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M. R. Mumpower

Publications and source records attributed to M. R. Mumpower.

52 records · Page 3Linked to original sources

$β$-Decay Half-Lives of 55 Neutron-Rich Isotopes beyond the N=82 Shell Gap

The $β$-decay half-lives of 55 neutron-rich nuclei $^{134-139}$Sn, $^{134-142}$Sb, $^{137-144}$Te, $^{140-146}$I, $^{142-148}$Xe, $^{145-151}$Cs, $^{148-153}$Ba, $^{151-155}$La were measured at the Radioactive Isotope Beam Factory (RIBF) employing the projectile fission fragments of $^{238}$U. The nuclear level structure, which relates to deformation, has a large effect on the half-lives. The impact of newly-measured half-lives on modeling the astrophysical origin of the heavy elements is studied in the context of $r$ process nucleosynthesis. For a wide variety of astrophysical conditions, including those in which fission recycling occurs, the half-lives have an important local impact on the second ($A$ $\approx$ 130) peak.

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First Exploration of Neutron Shell Structure Below Lead and Beyond $\boldsymbol{N=126}$

The nuclei below lead but with more than 126 neutrons are crucial to an understanding of the astrophysical $r$-process in producing nuclei heavier than $A\sim190$. Despite their importance, the structure and properties of these nuclei remain experimentally untested as they are difficult to produce in nuclear reactions with stable beams. In a first exploration of the shell structure of this region, neutron excitations in $^{207}$Hg have been probed using the neutron-adding ($d$,$p$) reaction in inverse kinematics. The radioactive beam of $^{206}$Hg was delivered to the new ISOLDE Solenoidal Spectrometer at an energy above the Coulomb barrier. The spectroscopy of $^{207}$Hg marks a first step in improving our understanding of the relevant structural properties of nuclei involved in a key part of the path of the $r$-process.

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Exploring the mass surface near the rare-earth abundance peak via precision mass measurements at JYFLTRAP

The JYFLTRAP double Penning trap at the Ion Guide Isotope Separator On-Line (IGISOL) facility has been used to measure the atomic masses of 13 neutron-rich rare-earth isotopes. Eight of the nuclides, $^{161}$Pm, $^{163}$Sm, $^{164,165}$Eu, $^{167}$Gd, and $^{165,167,168}$Tb, were measured for the first time. The systematics of the mass surface has been studied via one- and two-neutron separation energies as well as neutron pairing-gap and shell-gap energies. The proton-neutron pairing strength has also been investigated. The impact of the new mass values on the astrophysical rapid neutron capture process has been studied. The calculated abundance distribution results in a better agreement with the solar abundance pattern near the top of the rare-earth abundance peak at around $A\approx165$.

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Primary fission fragment mass yields across the chart of nuclides

We have calculated a complete set of primary fission fragment mass yields, $Y(A)$, for heavy nuclei across the chart of nuclides, including those of particular relevance to the rapid neutron capture process ($r$ process) of nucleosynthesis. We assume that the nuclear shape dynamics are strongly damped which allows for a description of the fission process via Brownian shape motion across nuclear potential-energy surfaces. The macroscopic energy of the potential was obtained with the Finite-Range Liquid-Drop Model (FRLDM), while the microscopic terms were extracted from the single-particle level spectra in the fissioning system by the Strutinsky procedure for the shell energies and the BCS treatment for the pairing energies. For each nucleus considered, the fission fragment mass yield, $Y(A)$, is obtained from 50,000 -- 500,000 random walks on the appropriate potential-energy surface. The full mass and charge yield, $Y(Z,A)$, is then calculated by invoking the Wahl systematics. With this method, we have calculated a comprehensive set of fission-fragment yields from over 3,800 nuclides bounded by $80\leq Z \leq 130$ and $A\leq330$; these yields are provided as an ASCII formatted database in the supplemental material. We compare our yields to known data and discuss general trends that emerge in low-energy fission yields across the chart of nuclides.

