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M. Rejmund

Publications and source records attributed to M. Rejmund.

At least 19 recordsLinked to original sources

Automated Physics-Informed Neural-Networks-Based Calibration of Highly Segmented Silicon Telescopes

Transfer and multi-nucleon transfer reactions are essential tools for probing nuclear structure and reaction dynamics, requiring precise determination of the identity, energy, and emission angles of reaction products. The increasing granularity of modern silicon telescope arrays enhances experimental capabilities but challenges detector calibration, as conventional channel-by-channel approaches become inefficient and difficult to scale. In this work, we present a fully automated, physics-informed calibration framework based on neural networks, specifically designed for highly segmented silicon detector arrays. The method formulates calibration as a global optimization problem, in which detector gains and geometrical corrections are determined simultaneously by minimizing the width of the reconstructed excitation energy under two-body kinematics constraints. The approach relies exclusively on experimental data and well-established physical principles, without requiring explicit modeling of detector response. A distinctive feature is the use of multiple neural network sub-models sharing a common loss function with embedded physics constraints, enabling coherent and self-consistent calibration across all detector channels. This strategy ensures scalability, robustness, and reproducibility, making it particularly suitable for next-generation detector systems with increasing complexity. The performance of the method is demonstrated using experimental data from the Particle-Identification Silicon-Telescope Array (PISTA) in high-resolution fission studies in inverse kinematics. The results show excellent agreement with theoretical kinematics, high-quality particle identification, and a significant improvement in calibration efficiency. The proposed framework provides a general and adaptable solution for the calibration of complex detector systems in modern nuclear physics experiments.

physics.ins-det

Self-Supervised Calibration of Scientific Instruments Using Physical Consistency Constraints

Calibration remains one of the principal obstacles to the deployment of machine learning in scientific instrumentation because it typically relies on expert intervention, dedicated procedures, and manually labelled data. We introduce a physics-informed self-supervised framework that jointly learns latent detector calibration parameters and task-specific predictions directly from raw measurements without requiring pre-calibrated signals or external labels. The method exploits known physical constraints to generate pseudo-labels iteratively, transforming calibration into a self-supervised optimization problem. The approach is demonstrated for ionic charge-state determination in the VAMOS++ magnetic spectrometer, where the calibration of a segmented ionization chamber and the inference of ionic charge states are learned simultaneously. Starting from a weak prior on the mean ionic charge state, the model progressively refines its predictions through iterative fractional pseudo-labelling driven by the discrete nature of atomic masses. Beyond accurate ionic charge-state reconstruction, the inferred calibration coefficients provide a compact representation of the detector state that enables automated monitoring of gain drifts, pressure variations, and detector aging. The resulting labels can subsequently be transferred to specialized models that quantify detector imperfections and track their spatial and temporal evolution. These results establish a general paradigm for self-calibrating and self-monitoring scientific instruments and represent a step toward intelligent experimental systems capable of autonomous calibration, analysis, and performance optimization.

cs.LG

Isotopic fission yields of ${}^{240}$Pu as a function of the excitation energy

Complete isotopic fission yields distributions of $^{240}$Pu have been measured as a function of the initial excitation energy. The $^{240}$Pu fissioning system was produced through a two-proton transfer reaction between a $^{238}$U beam and a $^{12}$C target. The reaction was measured in inverse kinematics at Coulomb barrier energies, allowing for the full distribution of fission fragments to be isotopically identified with the VAMOS++ Spectrometer. The excitation energy of the system was measured on an event-by-event basis by detecting the target-like recoil $^{10}$Be in a segmented silicon telescope. This manuscript reports on the evolution of the fission yields as a function of the excitation energy of the system between 8.2 to 11.9 MeV. The influence of the excitation energy is manifested in the damping of shell effects that feed the yields in the symmetry valley, as well as in a reduction of the neutron content of the fragments. This reduction, however, is observed only in the heavy fragment, while the neutron content of the light fragment remains unaffected. The comparison with previous measurements, models, and evaluations highlights the importance of correlated observables for improving fission models.

