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M. W. Wu

Publications and source records attributed to M. W. Wu.

At least 55 records · Page 3Linked to original sources

Energy spectra of three electrons in SiGe/Si/SiGe laterally coupled triple quantum dots

We investigate the energy spectra of three electrons in SiGe/Si/SiGe equilateral triangular and symmetric linear triple quantum dots in the presence of magnetic (in either Faraday or Voigt configuration) and electric fields with single valley approximation by using the real-space configuration interaction method. The strong electron-electron Coulomb interaction, which is crucial to the energy spectra, is explicitly calculated whereas the weak spin-orbit coupling is treated perturbatively. In both equilateral triangular and symmetric linear triple quantum dots, we find doublet-quartet transition of ground-state spin configuration by varying dot size or interdot distance in the absence of external fields. This transition has not been reported in the literature on triple quantum dots. In the magnetic-field (Faraday configuration) dependence of energy spectra, we find anticrossings with large energy splittings between the energy levels with the same spin state in the absence of the spin-orbit coupling. This anticrossing behavior originates from the triple quantum dot confinement potential. In addition, with the inclusion of the spin-orbit coupling, we find that all the intersections shown in the equilateral triangular case become anticrossing whereas only part of the intersections in symmetric linear case show anticrossing behavior in the presence of magnetic field in either the Faraday or Voigt configuration. All the anticrossing behaviors are analyzed based on symmetry consideration. Moreover, we show that the electric field can effectively influence the energy levels and the charge configurations.

cond-mat.mes-hall↗

Anomalous D'yakonov-Perel' spin relaxation in semiconductor quantum wells under strong magnetic field in Voigt configuration

We report an anomalous scaling of the D'yakonov-Perel' spin relaxation with the momentum relaxation in semiconductor quantum wells under a strong magnetic field in the Voigt configuration. We focus on the case that the external magnetic field is perpendicular to the spin-orbit-coupling--induced effective magnetic field and its magnitude is much larger than the later one. It is found that the longitudinal spin relaxation time is proportional to the momentum relaxation time even in the strong scattering limit, indicating that the D'yakonov-Perel' spin relaxation shows the Elliott-Yafet-like behaviour. Moreover, the transverse spin relaxation time is inversely proportional (proportional) to the momentum relaxation time in the weak (strong) scattering limit, both in the opposite trends against the well-established conventional D'yakonov-Perel' spin relaxation behaviours. We further demonstrate that all the above anomalous scaling relations come from the unique form of the effective inhomogeneous broadening.

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Spin-dependent inter- and intra-valley electron-phonon scattering in germanium

We investigate the spin-dependent electron-phonon scatterings of the $L$ and $Γ$ valleys and the band structure near the conduction band minima in germanium. We first construct a $16\times16$ ${\bm k}\cdot{\bm p}$ Hamiltonian in the vicinity of the $L$ point in germanium, which ensures the correctness of the band structure of the lowest three conduction bands and highest two valence bands. This Hamiltonian facilitates the analysis of the spin-related properties of the conduction electrons. We then demonstrate the phonon-induced electron scatterings of the $L$ and $Γ$ valleys, i.e., the intra-$Γ$/ $L$ valley, inter--$Γ$-$L$ valley and inter--$L$-$L$ valley scatterings in germanium. The selection rules and complete scattering matrices for these scatterings are calculated, where the scattering matrices for the intra-$Γ$ valley scattering, inter--$Γ$-$L$ valley scattering and the optical-phonon and the separated transverse-acoustic- and longitudinal-acoustic-phonon contributions to the intra-$Γ$ valley scattering have not been reported in the literature. The coefficients in these scattering matrices are obtained via the pseudo-potential calculation, which also verifies our selection rules and wave-vector dependence. We further discuss the Elliott-Yafet mechanisms in these electron-phonon scatterings with the ${\bm k}$$\cdot$${\bm p}$ eigenstates at the $L$ and $Γ$ valleys. Our investigation of these electron-phonon scatterings are essential for the study of the optical orientation of spin and hot-electron relaxation in germanium.

cond-mat.mtrl-sci↗

Electron spin relaxation in bilayer graphene

Electron spin relaxation due to the D'yakonov-Perel' mechanism is investigated in bilayer graphene with only the lowest conduction band being relevant. The spin-orbit coupling is constructed from the symmetry group analysis with the parameters obtained by fitting to the numerical calculation according to the latest report by Konschuh {\it et al.} [Phys. Rev. B {\bf 85}, 115423 (2012)] from first principles. In contrast to single-layer graphene, the leading term of the out-of-plane component of the spin-orbit coupling in bilayer graphene shows a Zeeman-like term with opposite effective magnetic fields in the two valleys. This Zeeman-like term opens a spin relaxation channel in the presence of intervalley scattering. It is shown that the intervalley electron-phonon scattering, which has not been reported in the previous literature, strongly suppresses the in-plane spin relaxation time at high temperature whereas the intervalley short-range scattering plays an important role in the in-plane spin relaxation especially at low temperature. A marked nonmonotonic dependence of the in-plane spin relaxation time on temperature with a minimum of several hundred picoseconds is predicted in the absence of the short-range scatterers. This minimum is comparable to the experimental data. Moreover, a peak in the electron density dependence of the in-plane spin relaxation time at low temperature, which is very different from the one in semiconductors, is predicted. We also find a rapid decrease in the in-plane spin relaxation time with increasing initial spin polarization at low temperature, which is opposite to the situation in both semiconductors and single-layer graphene. ......(The remaining is cut due to the limit of space)

cond-mat.mes-hall↗

Microscopic theory of ultrafast dynamics of carriers photoexcited by THz and near-infrared linearly-polarized laser pulses in graphene

