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M. W. Ahmed

Publications and source records attributed to M. W. Ahmed.

At least 19 recordsLinked to original sources
arXiv2026

Photonuclear Cross Sections for the $^{197}$Au($γ$,pn)$^{195m}$Pt Reaction Near Threshold

Platinum radioisotopes are of growing interest for targeted cancer therapy and diagnostic imaging because their decay delivers highly localized radiation doses in tissue, herewith enabling precise DNA damage through Auger-electron emission. Developing production technologies that provide platinum isotopes with high specific activity is therefore essential, and photonuclear reactions on stable nuclei offer a viable accelerator-based route when supported by reliable cross-section data. We report photonuclear cross-section measurements for the $^{197}$Au($γ$,pn)$^{195m}$Pt reaction at incident $γ$-ray energies of 27, 29, and 31 MeV using the activation method. The measurements were performed by irradiating a stack of concentric-ring gold targets with a quasi-monoenergetic $γ$-ray beam provided by the High Intensity Gamma-ray Source (HI$γ$S). The induced $^{195m}$Pt activity was quantified using off-line $γ$-ray spectroscopy. These data provide the first experimental constraints on the $^{197}$Au($γ$,pn)$^{195m}$Pt cross section in the near-threshold region. The measured excitation function is compared with PHITS and TALYS calculations and indicates that the reaction becomes measurable only near 30 MeV, with substantially higher bremsstrahlung end-point energies required for practically meaningful production.

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arXiv2024

Photo-nuclear cross sections on $^{197}$Au, an update on the gold standard

A method was developed for measuring photonuclear reactions concurrently at several discrete photon beam energies on a stack of different target materials via a single irradiation. Concentric ring targets of the materials (in order from front to back targets: Au, TiO$_2$, Zn, Os, and Au) were irradiated at the High Intensity Gamma-ray Source (HI$γ$S). As a proof of principle, we report the result of the cross section measurements from the front Au target. The excitation functions of the $^{197}$Au($γ$,n)$^{196}$Au and $^{197}$Au($γ$,3n)$^{194}$Au reactions were determined in the incident photon energy range of 13-31 MeV using quasi-monoenergetic photon beams provided at HI$γ$S. The cross sections of the combined ground state (2$^{-}$) and short-lived first isomeric state (m1, 5$^{+}$), and of the second isomeric state (m2, 12$^{-}$) in the $^{196}$Au production are obtained separately by subtracting the $γ$ rays from the internal conversion of the second isomeric state. The excitation function of the second isomeric state via the photon-induced reaction $^{197}$Au($γ$,n)$^{196m2}$Au was measured for the first time. By using the activation method rather than direct neutron counting, the exclusive cross sections for the ($γ$,n) and ($γ$,3n) reactions were determined. Comparing the yields from the front and back gold targets validates our ability to simulate the effect of photon scattering in the target stack and provides a method for assessing the systematic uncertainty of our technique.

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arXiv2022

Proton Compton Scattering from Linearly Polarized Gamma Rays

Differential cross sections for Compton scattering from the proton have been measured at scattering angles of $55^\circ$, $90^\circ$, and $125^\circ$ in the laboratory frame using quasimonoenergetic linearly (circularly) polarized photon beams with a weighted mean energy value of 83.4\,MeV (81.3\,MeV). These measurements were performed at the High Intensity Gamma-Ray Source facility at the Triangle Universities Nuclear Laboratory. The results are compared to previous measurements and are interpreted in the chiral effective field theory framework to extract the electromagnetic dipole polarizabilities of the proton, which gives $α_{E1}^p = 13.8\pm1.2_{\rm stat}\pm0.1_{\rm BSR}\pm0.3_{\rm theo}, β_{M1}^p = 0.2\mp1.2_{\rm stat}\pm0.1_{\rm BSR}\mp0.3_{\rm theo}$ in units of 10$^{-4}$\, fm$^3$.

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arXiv2020

International Workshop on Next Generation Gamma-Ray Source

A workshop on The Next Generation Gamma-Ray Sources sponsored by the Office of Nuclear Physics at the Department of Energy, was held November 17--19, 2016 in Bethesda, Maryland. The goals of the workshop were to identify basic and applied research opportunities at the frontiers of nuclear physics that would be made possible by the beam capabilities of an advanced laser Compton beam facility. To anchor the scientific vision to realistically achievable beam specifications using proven technologies, the workshop brought together experts in the fields of electron accelerators, lasers, and optics to examine the technical options for achieving the beam specifications required by the most compelling parts of the proposed research programs. An international assembly of participants included current and prospective $γ$-ray beam users, accelerator and light-source physicists, and federal agency program managers. Sessions were organized to foster interactions between the beam users and facility developers, allowing for information sharing and mutual feedback between the two groups. The workshop findings and recommendations are summarized in this whitepaper.

