arXiv subjects

M. V. Romalis

Publications and source records attributed to M. V. Romalis.

At least 19 recordsLinked to original sources

arXiv2024

Long spin-1/2 noble gas coherence times in mm-sized anodically bonded batch-fabricated $^{3}$He-$^{129}$Xe-$^{87}$Rb cells

As the only stable spin-1/2 noble gas isotopes, $^{3}$He and $^{129}$Xe are promising systems for inertial rotation sensing and searches for exotic spin couplings. Spin-1/2 noble gases have intrinsic coherence times on the order of hours to days, which allows for incredibly low frequency error of free-precession measurements. However relaxation in miniature cells is dominated by interactions with the cell wall, which limits the performance of a chip-scale sensor that uses noble gases. While $^{129}$Xe wall relaxation times have previously been limited to 10's of seconds in mm-sized cells, we demonstrate the first anodically bonded batch-fabricated cells with dual $^{3}$He-$^{129}$Xe isotopes and $^{87}$Rb in a 6~mm$^3$ volume with $^{3}$He and $^{129}$Xe $T_2$ coherence times of, respectively, 4 h and 300 s. We use these microfabricated cells in a dual noble-gas comagnetometer and discuss its limits.

physics.atom-ph↗

arXiv2023

Large-scale, Multi-pass, Two-chamber RF Atomic Magnetometer

We describe one of the largest radio-frequency RF atomic magnetometers presently operating. A total atomic volume of 128 $\mathrm{cm^3}$, with correspondingly large number of $^{87}$Rb atoms, can reduce atom noise. A total of 44 passes of the probe beam reduces photon-shot noise. The atomic vapor is divided between two chambers allowing for pumping of the cells individually; doing so with opposite-helicity light enables use as an intrinsic gradiometer. In this configuration, common-mode noise sources including light-shift noise can be reduced. Magnetic tuning fields can also be applied to the chambers individually, allowing simultaneous measurement of two frequencies. An application of this is in the search for contraband materials using Nuclear Quadrupole Resonance (NQR), for which simultaneous measurement can significantly reduce search times. We demonstrate dual-frequency measurement on an effective range of 423-531 kHz, corresponding to the NQR frequencies of ammonium nitrate NH$_4$NO$_3$ at the lowest value and potassium chlorate KClO$_3$ at the highest. We explore fundamental, as well as instrumental, noise contributions to the sensitivity in this system.

physics.atom-ph↗

arXiv2021

Femtotesla nearly quantum-noise-limited pulsed gradiometer at Earth-scale fields

We describe a finite fields magnetic gradiometer using an intense pulsed laser to polarize a $^{87}$Rb atomic ensemble and a compact VCSEL probe laser to detect paramagnetic Faraday rotation in a single multipass cell. We report differential magnetic sensitivity of $14$ fT/Hz$^{1/2}$ over a broad dynamic range including Earth's field magnitude and common-mode rejection ratio higher than $10^4$. We also observe a nearly quantum-noise-limited behaviour of the gradiometer, by comparing the experimental standard deviation of the estimated frequency difference against the Cramér-Rao lower bound in the presence of white photon shot-noise, atomic spin noise and atomic diffusion.

physics.atom-ph↗

arXiv2021

Comagnetometer probes of dark matter and new physics

We discuss the use of comagnetometry in studying new physics that couples to fermionic spin. Modern comagnetometry is -- in absolute energy units -- the most sensitive experimental technique for measuring the energy difference between quantum states, reaching sensitivities in the $10^{-26}\,$eV range. The technique suppresses the magnetic interactions of the spins, making searches for non-standard-model interactions possible. Many implementations have been developed and optimized for various uses. New physics scenarios which can be probed with comagnetometers include: EDMs, violations of Lorentz invariance, Goldstone bosons of new high-energy symmetries, CP-violating long-range forces, and axionic dark matter. We consider the prospects for improvements in the technique, and show -- based purely on signal-to-noise ratio with existing technology -- that there is room for several orders of magnitude in further improvement. We also evaluate several sources of systematic error and instability that may limit improvements.

