arXiv subjects

M. R. Wegewijs

Publications and source records attributed to M. R. Wegewijs.

At least 19 recordsLinked to original sources

arXiv2022

Renormalization group for open quantum systems using environment temperature as flow parameter

We present the $T$-flow renormalization group method, which computes the memory kernel for the density-operator evolution of an open quantum system by lowering the physical temperature $T$ of its environment. This has the key advantage that it can be formulated directly in real time, making it particularly suitable for transient dynamics, while automatically accumulating the full temperature dependence of transport quantities. We solve the $T$-flow equations numerically for the example of the single impurity Anderson model. We benchmark in the stationary limit, readily accessible in real-time for voltages on the order of the coupling or larger using results obtained by the functional renormalization group, density-matrix renormalization group and the quantum Monte Carlo method. Here we find quantitative agreement even in the worst case of strong interactions and low temperatures, indicating the reliability of the method. For transient charge currents we find good agreement with results obtained by the 2PI Green's function approach. Furthermore, we analytically show that the short-time dynamics of both local and non-local observables follow a universal temperature-independent behaviour when the metallic reservoirs have a flat wide band.

quant-ph↗

arXiv2021

The connection between time-local and time-nonlocal perturbation expansions

There exist two canonical approaches to describe open quantum systems by a time-evolution equation: the Nakajima-Zwanzig quantum master equation, featuring a time-nonlocal memory kernel $\mathcal{K}$, and the time-convolutionless equation with a time-local generator $\mathcal{G}$. These key quantities have recently been shown to be connected by an exact fixed-point relation [Phys. Rev. X 11, 021041 (2021)]. Here we show that this implies a recursive relation between their perturbative expansions, allowing a series for the kernel $\mathcal{K}$ to be translated directly into a corresponding series for the more complicated generator $\mathcal{G}$. This leads to an elegant way of computing the generator using well-developed, standard memory-kernel techniques for strongly interacting open systems. Moreover, it allows for an unbiased comparison of time-local and time-nonlocal approaches independent of the particular technique chosen to calculate expansions of $\mathcal{K}$ and $\mathcal{G}$ (Nakajima-Zwanzig projections, real-time diagrams, etc.). We illustrate this for leading and next-to-leading order calculations of $\mathcal{K}$ and $\mathcal{G}$ for the single impurity Anderson model using both the bare expansion in the system-environment coupling and a more advanced renormalized series. We compare the different expansions obtained, quantify the legitimacy of the generated dynamics (complete positivity) and benchmark with the exact result in the non-interacting limit.

quant-ph↗

arXiv2021

Fermionic duality: General symmetry of open systems with strong dissipation and memory

We consider the exact time-evolution of a broad class of fermionic open quantum systems with both strong interactions and strong coupling to wide-band reservoirs. We present a nontrivial fermionic duality relation between the evolution of states (Schrödinger) and of observables (Heisenberg). We show how this highly nonintuitive relation can be understood and exploited in analytical calculations within all canonical approaches to quantum dynamics, covering Kraus measurement operators, the Choi-Jamiołkowski state, time-convolution and convolutionless quantum master equations and generalized Lindblad jump operators. We discuss the insights this offers into the divisibility and causal structure of the dynamics and the application to nonperturbative Markov approximations and their initial-slip corrections. Our results underscore that predictions for fermionic models are already fixed by fundamental principles to a much greater extent than previously thought.

quant-ph↗

arXiv2019

Density-operator evolution: Complete positivity and the Keldysh real-time expansion

We study the reduced time-evolution of open quantum systems by combining quantum-information and statistical field theory. Inspired by prior work [EPL 102, 60001 (2013) and Phys. Rev. Lett. 111, 050402 (2013)] we establish the explicit structure guaranteeing the complete positivity (CP) and trace-preservation (TP) of the real-time evolution expansion in terms of the microscopic system-environment coupling. This reveals a fundamental two-stage structure of the coupling expansion: Whereas the first stage defines the dissipative timescales of the system --before having integrated out the environment completely-- the second stage sums up elementary physical processes described by CP superoperators. This allows us to establish the nontrivial relation between the (Nakajima-Zwanzig) memory-kernel superoperator for the density operator and novel memory-kernel operators that generate the Kraus operators of an operator-sum. Importantly, this operational approach can be implemented in the existing Keldysh real-time technique and allows approximations for general time-nonlocal quantum master equations to be systematically compared and developed while keeping the CP and TP structure explicit. Our considerations build on the result that a Kraus operator for a physical measurement process on the environment can be obtained by 'cutting' a group of Keldysh real-time diagrams 'in half'. This naturally leads to Kraus operators lifted to the system plus environment which have a diagrammatic expansion in terms of time-nonlocal memory-kernel operators. These lifted Kraus operators obey coupled time-evolution equations which constitute an unraveling of the original Schrödinger equation for system plus environment. Whereas both equations lead to the same reduced dynamics, only the former explicitly encodes the operator-sum structure of the coupling expansion.

