arXiv subjects

M. Spieker

Publications and source records attributed to M. Spieker.

35 records · Page 2Linked to original sources

arXiv2022

Investigation of octupole collectivity near the $A =72$ shape-transitional point

Enhanced octupole collectivity is expected in the neutron-deficient Ge, Se and Kr isotopes with neutron number $N \approx 40$ and has indeed been observed for $^{70,72}$Ge. Shape coexistence and configuration mixing are, however, a notorious challenge for theoretical models trying to reliably predict octupole collectivity in this mass region, which is known to feature rapid shape changes with changing nucleon number and spin of the system. To further investigate the microscopic configurations causing the prolate-oblate-triaxial shape transition at $A \approx 72$ and their influence on octupole collectivity, the rare isotopes $^{72}$Se and $^{74,76}$Kr were studied via inelastic proton scattering in inverse kinematics. While significantly enhanced octupole strength of $\sim 32$ Weisskopf units (W.u.) was observed for $^{72}$Se, only strengths of $\sim 15$ W.u. were observed for $^{74,76}$Kr. In combination with existing data, the new data clearly question a simple origin of enhanced octupole strengths around $N = 40$. The present work establishes two regions of distinct octupole strengths with a sudden strength increase around the $A=72$ shape transitional point.

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arXiv2020

Accessing the Single-Particle Structure of the Pygmy Dipole Resonance in $^{208}$Pb

New experimental data on the neutron single-particle character of the Pygmy Dipole Resonance (PDR) in $^{208}$Pb are presented. They were obtained from $(d,p)$ and resonant proton scattering experiments performed at the Q3D spectrograph of the Maier-Leibnitz Laboratory in Garching, Germany. The new data are compared to the large suite of complementary, experimental data available for $^{208}$Pb and establish $(d,p)$ as an additional, valuable, experimental probe to study the PDR and its collectivity. Besides the single-particle character of the states, different features of the strength distributions are discussed and compared to Large-Scale-Shell-Model (LSSM) and energy-density functional (EDF) plus Quasiparticle-Phonon Model (QPM) theoretical approaches to elucidate the microscopic structure of the PDR in $^{208}$Pb.

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arXiv2020

Collective 2p-2h intruder states in $^{118}$Sn studied via $β$-decay of $^{118}$In using GRIFFIN

The low-lying structure of semi-magic $^{118}$Sn has been investigated through the $β$-decay of $^{118}$In ($T_{1/2}=4.45$ min) to study shape coexistence via the reduced transition probabilities of states in the 2p-2h proton intruder band. This high-statistics study was carried out at TRIUMF-ISAC with the GRIFFIN spectrometer. In total, 99 transitions have been placed in the level scheme with 43 being newly observed. Three low-lying $γ$-ray transitions with energies near 285 keV have been resolved from which the 2$^+_{\mathrm{intr.}} \rightarrow 0^+_{\mathrm{intr.}}$ 284.52-keV transition was determined to have half of the previous branching fraction leading to a $B(E2;2^+_2\rightarrow 0^+_2)$ of 21(4) W.u. compared to 39(7) W.u. from the previous measurement. Calculations using $sd$ IBM-2 with mixing have also been made to compare the experimental $B(E2)$ values to the theoretical values and to make comparisons to the $^{114,116}$Sn isotopes previously studied using the same theoretical model.

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arXiv2020

Experimental identification of the $T = 1$, $J^π = 6^+$ state of $^{54}$Co and isospin symmetry in $A = 54$ studied via one-nucleon knockout reactions

New experimental data obtained from $γ$-ray tagged one-neutron and one-proton knockout from $^{55}$Co is presented. A candidate for the sought-after $T=1, T_z = 0, J^π = 6^+$ state in $^{54}$Co is proposed based on a comparison to the new data on $^{54}$Fe, the corresponding observables predicted by large-scale-shell-model (LSSM) calculations in the full $fp$-model space employing charge-dependent contributions, and isospin-symmetry arguments. Furthermore, possible isospin-symmetry breaking in the $A=54$, $T=1$ triplet is studied by calculating the experimental $c$ coefficients of the isobaric mass multiplet equation (IMME) up to the maximum possible spin $J=6$ expected for the $(1f_{7/2})^{-2}$ two-hole configuration relative to the doubly-magic nucleus $^{56}$Ni. The experimental quantities are compared to the theoretically predicted $c$ coefficients from LSSM calculations using two-body matrix elements obtained from a realistic chiral effective field theory potential at next-to-next-to-next-to-leading order (N$^3$LO).