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Propagation of Statistical Uncertainties of Skyrme Mass Models to Simulations of $r$-Process Nucleosynthesis

Uncertainties in nuclear models have a major impact on simulations that aim at understanding the origin of heavy elements in the universe through the rapid neutron capture process ($r$ process) of nucleosynthesis. Within the framework of the nuclear density functional theory, we use results of Bayesian statistical analysis to propagate uncertainties in the parameters of energy density functionals to the predicted $r$-process abundance pattern, by way not only of the nuclear masses but also through the influence of the masses on $β$-decay and neutron capture rates. We additionally make the first identifications of specific parameters of Skyrme-like energy density functionals which are correlated with particular aspects of the $r$-process abundance pattern. While previous studies have explored the reduction in the abundance pattern uncertainties due to anticipated new measurements of neutron-rich nuclei, here we point out that an even larger reduction will occur when these new measurements are used to reduce the uncertainty of model predictions of masses, which are then propagated through to the abundance pattern. We make a quantitative prediction for how large this reduction will be.

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FRIB and the GW170817 Kilonova

In July 2018 an FRIB Theory Alliance program was held on the implications of GW170817 and its associated kilonova for r-process nucleosynthesis. Topics of discussion included the astrophysical and nuclear physics uncertainties in the interpretation of the GW170817 kilonova, what we can learn about the astrophysical site or sites of the r process from this event, and the advances in nuclear experiment and theory most crucial to pursue in light of the new data. Here we compile a selection of scientific contributions to the workshop, broadly representative of progress in r-process studies since the GW170817 event.

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Californium-254 and kilonova light curves

Neutron star mergers offer unique conditions for the creation of the heavy elements and additionally provide a testbed for our understanding of this synthesis known as the $r$-process. We have performed dynamical nucleosynthesis calculations and identified a single isotope, $^{254}$Cf, which has a particularly high impact on the brightness of electromagnetic transients associated with mergers on the order of 15 to 250 days. This is due to the anomalously long half-life of this isotope and the efficiency of fission thermalization compared to other nuclear channels. We estimate the fission fragment yield of this nucleus and outline the astrophysical conditions under which $^{254}$Cf has the greatest impact to the light curve. Future observations in the middle-IR which are bright during this regime could indicate the production of actinide nucleosynthesis.

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r-Process Nucleosynthesis: Connecting Rare-Isotope Beam Facilities with the Cosmos

This is an exciting time for the study of r-process nucleosynthesis. Recently, a neutron star merger GW170817 was observed in extraordinary detail with gravitational waves and electromagnetic radiation from radio to gamma rays. The very red color of the associated kilonova suggests that neutron star mergers are an important r-process site. Astrophysical simulations of neutron star mergers and core collapse supernovae are making rapid progress. Detection of both, electron neutrinos and antineutrinos from the next galactic supernova will constrain the composition of neutrino-driven winds and provide unique nucleosynthesis information. Finally FRIB and other rare-isotope beam facilities will soon have dramatic new capabilities to synthesize many neutron-rich nuclei that are involved in the r-process. The new capabilities can significantly improve our understanding of the r-process and likely resolve one of the main outstanding problems in classical nuclear astrophysics. However, to make best use of the new experimental capabilities and to fully interpret the results, a great deal of infrastructure is needed in many related areas of astrophysics, astronomy, and nuclear theory. We will place these experiments in context by discussing astrophysical simulations and observations of r-process sites, observations of stellar abundances, galactic chemical evolution, and nuclear theory for the structure and reactions of very neutron-rich nuclei. This review paper was initiated at a three-week International Collaborations in Nuclear Theory program in June 2016 where we explored promising r-process experiments and discussed their likely impact, and their astrophysical, astronomical, and nuclear theory context.