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arXiv2020

First Measurement of the Asymmetry and the Gerasimov-Drell-Hearn Integrand from $\vec{{^3}He}(\vecγ,p)d$ reaction at the Incident Photon Energy of 29 MeV

The first measurement of the $\vec{^3He}(\vecγ,p)d$ process was performed at the High Intensity $γ$-ray Source (HI$γ$S) facility at Triangle Universities Nuclear Laboratory (TUNL) using a circularly polarized, monoenergetic $γ$-ray beam and a longitudinally polarized $^3$He target. The spin-dependent asymmetry and the contribution from the two-body photodisintegration to the $^3$He Gerasimov-Drell-Hearn integrand are extracted and compared with state-of-the-art three-nucleon system calculations at the incident photon energy of 29.0 MeV. The data are in general agreement with the various theoretical predictions based on the Siegert theorem or on explicit inclusion of meson-exchange currents.

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arXiv2020

Compton scattering from $^4$He at the TUNL HI$γ$S facility

Differential cross sections for elastic Compton scattering from $^4$He have been measured with high statistical precision at the High Intensity $γ$-ray Source at laboratory scattering angles of $55^\circ$, $90^\circ$, and $125^\circ$ using a quasi-monoenergetic photon beam with a weighted mean energy value of $81.3$ MeV. The results are compared to previous measurements and similar fore-aft asymmetry in the angular distribution of the differential cross sections is observed. This experimental work is expected to strongly motivate the development of effective-field-theory calculations of Compton scattering from $^4$He to fully interpret the data.

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arXiv2020

A stringent upper limit on the direct 3$α$ decay of the Hoyle State in $^{12}$C

We investigate an implication of the most recent observation of a second $J^π= 2^+$ state in $^{12}$C, which was measured using the $^{12}$C($γ$,$α$)$^8$Be$_{\textrm{(g.s.)}}$ reaction. In addition to the dissociation of $^{12}$C to an $α$-particle and $^8$Be in its ground state, a small fraction of events (2%) were identified as direct decays and decays to excited states in $^8$Be. This allowed a limit on the direct 3$α$ partial decay width to be determined as $Γ_{3α} < 32(4)$ keV. Since this 2$^+$ state is predicted by all theoretical models to be a collective excitation of the Hoyle state, the 3$α$ partial width of the Hoyle state is calculable from the ratio of 3$α$ decay penetrabilities of the Hoyle and 2$^+$ states. This was calculated using the semi-classical WKB approach and we deduce a stringent upper limit for the direct decay branching ratio of the Hoyle state of ${Γ_{3α} \over Γ} < 5.7 \times 10^{-6}$, over an order of magnitude lower than previously reported. This result places the direct measurement of this rare decay mode beyond current experimental capabilities.

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arXiv2019

A New Cryogenic Apparatus to Search for the Neutron Electric Dipole Moment

A cryogenic apparatus is described that enables a new experiment, nEDM@SNS, with a major improvement in sensitivity compared to the existing limit in the search for a neutron Electric Dipole Moment (EDM). It uses superfluid $^4$He to produce a high density of Ultra-Cold Neutrons (UCN) which are contained in a suitably coated pair of measurement cells. The experiment, to be operated at the Spallation Neutron Source at Oak Ridge National Laboratory, uses polarized $^3$He from an Atomic Beam Source injected into the superfluid $^4$He and transported to the measurement cells as a co-magnetometer. The superfluid $^4$He is also used as an insulating medium allowing significantly higher electric fields, compared to previous experiments, to be maintained across the measurement cells. These features provide an ultimate statistical uncertainty for the EDM of $2-3\times 10^{-28}$ e-cm, with anticipated systematic uncertainties below this level.

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arXiv2018

Time Projection Chamber (TPC) Detectors for Nuclear Astrophysics Studies With Gamma Beams

Gamma-Beams at the HIgS facility in the USA and anticipated at the ELI-NP facility, now constructed in Romania, present unique new opportunities to advance research in nuclear astrophysics; not the least of which is resolving open questions in oxygen formation during stellar helium burning via a precise measurement of the 12C(a,g) reaction. Time projection chamber (TPC) detectors operating with low pressure gas (as an active target) are ideally suited for such studies. We review the progress of the current research program and plans for the future at the HIγS facility with the optical readout TPC (O-TPC) and the development of an electronic readout TPC for the ELI-NP facility (ELITPC).