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arXiv2020

Two-neutron knockout as a probe of the composition of states in $^{22}$Mg, $^{23}$Al, and $^{24}$Si

Simpson and Tostevin proposed that the width and shape of exclusive parallel momentum distributions of the A-2 residue in direct two-nucleon knockout reactions carry a measurable sensitivity to the nucleon single-particle configurations and their couplings within the wave functions of exotic nuclei. We report here on the first benchmarks and use of this new spectroscopic tool. Exclusive parallel momentum distributions for states in the neutron-deficient nuclei $^{22}$Mg, $^{23}$Al, and $^{24}$Si populated in such direct two-neutron removal reactions were extracted and compared to predictions combining eikonal reaction theory and shell-model calculations. For the well-known $^{22}$Mg and $^{23}$Al nuclei, measurements and calculations were found to agree, supporting the dependence of the parallel momentum distribution width on the angular momentum composition of the shell-model two-neutron amplitudes. In $^{24}$Si, a level at 3439(9) keV, of relevance for the important $^{23}$Al(p,$γ$)$^{24}$Si astrophysical reaction rate, was confirmed to be the $2^+_2$ state, while the $4^+_1$ state, expected to be strongly populated in two-neutron knockout, was not observed. This puzzle is resolved by theoretical considerations of the Thomas-Ehrman shift, which also suggest that a previously reported 3471-keV state in $^{24}$Si is in fact the ($0^+_2$) level with one of the largest experimental mirror-energy shifts ever observed.

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arXiv2019

One-proton and one-neutron knockout reactions from $N = Z = 28$ $^{56}$Ni to the $A = 55$ mirror pair $^{55}$Co and $^{55}$Ni

We present a high-resolution in-beam $γ$-ray spectroscopy study of excited states in the mirror nuclei $^{55}$Co and $^{55}$Ni following one-nucleon knockout from a projectile beam of $^{56}$Ni. The newly determined partial cross sections and the $γ$-decay properties of excited states provide a test of state-of-the-art nuclear structure models and probe mirror symmetry in unique ways. A mirror asymmetry for the partial cross sections leading to the two lowest $3/2^-$ states in the $A = 55$ mirror pair was identified as well as a significant difference in the $E1$ decays from the $1/2^+_1$ state to the same two $3/2^-$ states. The mirror asymmetry in the partial cross sections cannot be reconciled with the present shell-model picture or small mixing introduced in a two-state model. The observed mirror asymmetry in the $E1$ decay pattern, however, points at stronger mixing between the two lowest $3/2^-$ states in $^{55}$Co than in its mirror $^{55}$Ni.

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arXiv2019

Spectroscopy and lifetime measurements near the proton drip line: $^{26,27,28}$P

We report on the observation of excited states in the neutron-deficient phosphorus isotopes $^{26,27,28}$P via in-beam gamma-ray spectroscopy with both high-efficiency and high-resolution detector arrays. In $^{26}$P, a previously-unobserved level has been identified at 244(3) keV, two new measurements of the astrophysically-important 3/2$^+$ resonance in $^{27}$P have been performed, gamma decays have been assigned to the proton-unbound levels at 2216 keV and 2483 keV in $^{28}$P, and the gamma-ray lineshape method has been used to make the first determination of the lifetimes of the two lowest-lying excited states in $^{28}$P. The expected Thomas-Ehrman shifts were calculated and applied to levels in the mirror nuclei. The resulting level energies from this procedure were then compared with the energies of known states in $^{26,27,28}$P.

