arXiv subjects

M. Rosenbusch

Publications and source records attributed to M. Rosenbusch.

26 records · Page 2Linked to original sources

arXiv2018

New mass anchor points for neutron-deficient heavy nuclei from direct mass measurements of radium and actinium isotopes

The masses of the exotic isotopes $^{210-214}$Ac and $^{210-214}$Ra have been measured with a multi-reflection time-of-flight mass spectrograph. These isotopes were obtained in flight as fusion-evaporation products behind the gas-filled recoil ion separator GARIS-II at RIKEN. The new direct mass measurements serve as an independent and direct benchmark for existing $α$-$γ$ spectroscopy data in this mass region. Further, new mass anchor points are set for U and Np nuclei close to the $N=126$ shell closure for a future benchmark of the $Z=92$ sub-shell for neutron-deficient heavy isotopes. Our mass results are in general in good agreement with the previously indirectly-determined mass values. Together with the measurement data, reasons for possible mass ambiguities from decay-data links between ground states are discussed.

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arXiv2018

Improving wide-band mass measurements in a multi-reflection time-of-flight mass spectrograph by usage of a concomitant measurement scheme

We introduce a new concomitant referencing mode for operating a multi-reflection time-of-flight mass spectrograph (MRTOF-MS), wherein the reference and analyte ions are interleaved on a cycle by cycle bases. Using this mode, we demonstrate an improved technique for performing wide bandwidth mass measurements via MRTOF-MS. This new technique offers a simplified analysis and high-accuracy.

physics.ins-det↗

arXiv2018

First direct mass measurements of nuclides around $Z=100$ with a Multireflection Time-of-Flight Mass Spectrograph

The masses of $^{246}$Es, $^{251}$Fm and the transfermium nuclei $^{249-252}$Md, and $^{254}$No, produced by hot- and cold-fusion reactions, in the vicinity of the deformed $N=152$ neutron shell closure, have been directly measured using a multireflection time-of-flight mass spectrograph. The masses of $^{246}$Es and $^{249,250,252}$Md were measured for the first time. Using the masses of $^{249,250}$Md as anchor points for $α$ decay chains, the masses of heavier nuclei, up to $^{261}$Bh and $^{266}$Mt, were determined. These new masses were compared with theoretical global mass models and demonstrated to be in good agreement with macroscopic-microscopic models in this region. The empirical shell gap parameter $δ_{2n}$ derived from three isotopic masses was updated with the new masses and corroborate the existence of the deformed $N=152$ neutron shell closure for Md and Lr.

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arXiv2018

Atomic masses of intermediate-mass neutron-deficient nuclei with relative uncertainty down to 35-ppb via multireflection time-of-flight mass spectrograph

High-precision mass measurements of $^{63}$Cu, $^{64-66}$Zn, $^{65}$Ga, $^{65-67}$Ge, $^{67}$As, $^{78,81}$Br, $^{80}$Rb, and $^{79}$Sr were performed utilizing a multireflection time-of-flight mass spectrograph combined with the gas-filled recoil ion separator GARIS-II. In the case of $^{65}$Ga, a mass uncertainty of 2.1 keV, corresponding to a relative precision of $δm / m = 3.5\times10^{-8}$, was obtained and the mass value is in excellent agreement with the 2016 Atomic Mass Evaluation. For $^{67}$Ge and $^{81}$Br, where masses were previously deduced through indirect measurements, discrepancies with literature values were found. The feasibility of using this device for mass measurements of nuclides more neutron-deficient side, which have significant impact on the $rp$-process pathway, is discussed.

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arXiv2017

Study of the long-lived excited state in the neutron deficient nuclides $^{195,197,199}$Po by precision mass measurement

Direct mass measurements of the low-spin $3/2^{(-)}$ and high-spin $13/2^{(+)}$ states in the neutron-deficient isotopes $^{195}$Po, $^{197}$Po, and high-spin $13/2^{(+)}$ state in $^{199}$Po were performed with the Penning-trap mass spectrometer ISOLTRAP at ISOLDE-CERN. These measurements allow the determination of the excitation energy of the isomeric state arising from the $ν$i$_{13/2}$ orbital in $^{195,197}$Po. Additionally, the excitation energy of isomeric states of lead, radon, and radium isotopes in this region were obtained from $α$-decay chains. The new excitation energies complete the knowledge of the energy systematics in the region and confirm for the first time that the $13/2^{(+)}$ states remain isomeric, independent of the number of valence neutrons.

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arXiv2015

Precision Mass Measurements of 129-131Cd and Their Impact on Stellar Nucleosynthesis via the Rapid Neutron Capture Process

Masses adjacent to the classical waiting-point nuclide 130Cd have been measured by using the Penning- trap spectrometer ISOLTRAP at ISOLDE/CERN. We find a significant deviation of over 400 keV from earlier values evaluated by using nuclear beta-decay data. The new measurements show the reduction of the N = 82 shell gap below the doubly magic 132Sn. The nucleosynthesis associated with the ejected wind from type-II supernovae as well as from compact object binary mergers is studied, by using state-of-the-art hydrodynamic simulations. We find a consistent and direct impact of the newly measured masses on the calculated abundances in the A = 128 - 132 region and a reduction of the uncertainties from the precision mass input data.

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arXiv2015

Probing the N = 32 shell closure below the magic proton number Z = 20: Mass measurements of the exotic isotopes 52,53K

The recently confirmed neutron-shell closure at N = 32 has been investigated for the first time below the magic proton number Z = 20 with mass measurements of the exotic isotopes 52,53K, the latter being the shortest-lived nuclide investigated at the online mass spectrometer ISOLTRAP. The resulting two-neutron separation energies reveal a 3 MeV shell gap at N = 32, slightly lower than for 52Ca, highlighting the doubly-magic nature of this nuclide. Skyrme-Hartree-Fock-Boguliubov and ab initio Gorkov-Green function calculations are challenged by the new measurements but reproduce qualitatively the observed shell effect.

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arXiv2011

Q-Value and Half-Lives for the Double-Beta-Decay Nuclide 110Pd

The 110Pd double-beta decay Q-value was measured with the Penning-trap mass spectrometer ISOLTRAP to be Q = 2017.85(64) keV. This value shifted by 14 keV compared to the literature value and is 17 times more precise, resulting in new phase-space factors for the two-neutrino and neutrinoless decay modes. In addition a new set of the relevant matrix elements has been calculated. The expected half-life of the two-neutrino mode was reevaluated as 1.5(6) E20 yr. With its high natural abundance, the new results reveal 110Pd to be an excellent candidate for double-beta decay studies.

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