hep-ph↗

arXiv2021

Heading errors in all-optical alkali-vapor magnetometers in geomagnetic fields

Alkali-metal atomic magnetometers suffer from heading errors in geomagnetic fields as the measured magnetic field depends on the orientation of the sensor with respect to the field. In addition to the nonlinear Zeeman splitting, the difference between Zeeman resonances in the two hyperfine ground states can also generate heading errors depending on initial spin polarization. We examine heading errors in an all-optical scalar magnetometer that uses free precession of polarized $^{87}\text{Rb}$ atoms by varying the direction and magnitude of the magnetic field at different spin polarization regimes. In the high polarization limit where the lower hyperfine ground state $F = 1$ is almost depopulated, we show that heading errors can be corrected with an analytical expression, reducing the errors by two orders of magnitude in Earth's field. We also verify the linearity of the measured Zeeman precession frequency with the magnetic field. With lower spin polarization, we find that the splitting of the Zeeman resonances for the two hyperfine states causes beating in the precession signals and nonlinearity of the measured precession frequency with the magnetic field. We correct for the frequency shifts by using the unique probe geometry where two orthogonal probe beams measure opposite relative phases between the two hyperfine states during the spin precession.

physics.atom-ph↗

arXiv2021

Femtotesla direct magnetic gradiometer using a single multipass cell

We describe a direct gradiometer using optical pumping with opposite circular polarization in two $^{87}$Rb atomic ensembles within a single multipass cell. A far-detuned probe laser undergoes a near-zero paramagnetic Faraday rotation due to the intrinsic subtraction of two contributions exceeding 3.5 rad from the highly-polarized ensembles. We develop analysis methods for the direct gradiometer signal and measure a gradiometer sensitivity of $10.1$ fT/cm$\sqrt{\mathrm{Hz}}$. We also demonstrate that our multipass design, in addition to increasing the optical depth, provides a fundamental advantage due to the significantly reduced effect of atomic diffusion on the spin noise time-correlation, in excellent agreement with theoretical estimate.

physics.atom-ph↗

arXiv2020

Portable magnetometry for detection of biomagnetism in ambient environments

We present a method of optical magnetometry with parts-per-billion resolution that is able to detect biomagnetic signals generated from the human brain and heart in Earth's ambient environment. Our magnetically silent sensors measure the total magnetic field by detecting the free-precession frequency of highly spin-polarized alkali metal vapor. A first-order gradiometer is formed from two magnetometers that are separated by a 3 cm baseline. Our gradiometer operates from a laptop consuming 5 W over a USB port, enabled by state-of-the-art micro-fabricated alkali vapor cells, advanced thermal insulation, custom electronics, and laser packages within the sensor head. The gradiometer obtains a sensitivity of 16 fT/cm/Hz$^{1/2}$ outdoors, which we use to detect neuronal electrical currents and magnetic cardiography signals. Recording of neuronal magnetic fields is one of a few available methods for non-invasive functional brain imaging that usually requires extensive magnetic shielding and other infractructure. This work demonstrates the possibility of a dense array of portable biomagnetic sensors that are deployable in a variety of natural environments.

physics.med-ph↗

arXiv2018

Dipolar and scalar $^3$He and $^{129}$Xe frequency shifts in mm-sized cells

We describe a $^{3}$He-$^{129}$Xe comagnetometer operating in stemless anodically bonded cells with a 6 mm$^3$ volume and a $^{129}$Xe spin coherence time of 300 sec. We use a $^{87}$Rb pulse-train magnetometer with co-linear pump and probe beams to study the nuclear spin frequency shifts caused by spin polarization of $^{3}$He. By systematically varying the cell geometry in a batch cell fabrication process we can separately measure the cell shape dependent and independent frequency shifts. We find that a certain aspect ratio of the cylindrical cell can cancel the effects of $^3$He magnetization that limit the stability of vapor-cell comagnetometers. Using this control we also observe for the first time a scalar $^{3}$He-$^{129}$Xe collisional frequency shift characterized by an enhancement factor $κ_{\text{HeXe}} = -0.011\pm0.001$.

