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M. Ramalho

Publications and source records attributed to M. Ramalho.

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Electron spectral shape of the third-forbidden $\beta$-decay of $^{87}$Rb measured using a Rb$_2$ZrCl$_6$ crystal scintillator

In recent years, interest in experimental studies of $\beta$-decay electron spectra -- often referred to as $\beta$ spectra -- has been growing. This is particularly true for $\beta$ transitions where the electron spectra are sensitive to the effective value of the weak axial coupling, $g_{\rm A}$. Such measurements serve as important benchmarks for nuclear physics calculations and can also be used to characterize background in astroparticle physics experiments. In this work, a dedicated experiment has been carried out to investigate the spectral shape of the third-forbidden $^{87}$Rb $\beta$-decays, with the goal of estimating the effective $g_{\rm A}$ value for this transition and of deriving the T$_{1/2}$ value. This was done by comparing the experimental spectral shape with the estimates from various phenomenological models. The $^{87}$Rb source was embedded directly within the detector material of a new Rb$_2$ZrCl$_6$ crystal scintillator; the data taking was performed deep underground at Gran Sasso National Laboratory. The obtained experimental half-life value for the studied process is T$_{1/2} = 5.08(13) \times$ 10$^{10}$ yr; while a $g_{\rm A}$ value in the range 0.4 to 0.6 is obtained when accounting for uncertainties and depending on the model adopted as discussed in detail in the text.

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The measurement of the $^{99}$Tc $\beta$-decay spectrum and its implications for the effective value of weak axial coupling

Measurements of $\beta$-spectral shapes is an important way to examine the effective value of the weak axial coupling $g_{\rm A}$. These stu\ dies focus specifically on forbidden non-unique $\beta^-$ transitions, as only in these cases is the spectral shape directly sensitive to th\ e ratio $g_{\rm A}/g_{\rm V}$. Here, the value of the weak vector coupling constant, $g_{\rm V}$, is fixed at 1.0 according to the Conserve\ d Vector Current (CVC) hypothesis. In previous studies for the fourth-forbidden non-unique $\beta^-$ decays of $^{113}$Cd [J.~Kostensalo \textit{et al.}, Phys. Lett. B 822, 136652 (2021)] and $^{115}$In [A.~F. Leder \textit{et al.}, Phys. Rev. Lett. 129, 232502 \ (2022) and L. Pagnanini \textit{et al.}, Phys. Rev. Lett. 133, 122501 (2024)] a quenched value was determined for the ratio $g_{\rm A}/g_{\rm V}$ using $g_{\rm V}=1.0$. A notable exception is the recent measurement and analysis of the second-forbidden non-unique $\ \beta$-decay transition in $^{99}$Tc, performed by M. Paulsen \textit{et al.}, Phys. Rev. C 110, 05503(2024). Where an enhanced ratio $g_{\\ rm A}/g_{\rm V}=1.526(92)$ was suggested. To resolve this apparently contradictory situation with the effective value of $g_{\rm A}$, we hav\ e performed calculations based on the nuclear shell model (NSM) Hamiltonians glekpn, jj45pnb, and the MQPM approach with a careful considera\ tion of the small relativistic vector nuclear matrix element (sNME). The theoretical spectra were compared to the $^{99}$Tc $\beta$-decay sp\ ectrum by using the 4$\pi$ gold absorber with a Metallic Magnetic Calorimeter (MMC). In all cases, we found that the data matches well with \ reduced $g_{\rm A}$/$g_{\rm V}$ values of 1.0--1.2. Our result contradicts the previously reported measurement for $^{99}$Tc and instead sup\ ports a quenched axial coupling as reported for other isotopes.