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arXiv2018

Fine structure of the pygmy quadrupole resonance in $^{112,114}$Sn isotopes

The electric quadrupole response in $^{112,114}$Sn isotopes is investigated by energy-density functional (EDF) and three-phonon quasiparticle-phonon model (QPM) theory with special emphasis on 2$^+$ excitations located above the first collective quadrupole state and below 5 MeV. Additional quadrupole strength clustering as a sequence of states similar to the recently observed pygmy quadrupole resonance in $^{124}$Sn is found. The spectral distributions and transition densities of these 2$^+$ states show special features being compatible with oscillations of a neutron skin against the isospin-symmetric nuclear core. Furthermore, two new ($p$, $p' γ$) Doppler-shift attenuation (DSA) coincidence experiments were performed at the SONIC@HORUS setup. Quadrupole states with excitation energies up to 4.2 MeV were populated in $^{112,114}$Sn. Lifetimes and branching ratios were measured allowing for the determination of the reduced quadrupole transition strengths to the ground state. A stringent comparison of the new data to EDF+QPM theory in $^{112}$Sn and $^{114}$Sn isotopes hints at the occurrence of a low-energy quadrupole mode of unique character which could be interpreted as pygmy quadrupole resonance.

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arXiv2018

Shape coexisistence and collective low-spin states in $^{112,114}$Sn studied with the $(p,p'γ)$ DSA coincidence technique

Proton-scattering experiments followed by the coincident spectroscopy of $γ$ rays have been performed at the Institute for Nuclear Physics of the University of Cologne to excite low-spin states in $^{112}$Sn and $^{114}$Sn, to determine their lifetimes and extract reduced transitions strengths $B(ΠL)$. The combined spectroscopy setup SONIC@HORUS has been used to detect the scattered protons and the emitted $γ$ rays of excited states in coincidence. The novel $(p,p'γ)$ DSA coincidence technique was employed to measure sub-ps nuclear level lifetimes. 74 level lifetimes $τ$ of states with $J = 0 - 6$ were determined. In addition, branching ratios were deduced which allowed the investigation of the intruder configuration in both nuclei. Here, $sd$ IBM-2 mixing calculations were added which support the coexistence of the two configurations. Furthermore, members of the expected QOC quintuplet are proposed in $^{114}$Sn for the first time. The $1^-$ candidate in $^{114}$Sn fits perfectly into the systematics observed for the other stable Sn isotopes. The $E2$ transition strengths observed for the low-spin members of the so-called intruder band support the existence of shape coexistence in $^{112,114}$Sn. The collectivity in this configuration is comparable to the one observed in the Pd nuclei, i.e. the 0p-4h nuclei. Strong mixing between the $0^+$ states of the normal and intruder configuration might be observed in $^{114}$Sn. The general existence of QOC states in $^{112,114}$Sn is supported by the observation of QOC candidates with $J \neq 1$.

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arXiv2018

High-resolution $(p,t)$ study of low-spin states in $^{240}$Pu: Octupole excitations, $α$ clustering, and other structure features

A high-resolution $(p,t)$ experiment at $E_{p}$= 24 MeV was performed to populate low-spin states in the actinide nucleus ${}^{240}$Pu. The Q3D magnetic spectrograph of the Maier-Leibnitz Laboratory (MLL) in Munich (Germany) was used to identify the ejected tritons via $dE/E$ particle identification with its focal-plane detection system. Angular distributions were measured at nine different Q3D angles to assign spin and parity to the excited states based on a comparison with coupled-channels DWBA calculations. In total, 209 states have been excited in $^{240}$Pu up to an excitation energy of 3 MeV. Many previously known states have also been observed and their spin-parity assignments were confirmed. However, many of the populated states have been seen for the first time. The low-spin one-octupole phonon excitations, i.e. $K^π = 0^-,1^-,2^-,3^-$, could be observed and a new candidate for the $K = 3$ projection is proposed. Furthermore, the double-octupole or $α$-cluster structure of the $0^+_2$ state in $^{240}$Pu has been studied in more detail. It is shown that the $0^+_2$ state in $^{230}$Th has a distinctly different structure. In addition, strongly excited $1^-$ states have been observed at 1.5\,MeV and 1.8\,MeV in $^{240}$Pu. The present study suggests that similar states might be observed in $^{230}$Th. At least two different and distinct structures for $J^π = 0^+$ states are present in the actinides. These are pairing states and states with enhanced octupole correlations. We have shown that it is crucial to consider negative-parity single-particle states being admixed to some $K^π = 0^+_2$ rotational bands to understand the $α$-decay hindrance factors and enhanced $E1$-decay rates. Based on our analysis, we have identified the double-octupole or $α$-cluster $K^π = 0^+$ candidates from $^{224}$Ra to $^{240}$Pu.