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Precision mass measurements on neutron-rich rare-earth isotopes at JYFLTRAP - reduced neutron pairing and implications for the $r$-process calculations

The rare-earth peak in the $r$-process abundance pattern depends sensitively on both the astrophysical conditions and subtle changes in nuclear structure in the region. This work takes an important step elucidating the nuclear structure and reducing the uncertainties in $r$-process calculations via precise atomic mass measurements at the JYFLTRAP double Penning trap. $^{158}$Nd, $^{160}$Pm, $^{162}$Sm, and $^{164-166}$Gd have been measured for the first time and the precisions for $^{156}$Nd, $^{158}$Pm, $^{162,163}$Eu, $^{163}$Gd, and $^{164}$Tb have been improved considerably. Nuclear structure has been probed via two-neutron separation energies $S_{2n}$ and neutron pairing energy metrics $D_n$. The data do not support the existence of a subshell closure at $N=100$. Neutron pairing has been found to be weaker than predicted by theoretical mass models. The impact on the calculated $r$-process abundances has been studied. Substantial changes resulting in a smoother abundance distribution and a better agreement with the solar $r$-process abundances are observed.

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$β$-delayed fission in $r$-process nucleosynthesis

We present $β$-delayed neutron emission and $β$-delayed fission calculations for heavy, neutron-rich nuclei using the coupled Quasi-Particle Random Phase Approximation plus Hauser-Feshbach (QRPA+HF) approach. From the initial population of a compound nucleus after $β$-decay, we follow the statistical decay taking into account competition between neutrons, $γ$-rays, and fission. We find a region of the chart of nuclides where the probability of $β$-delayed fission is $\sim100$%, that likely prevents the production of superheavy elements in nature. For a subset of nuclei near the neutron dripline, neutron multiplicity and the probability of fission are both large, leading to the intriguing possibility of multi-chance $β$-delayed fission, a new decay mode for extremely neutron-rich heavy nuclei. In this new decay mode, $β$-decay can be followed by multiple neutron emission leading to subsequent daughter generations which each have a probability to fission. We explore the impact of $β$-delayed fission in rapid neutron capture process ($r$-process) nucleosynthesis in the tidal ejecta of a neutron star--neutron star merger and show that it is a key fission channel that shapes the final abundances near the second $r$-process peak.

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Estimation of M1 scissors mode strength for deformed nuclei in the medium to heavy mass region by statistical Hauser-Feshbach model calculations

Radiative neutron capture is an important nuclear reaction whose accurate description is needed for many applications ranging from nuclear technology to nuclear astrophysics. The description of such a process relies on the Hauser-Feshbach theory which requires the nuclear optical potential, level density and $γ$-strength function as model inputs. It has recently been suggested that the M1 scissors mode may explain discrepancies between theoretical calculations and evaluated data. We explore statistical model calculations with the strength of the M1 scissors mode estimated to be dependent on the nuclear deformation of the compound system. We show that the form of the M1 scissors mode improves the theoretical description of evaluated data and the match to experiment in both the fission product and actinide regions. Since the scissors mode occurs in the range of a few keV $\sim$ a few MeV, it may also impact the neutron capture cross sections of neutron-rich nuclei that participate in the rapid neutron capture process of nucleosynthesis. We comment on the possible impact to nucleosynthesis by evaluating neutron capture rates for neutron-rich nuclei with the M1 scissors mode active.

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Reverse engineering nuclear properties from rare earth abundances in the $r$ process