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Ultra-low $Q_\beta$ value for the allowed decay of $^{110}$Ag$^m$ confirmed via mass measurements

The mass of the electron-antineutrino can be determined in dedicated measurements of the $\beta$ spectral shape near the $\beta$ endpoint of a $\beta^-$ transition, with a low $Q$ value enhancing the sensitivity of the measurement. One such low-$Q$-value candidate is the transition between the $6^+$ isomer of $^{110}$Ag and the $5^+_2$ state in $^{110}$Cd ($Q^{\ast}_{\beta,m}=-0.12(131)$ keV). To reduce the uncertainty of the $Q$ value, we have used the phase-imaging ion-cyclotron-resonance technique with the JYFLTRAP double Penning trap and performed a high-precision atomic-mass measurement of $^{109}$Ag with $^{110}$Cd as a reference. Combined with the known spectroscopic data, we obtain a re-evaluated value $Q^{\ast}_{\beta,m}=405(135)$ eV, for the $^{110}\text{Ag}(6^+_\text{m}) \rightarrow {^{110}\text{Cd}}(5^+_2)$ transition. This represents the lowest $Q_{\beta}$ value for any allowed transition observed to date. In order to estimate the partial half-life ($t_{1/2}$) and branching ratio (Br) of the transition, nuclear shell-model calculations were performed using the $jj45pnb$ Hamiltonian in combination with state-of-the-art atomic calculations. The computed values $t_{1/2} = 2.23^{+5.24}_{-1.28} \times 10^7$ years and $\textrm{Br} = 3.07^{+4.16}_{-2.15} \times 10^{-8}$, along with the thermal-neutron capture on stable $^{109}$Ag as a viable production method, make $^{110}\textrm{Ag}^m$ a promising candidate for future antineutrino-mass measurements.

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Direct high-precision measurement of the mass difference of $^{77}$As-$^{77}$Se related to neutrino mass determination

The first direct determination of the ground-state-to-ground-state ${β^{-}}$-decay $Q$-value of $^{77}$As to $^{77}$Se was performed by measuring their atomic mass difference utilizing the double Penning trap mass spectrometer, JYFLTRAP. The resulting $Q$-value is 684.463(70) keV, representing a remarkable 24-fold improvement in precision compared to the value reported in the most recent Atomic Mass Evaluation (AME2020). With the significant reduction of the uncertainty of the ground-state-to-ground-state $Q$-value and knowledge of the excitation energies in $^{77}$Se from $γ$-ray spectroscopy, the ground-state-to-excited-state $Q$-value of the transition $^{77}$As (3/2$^{-}$, ground state) $\rightarrow$ $^{77}$Se$^{*}$ (5/2$^{+}$, 680.1035(17) keV) was refined to be 4.360(70) keV. We confirm that this potential low $Q$-value ${β^{-}}$-decay transition for neutrino mass determination is energetically allowed at a confidence level of about 60$σ$. Nuclear shell-model calculations with two well-established effective Hamiltonians were used to estimate the partial half-life for the low $Q$-value transition. The half-life was found to be of the order of 10$^{9}$ years for this first-forbidden non-unique transition, which rules out this candidate a potential source for rare-event experiments searching for the electron antineutrino mass.

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Isomeric states of fission fragments explored via Penning trap mass spectrometry at IGISOL

The masses of $^{84}$Br, $^{105}$Mo, $^{115,119,121}$Pd, $^{122}$Ag, $^{127,129}$In, $^{132}$Sb and their respective isomeric states have been measured with the JYFLTRAP Penning trap mass spectrometer using the phase-imaging ion-cyclotron-resonance technique. The excitation energies of the isomeric states in $^{132}$Sb and $^{119}$Pd were experimentally determined for the first time, while for $^{84}$Br, $^{115}$Pd and $^{127,129}$In, the precision of the mass values was substantially improved. In $^{105}$Mo and $^{121}$Pd there were no signs of a long-lived isomeric state. The ground-state measurements of $^{119}$Pd and $^{122}$Ag indicated that both are significantly more bound than the literature values. For $^{122}$Ag, there was no indication of a proposed third long-lived state. The results for the $N=49$ nucleus $^{84}$Br and isomers close to doubly magic $^{132}$Sn have been compared to the shell-model and the microscopic quasiparticle-phonon model calculations.