nucl-ex

Performance of the Particle-Identification Silicon-Telescope Array Coupled with the VAMOS++ Magnetic Spectrometer

The Particle-Identification Silicon-Telescope Array (PISTA) is a new detection system designed for high-resolution studies of the fission process induced by multi-nucleon transfer in inverse kinematics. It is specifically optimized for experiments with the VAMOS++ magnetic spectrometer at GANIL (Grand Accélérateur National d'Ions Lourds). The array comprises eight trapezoidal $Δ$E-E silicon telescopes arranged in a corolla configuration. Each telescope integrates two single-sided stripped silicon detectors, enabling target-like recoil identification, energy loss measurements, and trajectory reconstruction. Positioned in close proximity to the target, PISTA's compact geometry achieves high-efficiency tracking of target-like recoils produced in multi-nucleon transfer reactions at Coulomb barrier energies. The spatial segmentation of the array allows precise determination of the mass and charge of the target-like nucleus, and excitation energy of fissioning systems. This work presents the particle identification and excitation energy reconstruction performances for the interactions of $^{238}$U beam with $^{12}$C target. An excitation energy resolution of 800 keV (FWHM) was determined together with mass resolution of 1.1% (FWHM). The combination of PISTA and VAMOS++ magnetic spectrometer enables unprecedented investigations of the fission process as a function of the excitation energy of the fissioning nucleus, particularly for exotic systems produced in transfer-induced reactions.

physics.ins-det

Hindered Prompt-Neutron Evaporation in Surrogate Reactions for $^{239}$Pu(n,f)

Isotopic fission-fragment distributions of $^{240}$Pu have been measured, for the first time, as a function of the initial excitation energy, and the prompt neutron multiplicity has been derived from these data. The $^{240}$Pu fissioning system was produced through the two-proton transfer reaction between $^{238}$U and $^{12}$C, a surrogate reaction for the neutron-capture-induced fission $^{239}$Pu(n,f). The reaction was measured in inverse kinematics, allowing the fission fragments to be fully identified with the VAMOS Spectrometer. When compared to neutron-capture-induced reactions, the observed prompt neutron multiplicity shows a clear reduction in the surrogate two-proton transfer, revealing an unexpected influence of the entrance channel in the fission output. At the same time, fission-fragment yield distributions obtained in neutron-capture-induced reactions show a relative fission-fragment production in the symmetry region similar to that measured in this work. The discrepancy in neutron multiplicity is attributed to the additional angular momentum induced in the multi-nucleon transfer reactions, which excites the fissioning system to higher-spin states, increasing the probability of gamma emission that competes with neutron evaporation, in particular from the fission barrier to the scission point. This observation underlines the limitations in the utilisation of properties derived from surrogate reactions in nuclear technology and other applications of nuclear fission.

nucl-ex

First observation of multi-phonon $γ$-vibrations in an odd-odd nuclear system

The identification of the first multi-phonon $γ$-vibrational bands in an odd-odd neutron-rich nucleus of the nuclear chart is presented. These high spin structures of hard to access $^{104}_{41}$Nb$_{63}$, produced in fission, were studied by combining a spectrometer with isotopic resolution coupled to a $γ$-ray tracking array and independently high-fold $γ$ coincidence measurements. Triaxial Projected Shell Model calculations for the high-spin states are in good agreement with the measured observables for the yrast, one-phonon and two-phonon $γ$ bands. The possibility of an oblate shape of an isomeric state and coexistence of triaxial and oblate configurations are investigated from the decay of the 141 keV isomer. The present work illustrates the robustness of vibration excitations in the presence of odd valence proton and neutron as well as the possibly coexisting shapes beyond the $N=60$ transitional region.

