arXiv subjects

M. S. Laad

Publications and source records attributed to M. S. Laad.

61 records · Page 4Linked to original sources

arXiv2002

On the Normal State Electronic properties of Layered Sr_2 RuO_4

Based on a comprehensive perusal of experimental results, we construct a microscopic model describing the normal state of layered 4d oxide Sr_2 RuO_4 incorporating relevant quantum chemical features of the material. The high-T anomalies are explained within a Luttinger liquid (LL) picture. Interlayer one-particle hopping drives a dimensional crossover to a correlated Fermi liquid below a scale E^{*} << t_{perp}. Using recently developed chain-dynamical mean field theory, the low value of E^{*}, as well as various puzzling features of the low-T normal state are explained as manifestations of the crossover from the high-T Luttinger liquid state in a consistent way.

cond-mat↗

arXiv2002

On the heavy-fermion behavior of the pyrochlore transition-metal oxide $LiV_{2}O_{4}$

Motivated by the heavy fermion Fermi liquid (HFFL) features observed at low-$T$ in the pyrochlore $LiV_{2}O_{4}$, we consider a material-specific model that includes aspects of the local quantum chemistry, the geometrically frustrated lattice structure, and strong correlations in a {\it single} approach. In particular, we show how geometrical frustration (GF) gives rise to a crossover scale, $T^{*}<<J$, the intersite (AF) exchange, below which the metallic system shows HFFL features. Our scenario is a specific realization of the importance of GF effects in driving HFFL behavior in $LiV_{2}O_{4}$, and provides a natural understanding of various puzzling features observed experimentally.

cond-mat.str-el↗

arXiv2001

Dynamical correlations in half-metallic manganites

Motivated by the recent optical and photoemission measurements on half-metallic ferromagnetic three-dimensional manganites, we combine a tight-binding fit of the one-particle bandstructure with the dynamical mean-field theory, which treats the dynamical orbital correlations and the combination of Jahn-Teller and doping-induced disorder on the same footing. We show how all of the above effects are necessary to obtain good semiquantitative agreement with experimental features. As applications, we show how modest external magnetic fields drive drastic changes in the optical spectrum, demonstrating the {\it colossal ac magnetoconductivity}. The photoemission lineshape contribution is evaluated, and good agreement with published experimental work is found.

cond-mat.str-el↗

arXiv2001

On the Origin of the Non-Fermi Liquid Behavior of SrRuO_{3}

Motivated by the unusual features observed in the transport properties of the ferromagnetic "bad metal" $SrRuO_{3}$, we construct a model incorporating essential features of the realistic structure of this nearly cubic material. In particular, we show how the $t_{2g}$orbital {\it orientation} in the perfectly cubic structure determines the peculiar structure of the hybridization matrix, and demonstrate how the local non-Fermi liquid features arise when interactions are switched on. we discuss the effect of the slight deviation from the cubic structure (at low-$T$) qualitatively. The model provides a consistent explanation of the features observed recently in the optical response of $SrRuO_{3}$.

cond-mat.str-el↗

arXiv2001

Orbital Correlations in the Ferromagnetic Half-Metal $CrO_{2}

We deduce a model relevant for the description of the ferromagnetic half-metal Chromium dioxide ($CrO_{2}$), widely used in magnetic recording technology. The model describes the effect of dynamical, local orbital correlations arising from local quantum chemistry of the material. A finite temperature solution of the model in $d=\infty$ provides a natural explanation of the optical response, photoemission, resistivity and the large Woods-Saxon ratio observed in experiments. Our study confirms the important role of many body dynamical correlation effects for a proper understanding of the metallic phase of $CrO_{2}$.

cond-mat.str-el↗

arXiv2000

Role of Orbital Degeneracy in Double Exchange Systems

We investigate the role of orbital degeneracy in the double exchange (DE) model. In the $J_{H}\to\infty$ limit, an effective generalized ``Hubbard'' model incorporating orbital pseudospin degrees of freedom is derived. The model possesses an exact solution in one- and in infinite dimensions. In 1D, the metallic phase off ``half-filling'' is a Luttinger liquid with pseudospin-charge separation. Using the $d=\infty$ solution for our effective model, we show how many experimental observations for the well-doped ($x\simeq 0.3$) three-dimensional manganites $La_{1-x}Sr_{x}MnO_{3}$ can be qualitatively explained by invoking the role of orbital degeneracy in the DE model.

cond-mat.str-el↗

arXiv1999

Disordered Hubbard model in $d=\infty$

We investigate the effects of static, diagonal disorder in the $d=\infty$ Hubbard model by treating the dynamical effects of local Hubbard correlations and disorder on an equal footing. This is achieved by a proper combination of the iterated perturbation theory and the coherent potential approximation. Within the paramagnetic phase, we find that the renormalized Fermi liquid metal phase of the pure Hubbard model is stable against disorder for small disorder strengths. With increasing disorder, strong resonant scattering effects destroy low-energy Fermi liquid coherence, leading to an {\it incoherent} metallic non-FL state off half-filling. Finally, for large enough disorder, a {\it continuous} transition to the Mott-Anderson insulating phase occurs. The nature of the non-FL metallic phase, as well as the effects of the low energy coherence (incoherence) on optical conductivity and electronic Raman spectra, are considered in detail.

cond-mat.str-el↗