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arXiv2015

Measurement of the Doubly-Polarized $\vec{{^3}He}(\vecγ,n)pp$ Reaction at 16.5 MeV and Its Implications for the GDH Sum Rule

We report new measurements of the doubly-polarized photodisintegration of $^3$He at an incident photon energy of 16.5 MeV, carried out at the High Intensity $γ$-ray Source (HI$γ$S) facility located at Triangle Universities Nuclear Laboratory (TUNL). The spin-dependent double-differential cross sections and the contribution from the three--body channel to the Gerasimov-Drell-Hearn (GDH) integrand were extracted and compared with the state-of-the-art three--body calculations. The calculations, which include the Coulomb interaction and are in good agreement with the results of previous measurements at 12.8 and 14.7 MeV, can no longer describe the cross section results at 16.5 MeV. The GDH integrand was found to be about one standard deviation larger than the maximum value predicted by the theories.

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arXiv2014

Compton Scattering from \nuc{6}{Li} at 86 MeV

Cross sections for \nuc{6}{Li}($γ$,$γ$)\nuc{6}{Li} have been measured at the High Intensity Gamma-Ray Source (\HIGS) and the sensitivity of these cross sections to the nucleon isoscalar polarizabilities was studied. Data were collected using a quasi-monoenergetic 86 MeV photon beam at photon scattering angles of 40$^{\circ}$--160$^{\circ}$. These results are an extension of a previous measurement at a lower energy. The earlier work indicated that the \nuc{6}{Li}($γ$,$γ$)\nuc{6}{Li} reaction at 60 MeV provides a means of extracting the nucleon polarizabilities; this work demonstrates that the sensitivity of the cross section to the polarizabilities is increased at 86 MeV. A full theoretical treatment is needed to verify this conclusion and produce values of the polarizabilities.

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arXiv2013

A Segmented, Enriched N-type Germanium Detector for Neutrinoless Double Beta-Decay Experiments

We present data characterizing the performance of the first segmented, N-type Ge detector, isotopically enriched to 85% $^{76}$Ge. This detector, based on the Ortec PT6x2 design and referred to as SEGA (Segmented, Enriched Germanium Assembly), was developed as a possible prototype for neutrinoless double beta-decay measurements by the {\sc Majorana} collaboration. We present some of the general characteristics (including bias potential, efficiency, leakage current, and integral cross-talk) for this detector in its temporary cryostat. We also present an analysis of the resolution of the detector, and demonstrate that for all but two segments there is at least one channel that reaches the {\sc Majorana} resolution goal below 4 keV FWHM at 2039 keV, and all channels are below 4.5 keV FWHM.

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arXiv2013

First Measurements of Spin-Dependent Double-Differential Cross Sections and the GDH Integrand from \vec{^3He}(\vecγ,n)pp at Incident Photon Energies of 12.8 and 14.7 MeV

The first measurement of the three-body photodisintegration of longitudinally-polarized ^3He with a circularly-polarized γ-ray beam was carried out at the High Intensity γ-ray Source (HIγS) facility located at Triangle Universities Nuclear Laboratory (TUNL). The spin-dependent double-differential cross sections and the contributions from the three-body photodisintegration to the ^3He GDH integrand are presented and compared with state-of-the-art three-body calculations at the incident photon energies of 12.8 and 14.7 MeV. The data reveal the importance of including the Coulomb interaction between protons in three-body calculations.

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arXiv2013

Unambiguous Identification of the Second 2+ State in 12C and the Structure of the Hoyle State

The second 2+ state of 12C, predicted over fifty years ago as an excitation of the Hoyle state, has been unambiguously identified using the 12C(g,a_0)8Be reaction. The alpha particles produced by the photodisintegration of 12C were detected using an Optical Time Projection Chamber (O-TPC). Data were collected at beam energies between 9.1 and 10.7 MeV using the intense nearly mono-energetic gamma-ray beams at the HIgS facility. The measured angular distributions determine the cross section and the E1-E2 relative phases as a function of energy leading to an unambiguous identification of the second 2+ state in 12C at 10.03(11) MeV, with a total width of 800(130) keV and a ground state gamma-decay width of 60(10) meV; B(E2: 2+ ---> gs) = 0.73(13) e2fm4 [or 0.45(8) W.u.]. The Hoyle state and its rotational 2+ state that are more extended than the ground state of 12C presents a challenge and constraints for models attempting to reveal the nature of three alpha particle states in 12C. Specifically it challenges the ab-initio Lattice Effective Field Theory (L-EFT) calculations that predict similar r.m.s. radii for the ground state and the Hoyle state.