cond-mat.stat-mech↗

arXiv2018

Duality for open fermion systems: energy-dependent weak coupling and quantum master equations

Open fermion systems with energy-independent bilinear coupling to a fermionic environment have been shown to obey a general duality relation [Phys. Rev. B 93, 81411 (2016)] which allows for a drastic simplification of time-evolution calculations. In the weak-coupling limit, such a system can be associated with a unique dual physical system in which all energies are inverted, in particular the internal interaction. This paper generalizes this fermionic duality in two ways: we allow for weak coupling with arbitrary energy dependence and describe both occupations and coherences coupled by a quantum master equation for the density operator. We also show that whenever generalized detailed balance holds (Kolmogorov criterion), the stationary probabilities for the dual system can be expressed explicitly in terms of the stationary recurrence times of the original system, even at large bias. We illustrate the generalized duality by a detailed analysis of the rate equation for a quantum dot with strong onsite Coulomb repulsion, going beyond the commonly assumed wideband limit. We present predictions for (i) the decay rates for transient charge and heat currents after a gate-voltage quench and (ii) the thermoelectric linear response coefficients in the stationary limit. We show that even for pronouncedly energy-dependent coupling, all nontrivial parameter dependence in these problems is entirely captured by just two well-understood stationary variables, the average charge of the system and of the dual system. Remarkably, it is the latter that often dictates the most striking features of the measurable quantities (e.g., positions of resonances), underscoring the importance of the dual system for understanding the actual one.

cond-mat.mes-hall↗

arXiv2018

Attractive and driven interaction in quantum dots: mechanisms for geometric pumping

We analyze time-dependent transport through a quantum dot with electron-electron interaction that is statically tunable to both repulsive and attractive regimes, or even dynamically driven. Motivated by the recent experimental realization [Hamo et. al, Nature 535, 395 (2016)] of such a system in a static double quantum dot we compute the geometric pumping of charge in the limit of weak tunneling, high temperature and slow driving. We analyze the pumping responses for all pairs of driving parameters (gate voltage, bias voltage, tunnel coupling, electron-electron interaction). We show that the responses are analytically related when these different driving protocols are governed by the same pumping mechanism, which is characterized by effective driving parameters that differ from the experimental ones. For static attractive interaction we find a characteristic pumping resonance despite the 'attractive Coulomb blockade' that hinders stationary transport. Moreover, we identify a pumping mechanism that is unique to driving of the interaction. Finally, although a single-dot model with orbital pseudo-spin describes most of the physics of the mentioned experimental setup, it is crucial to account for the additional (real-) spin degeneracies of the double dot and the associated electron-hole symmetry breaking. This is necessary because the pumping response is more sensitive than DC transport measurements and detects this difference through pronounced qualitative effects.

cond-mat.mes-hall↗

arXiv2017

Meter calibration and the geometric pumping process in open quantum systems

We consider the process of pumping charge through an open quantum system, motivated by the example of a quantum dot with strong repulsive or attractive electron-electron interaction. Using the geometric formulation of adiabatic nonunitary evolution put forward by Sarandy and Lidar, we derive an encompassing approach to ideal charge measurements of time-dependently driven transport, that stays near the familiar approach to closed systems. Following Schaller, Kießlich and Brandes we explicitly account for a meter that registers the transported charge outside the system. The gauge freedom underlying geometric pumping effects in all moments of the transported charge emerges naturally as the calibration of this meter. Remarkably, we find that geometric and physical considerations cannot be applied independently as done in closed systems: physical recalibrations do not form a group due to constraints of positivity (Bochner's theorem). This complication goes unnoticed when considering only the average charge but it is relevant for understanding the origin of geometric effects in the higher moments of the charge-transport statistics. As an application we derive two prominent existing approaches to pumping, based on full-counting-statistics (FCS) and adiabatic-response (AR), respectively, from our approach in a transparent way. This allows us to reconcile all their apparent incompatibilities, in particular the puzzle how for the average charge the nonadiabatic stationary-state AR result can exactly agree with the adiabatic nonstationary FCS result. We relate this and other difficulties to a single characteristic of geometric approaches to open systems: the system-environment boundary can always be chosen to either include or exclude the ideal charge meter. This leads to a physically motivated relation between the mixed-state Berry phase and the entirely different geometric phase of Landsberg.