physics.atom-ph↗

arXiv2017

Correlation function of spin noise due to atomic diffusion

We use paramagnetic Faraday rotation to study spin noise spectrum from unpolarized Rb vapor in a tightly focused probe beam in the presence of N$_2$ buffer gas. We derive an analytical form for the diffusion component of the spin noise time-correlation function in a Gaussian probe beam. We also obtain analytical forms for the frequency spectrum of the spin noise in the limit of a tightly focused or a collimated Gaussian beam in the presence of diffusion. In particular, we find that in a tightly focused probe beam the spectral lineshape can be independent of the buffer gas pressure. Experimentally, we find good agreement between the calculated and measured spin noise spectra for N$_2$ gas pressures ranging from 56 to 820 torr.

quant-ph↗

arXiv2017

$^{3}$He-$^{129}$Xe Comagnetometery using $^{87}$Rb Detection and Decoupling

We describe a $^{3}$He-$^{129}$Xe comagnetometer using $^{87}$Rb atoms for noble-gas spin polarization and detection. We use a train of $^{87}$Rb $π$ pulses and $σ^+/σ^-$ optical pumping to realize a finite-field Rb magnetometer with suppression of spin-exchange relaxation. We suppress frequency shifts from polarized Rb by measuring the $^{3}$He and $^{129}$Xe spin precession frequencies in the dark, while applying $π$ pulses along two directions to depolarize Rb atoms. The plane of the $π$ pulses is rotated to suppress the Bloch-Siegert shifts for the nuclear spins. We measure the ratio of $^{3}$He to $^{129}$Xe spin precession frequencies with sufficient absolute accuracy to resolve the Earth's rotation without changing the orientation of the comagnetometer. A frequency resolution of 7 nHz is achieved after integration for 8 hours without evidence of significant drift.

physics.atom-ph↗

arXiv2017

Nuclear Matrix Elements for Tests of Local Lorentz Invariance Violation

The nuclear matrix elements for the momentum quadrupole operator are important for the interpretation of precision atomic physics experiments that search for violations of local Lorentz and CPT symmetry and for new spin-dependent forces. We use the configuration-interaction nuclear shell model and self-consistent mean field theory to calculate these matrix elements in $^{21}$Ne, $^{23}$Na, $^{131}$Xe, $^{173}$Yb and $^{201}$Hg. These are the first microscopic calculations of the nuclear matrix elements for the momentum quadrupole tensor that go beyond the single-particle estimate. We show that they are strongly suppressed by the many-body correlations, in contrast to the well known enhancement of the spatial quadrupole nuclear matrix elements.

nucl-th↗

arXiv2017

Effects of the Lorentz invariance violation in Coulomb interaction in nuclei and atoms

Anisotropy in the speed of light that has been constrained by Michelson-Morley-type experiments also generates anisotropy in the Coulomb interactions. This anisotropy can manifest itself as an energy anisotropy in nuclear and atomic experiments. Here the experimental limits on Lorentz violation in 21Ne are used to improve the limits on the Lorentz symmetry in the photon sector, namely the anisotropy of the speed of light and the Coulomb interactions, by 7 orders of magnitude in comparison with previous experiments: the speed of light is isotropic to a part in E-28.

nucl-th↗

arXiv2012

Sub-femtotesla scalar atomic magnetometer using multipass cells

Scalar atomic magnetometers have many attractive features but their sensitivity has been relatively poor. We describe a Rb scalar gradiometer using two multi-pass optical cells. We use a pump-probe measurement scheme to suppress spin-exchange relaxation and two probe pulses to find the spin precession zero crossing times with a resolution of 1 psec. We realize magnetic field sensitivity of 0.54 fT/Hz$^{1/2}$, which improves by an order of magnitude the best scalar magnetometer sensitivity and surpasses the quantum limit set by spin-exchange collisions for a scalar magnetometer with the same measurement volume operating in a continuous regime.

