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M. Patra

Publications and source records attributed to M. Patra.

18 recordsLinked to original sources

Glassy magnetic phase driven by short range charge and magnetic ordering in nanocrystalline La$_{1/3}$Sr$_{2/3}$FeO$_{3-δ}$: Magnetization, Mossbauer, and polarised neutron studies

The charge ordered La$_{1/3}$Sr$_{2/3}$FeO$_{3-δ}$ (LSFO) in bulk and nanocrystalline forms are investigated using ac and dc magnetization, Mössbauer, and polarised neutron studies. A complex scenario of short range charge and magnetic ordering is realized from the polarised neutron studies in nanocrystalline specimen. This short range ordering does not involve any change in spin state and modification in the charge disproportion between Fe$^{3+}$ and Fe$^{5+}$ compared to bulk counterpart as evident in the Mössbauer results. The refinement of magnetic diffraction peaks provides magnetic moments of Fe$^{3+}$ and Fe$^{5+}$ are about 3.15$μ_B$ and 1.57$μ_B$ for bulk, and 2.7$μ_B$ and 0.53$μ_B$ for nanocrystalline specimen, respectively. The destabilization of charge ordering leads to magnetic phase separation, giving rise to the robust exchange bias (EB) effect. Strikingly, EB field at 5 K attains a value as high as 4.4 kOe for average size $\sim$ 70 nm, which is zero for the bulk counterpart. A strong frequency dependence of ac susceptibility reveals cluster-glass like transition around $\sim$ 65 K, below which EB appears. Overall results propose that finite size effect directs the complex glassy magnetic behavior driven by unconventional short range charge and magnetic ordering, and magnetic phase separation appears in nanocrystalline LSFO.

cond-mat.mtrl-sci

Magnetic and magnetoresistive properties of cubic Laves phase HoAl$_2$ single crystal

We report the magnetization ($M$) and magnetoresistance (MR) results of HoAl$_2$ single crystals oriented along $<100>$ and $<110>$ directions. Although HoAl$_2$ has cubic Laves phase structure, a large anisotropy is observed in $M$ and MR results below Curie temperature ($T_C$) at 31.5 K. A satisfactory correlation between magnetic entropy change ($ΔS_M$) and MR could be established along $<110>$ direction and in $<100>$ direction except for the temperature ($T$) region, around which spin reorientation takes place. Large inverse magnetocaloric effect is observed at low-$T$ which is associated with the spin reorientation process in $<100>$ direction. A theoretical model based on Landau theory of phase transition can describe $T$-variation of -$ΔS_M$ for $T > T_C$.

cond-mat.mtrl-sci

Exchange bias effect and intragranular magnetoresistance in Nd$_{0.84}Sr_{0.16}CoO_3

Electrical transport properties as a function of magnetic field and time have been investigated in polycrystalline, Nd_{0.84}Sr_{0.16}CoO_3. A strong exchange bias (EB) effect is observed associated with the fairly large intragranular magnetoresistance (MR). The EB effect observed in the MR curve is compared with the EB effect manifested in magnetic hysteresis loop. Training effect, described as the decrease of EB effect when the sample is successively field-cycled at a particular temperature, has been observed in the shift of the MR curve. Training effect could be analysed by the successful models. The EB effect, MR and a considerable time dependence in MR are attributed to the intrinsic nanostructure giving rise to the varieties of magnetic interfaces in the grain interior.

cond-mat.str-el

Exchange bias effect involved with tunneling magnetoresistance in polycrystalline La_{0.88}Sr_{0.12}CoO_3

We report the exchange bias (EB) effect along with tunneling magnetoresistance (MR) in polycrystalline La_{0.88}Sr_{0.12}CoO_3. Analogous to the shift in the magnetic hysteresis loop along the field (H)-axis a shift is clearly observed in the MR-H curve when the sample is cooled in a static magnetic field. Training effect (TE) is a significant manifestation of EB effect which describes the decrease of EB effect when sample is successively field-cycled at a particular temperature. We observe TE in the shift of the MR-H curve which could be interpreted by the spin configurational relaxation model. A strong field-cooled (FC) effect in the temperature as well as time dependence of resistivity is observed below spin freezing temperature. The unusual MR results measured in FC mode are interpreted in terms of intragranular interface effect between short range ferromagnetic clusters and spin-glass matrix giving rise to the EB effect. EB effect in MR has been observed in bilayer or multilayer films which has not yet seen in a polycrystalline compound. EB effect involved with tunneling MR and semiconducting transport property attributed to the intragranular intrinsic nanostructure is promising for the spintronic applications.

cond-mat.str-el

Exchange bias effect in the phase separated Nd_{1-x}Sr_{x}CoO_3 at the spontaneous ferromagnetic/ferrimagnetic interface

