arXiv subjects

M. S. Ferreira

Publications and source records attributed to M. S. Ferreira.

At least 37 records · Page 2Linked to original sources

arXiv2011

Magnetization profile for impurities in graphene nanoribbons

The magnetic properties of graphene-related materials and in particular the spin-polarised edge states predicted for pristine graphene nanoribbons (GNRs) with certain edge geometries have received much attention recently due to a range of possible technological applications. However, the magnetic properties of pristine GNRs are not predicted to be particularly robust in the presence of edge disorder. In this work, we examine the magnetic properties of GNRs doped with transition-metal atoms using a combination of mean-field Hubbard and Density Functional Theory techniques. The effect of impurity location on the magnetic moment of such dopants in GNRs is investigated for the two principal GNR edge geometries - armchair and zigzag. Moment profiles are calculated across the width of the ribbon for both substitutional and adsorbed impurities and regular features are observed for zigzag-edged GNRs in particular. Unlike the case of edge-state induced magnetisation, the moments of magnetic impurities embedded in GNRs are found to be particularly stable in the presence of edge disorder. Our results suggest that the magnetic properties of transition-metal doped GNRs are far more robust than those with moments arising intrinsically due to edge geometry.

cond-mat.mes-hall↗

arXiv2011

Graphene as a non-magnetic spin-current lens

In spintronics, the ability to transport magnetic information often depends on the existence of a spin current traveling between two different magnetic objects acting as source and probe. A large fraction of this information never reaches the probe and is lost because the spin current tends to travel omni-directionally. We propose that a curved boundary between a gated and a non-gated region within graphene acts as an ideal lens for spin currents despite being entirely of non-magnetic nature. We show as a proof of concept that such lenses can be utilized to redirect the spin current that travels away from a source onto a focus region where a magnetic probe is located, saving a considerable fraction of the magnetic information that would be otherwise lost.

cond-mat.mes-hall↗

arXiv2010

Monte-Carlo phase diagram of a Hubbard-Peierls model in the search for spin crossover transition in $π$-conjugated polymers

We present a Monte Carlo study of the finite temperature properties of an extended Hubbard-Peierls model describing one dimensional $π$-conjugated polymers. The model incorporates electron-phonon and hyperfine interaction and it is solved at the mean field level for half filling. In particular we explore the model as a function of the strength of electron-electron and electron-phonon interactions. At low temperature the system presents a diamagnetic to antiferromagnetic transition as the electron-electron interaction strength increases. At the same time by increasing the electron-phonon coupling there is a transition from a homogeneous to a Peierls dimerized geometry. As expected such a Peierls dimerized phase disappears at finite temperature as a result of thermal vibrations. More intriguing is the interplay between the electron-phonon and the electron-electron interactions at finite temperature. In particular we demonstrate that for a certain region of the parameter space there is a spin-crossover, where the system transits from a low-spin to a high-spin state as the temperature increases. In close analogy to standard spin-crossover in divalent magnetic molecules such a transition is entropy driven. Finally we discuss the role played by the hyperfine interaction over the phase diagram.

cond-mat.mes-hall↗

arXiv2010

A computationally efficient method for calculating the maximum conductance of disordered networks: Application to 1-dimensional conductors

Random networks of carbon nanotubes and metallic nanowires have shown to be very useful in the production of transparent, conducting films. The electronic transport on the film depends considerably on the network properties, and on the inter-wire coupling. Here we present a simple, computationally efficient method for the calculation of conductance on random nanostructured networks. The method is implemented on metallic nanowire networks, which are described within a single-orbital tight binding Hamiltonian, and the conductance is calculated with the Kubo formula. We show how the network conductance depends on the average number of connections per wire, and on the number of wires connected to the electrodes. We also show the effect of the inter-/intra-wire hopping ratio on the conductance through the network. Furthermore, we argue that this type of calculation is easily extendable to account for the upper conductivity of realistic films spanned by tunneling networks. When compared to experimental measurements, this quantity provides a clear indication of how much room is available for improving the film conductivity.

cond-mat.mes-hall↗

arXiv2010

Graphene-based spin-pumping transistor

We demonstrate with a fully quantum-mechanical approach that graphene can function as gate-controllable transistors for pumped spin currents, i.e., a stream of angular momentum induced by the precession of adjacent magnetizations, which exists in the absence of net charge currents. Furthermore, we propose as a proof of concept how these spin currents can be modulated by an electrostatic gate. Because our proposal involves nano-sized systems that function with very high speeds and in the absence of any applied bias, it is potentially useful for the development of transistors capable of combining large processing speeds, enhanced integration and extremely low power consumption.