nucl-ex

Level structure of light neutron-rich La isotopes beyond the N=82 shell closure

The high spin excited states of Lanthanum isotopes $^{140-143}$La, above the $N=82$ closed shell, have been populated in fission reactions. The prompt $γ$-ray transitions were measured using two complementary methods; a) in coincidence with the isotopically identified fragments produced in the fission of the $^{238}$U+$^{9}$Be system using the VAMOS++ and the AGATA spectrometers and b) high statistics three-fold $γ-γ-γ$ and four-fold $γ-γ-γ-γ$ coincidence data from the spontaneous fission of $^{252}$Cf using the Gammasphere. This work reports the first identification of a pair of parity doublet structures in $^{143}$La and the new high spin level structure in $^{140-142}$La from prompt $γ$-ray spectroscopy. The level structures are interpreted in terms of the systematics of neighbouring odd-$Z$ nuclei above $Z=50$ shell closure and large-scale shell model calculations. The present results indicate the presence of stable octupole deformation, in $^{143}$La. The excitation energy pattern and their comparison with neighbouring isotones, moving away from the N=82 closed shell, point towards a transition from single particle structures to an alternating parity rotational band structure in the La isotopic chain.

nucl-ex

Direct transfer to $^{46,48}$K as a survey of the $π(s_{1/2})$$-ν(sdpf)$ interaction

The collapse of the canonical $N=28$ magic number in nuclei with $Z<20$ has drawn significant interest as it relates to the emergence of an island of inversion centered on $^{42}$Si and $^{44}$S. In particular, interactions between the $πs_{1/2}$ orbital -- empty in $^{42}$Si and full in $^{44}$S -- and the neutron orbitals just above and below the $N=28$ gap are expected to be critical in this region, but remain relatively unexplored. In this paper, we expand upon the results of our previous study of the direct transfer reaction $^{47}$K(d,p$γ$)$^{48}$K [C.\,J.~Paxman \textit{et al.}, Phys. Rev. Lett. 134, 162504 (2025)] with the results of the complementary $^{47}$K(d,t$γ$)$^{46}$K reaction. Through this study, we present a comprehensive scan of the interaction between the critical $πs_{1/2}$ orbital and a broad range of neutron orbitals spanning nearly two full shells. We identify several discrepancies between the experimental results and state-of-the-art shell model calculations, which suggest a deficiency of the shell model to fully capture the complex proton configuration mixing in this region, highlighting a significant challenge for single-particle descriptions of the island of inversion.

nucl-ex

Analysis of Atomic Charge State and Atomic Number for VAMOS++ Magnetic Spectrometer using Deep Neural Networks and Fractionally Labelled Events

The VAMOS++ magnetic spectrometer is a multi-parametric system that integrates ion optical magnetic elements with a multi-detector stack. The magnetic elements, along with the tracking and timing detectors and the trajectory reconstruction method, provide the analysis of the magnetic rigidity, the trajectory length between the beam interaction point and the focal plane of the spectrometer, and the related velocity and mass-over-charge ratio. The segmented ionization chamber provides the energy measurements necessary to analyze the atomic charge state and atomic number. However, this analysis critically suffers from inherent limitations due to the variable thickness and non-uniformity of the entrance window of the ionization chamber and other detector imperfections. Conventionally, this meticulous, detailed analysis is exceptionally tedious, often requiring several months to complete. We present a novel method utilizing deep neural networks, trained on an experimental dataset with only a small fraction of precisely labeled events for the lowest and best-resolved atomic charge states or numbers. This innovative approach enables the networks to autonomously and accurately classify the remaining events. This method drastically accelerates the acquisition of high-resolution atomic charge state and atomic number spectra, reducing analysis time from months to mere hours. Crucially, by discarding human bias, this approach ensures standardized, optimal, and reproducible results with unprecedented efficiency.

