multiple ion implantation stages using 150 keV, 100 keV and 50 keV incident He+ ion beams with a total fluence of 5 x 1017 ion/cm^2, significant amounts of He were identified in porous coatings by Rutherford backscattering (RBS). Time-of-flight elastic recoil detection (TOF-ERDA) measurements showed that most of the implanted He was already released from the porous coatings five month after implantation while for the case of amorphous ones the He content remains significant at deeper layers and smoothly decrease towards the surface, as result of a different morphology and nanostructure. The proposed method involving PLD and ion implantation seems adequate to produce W-O-He reference samples for fusion investigations.

physics.app-ph↗

arXiv2018

Tunable out-of-plane excitons in 2D single crystal perovskites

Hybrid organic-inorganic perovskites have emerged as very promising materials for photonic applications, thanks to the great synthetic versatility that allows to tune their optical properties. In the two-dimensional (2D) crystalline form, these materials behave as multiple quantum-well heterostructures with stable excitonic resonances up to room temperature. In this work strong light-matter coupling in 2D perovskite single-crystal flakes is observed, and the polarization-dependent exciton-polariton response is used to disclose new excitonic features. For the first time, an out-of-plane component of the excitons is observed, unexpected for such 2D systems and completely absent in other layered materials, such as transition-metal dichalcogenides. By comparing different hybrid perovskites with the same inorganic layer but different organic interlayers, it is shown how the nature of the organic ligands controllably affects the out-of-plane exciton-photon coupling. Such vertical dipole coupling is particularly sought in those systems, e.g. plasmonic nanocavities, in which the direction of the field is usually orthogonal to the material sheet. Organic interlayers are shown to affect also the strong birefringence associated to the layered structure, which is exploited in this work to completely rotate the linear polarization degree in only few microns of propagation, akin to what happens in metamaterials.

cond-mat.mes-hall↗

arXiv2017

Coefficient of thermal expansion of nanostructured tungsten based coatings assessed by thermally induced substrate curvature method

The in plane coefficient of thermal expansion (CTE) and the residual stress of nanostructured W based coatings are extensively investigated. The CTE and the residual stresses are derived by means of an optimized ad-hoc developed experimental setup based on the detection of the substrate curvature by a laser system. The nanostructured coatings are deposited by Pulsed Laser Deposition. Thanks to its versatility, nanocrystalline W metallic coatings, ultra-nano-crystalline pure W and W-Tantalum coatings and amorphous-like W coatings are obtained. The correlation between the nanostructure, the residual stress and the CTE of the coatings are thus elucidated. We find that all the samples show a compressive state of stress that decreases as the structure goes from columnar nanocrystalline to amorphous-like. The CTE of all the coatings is higher than the one of the corresponding bulk W form. In particular, as the grain size shrinks, the CTE increases from 5.1 10$^{-6}$ K$^{-1}$ for nanocrystalline W to 6.6 10$^{-6}$ K$^{-1}$ in the ultra-nano-crystalline region. When dealing with amorphous W, the further increase of the CTE is attributed to a higher porosity degree of the samples. The CTE trend is also investigated as function of materials stiffness. In this case, as W coatings become softer, the easier they thermally expand.

cond-mat.mtrl-sci↗

arXiv2017

Amorphous, ultra-nano- and nano-crystalline tungsten-based coatings grown by Pulsed Laser Deposition: mechanical characterization by Surface Brillouin Spectroscopy

Pulsed Laser Deposition allows to obtain W and W-Ta alloy coatings with different nanostructures, monitored by X-ray diffraction. The correlation between such structures and the elastic properties is investigated for amorphous-like, ultra-nano- and nano-crystalline coatings obtained by tuning the gas pressure during deposition, annealing temperature and Ta concentration. The full elastic characterization is achieved by surface Brillouin spectroscopy, interpreted by isotropic and anisotropic film models. Amorphous like coatings are obtained with He pressures of tens of Pa. In comparison with bulk W, they have lower stiffness, by about 60\%, closely correlated to the mass density (lower by about 40\%). In the nanocrystalline regime the stiffness is more correlated to the average grain size, approaching the bulk values for increasing crystallite size. Vacuum annealing of amorphous like coatings leads to the nucleation of ultra-nano crystalline seeds, embedded in an amorphous matrix with intermediate values for mass density and stiffness. Here, the stiffness results from an interplay between the crystal size and the density. Alloying with Ta leads to properties which are consistent with the lever rule in the nanocrystalline regime, and deviate from it when the higher Ta concentration, interfering with crystal growth, induces an ultra-nano crystalline structure.

cond-mat.mtrl-sci↗

arXiv2015

Two-dimensional TiOx nanostructures on Au(111): a Scanning Tunneling Microscopy and Spectroscopy investigation