We report the new results of exchange bias effect in Nd_{1-x}Sr_{x}CoO_3 for x = 0.20 and 0.40, where the exchange bias phenomenon is involved with the ferrimagnetic (FI) state in a spontaneously phase separated system. The zero-field cooled magnetization exhibits the FI (T_{FI}) and ferromagnetic (T_C) transitions at ~ 23 and \sim 70 K, respectively for x = 0.20. The negative horizontal and positive vertical shifts of the magnetic hysteresis loops are observed when the system is cooled through T_{FI} in presence of a positive static magnetic field. Training effect is observed for x = 0.20, which could be interpreted by a spin configurational relaxation model. The unidirectional shifts of the hysteresis loops as a function of temperature exhibit the absence of exchange bias above T_{FI} for x = 0.20. The analysis of the cooling field dependence of exchange bias field and magnetization indicates that the ferromagnetic (FM) clusters consist of single magnetic domain with average size around \sim 20 and ~ 40 Å~ for x = 0.20 and 0.40, respectively. The sizes of the FM clusters are close to the percolation threshold for x = 0.20, which grow and coalesce to form the bigger size for x = 0.40 resulting in a weak exchange bias effect.

cond-mat.str-el

Exchange bias with Fe substitution in LaMnO_3

The exchange bias (EB) in LaMn_{0.7}Fe_{0.3}O_3 is observed by the negative shift and training effect of the hysteresis loops, while the sample was cooled in external magnetic field. The analysis of cooling field dependence of EB gives the size of the ferromagnetic (FM) cluster ~ 25 Angstrom, where the magnetic anisotropy of FM cluster is found two order of magnitude higher than the FM bulk manganites. We propose that the nanoscale FM clusters are embedded in the glassy magnetic host with EB at the FM/glassy magnetic interface.

cond-mat.str-el

Molecular Dynamics Simulations of Lipid Bilayers: Major Artifacts due to Truncating Electrostatic Interactions

We study the influence of truncating the electrostatic interactions in a fully hydrated pure dipalmitoylphosphatidylcholine (DPPC) bilayer through 20 ns molecular dynamics simulations. The computations in which the electrostatic interactions were truncated are compared to similar simulations using the Particle-Mesh Ewald (PME) technique. All examined truncation distances (1.8 to 2.5 nm) lead to major effects on the bilayer properties, such as enhanced order of acyl chains together with decreased areas per lipid. The results obtained using PME, on the other hand, are consistent with experiments. These artifacts are interpreted in terms of radial distribution functions $g(r)$ of molecules and molecular groups in the bilayer plane. Pronounced maxima or minima in g(r) appear exactly at the cutoff distance indicating that the truncation gives rise to artificial ordering between the polar phosphatidyl and choline groups of the DPPC molecules. In systems described using PME, such artificial ordering is not present.

cond-mat.soft

Decay Rate Distributions of Disordered Slabs and Application to Random Lasers

We compute the distribution of the decay rates (also referred to as residues) of the eigenstates of a disordered slab from a numerical model. From the results of the numerical simulations, we are able to find simple analytical formulae that describe those results well. This is possible for samples both in the diffusive and in the localised regime. As example of a possible application, we investigate the lasing threshold of random lasers.

cond-mat.mes-hall

Theory for the photon statistics of random lasers

A theory for the photon statistics of a random laser is presented. Noise is described by Langevin operators, where both fluctuations of the electromagnetic field and of the medium are included. The theory is valid for all lasers with small outcoupling when the laser cavity is large compared to the wavelength of the radiation. The theory is applied to a chaotic laser cavity with a small opening. It is known that a large number of modes can be above threshold simultaneously in such a cavity. It is shown the amount of fluctuations is increased compared to the Poissonian value by an amount that depends on that number.

quant-ph

Frequency dependence of the photonic noise spectrum in an absorbing or amplifying diffusive medium

A theory is presented for the frequency dependence of the power spectrum of photon current fluctuations originating from a disordered medium. Both the cases of an absorbing medium (``grey body'') and of an amplifying medium (``random laser'') are considered in a waveguide geometry. The semiclassical approach (based on a Boltzmann-Langevin equation) is shown to be in complete agreement with a fully quantum mechanical theory, provided that the effects of wave localization can be neglected. The width of the peak in the power spectrum around zero frequency is much smaller than the inverse coherence time, characteristic for black-body radiation. Simple expressions for the shape of this peak are obtained, in the absorbing case, for waveguide lengths large compared to the absorption length, and, in the amplifying case, close to the laser threshold.

