arXiv subjects

M. S. Grbić

Publications and source records attributed to M. S. Grbić.

6 recordsLinked to original sources

arXiv2026

Magnetic-field-induced Tomonaga-Luttinger liquid and Bose-Einstein condensate phases in an organic S=1 Haldane chain

We present a comprehensive low-temperature $^1$H nuclear magnetic resonance (NMR) study of magnetic field-induced phases and spin fluctuations in an isotropic Haldane chain system $m$-NO$_2$PhBNO (BoNO) in fields up to 34 T. NMR spectral and $T_1^{-1}$ relaxation rate data are used to map out the transition temperature $T_c(B)$ and we show that it defines a complete phase boundary between the field-induced Bose-Einstein condensate (BEC) and Tomonaga-Luttinger liquid (TLL) phases by reproducing its shape via quantum Monte Carlo calculations. We also observe the theoretical critical behavior $T_c (B) \propto (B-B_\text{c2})^ν$ with $ν= 2/3$ and universal quasiparticle scaling in the low-temperature limit close to $B_\text{c2}$. The extensive Bayesian inference analysis of the temperature and field dependence of $T_1 ^{-1} (T,B)$ reveals attractive interactions across the TLL phase of a Haldane chain. Our results are further corroborated by magnetostriction measurements in pulsed magnetic fields and density matrix renormalization group calculations.

cond-mat.str-el↗

arXiv2026

Discovery of BKT correlations in the quantum kagome compound Cs$_2$Cu$_3$SnF$_{12}$

We investigate the microscopic properties of the kagome compound Cs$_2$Cu$_3$SnF$_{12}$ using $^{63,65}$Cu nuclear quadrupolar resonance (NQR). Analysis of the local hyperfine fields below the Néel temperature $T_N = 20$ K indicates a spin structure consistent with $P2_1/n$ symmetry of negative vector chirality. Measurements of the spin-lattice relaxation rate $T_1 ^{-1}$ reveal signatures of a gapless ground state and two-dimensional Berezinskii-Kosterlitz-Thouless (BKT)-type correlations above $T_N$, extending over a broad temperature range of approximately 130 K in zero magnetic field. Within the same temperature range, the observed increase in the NQR linewidth is consistent with short-range chiral order recently identified by neutron scattering. Our results establish Cs$_2$Cu$_3$SnF$_{12}$ as a unique quantum kagome system exhibiting BKT behavior.

cond-mat.str-el↗

arXiv2013

Microscopic properties of the "pinwheel" kagome compound Rb_2Cu_3SnF_{12}

Using $^{63,65}$Cu nuclear magnetic resonance (NMR) in magnetic fields up to 30 T we study the microscopic properties of the 12-site valence-bond-solid ground state in the "pinwheel" kagome compound Rb$_2$Cu$_3$SnF$_{12}$. We find that the ground state is characterized by a strong transverse staggered spin polarization whose temperature and field dependence points to a mixing of the singlet and triplet states. This is further corroborated by the field dependence of the gap $Δ(H)$, which has a level anticrossing with a large minimum gap value of $\approx Δ(0)/2$, with no evidence of a phase transition down to 1.5\,K. By the exact diagonalization of small clusters, we show that the observed anticrossing is mainly due to staggered tilts of the $g$-tensors defined by the crystal structure, and reveal symmetry properties of the low-energy excitation spectrum compatible with the absence of level crossing.

cond-mat.str-el↗

arXiv2012

Field-induced quantum soliton lattice in a frustrated two-leg spin-1/2 ladder

The field-induced quantum phase transitions (QPT) of the spin ladder material Bi(Cu(1-x)Znx)2PO6 have been investigated via 31P nuclear magnetic resonance (NMR) on single-crystal samples with x = 0 and x = 0.01. Measurements at temperatures between 0.25 K and 20 K in magnetic fields up to 31 T served to establish the nature of the various phases. In BiCu2PO6, an incommensurate (IC) magnetic order develops above a critical field mu0*H(c1) ~ 21 T; the field and temperature dependences of the NMR lines and the resulting model for the spin structure are discussed. Supported by results of Density-Matrix Renormalization Group (DMRG) calculations it is argued that the observed field-induced IC order involves the formation of a magnetic-soliton lattice. An additional QPT is predicted to occur at H > H(c1). For x = 0.01, this IC order is found to be stable against site disorder, although with a renormalized critical field.

cond-mat.str-el↗

arXiv2012

Quantum-critical spin dynamics in quasi-one-dimensional antiferromagnets

By means of nuclear spin-lattice relaxation rate 1/T1, we follow the spin dynamics as a function of the applied magnetic field in two gapped one-dimensional quantum antiferromagnets: the anisotropic spin-chain system NiCl2-4SC(NH2)2 and the spin-ladder system (C5H12N)2CuBr4. In both systems, spin excitations are confirmed to evolve from magnons in the gapped state to spinons in the gapples Tomonaga-Luttinger-liquid state. In between, 1/T1 exhibits a pronounced, continuous variation, which is shown to scale in accordance with quantum criticality. We extract the critical exponent for 1/T1, compare it to the theory, and show that this behavior is identical in both studied systems, thus demonstrating the universality of quantum critical behavior.

cond-mat.str-el↗

arXiv2008

Upper critical field, penetration depth, and depinning frequency of the novel high-temperature superconductor LaFeAsO$_{0.9}$F$_{0.1}$ studied by microwave surface impedance

Temperature and magnetic field dependent measurements of the microwave surface impedance of superconducting LaFeAsO$_{0.9}$F$_{0.1}$ (\Tc $\approx$ 26K) reveal a very large upper critical field ($B_{\rm c2} \approx 56$T) and a large value of the depinning frequency ($f_{0}\approx 6$GHz); together with an upper limit for the effective London penetration depth, $λ_{\rm eff} \le 200 \rm nm$, our results indicate a strong similarity between this system and the high-$T_{\rm c}$ superconducting cuprates.

cond-mat.supr-con↗