cond-mat.mes-hall↗

arXiv2010

Carbon nanotube: a low-loss spin-current waveguide

We demonstrate with a quantum-mechanical approach that carbon nanotubes are excellent spin-current waveguides and are able to carry information stored in a precessing magnetic moment for long distances with very little dispersion and with tunable degrees of attenuation. Pulsed magnetic excitations are predicted to travel with the nanotube Fermi velocity and are able to induce similar excitations in remote locations. Such an efficient way of transporting magnetic information suggests that nanotubes are promising candidates for memory devices with fast magnetization switchings.

cond-mat.mes-hall↗

arXiv2009

Impurity segregation in graphene nanoribbons

The electronic properties of low-dimensional materials can be engineered by doping, but in the case of graphene nanoribbons (GNR) the proximity of two symmetry-breaking edges introduces an additional dependence on the location of an impurity across the width of the ribbon. This introduces energetically favorable locations for impurities, leading to a degree of spatial segregation in the impurity concentration. We develop a simple model to calculate the change in energy of a GNR system with an arbitrary impurity as that impurity is moved across the ribbon and validate its findings by comparison with ab initio calculations. Although our results agree with previous works predicting the dominance of edge disorder in GNR, we argue that the distribution of adsorbed impurities across a ribbon may be controllable by external factors, namely an applied electric field. We propose that this control over impurity segregation may allow manipulation and fine-tuning of the magnetic and transport properties of GNRs.

cond-mat.mes-hall↗

arXiv2009

Upper bound for the conductivity of nanotube networks

Films composed of nanotube networks have their conductivities regulated by the junction resistances formed between tubes. Conductivity values are enhanced by lower junction resistances but should reach a maximum that is limited by the network morphology. By considering ideal ballistic-like contacts between nanotubes we use the Kubo formalism to calculate the upper bound for the conductivity of such films and show how it depends on the nanotube concentration as well as on their aspect ratio. Highest measured conductivities reported so far are approaching this limiting value, suggesting that further progress lies with nanowires other than nanotubes.

cond-mat.mes-hall↗

arXiv2009

Emergence of local magnetic moments in doped graphene-related materials

Motivated by recent studies reporting the formation of localized magnetic moments in doped graphene, we investigate the energetic cost for spin polarizing isolated impurities embedded in this material. When a well-known criterion for the formation of local magnetic moments in metals is applied to graphene we are able to predict the existence of magnetic moments in cases that are in clear contrast to previously reported Density Functional Theory (DFT) results. When generalized to periodically repeated impurities, a geometry so commonly used in most DFT-calculations, this criterion shows that the energy balance involved in such calculations contains unavoidable contributions from the long-ranged pairwise magnetic interactions between all impurities. This proves the fundamental inadequacy of the DFT-assumption of independent unit cells in the case of magnetically doped low-dimensional graphene-based materials. We show that this can be circumvented if more than one impurity per unit cell is considered, in which case the DFT results agree perfectly well with the criterion-based predictions for the onset of localized magnetic moments in graphene. Furthermore, the existence of such a criterion determining whether or not a magnetic moment is likely to arise within graphene will be instrumental for predicting the ideal materials for future carbon-based spintronic applications.

cond-mat.mtrl-sci↗

arXiv2008

Indirect exchange coupling between localized magnetic moments in carbon nanotubes: a dynamic approach

Magnetic moments dilutely dispersed in a metallic host tend to be coupled through the conduction electrons of the metal. This indirect exchange coupling, known to occur for a variety of magnetic materials embedded in several different metallic structures, is of rather long range, especially for low-dimensional structures like carbon nanotubes. Motivated by recent claims that the indirect coupling between magnetic moments in precessional motion has a much longer range than its static counterpart, here we consider how magnetic atoms adsorbed to the walls of a metallic nanotube respond to a time-dependent perturbation that induces their magnetic moments to precess. By calculating the frequency-dependent spin susceptibility we are able to identify resonant peaks whose respective widths provide information about the dynamic aspect of the indirect exchange coupling. We show that by departing from a purely static representation to another in which the moments are allowed to precess, we change from what is already considered a long range interaction to another whose range is far superior. In other words, localized magnetic moments embedded in a metallic structure can feel each other's presence more easily when they are set in precessional motion. We argue that such an effect can have useful applications leading to large-scale spintronics devices.

cond-mat.str-el↗

arXiv2007

Non-collinear coupling between magnetic adatoms in carbon nanotubes

The long range character of the exchange coupling between localized magnetic moments indirectly mediated by the conduction electrons of metallic hosts often plays a significant role in determining the magnetic order of low-dimensional structures. In addition to this indirect coupling, here we show that the direct exchange interaction that arises when the moments are not too far apart may induce a non-collinear magnetic order that cannot be characterized by a Heisenberg-like interaction between the magnetic moments. We argue that this effect can be manipulated to control the magnetization alignment of magnetic dimers adsorbed to the walls of carbon nanotubes.