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arXiv2017

Combining γ-ray and particle spectroscopy with SONIC@HORUS

The particle spectrometer SONIC for particle-$γ$ coincidence measurements was commissioned at the Institute for Nuclear Physics in Cologne, Germany. SONIC consists of up to 12 silicon $\mathitΔE$-$E$ telescopes with a total solid angle coverage of 9%, and will complement HORUS, a $γ$-ray spectrometer with 14 HPGe detectors. The combined setup SONIC@HORUS is used to investigate the $γ$-decay behaviour of low-spin states up to the neutron separation threshold excited by light-ion inelastic scattering and transfer reactions using beams provided by a 10 MV FN Tandem accelerator. The particle-$γ$ coincidence method will be presented using data from a $^{92}$Mo(p,p'$γ$) experiment. In a $^{119}$Sn(d,X) experiment, excellent particle identification has been achieved because of the good energy resolution of the silicon detectors of approximately 20 keV. Due to the non-negligible momentum transfer in the reaction, a Doppler correction of the detected $γ$-ray energy has to be performed, using the additional information from measuring the ejectile energy and direction. The high sensitivity of the setup is demonstrated by the results from a $^{94}$Mo(p,p'$γ$) experiment, where small $γ$-decay branching ratios have been deduced.

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arXiv2015

Lifetime measurement of excited low-spin states via the $(p,p^{\prime}γ$) reaction

In this article a method for lifetime measurements in the sub-picosecond regime via the Doppler-shift attenuation method (DSAM) following the inelastic proton scattering reaction is presented. In a pioneering experiment we extracted the lifetimes of 30 excited low-spin states of $^{96}$Ru, taking advantage of the coincident detection of scattered protons and de-exciting $γ$-rays as well as the large number of particle and $γ$-ray detectors provided by the SONIC@HORUS setup at the University of Cologne. The large amount of new experimental data shows that this technique is suited for the measurement of lifetimes of excited low-spin states, especially for isotopes with a low isotopic abundance, where $(n,n^{\prime}γ$) or - in case of investigating dipole excitations - ($γ,γ^{\prime}$) experiments are not feasible due to the lack of sufficient isotopically enriched target material.

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arXiv2015

Origin of Low-Lying Enhanced E1 Strength in Rare-Earth Nuclei

The experimental $E1$ strength distribution below 4 MeV in rare-earth nuclei suggests a local breaking of isospin symmetry. In addition to the octupole states, additional $1^-$ states with enhanced E1 strength have been observed in rare-earth nuclei by means of ($γ,γ'$) experiments. By reproducing the experimental results, the spdf interacting boson model calculations provide further evidence for the formation of an $α$ cluster in medium-mass nuclei and might provide a new understanding of the origin of low-lying E1 strength.