cond-mat.mes-hall↗

arXiv2017

Gauge freedom in observables and Landsbergs nonadiabatic geometric phase: pumping spectroscopy of interacting open quantum systems

We set up a general density-operator approach to geometric steady-state pumping through slowly driven open quantum systems. This approach applies to strongly interacting systems that are weakly coupled to multiple reservoirs at high temperature, illustrated by an Anderson quantum dot, but shows potential for generalization. Pumping gives rise to a nonadiabatic geometric phase that can be described by a framework originally developed for classical dissipative systems by Landsberg. This geometric phase is accumulated by the transported observable (charge, spin, energy) and not by the quantum state. It thus differs radically from the adiabatic Berry-Simon phase, even when generalizing it to mixed states, following Sarandy and Lidar. Importantly, our geometric formulation of pumping stays close to a direct physical intuition (i) by tying gauge transformations to calibration of the meter registering the transported observable and (ii) by deriving a geometric connection from a driving-frequency expansion of the current. Our approach provides a systematic and efficient way to compute the geometric pumping of various observables, including charge, spin, energy and heat. Our geometric curvature formula reveals a general experimental scheme for performing geometric transport spectroscopy that enhances standard nonlinear spectroscopies based on measurements for static parameters. We indicate measurement strategies for separating the useful geometric pumping contribution to transport from nongeometric effects. Finally, we highlight several advantages of our approach in an exhaustive comparison with the Sinitsyn-Nemenmann full-counting statistics (FCS) approach to geometric pumping of an observable`s first moment. We explain how in the FCS approach an "adiabatic" approximation leads to a manifestly nonadiabatic result involving a finite retardation time of the response to parameter driving.

cond-mat.mes-hall↗

arXiv2016

Qubit quantum-dot sensors: noise cancellation by coherent backaction, initial slips, and elliptical precession

We theoretically investigate the backaction of a sensor quantum dot with strong local Coulomb repulsion on the transient dynamics of a qubit that is probed capacitively. We show that the measurement backaction induced by the noise of electron cotunneling through the sensor is surprisingly mitigated by the recently identified coherent backaction [PRB 89, 195405] arising from quantum fluctuations. This renormalization effect is missing in semiclassical stochastic fluctuator models and typically also in Born-Markov approaches, which try to avoid the calculation of the nonstationary, nonequilibrium state of the qubit plus sensor. Technically, we integrate out the current-carrying electrodes to obtain kinetic equations for the joint, nonequilibrium detector-qubit dynamics. We show that the sensor-current response, level renormalization, cotunneling, and leading non-Markovian corrections always appear together and cannot be turned off individually in an experiment or ignored theoretically. We analyze the backaction on the reduced qubit state - capturing the full non-Markovian effects imposed by the sensor quantum dot on the qubit - by applying a Liouville-space decomposition into quasistationary and rapidly decaying modes. Importantly, the sensor cannot be eliminated completely even in the simplest high-temperature, weak-measurement limit: The qubit state experiences an initial slip that persists over many qubit cycles and depends on the initial preparation of qubit plus sensor quantum dot. A quantum-dot sensor can thus not be modeled as a 'black box' without accounting for its dynamical variables. We furthermore find that the Bloch vector relaxes (T1) along an axis that is not orthogonal to the plane in which the Bloch vector dephases (T2), blurring the notions of T1 and T2 times. Finally, the precessional motion of the Bloch vector is distorted into an ellipse in the tilted dephasing plane.

