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M. Taniguchi

Publications and source records attributed to M. Taniguchi.

65 records · Page 4Linked to original sources

High-energy scale revival and giant kink in the dispersion of a cuprate superconductor

In the present photoemission study of a cuprate superconductor Bi1.74Pb0.38Sr1.88CuO6+delta, we discovered a large scale dispersion of the lowest band, which unexpectedly follows the band structure calculation very well. The incoherent nature of the spectra suggests that the hopping-dominated dispersion occurs possibly with the assistance of local spin correlations. A giant kink in the dispersion is observed, and the complete self-energy containing all interaction information is extracted for a doped cuprate in the low energy region. These results recovered significant missing pieces in our current understanding of the electronic structure of cuprates.

cond-mat.supr-con↗

Normal state electronic structure in the heavily overdoped regime of Bi1.74Pb0.38Sr1.88CuO6+delta single-layer cuprate superconductors

We explore the electronic structure in the heavily overdoped regime of the single layer cuprate superconductor Bi1.74Pb0.38Sr1.88CuO6+delta. We found that the nodal quasiparticle behavior is dominated mostly by phonons, while the antinodal quasiparticle lineshape is dominated by spin fluctuations. Moreover, while long range spin fluctuations diminish at very high doping, the local magnetic fluctuations still dominate the quasiparticle dispersion, and the system exhibits a strange metal behavior in the entire overdoped regime.

cond-mat.supr-con↗

Electronic Structure of Charge- and Spin-controlled Sr_{1-(x+y)}La_{x+y}Ti_{1-x}Cr_{x}O_{3}

We present the electronic structure of Sr_{1-(x+y)}La_{x+y}Ti_{1-x}Cr_{x}O_{3} investigated by high-resolution photoemission spectroscopy. In the vicinity of Fermi level, it was found that the electronic structure were composed of a Cr 3d local state with the t_{2g}^{3} configuration and a Ti 3d itinerant state. The energy levels of these Cr and Ti 3d states are well interpreted by the difference of the charge-transfer energy of both ions. The spectral weight of the Cr 3d state is completely proportional to the spin concentration x irrespective of the carrier concentration y, indicating that the spin density can be controlled by x as desired. In contrast, the spectral weight of the Ti 3d state is not proportional to y, depending on the amount of Cr doping.

cond-mat.str-el↗

Bulk and surface-sensitive high-resolution photoemission study of Mott-Hubbard systems SrVO$_3$ and CaVO$_3$

We study the electronic structure of Mott-Hubbard systems SrVO$_{3}$ and CaVO$_3$ with bulk and surface-sensitive high-resolution photoemission spectroscopy (PES), using a VUV laser, synchrotron radiation and a discharge lamp ($hν$ = 7 - 21 eV). A systematic suppression of the density of states (DOS) within $\sim$ 0.2 eV of the Fermi level ($E_F$) is found on decreasing photon energy i.e. on increasing bulk sensitivity. The coherent band in SrVO$_{3}$ and CaVO$_3$ is shown to consist of surface and bulk derived features, separated in energy. The stronger distortion on surface of CaVO$_{3}$ compared to SrVO$_{3}$ leads to higher surface metallicity in the coherent DOS at $E_F$, consistent with recent theory.

cond-mat.str-el↗

Orbital selectivity of the kink in the dispersion of Sr2RuO4

We present detailed energy dispersions near the Fermi level on the monolayer perovskite ruthenate Sr2RuO4, determined by high-resolution angle-resolved photoemission spectroscopy. An orbital selectivity of the kink in the dispersion of Sr2RuO4 has been found: A kink for the Ru 4d_xy orbital is clearly observed, but not for the Ru 4d_yz and 4d_zx ones. The result provides insight into the origin of the kink.

cond-mat.supr-con↗

Nature of Well-Screened State in Hard X-ray Mn 2$p$ Core-Level Photoemission of La$_{1-x}$Sr$_x$MnO$_3$ Films

Using hard x-ray (HX ; $hν$ = 5.95 keV) synchrotron photoemission spectroscopy (PES), we study the intrinsic electronic structure of La$_{1-x}$Sr$_x$MnO$_3$ (LSMO) thin films. Comparison of Mn 2$p$ core-levels with Soft x-ray (SX ; $hν$ $\sim$ 1000 eV) -PES shows a clear additional well-screened feature only in HX-PES. Take-off-angle dependent data indicate its bulk ($\ge$ 20 Å) character. The doping and temperature dependence track the ferromagnetism and metallicity of the LSMO series. Cluster model calculations including charge transfer from doping induced states show good agreement, confirming this picture of bulk properties reflected in Mn 2$p$ core-levels using HX-PES.