cond-mat.other↗

arXiv2005

Indirect exchange coupling between magnetic adatoms in carbon nanotubes

The long range character of the exchange coupling between localized magnetic moments indirectly mediated by the conduction electrons of metallic hosts can play a significant role in determining the magnetic order of low-dimensional structures. Here we consider how this indirect coupling influences the magnetic alignment of adatoms attached to the walls of carbon nanotubes. A general expression for the indirect coupling in terms of single-particle Green functions is presented. Contrary to the general property that magnetic moments embedded in a metal display Friedel-like oscillations in their magnetic response, calculated values for the coupling across metallic zigzag nanotubes show monotonic behaviour as a function of the adatom separation. Rather than an intrinsic property, the monotonicity is shown to reflect a commensurability effect in which the coupling oscillates with periods that coincide with the lattice parameter of the nanotube host. Such a commensurability effect does not dominate the coupling across semiconducting zigzag or metallic armchair nanotubes. We argue that such a long-range character in the magnetic interaction can be used in future spintronic devices.

cond-mat.other↗

arXiv2002

Multi-band quantum ratchets

We investigate directed motion in non-adiabatically rocked ratchet systems sustaining few bands below the barrier. Upon restricting the dynamics to the lowest M bands, the total system-plus-bath Hamiltonian is mapped onto a discrete tight-binding model containing all the information both on the intra- and inter-well tunneling motion. A closed form for the current in the incoherent tunneling regime is obtained. In effective single-band ratchets, no current rectification occurs. We apply our theory to describe rectification effects in vortex quantum ratchets devices. Current reversals upon variation of the ac-field amplitude or frequency are predicted.

cond-mat.mes-hall↗

arXiv1998

Exponential behavior of the interlayer exchange coupling across non-magnetic metallic superlattices

It is shown that the coupling between magnetic layers separated by non-magnetic metallic superlattices can decay exponentially as a function of the spacer thickness $N$, as opposed to the usual $N^{-2}$ decay. This effect is due to the lack of constructive contributions to the coupling from extended states across the spacer. The exponential behavior is obtained by properly choosing the distinct metals and the superlattice unit cell composition.

cond-mat.mes-hall↗

arXiv1997

Exchange coupling between magnetic layers across non-magnetic superlattices

The oscillation periods of the interlayer exchange coupling are investigated when two magnetic layers are separated by a metallic superlattice of two distinct non-magnetic materials. In spite of the conventional behaviour of the coupling as a function of the spacer thickness, new periods arise when the coupling is looked upon as a function of the number of cells of the superlattice. The new periodicity results from the deformation of the corresponding Fermi surface, which is explicitly related to a few controllable parameters, allowing the oscillation periods to be tuned.

cond-mat↗

arXiv1996

Fundamental Oscillation Periods of the Interlayer Exchange Coupling beyond the RKKY Approximation

A general method for obtaining the oscillation periods of the interlayer exchange coupling is presented. It is shown that it is possible for the coupling to oscillate with additional periods beyond the ones predicted by the RKKY theory. The relation between the oscillation periods and the spacer Fermi surface is clarified, showing that non-RKKY periods do not bear a direct correspondence with the Fermi surface. The interesting case of a FCC(110) structure is investigated, unmistakably proving the existence and relevance of non-RKKY oscillations. The general conditions for the occurrence of non-RKKY oscillations are also presented.

cond-mat.str-el↗

arXiv1996

Exchange Coupling Between Iron Layers Separated by BCC Copper

The exchange coupling between Fe layers separated by BCC Cu is calculated for Fe/Cu/Fe (001) trilayers. It is shown that the coupling is basically regulated by three extrema of the bulk BCC Cu Fermi surface. The contributions from those extrema are all of the same order of magnitude, but that associated with the ``belly'' at the $Γ$-point dominates. The calculated temperature dependence of the coupling varies considerably with spacer layer thickness. Individually, the amplitudes of these extrema contribution decrease with temperature, each according to a different rate. Such an effect may cause an actual increase of coupling with temperature for some Cu thicknesses.

cond-mat↗

arXiv1995

Non-RKKY oscillations of exchange coupling in magnetic multilayers

It is shown how the exchange coupling between two ferromagnetic planes embedded in an infinite non-magnetic metal, regarded as a function of the distance between the planes, may contain important components which oscillate with periods not predicted by RKKY theory. The interesting case of a FCC(110) structure with a Cu-like Fermi surface is discussed in detail.

cond-mat↗