cond-mat.mes-hall↗

arXiv2016

Coherent Backaction of Quantum Dot Detectors: Qubit Isospin Precession

A sensitive technique for the readout of the state of a qubit is based on the measurement of the conductance through a proximal sensor quantum dot (SQD). Here, we theoretically study the coherent backaction of such a measurement on a coupled SQD-charge-qubit system. We derive Markovian kinetic equations for the ensemble-averaged state of the SQD-qubit system, expressed in the coupled dynamics of two charge-state occupations of the SQD and two qubit isospin vectors, one for each SQD charge state. We find that aside from introducing dissipation, the detection also renormalizes the coherent evolution of the SQD-qubit system. Basically, if the electron on the detector has time to probe the qubit, then it also has time to fluctuate and thereby renormalize the system parameters. In particular, this induces torques on the qubit isospins, similar to the spin torque generated by the spintronic exchange field in noncollinear spin-valve structures. Secondly, we show that for a consistent description of the detection, one must also include the renormalization effects in the next-to-leading order in the electron tunneling rates, especially at the point of maximal sensitivity of the detector. Although we focus on a charge-qubit model, our findings are generic for qubit readout schemes that are based on spin-to-charge conversion using a quantum-dot detector. Furthermore, our study of the stationary current through the SQD, a test measurement verifying that the qubit couples to the detector current, already reveals various significant effects of the isospin torques on the qubit. Our kinetic equations provide a starting point for further studies of the time evolution in charge-based qubit readout. Finally, we provide a rigorous sum rule that constrains such approximate descriptions of the qubit isospin dynamics and show that it is obeyed by our kinetic equations.

cond-mat.mes-hall↗

arXiv2016

Spin resonance without spin splitting

We predict that a single-level quantum dot without discernible splitting of its spin states develops a spin-precession resonance in charge transport when embedded into a spin valve. The resonance occurs in the generic situation of Coulomb blockaded transport with ferromagnetic leads whose polarizations deviate from perfect antiparallel alignment. The resonance appears when electrically tuning the interaction-induced exchange field perpendicular to one of the polarizations -- a simple condition relying on vectors in contrast to usual resonance conditions associated with energy splittings. The spin resonance can be detected by stationary dI/dV spectroscopy and by oscillations in the time-averaged current using a gate-pulsing scheme. The generic noncollinearity of the ferromagnets and junction asymmetry allow for an all-electric determination of the spin-injection asymmetry, the anisotropy of spin relaxation, and the magnitude of the exchange field. We also investigate the impact of a nearby superconductor on the resonance position. Our simplistic model turns out to be generic for a broad class of coherent few-level quantum systems.

cond-mat.mes-hall↗

arXiv2016

Fermion-parity duality and energy relaxation in interacting open systems

We study the transient heat current out of a confined electron system into a weakly coupled electrode in response to a voltage switch. We show that the decay of the Coulomb interaction energy for this repulsive system exhibits signatures of electron-electron attraction, and is governed by an interaction-independent rate. This can only be understood from a general duality that relates the non-unitary evolution of a quantum system to that of a dual model with inverted energies. Deriving from the fermion-parity superselection postulate, this duality applies to a large class of open systems.

cond-mat.mes-hall↗

arXiv2015

Probing Transverse Magnetic Anisotropy by Electronic Transport through a Single-Molecule Magnet

By means of electronic transport, we study the transverse magnetic anisotropy of an individual Fe$_4$ single-molecule magnet (SMM) embedded in a three-terminal junction. In particular, we determine in situ the transverse anisotropy of the molecule from the pronounced intensity modulations of the linear conductance, which are observed as a function of applied magnetic field. The proposed technique works at temperatures exceeding the energy scale of the tunnel splittings of the SMM. We deduce that the transverse anisotropy for a single Fe$_4$ molecule captured in a junction is substantially larger than the bulk value.

cond-mat.mes-hall↗

arXiv2015

Switchable Coupling of Vibrations to Two-Electron Carbon-Nanotube Quantum Dot States

We report transport measurements on a quantum dot in a partly suspended carbon nanotube. Electrostatic tuning allows us to modify and even switch 'on' and 'off' the coupling to the quantized stretching vibration across several charge states. The magnetic-field dependence indicates that only the two-electron spin-triplet excited state couples to the mechanical motion, indicating mechanical coupling to both the valley degree of freedom and the exchange interaction, in contrast to standard models.

cond-mat.mes-hall↗

arXiv2014

Time-dependent quantum transport: causal superfermions, exact fermion-parity protected decay mode, and Pauli exclusion principle for mixed quantum states