The bulk of the rare earth elements are believed to be synthesized in the rapid neutron capture process or $r$ process of nucleosynthesis. The solar $r$-process residuals show a small peak in the rare earths around $A\sim 160$, which is proposed to be formed dynamically during the end phase of the $r$ process by a pileup of material. This abundance feature is of particular importance as it is sensitive to both the nuclear physics inputs and the astrophysical conditions of the main $r$ process. We explore the formation of the rare earth peak from the perspective of an inverse problem, using Monte Carlo studies of nuclear masses to investigate the unknown nuclear properties required to best match rare earth abundance sector of the solar isotopic residuals. When nuclear masses are changed, we recalculate the relevant $β$-decay properties and neutron capture rates in the rare earth region. The feedback provided by this observational constraint allows for the reverse engineering of nuclear properties far from stability where no experimental information exists. We investigate a range of astrophysical conditions with this method and show how these lead to different predictions in the nuclear properties influential to the formation of the rare earth peak. We conclude that targeted experimental campaigns in this region will help to resolve the type of conditions responsible for the production of the rare earth nuclei, and will provide new insights into the longstanding problem of the astrophysical site(s) of the $r$ process.

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The link between rare earth peak formation and the astrophysical site of the $r$ process

The primary astrophysical source of the rare earth elements is the rapid neutron capture process ($r$ process). The rare earth peak that is seen in the solar $r$-process residuals has been proposed to originate as a pile-up of nuclei during the end of the $r$ process. We introduce a new method utilizing Monte Carlo studies of nuclear masses in the rare earth region, that includes self-consistently adjusting $β$-decay rates and neutron capture rates, to find the mass surfaces necessary for the formation of the rare earth peak. We demonstrate our method with two types of astrophysical scenarios, one corresponding conditions typical of core-collapse supernova winds and one corresponding to conditions typical of the ejection of the material from the tidal tails of neutron star mergers. In each type of astrophysical conditions, this method successfully locates a region of enhanced stability in the mass surface that is responsible for the rare earth peak. For each scenario, we find that the change in the mass surface has qualitatively different features, thus future measurements can shed light on the type of environment in which the $r$ process occurred.

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The impact of individual nuclear properties on $r$-process nucleosynthesis

The astrophysical rapid neutron capture process or `$r$ process' of nucleosynthesis is believed to be responsible for the production of approximately half the heavy element abundances found in nature. This multifaceted problem remains one of the greatest open challenges in all of physics. Knowledge of nuclear physics properties such as masses, $β$-decay and neutron capture rates, as well as $β$-delayed neutron emission probabilities are critical inputs that go into calculations of $r$-process nucleosynthesis. While properties of nuclei near stability have been established, much still remains unknown regarding neutron-rich nuclei far from stability that may participate in the $r$ process. Sensitivity studies gauge the astrophysical response of a change in nuclear physics input(s) which allows for the isolation of the most important nuclear properties that shape the final abundances observed in nature. This review summarizes the extent of recent sensitivity studies and highlights how these studies play a key role in facilitating new insight into the $r$ process. The development of these tools promotes a focused effort for state-of-the-art measurements, motivates construction of new facilities and will ultimately move the community towards addressing the grand challenge of `How were the elements from iron to uranium made?'.

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The impact of individual nuclear masses on $r$-process abundances

We have performed for the first time a comprehensive study of the sensitivity of $r$-process nucleosynthesis to individual nuclear masses across the chart of nuclides. Using the latest version (2012) of the Finite-Range Droplet Model, we consider mass variations of $\pm0.5$ MeV and propagate each mass change to all affected quantities, including $Q$-values, reaction rates, and branching ratios. We find such mass variations can result in up to an order of magnitude local change in the final abundance pattern produced in an $r$-process simulation. We identify key nuclei whose masses have a substantial impact on abundance predictions for hot, cold, and neutron star merger $r$-process scenarios and could be measured at future radioactive beam facilities.

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The Influence Of Neutron Capture Rates On The Rare Earth Region Of The r-Process Abundance Pattern

We study the sensitivity of the r-process abundance pattern to neutron capture rates along the rare earth region (A~150 to A~180). We introduce the concepts of large nuclear flow and flow saturation which determine the neutron capture rates that are influential in setting the rare earth abundances. We illustrate the value of the two concepts by considering high entropy conditions favorable for rare earth peak production and identifying important neutron capture rates among the rare earth isotopes. We also show how these rates influence nuclear flow and specific sections of the abundance pattern.

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