cond-mat.str-el↗

Electronic structures of Cr$_{1-δ}$X (X=S, Te) studied by Cr 2p soft x-ray magnetic circular dichroism

Cr 2p core excited XAS and XMCD spectra of ferromagnetic Cr$_{1-δ}$Te with several concentrations of $δ$=0.11-0.33 and ferrimagnetic Cr$_{5}$S$_{6}$ have been measured. The observed XMCD lineshapes are found to very weakly depend on $δ$ for Cr$_{1-δ}$Te. The experimental results are analyzed by means of a configuration-interaction cluster model calculation with consideration of hybridization and electron correlation effects. The obtained values of the spin magnetic moment by the cluster model analyses are in agreement with the results of the band structure calculation.The calculated result shows that the doped holes created by the Cr deficiency exist mainly in the Te 5porbital of Cr$_{1-δ}$Te, whereas the holes are likely to be in Cr 3d state for Cr$_{5}$S$_{6}$.

cond-mat.mtrl-sci↗

Bulk Electronic structure of Na$_{0.35}$CoO$_{2}$.1.3H$_{2}$O

High-energy (h$ν$ = 5.95 keV) synchrotron Photoemission spectroscopy (PES) is used to study bulk electronic structure of Na$_{0.35}$CoO$_{2}$.1.3H$_{2}$O, the layered superconductor. In contrast to 3-dimensional doped Co oxides, Co $\it{2p}$ core level spectra show well-separated Co$^{3+}$ and Co$^{4+}$ ions. Cluster calculations suggest low spin Co$^{3+}$ and Co$^{4+}$ character, and a moderate on-site Coulomb correlation energy U$_{dd}\sim$3-5.5 eV. Photon dependent valence band PES identifies Co $\it{3d}$ and O $\it{2p}$ derived states, in near agreement with band structure calculations.

cond-mat.mtrl-sci↗

Soft X-ray magnetic circular dichroism study of the ferromagnetic Cr$_{1-δ}$Te

The 2p core excited XAS and XMCD spectra of Cr$_{1-δ}$Te with several concentrations of $δ$=0.11-0.33 have been measured. The observed XMCD lineshapes are found to very weakly depend on $δ$. The experimental results are analyzed in terms of the configuration-interaction picture with consideration of hybridization and electron correlation effects. The calculated result shows that CrTe can be classified into a charge transfer type material and created holes preferably exist in Te 5p orbitals in Cr deficient materials Cr$_{1-δ}$Te, which are in consistence with the observed XMCD feature and the reported band structure calculation.

cond-mat.mtrl-sci↗

Soft X-ray Magnetic Circular Dichroism of c(2x2) CuMn Ordered Surface Alloy

Mn 2p soft X-ray absorption (XAS) spectroscopy excited with circularly polarized synchrotron radiation has been applied to a new class of material, c(2x2)CuMn/Cu(001) two-dimensional ordered surface alloy. A significant X-ray magnetic circular dichroism (XMCD) signal has been clearly observed at T=25K, indicating the existence of the ferromagnetic state under the external magnetic field of 1.4 Tesla. The lineshape analyses of the XAS and XMCD spectra clearly show that the Mn 3d state is rather localized and has a high spin magnetic moment due to its half-filled character.

cond-mat.mtrl-sci↗

Electronic structure of Cr1-dS (d=0,0.17) with NiAs-type crystal structure

Valence-band and conduction-band electronic structure of CrS (d=0) and Cr5S6 (d=0.17) has been investigated by means of photoemission and inverse-photoemission spectroscopies. Bandwidth of the valence bands of Cr5S6 (8.5 eV) is wider than that of CrS (8.1 eV), though the Cr 3d partial density of states evaluated from the Cr 3p-3d resonant photoemission spectroscopy is almost unchanged between the two compounds with respect to the shapes including binding energies. The Cr 3d (t2g) exchange splitting energies of CrS and Cr5S6 are determined to be 3.9 and 3.3 eV, respectively.

cond-mat.mtrl-sci↗