physics.atom-ph↗

arXiv2011

A new test of local Lorentz invariance using $^{21}$Ne-Rb-K comagnetometer

We develop a new comagnetometer using $^{21}$Ne atoms with nuclear spin $I=3/2$ and Rb atoms polarized by spin-exchange with K atoms to search for tensor interactions that violate local Lorentz invariance. We frequently reverse orientation of the experiment and search for signals at the first and second harmonics of the sidereal frequency. We constrain 4 of the 5 spatial Lorentz-violating coefficients $c^n_{jk}$ that parameterize anisotropy of the maximum attainable velocity of a neutron at a level of $10^{-29}$, improving previous limits by 2 to 4 orders of magnitude and placing the most stringent constrain on deviations from local Lorentz invariance.

physics.atom-ph↗

arXiv2011

Very large optical rotation generated by Rb vapor in a multi-pass cell

Paramagnetic Faraday rotation is a powerful technique for atom sensing widely used in quantum non-demolition measurements, fundamental symmetry tests, and other precision measurements. We demonstrate the use of a multi-pass optical cell for Faraday rotation spectroscopy and observe polarization rotation in excess of 100 radians from spin-polarized Rb vapor. Unlike optical cavities, multi-pass cells have a deterministic number of light passes and can be used to measure large optical rotations. We also observe a 10-fold suppression of transverse spin relaxation when Rb atoms are placed in a coherent superposition state immune to spin-exchange collisions.

physics.atom-ph↗

arXiv2011

Measurement of Linear Stark Interference in 199Hg

We present measurements of Stark interference in the 6$^1S_0$ $\rightarrow$ 6$^3P_1$ transition in $^{199}$Hg, a process whereby a static electric field $E$ mixes magnetic dipole and electric quadrupole couplings into an electric dipole transition, leading to $E$-linear energy shifts similar to those produced by a permanent atomic electric dipole moment (EDM). The measured interference amplitude, $a_{SI}$ = $(a_{M1} + a_{E2})$ = (5.8 $\pm$ 1.5)$\times 10^{-9}$ (kV/cm)$^{-1}$, agrees with relativistic, many-body predictions and confirms that earlier central-field estimates are a factor of 10 too large. More importantly, this study validates the capability of the $^{199}$Hg EDM search apparatus to resolve non-trivial, controlled, and sub-nHz Larmor frequency shifts with EDM-like characteristics.

physics.atom-ph↗

arXiv2010

Stroboscopic back-action evasion in a dense alkali-metal vapor

We explore experimentally quantum non-demolition (QND) measurements of atomic spin in a hot potassium vapor in the presence of spin-exchange relaxation. We demonstrate a new technique for back-action evasion by stroboscopic modulation of the probe light. With this technique we study spin noise as a function of polarization for atoms with spin greater than 1/2 and obtain good agreement with a simple theoretical model. We point that in a system with fast spin-exchange, where the spin relaxation rate is changing with time, it is possible to improve the long-term sensitivity of atomic magnetometry by using QND measurements.

quant-ph↗

arXiv2010

Hybrid optical pumping of optically dense alkali-metal vapor without quenching gas

Optical pumping of an optically thick atomic vapor typically requires a quenching buffer gas, such as N$_{2}$, to prevent radiation trapping of unpolarized photons which would depolarize the atoms. We show that optical pumping of a trace contamination of Rb present in K metal results in a 4.5 times higher polarization of K than direct optical pumping of K in the absence of N$_{2}$. Such spin-exchange polarization transfer from optically-thin species is useful in a variety of areas, including spin-polarized nuclear scattering targets and electron beams, quantum-non-demolition spin measurements, and ultra-sensitive magnetometry.

physics.atom-ph↗