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arXiv2011

Search for the Neutron Electric Dipole Moment: Contributions from the Triangle Universities Nuclear Laboratory

A significant fraction of the research effort at the Triangle Universities Nuclear Laboratory (TUNL) focuses on weak interaction studies and searches for physics beyond the Standard Model. One major effort is the development of a new experimental technique to search for the neutron electric dipole moment (nEDM) that offers the potential for a factor of 100 increase in sensitivity over existing measurements. The search for this moment has the potential to reveal new sources of time reversal (T) and charge-conjugation-and-parity (CP) violation and to challenge calculations that propose extensions to the Standard Model. We provide a brief overview of the experiment as a whole and discuss the work underway at TUNL as part of this effort.

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arXiv2011

An Optical Readout TPC (O-TPC) for Studies in Nuclear Astrophysics With Gamma-Ray Beams at HIgS

We report on the construction, tests, calibrations and commissioning of an Optical Readout Time Projection Chamber (O-TPC) detector operating with a CO2(80%) + N2(20%) gas mixture at 100 and 150 Torr. It was designed to measure the cross sections of several key nuclear reactions involved in stellar evolution. In particular, a study of the rate of formation of oxygen and carbon during the process of helium burning will be performed by exposing the chamber gas to intense nearly mono-energetic gamma-ray beams at the High Intensity Gamma Source (HIgS) facility. The O-TPC has a sensitive target-drift volume of 30x30x21 cm^3. Ionization electrons drift towards a double parallel grid avalanche multiplier, yielding charge multiplication and light emission. Avalanche induced photons from N2 emission are collected, intensified and recorded with a Charge Coupled Device (CCD) camera, providing two-dimensional track images. The event's time projection (third coordinate) and the deposited energy are recorded by photomultipliers and by the TPC charge-signal, respectively. A dedicated VME-based data acquisition system and associated data analysis tools were developed to record and analyze these data. The O-TPC has been tested and calibrated with 3.183 MeV alpha-particles emitted by a 148Gd source placed within its volume with a measured energy resolution of 3.0%. Tracks of alpha and 12C particles from the dissociation of 16O and of three alpha-particles from the dissociation of 12C have been measured during initial in-beam test experiments performed at the HIgS facility at Duke University. The full detection system and its performance are described and the results of the preliminary in-beam test experiments are reported.

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arXiv2006

In Beam Tests of Implanted Helium Targets

Targets consisting of 3,4He implanted into thin aluminum foils (approximately 100, 200 or 600 ug/cm^2) were prepared using intense (a few uA) helium beams at low energy (approximately 20, 40 or 100 keV). Uniformity of the implantation was achieved by a beam raster across a 12 mm diameter tantalum collimator at the rates of 0.1 Hz in the vertical direction and 1 Hz in the horizontal direction. Helium implantation into the very thin (approximately 80-100 ug/cm^2) aluminum foils failed to produce useful targets (with only approximately 10% of the helium retained) due to an under estimation of the range by the code SRIM. The range of low energy helium in aluminum predicted by Northcliffe and Shilling and the NIST online tabulation are observed on the other hand to over estimate the range of low energy helium ions in aluminum. An attempt to increase the amount of helium by implanting a second deeper layer was also carried out, but it did not significantly increase the helium content beyond the blistering limit (approximately 6 x 10^17 helium/cm^2). The implanted targets were bombarded with moderately intense 4He and 16O beams of 50-100 particle nA . Rutherford Back Scattering of 1.0 and 2.5 MeV proton beams and recoil helium from 15.0 MeV oxygen beams were used to study the helium content and profile before, during and after bombardments. We observed the helium content and profile to be very stable even after a prolonged bombardment (up to two days) with moderately intense beams of 16O or 4He. Helium implanted into thin (aluminum) foils is a good choice for thin helium targets needed, for example, for a measurement of the 3he(a,g)7Be reaction and the associated S34 astrophysical cross section factor (S-factor).

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