We extend the recently developed causal superfermion approach to the real-time transport theory to time-dependent decay problems.Its usefulness is illustrated for the Anderson model of a quantum dot with tunneling rates depending on spin due to the ferromagnetic electrodes and/or spin polarization of the tunnel junction. We set up a second quantization scheme for density operators in the Liouville-Fock space constructing causal field superoperators using the fundamental physical principles of causality/probability conservation and the fermion-parity superselection (univalence). The time-dependent perturbation series for the time-evolution is renormalized by explicitly performing the wide-band limit on the superoperator level. The short and long-time reservoir correlations are shown to be tightly linked to the occurrence of causal field destruction and creation superoperators, respectively. The effective theory takes as a reference a damped local system, providing an interesting starting point for numerical calculations of memory kernels in real-time. A remarkable feature of this approach is the natural appearance of a measurable fermion-parity protected decay mode. It already can be calculated exactly in the Markovian, infinite temperature limit by leading order perturbation theory, yet persists unaltered for the finite temperature, interaction and tunneling spin polarization. Furthermore, we show how a Liouville-space analog of the Pauli principle directly leads to the exact result in the noninteracting limit: surprisingly, it is obtained in finite (second) order renormalized perturbation theory, both for the self-energy as well as the time-evolution propagator. For this limit we calculate the time-evolution of the full density operator starting from an arbitrary initial state on the quantum dot, including spin and pairing coherences and two-particle correlations.

cond-mat.str-el↗

arXiv2013

Heat, molecular vibrations, and adiabatic driving in non-equilibrium transport through interacting quantum dots

In this article we review aspects of charge and heat transport in interacting quantum dots and molecular junctions under stationary and time-dependent non-equilibrium conditions due to finite electrical and thermal bias. In particular, we discuss how a discrete level spectrum can be beneficial for thermoelectric applications, and investigate the detrimental effects of molecular vibrations on the efficiency of a molecular quantum dot as an energy converter. In addition, we consider the effects of a slow time-dependent modulation of applied voltages on the transport properties of a quantum dot and show how this can be used as a spectroscopic tool complementary to standard dc-measurements. Finally, we combine time-dependent driving with thermoelectrics in a double-quantum dot system - a nanoscale analogue of a cyclic heat engine - and discuss its operation and the main limitations to its performance.

cond-mat.mes-hall↗

arXiv2012

Fermionic superoperators for zero-temperature non-linear transport: real-time perturbation theory and renormalization group for Anderson quantum dots

We study the transport through a strongly interacting Anderson quantum dot at zero-temperature using the real-time renormalization group (RT-RG) in the framework of a kinetic equation for the reduced density operator. We further develop the general finite temperature real-time transport formalism by introducing field superoperators that obey fermionic statistics. This direct second quantization in Liouville-Fock space strongly simplifies the construction of operators and superoperators which transform irreducibly under the Anderson-model symmetry transformations. The fermionic field superoperators naturally arise from the univalence (fermion-parity) superselection rule for the total system. Expressed in these field superoperators, the causal structure of the perturbation theory for the effective time-evolution superoperator-kernel becomes explicit. The causal structure also implies the existence of a fermion-parity protected eigenvector of the exact Liouvillian, explaining a recently reported result on adiabatic driving [Phys. Rev. B 85, 075301 (2012)] and generalizing it to arbitrary order in the tunnel coupling. Furthermore, in the WBL the causal representation exponentially reduces the number of diagrams for the time-evolution kernel. We perform a complete 2-loop RG analysis at finite voltage and magnetic field, while systematically accounting for the dependence on both the quantum dot and reservoir frequencies. Using the second quantization in Liouville-space and symmetry restrictions we obtain analytical RT-RG equations with an efficient numerical solution and we extensively study the model parameter space, excluding the Kondo regime. The incorporated renormalization effects result in an enhancement of the inelastic cotunneling peak. Moreover, we find a tunnel-induced non-linearity of the stability diagrams at finite voltage, both in the SET and ICT regime.

cond-mat.mes-hall↗

arXiv2011

Interaction of spin and vibrations in transport through single-molecule magnets

We study linear electron transport through a single-molecule magnet (SMM) and the interplay of its anisotropic spin with quantized vibrational distortions of the molecule. We show that, despite the longitudinal anisotropy barrier and small transverse anisotropy, vibrational fluctuations can induce quantum spin-tunneling (QST) and a QST-Kondo effect. The interplay of spin scattering, QST and molecular vibrations can strongly enhance the Kondo effect and induce an anomalous magnetic field dependence of vibrational Kondo side-bands.

cond-mat.mes-hall↗