physics.ins-det

Seven-dimensional Trajectory Reconstruction for VAMOS++

The VAMOS++ magnetic spectrometer is characterized by a large angular and momentum acceptance and highly non-linear ion optics properties requiring the use of software ion trajectory reconstruction methods to measure the ion magnetic rigidity and the trajectory length between the beam interaction point and the focal plane of the spectrometer. Standard measurements, involving the use of a thin target and a narrow beam spot, allow the assumption of a point-like beam interaction volume for ion trajectory reconstruction. However, this represents a limitation for the case of large beam spot size or extended gaseous target volume. To overcome this restriction, a seven-dimensional reconstruction method incorporating the reaction position coordinates was developed, making use of artificial deep neural networks. The neural networks were trained on a theoretical dataset generated by standard magnetic ray-tracing code. Future application to a voluminous gas target, necessitating the explicit inclusion of the three-dimensional position of the beam interaction point within the target in the trajectory reconstruction method, is discussed. The performances of the new method are presented along with a comparison of mass resolution obtained with previously reported model for the case of thin-target experimental data.

physics.ins-det

Probing exotic cross-shell interactions at N=28 with single-neutron transfer on 47K

We present the first measurement of the $^{47}$K($d,pγ$)$^{48}$K transfer reaction, performed in inverse kinematics using a reaccelerated beam of $^{47}$K. The level scheme of $^{48}$K has been greatly extended with nine new bound excited states identified and spectroscopic factors deduced. Detailed comparisons with SDPF-U and SDPF-MU shell-model calculations reveal a number of discrepancies with these results, and a preference for SDPF-MU is found. Intriguingly, an apparent systematic overestimation of spectroscopic factors and a poor reproduction of the energies for 1$^-$ states suggests that the mixing between the $πs^{\,\,\,1}_{1/2} d^{\,\,\,4}_{3/2}$ and $πs^{\,\,\,2}_{1/2} d^{\,\,\,3}_{3/2}$ proton configurations in $^{48}$K is not correctly described using current interactions, challenging our descriptions of light $N=28$ nuclei.

nucl-ex

Mirror nucleon-transfer reactions from $^{18}$Ne and $^{18}$O

The $^{18}$Ne(d,t)$^{17}$Ne and $^{18}$Ne(d,$^3$He)$^{17}$F single-nucleon pickup reactions were measured at 16.5 MeV/nucleon in inverse kinematics together with elastic and inelastic scattering channels. The full set of measured exclusive differential cross sections was compared with the mirror reaction channels on stable $^{18}$O after consistent reanalysis using coupled reaction channels calculations. Within this interpretation scheme, most of the spectroscopic factors extracted for the population of unbound states in $^{17}$F match within uncertainties with their mirror partners in $^{17}$O. However, for the deeply-bound neutron removal channel to $^{17}$Ne, a significant symmetry breaking with the mirror proton-removal channel leading to $^{17}$N is evidenced by an overall single-particle strength reduction.

nucl-ex

High-resolution spectroscopy of neutron-rich Br isotopes and signatures for a prolate-to-oblate shape transition at N=56

The first systematic experimental study of the neutron-rich Br isotopes with two complementary state-of-the-art techniques is presented. These isotopes have been populated in the fission process at two different facilities, GANIL and ILL. New spectroscopic information has been obtained for odd-even $^{87-93}$Br isotopes and the experimental results have been compared with state-of-the-art Large-Scale Shell-Model and DNO Shell-Model calculations. As a result of such theoretical approaches, a transition from prolate ($^{87,89}$Br) to oblate ($^{91,93}$Br) shapes is obtained from the subtle balance between proton and neutron quadrupole deformations, as a clear signature of pseudo-SU3 quadrupole regime.

nucl-ex

High-precision spectroscopy of $^{20}$O benchmarking ab-initio calculations in light nuclei