cond-mat.mes-hall

Photonic excess noise and wave localization

This is a theory for the effect of localization on the super-Poissonian noise of radiation propagating through an absorbing disordered waveguide. Localization suppresses both the mean photon current I and the noise power P, but the Fano factor P/I is found to remain unaffected. For strong absorption the Fano factor has the universal value 1+3f/2 (with f the Bose-Einstein function), regardless of whether the waveguide is long or short compared to the localization length.

cond-mat.dis-nn

Quantum limit of the laser linewidth in chaotic cavities and statistics of residues of scattering matrix poles

The quantum-limited linewidth of a laser cavity is enhanced above the Schawlow-Townes value by the Petermann factor K, due to the non-orthogonality of the cavity modes. We derive the relation between the Petermann factor and the residues of poles of the scattering matrix and investigate the statistical properties of the Petermann factor for cavities in which the radiation is scattered chaotically. For a single scattering channel we determine the complete probability distribution of K and find that the average Petermann factor $ $ depends non-analytically on the area of the opening, and greatly exceeds the most probable value. For an arbitrary number N of scattering channels we calculate $ $ as a function of the decay rate $Γ$ of the lasing mode. We find for $N\gg 1$ that for typical values of $Γ$ the average Petermann factor $ \propto \sqrt{N}\gg 1$ is parametrically larger than unity.

chao-dyn

Propagation of squeezed radiation through amplifying or absorbing random media

We analyse how nonclassical features of squeezed radiation (in particular the sub-Poissonian noise) are degraded when it is transmitted through an amplifying or absorbing medium with randomly located scattering centra. Both the cases of direct photodetection and of homodyne detection are considered. Explicit results are obtained for the dependence of the Fano factor (the ratio of the noise power and the mean current) on the degree of squeezing of the incident state, on the length and the mean free path of the medium, the temperature, and on the absorption or amplification rate.

quant-ph

Large Petermann factor in chaotic cavities with many scattering channels

The quantum-limited linewidth of a laser cavity is enhanced above the Schawlow-Townes value by the Petermann factor K, due to the non-orthogonality of the cavity modes. The average Petermann factor $ $ in an ensemble of cavities with chaotic scattering and broken time-reversal symmetry is calculated non-perturbatively using random-matrix theory and the supersymmetry technique, as a function of the decay rate $Γ$ of the lasing mode and the number of scattering channels N. We find for $N\gg 1$ that for typical values of $Γ$ the average Petermann factor $ \propto \sqrt{N}\gg 1$ is parametrically larger than unity.

chao-dyn

Photon shot noise

A recent theory is reviewed for the shot noise of coherent radiation propagating through a random medium. The Fano factor P/I (the ratio of the noise power and the mean transmitted current) is related to the scattering matrix of the medium. This is the optical analogue of Buttiker's formula for electronic shot noise. Scattering by itself has no effect on the Fano factor, which remains equal to 1 (as for a Poisson process). Absorption and amplification both increase the Fano factor above the Poisson value. For strong absorption P/I has the universal limit 1+3f/2 with f the Bose-Einstein function at the frequency of the incident radiation. This is the optical analogue of the one-third reduction factor of electronic shot noise in diffusive conductors. In the amplifying case the Fano factor diverges at the laser threshold, while the signal-to-noise ratio I^2/P reaches a finite, universal limit.

cond-mat.mes-hall

Quantum-limited linewidth of a chaotic laser cavity

A random-matrix theory is presented for the linewidth of a laser cavity in which the radiation is scattered chaotically. The linewidth is enhanced above the Schawlow-Townes value by the Petermann factor K, due to the non-orthogonality of the cavity modes. The factor K is expressed in terms of a non-Hermitian random matrix and its distribution is calculated exactly for the case that the cavity is coupled to the outside via a small opening. The average of K is found to depend non-analytically on the area of the opening, and to greatly exceed the most probable value.

chao-dyn

Excess noise for coherent radiation propagating through amplifying random media

A general theory is presented for the photodetection statistics of coherent radiation that has been amplified by a disordered medium. The beating of the coherent radiation with the spontaneous emission increases the noise above the shot-noise level. The excess noise is expressed in terms of the transmission and reflection matrices of the medium, and evaluated using the methods of random-matrix theory. Inter-mode scattering between $N$ propagating modes increases the noise figure by up to a factor of $N$, as one approaches the laser threshold. Results are contrasted with those for an absorbing medium.

quant-ph

Long-range correlation of thermal radiation

A general theory is presented for the spatial correlations in the intensity of the radiation emitted by a random medium in thermal equilibrium. We find that a non-zero correlation persists over distances large compared to the transverse coherence length of the thermal radiation. This long-range correlation vanishes in the limit of an ideal black body. We analyze two types of systems (a disordered waveguide and an optical cavity with chaotic scattering) where it should be observable.

quant-ph