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High-precision measurements of low-lying isomeric states in $^{120-124}$In with JYFLTRAP double Penning trap

Neutron-rich $^{120-124}$In isotopes have been studied utilizing the double Penning trap mass spectrometer JYFLTRAP at the IGISOL facility. Using the phase-imaging ion-cyclotron-resonance technique, the isomeric states were resolved from ground states and their excitation energies measured with high precision in $^{121,123,124}$In. In $^{120,122}$In, the $1^+$ states were separated and their masses were measured while the energy difference between the unresolved $5^+$ and $8^-$ states, whose presence was confirmed by post-trap decay spectroscopy was determined to be $\leq15$ keV. In addition, the half-life of $^{122}$Cd, $T_{1/2} = 5.98(10)$ s, was extracted. Experimental results were compared with energy density functionals, density functional theory and shell-model calculations.

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$\beta^-$ decay $Q$-value measurement of $^{136}$Cs and its implications to neutrino studies

The $\beta^-$ decay $Q$-value of $^{136}$Cs ($J^\pi = 5^+$, $t_{1/2} \approx 13$~days) was measured with the JYFLTRAP Penning trap setup at the Ion Guide Isotope Separator On-Line (IGISOL) facility of the University of Jyv\"askyl\"a, Finland. The mono-isotopic samples required in the measurements were prepared with a new scheme utilised for the cleaning, based on the coupling of dipolar excitation with Ramsey's method of time-separated oscillatory fields and the phase-imaging ion-cyclotron-resonance (PI-ICR) technique. The $Q$ value is determined to be 2536.83(45) keV, which is $\sim$4 times more precise and 11.4(20) keV ($\sim$ 6$\sigma$) smaller than the adopted value in the most recent Atomic Mass Evaluation AME2020. The daughter, $^{136}$Ba, has a 4$^+$ state at 2544.481(24) keV and a $3^-$ state at 2532.653(23) keV, both of which can potentially be ultralow $Q$-value end-states for the $^{136}$Cs decay. With our new ground-to-ground state $Q$ value, the decay energies to these two states become -7.65(45) keV and 4.18(45) keV, respectively. The former is confirmed to be negative at the level of $\sim$ 17$\sigma$, which verifies that this transition is not a suitable candidate for neutrino mass determination. On the other hand, the slightly negative $Q$ value makes this transition an interesting candidate for the study of virtual $\beta$-$\gamma$ transitions. The decay to the 3$^{-}$ state is validated to have a positive low $Q$ value which makes it a viable candidate for neutrino mass determination. For this transition, we obtained a shell-model-based half-life estimate of $2.1_{-0.8}^{+1.6}\times10^{12}$ yr.

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Observation of an ultra-low $Q$-value electron-capture channel decaying to $^{75}$As via high-precision mass measurement

A precise determination of the atomic mass of $^{75}$As has been performed utilizing the double Penning trap mass spectrometer, JYFLTRAP. The mass excess is measured to be -73035.519(42) keV/c$^2$, which is a factor of 21 more precise and 1.3(9) keV/c$^2$ lower than the adopted value in the newest Atomic Mass Evaluation (AME2020). This value has been used to determine the ground-state-to-ground-state electron-capture decay $Q$ value of $^{75}$Se and $β^-$ decay $Q$ value of $^{75}$Ge, which are derived to be 866.041(81) keV and 1178.561(65) keV, respectively. Using the nuclear energy-level data of 860.00(40) keV, 865.40(50) keV (final states of electron capture) and 1172.00(60) keV (final state of $β^-$ decay) for the excited states of $^{75}$As$^*$, we have determined the ground-state-to-excited-state $Q$ values for two transitions of $^{75}$Se $\rightarrow$ $^{75}$As$^*$ and one transition of $^{75}$Ge $\rightarrow$ $^{75}$As$^*$. The ground-state-to-excited-state $Q$ values are determined to be 6.04(41) keV, 0.64(51) keV and 6.56(60) keV, respectively, thus confirming that the three low $Q$-value transitions are all energetically valid and one of them is a possible candidate channel for antineutrino mass determination. Furthermore, the ground-state-to-excited-state $Q$ value of transition $^{75}$Se $\rightarrow$ $^{75}$As$^*$ (865.40(50) keV) is revealed to be ultra-low (< 1 keV) and the first-ever confirmed EC transition possessing an ultra-low $Q$ value from direct measurements.

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