The excited states of unstable $^{20}$O were investigated via $γ$-ray spectroscopy following the $^{19}$O$(d,p)^{20}$O reaction at 8 $A$MeV. By exploiting the Doppler Shift Attenuation Method, the lifetime of the 2$^+_2$ and 3$^+_1$ states were firmly established. From the $γ$-ray branching and E2/M1 mixing ratios for transitions deexciting the 2$^+_2$ and 3$^+_1$ states, the B(E2) and B(M1) were determined. Various chiral effective field theory Hamiltonians, describing the nuclear properties beyond ground states, along with a standard USDB interaction, were compared with the experimentally obtained data. Such a comparison for a large set of $γ$-ray transition probabilities with the valence space in medium similarity renormalization group ab-initio calculations was performed for the first time in a nucleus far from stability. It was shown that the ab-initio approaches using chiral EFT forces are challenged by detailed high-precision spectroscopic properties of nuclei. The reduced transition probabilities were found to be a very constraining test of the performance of the ab-initio models.

nucl-ex

Search for the origin of wobbling motion in the $ A \approx 130 $ region: The case of $^{131}$Xe

In-beam $ γ$-ray spectroscopy of $^{131}$Xe has been carried out to study the structure of the intruder $ νh_{11/2} $ band. Excited states were populated via an $ α$-induced fusion-evaporation reaction at E$ _α = 38 $ MeV. Inspection of $ γγ$-coincidence data resulted in the identification of a new rotational sequence. Based on the systematics of excitation energy, assigned spin-parity, decay pattern, and the electromagnetic character of the inter-band $ ΔI = 1 $ $ γ$-transitions, this sequence is proposed as the unfavoured signature partner of the $ νh_{11/2} $ band. The structure of this band is further illuminated in the light of the triaxial particle rotor model (TPRM). The possibility of wobbling excitation in $ N = 77 $ Xe-Ba-Ce isotones has been explored in a systematic manner.

nucl-ex

Particle Identification at VAMOS++ with Machine Learning Techniques

Multi-nucleon transfer reaction between 136Xe beam and 198Pt target was performed using the VAMOS++ spectrometer at GANIL to study the structure of n-rich nuclei around N=126. Unambiguous charge state identification was obtained by combining two supervised machine learning methods, deep neural network (DNN) and positional correction using a gradient-boosting decision tree (GBDT). The new method reduced the complexity of the kinetic energy calibration and outperformed the conventional method, improving the charge state resolution by 8%

physics.ins-det

CATLIFE (Complementary Arm for Target LIke FragmEnts): Spectrometer for Target like fragments at VAMOS++

The multi-nucleon transfer reaction between 136Xe beam and 198Pt target at the beam energy 7 MeV/u was studied using the large acceptance spectrometer VAMOS++ coupled with the newly installed second arm time-of-flight and delayed $γ$-ray spectrometer CATLIFE (Complementary Arm for Target LIke FragmEnts). The CATLIFE detector is composed of a large area multi-wire proportional chamber and the EXOGAM HPGe clover detectors with an ion flight length of 1230 mm. Direct measurement of the target-like fragments (TLF) and the delayed $γ$-rays from the isomeric state helps to improve TLF identification. The use of the velocity of TLFs and the delayed $γ$-ray demonstrate the proof of principle and effectiveness of the new setup.

physics.ins-det

Advancements of $γ$-ray spectroscopy of isotopically identified fission fragments with AGATA and VAMOS++

$γ$-ray spectroscopy of fission fragments is a powerful method for studies of nuclear structure properties. Recent results on the spectroscopy of fission fragments, using the combination of the AGATA $γ$-ray tracking array and the VAMOS++ large acceptance magnetic spectrometer at GANIL, are reported. A comparison of the performance of the large germanium detector arrays EXOGAM and AGATA illustrates the advances in $γ$-ray spectroscopy of fission fragments. Selected results are highlighted for prompt $γ$-ray spectroscopy studies, measurements of short lifetimes of excited states with the Recoil Distance Doppler-Shift method, using both AGATA and VAMOS++ and prompt-delayed $γ$-ray spectroscopy studies using AGATA, VAMOS++ and EXOGAM.

nucl-ex