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arXiv2015

Experimental constraints on the $γ$-ray strength function in $^{90}$Zr using partial cross sections of the $^{89}$Y(p,$γ$)$^{90}$Zr reaction

Partial cross sections of the $^{89}$Y(p,$γ$)$^{90}$Zr reaction have been measured to investigate the $γ$-ray strength function in the neutron-magic nucleus $^{90}$Zr. For five proton energies between $E_p=3.65$ MeV and $E_p=4.70$ MeV, partial cross sections for the population of seven discrete states in $^{90}$Zr have been determined by means of in-beam $γ$-ray spectroscopy. Since these $γ$-ray transitions are dominantly of $E1$ character, the present measurement allows an access to the low-lying dipole strength in $^{90}$Zr. A $γ$-ray strength function based on the experimental data could be extracted, which is used to describe the total and partial cross sections of this reaction by Hauser-Feshbach calculations successfully. Significant differences with respect to previously measured strength functions from photoabsorption data point towards deviations from the Brink-Axel hypothesis relating the photo-excitation and de-excitation strength functions.

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arXiv2015

Mixed-symmetry octupole and hexadecapole excitations in the N=52 isotones

Background: Excitations with mixed proton-neutron symmetry have been previously observed in the $N=52$ isotones. Besides the well established quadrupole mixed-symmetry states (MSS), octupole and hexadecapole MSS have been recently proposed for the nuclei $^{92}$Zr and $^{94}$Mo. Purpose: The heaviest stable $N=52$ isotone $^{96}$Ru was investigated to study the evolution of octupole and hexadecapole MSS with increasing proton number. Methods: Two inelastic proton-scattering experiments on $^{96}$Ru were performed to extract branching ratios, multipole mixing ratios, and level lifetimes. From the combined data, absolute transition strengths were calculated. Results: Strong $M1$ transitions between the lowest-lying $3^-$ and $4^+$ states were observed, providing evidence for a one-phonon mixed-symmetry character of the $3^{(-)}_2$ and $4^+_2$ states. Conclusions: $sdg$-IBM-2 calculations were performed for $^{96}$Ru. The results are in excellent agreement with the experimental data, pointing out a one-phonon hexadecapole mixed-symmetry character of the $4^+_2$ state. The $\big< 3^-_1||M1||3^{(-)}_2\big>$ matrix element is found to scale with the $<2^+_{\mathrm{s}}||M1||2^+_{\mathrm{ms}}>$ matrix element.

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arXiv2014

The gamma-ray spectrometer HORUS and its applications for nuclear astrophysics

A dedicated setup for the in-beam measurement of absolute cross sections of astrophysically relevant charged-particle induced reactions is presented. These, usually very low, cross sections at energies of astrophysical interest are important to improve the modeling of the nucleosynthesis processes of heavy nuclei. Particular emphasis is put on the production of the $p$ nuclei during the astrophysical $γ$ process. The recently developed setup utilizes the high-efficiency $γ$-ray spectrometer HORUS, which is located at the 10 MV FN tandem ion accelerator of the Institute for Nuclear Physics in Cologne. The design of this setup will be presented and results of the recently measured $^{89}$Y(p,$γ$)$^{90}$Zr reaction will be discussed. The excellent agreement with existing data shows, that the HORUS spectrometer is a powerful tool to determine total and partial cross sections using the in-beam method with high-purity germanium detectors.

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arXiv2013

Possible experimental signature of octupole correlations in the 0$^+_2$ states of the actinides

$J^π$= 0$^+$ states have been investigated in the actinide nucleus ${}^{240}$Pu up to an excitation energy of 3 MeV with a high-resolution (p,t) experiment at $E_{p}$= 24 MeV. To test the recently proposed $J^π$= 0$^+_2$ double-octupole structure, the phenomenological approach of the spdf-interacting boson model has been chosen. In addition, the total 0$^+$ strength distribution and the $0^+$ strength fragmentation have been compared to the model predictions as well as to the previously studied (p,t) reactions in the actinides. The results suggest that the structure of the 0$^+_2$ states in the actinides might be more complex than the usually discussed pairing isomers. Instead, the octupole degree of freedom might contribute significantly. The signature of two close-lying 0$^+$ states below the 2-quasiparticle energy is presented as a possible manifestation of strong octupole correlations in the structure of the 0$^+_2$ states in the actinides.

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