We investigated the growth of titanium oxide two-dimensional (2D) nanostructures on Au(111), produced by Ti evaporation and post-deposition oxidation. Scanning tunneling microscopy and spectroscopy (STM and STS) and low-energy electron diffraction (LEED) measurements characterized the morphological, structural and electronic properties of the observed structures. Five distinct TiO\sub{x} phases were identified: the \emph{honeycomb} and \emph{pinwheel} phases appear as monolayer films wetting the gold surface, while nanocrystallites of the \emph{triangular}, \emph{row} and \emph{needle} phases grow mainly over the honeycomb or pinwheel layers. Density Functional Theory (DFT) investigation of the honeycomb structure supports a $(2\times 2)$ structural model based on a Ti-O bilayer having $\text{Ti}_2\text{O}_3$ stoichiometry. The pinwheel phase was observed to evolve, for increasing coverage, from single triangular crystallites to a well-ordered film forming a $(4\sqrt{7}\times 4\sqrt{7})R19.1^\circ$ superstructure, which can be interpreted within a moir\~A\c{opyright}-like model. Structural characteristics of the other three phases were disclosed from the analysis of high-resolution STM measurements. STS measurements revealed a partial metallization of honeycomb and pinwheel and a semiconducting character of row and triangular phases.

cond-mat.mtrl-sci↗

arXiv2013

Evidence of resonant surface wave excitation in the relativistic regime through measurements of proton acceleration from grating targets

The interaction of laser pulses with thin grating targets, having a periodic groove at the irradiated surface, has been experimentally investigated. Ultrahigh contrast ($\sim 10^{12}$) pulses allowed to demonstrate an enhanced laser-target coupling for the first time in the relativistic regime of ultra-high intensity $>10^{19} \mbox{W/cm}^{2}$. A maximum increase by a factor of 2.5 of the cut-off energy of protons produced by Target Normal Sheath Acceleration has been observed with respect to plane targets, around the incidence angle expected for resonant excitation of surface waves. A significant enhancement is also observed for small angles of incidence, out of resonance.

physics.plasm-ph↗

arXiv2013

Advanced strategies for ion acceleration using high power lasers

A short overview of laser-plasma acceleration of ions is presented. The focus is on some recent experimental results and related theoretical work on advanced regimes. These latter include in particular target normal sheath acceleration using ultrashort low-energy pulses and structured targets, radiation pressure acceleration of both thick and ultrathin targets, and collisionless shock acceleration in moderate density plasmas. For each approach, open issues and the need and potential for further developments are briefly discussed.

physics.plasm-ph↗

arXiv2009

Direct observation of the basic mechanisms of Pd island nucleation on Au(111)

The formation mechanisms of evaporated Pd islands on the reconstructed Au(111) $22 /times /sqrt{3}$ herringbone surface have been here studied by Scanning Tunneling Microscopy (STM) at room temperature. Atomically resolved STM images at the very early stages of growth provide a direct observation of the mechanisms involved in preferential Pd islands nucleation at the elbows of the herringbone structure. At low Pd coverage the Au(111) herringbone structure remains substantially unperturbed and isolated Pd atoms settled in hollow sites between Au atoms are found nearby the elbows and the distortions of the reconstructed surface. In the same regions, at extremely low coverage (0.003 ML), substituted Pd atoms in lattice sites of the Au(111) surface are also observed, revealing the occurrence of a place exchange mechanism. Substitution seems to play a fundamental role in the nucleation process, forming aggregation centers for incoming atoms and thus leading to the ordered growth of Pd islands on Au(111). Atomically resolved STM images of Pd islands reveal a close-packed arrangement with lattice parameter close to the interatomic distance between gold atoms in the fcc regions of the Au(111) surface. Distortion of the herringbone structure for Pd coverages higher than 0.25 ML indicates strong interaction between the growing islands and the topmost Au(111) layer.

cond-mat.mtrl-sci↗

arXiv2007

Bulk Cr tips for scanning tunneling microscopy and spin-polarized scanning tunneling microscopy

A simple, reliable method for preparation of bulk Cr tips for Scanning Tunneling Microscopy (STM) is proposed and its potentialities in performing high-quality and high-resolution STM and Spin Polarized-STM (SP-STM) are investigated. Cr tips show atomic resolution on ordered surfaces. Contrary to what happens with conventional W tips, rest atoms of the Si(111)-7x7 reconstruction can be routinely observed, probably due to a different electronic structure of the tip apex. SP-STM measurements of the Cr(001) surface showing magnetic contrast are reported. Our results reveal that the peculiar properties of these tips can be suited in a number of STM experimental situations.

cond-mat.mtrl-sci↗

arXiv2007

Different W cluster deposition regimes in pulsed laser ablation observed by in situ Scanning Tunneling Microscopy

We report on how different cluster deposition regimes can be obtained and observed by in situ Scanning Tunneling Microscopy (STM) by exploiting deposition parameters in a pulsed laser deposition (PLD) process. Tungsten clusters were produced by nanosecond Pulsed Laser Ablation in Ar atmosphere at different pressures and deposited on Au(111) and HOPG surfaces. Deposition regimes including cluster deposition-diffusion-aggregation (DDA), cluster melting and coalescence and cluster implantation were observed, depending on background gas pressure and target-to-substrate distance which influence the kinetic energy of the ablated species. These parameters can thus be easily employed for surface modification by cluster bombardment, deposition of supported clusters and growth of films with different morphologies. The variation in cluster mobility on different substrates and its influence on aggregation and growth mechanisms has also been investigated.

cond-mat.mtrl-sci↗