We investigate the dynamics of photoexcited carriers and nonequilibrium phonons in graphene by solving the microscopic kinetic Bloch equations. The pump and drift effects from the laser field as well as the relevant scatterings (including the Coulomb scattering with dynamic screening) are explicitly included. When the pump-photon energy is high enough, the influence of the drift term is shown to be negligible and the isotropic hot-electron Fermi distribution is established under the scattering during the linearly polarized laser pulse investigated here. However, in the case with low pump-phonon energy, the drift term is important and leads to a net momentum transfer from the electric field to electrons. Due to this net momentum and the dominant Coulomb scattering, a drifted Fermi distribution different from the one established under static electric field is found to be established in several hundred femtoseconds. We also show that the Auger process investigated in the literature involving only the diagonal terms of density matrices is forbidden by the dynamic screening. However, we propose an Auger process involving the interband coherence and show that it contributes to the dynamics of carriers when the pump-photon energy is low. In addition, the anisotropically momentum-resolved hot-phonon temperatures due to the linearly polarized light are also investigated, with the underlying physics revealed.

cond-mat.mes-hall↗

Kinetic theory of surface plasmon polariton in semiconductor nanowires

Based on the semiclassical model Hamiltonian of the surface plasmon polariton and the nonequilibrium Green-function approach, we present a microscopic kinetic theory to study the influence of the electron scattering on the dynamics of the surface plasmon polariton in semiconductor nanowires. The damping of the surface plasmon polariton originates from the resonant absorption by the electrons (Landau damping), and the corresponding damping exhibits size-dependent oscillations and distinct temperature dependence without any scattering. The scattering influences the damping by introducing a broadening and a shifting to the resonance. To demonstrate this, we investigate the damping of the surface plasmon polariton in InAs nanowires in the presence of the electron-impurity, electron-phonon and electron-electron Coulomb scatterings. The main effect of the electron-impurity and electron-phonon scatterings is to introduce a broadening, whereas the electron-electron Coulomb scattering can not only cause a broadening, but also introduce a shifting to the resonance. For InAs nanowires under investigation, the broadening due to the electron-phonon scattering dominates. As a result, the scattering has a pronounced influence on the damping of the surface plasmon polariton: The size-dependent oscillations are smeared out and the temperature dependence is also suppressed in the presence of the scattering. These results demonstrate the the important role of the scattering on the surface plasmon polariton damping in semiconductor nanowires.

cond-mat.mes-hall↗

Hot-carrier transport and spin relaxation on the surface of topological insulator

We study the charge and spin transport under high electric field (up to several kV/cm) on the surface of topological insulator Bi$_2$Se$_3$, where the electron-surface optical phonon scattering dominates except at very low temperature. Due to the spin mixing of conduction and valence bands, the electric field not only accelerates electrons in each band, but also leads to inter-band precession. In the presence of the electric field, electrons can transfer from the valence band to the conduction one via the inter-band precession and inter-band electron-phonon scattering. The electron density in each band varies with the electric field linearly when the electric field is strong. Due to the spin-momentum locking, a transverse spin polarization, with the magnitude proportional to the momentum scattering time, is induced by the electric field. The induced spin polarization depends on the electric field linearly when the latter is small. Moreover, its magnitude is inversely proportional to the temperature and is insensitive to the electron density at high temperature. Our investigation also reveals that due to the large relative static dielectric constant, the Coulomb scattering is too weak to establish a drifted Fermi distribution with a unified hot-electron temperature in the steady state under the electric field. After turning off the electric field in the steady state, the hot carriers cool down in a time scale of energy relaxation which is very long (of the order of 100-1000 ps) while the spin polarization relaxes in a time scale of momentum scattering which is quite short (of the order of 0.01-0.1 ps).

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Microscopic theory for the Doppler velocimetry of spin propagation in semiconductor quantum wells

We provide a microscopic theory for the Doppler velocimetry of spin propagation in the presence of spatial inhomogeneity, driving electric field and the spin orbit coupling in semiconductor quantum wells in a wide range of temperature regime based on the kinetic spin Bloch equation. It is analytically shown that under an applied electric field, the spin density wave gains a time-dependent phase shift $ϕ(t)$. Without the spin-orbit coupling, the phase shift increases linearly with time and is equivalent to a normal Doppler shift in optical measurements. Due to the joint effect of spin-orbit coupling and the applied electric field, the phase shift behaviors differently at the early and the later stages. At the early stage, the phase shifts are the same with or without the spin-orbit coupling. While at the later stage, the phase shift deviates from the normal Doppler one when the spin-orbit coupling is present. The crossover time from the early normal Doppler behavior to the anomalous one at the later stage is inversely proportional to the spin diffusion coefficient, wave vector of the spin density wave and the spin-orbit coupling strength. In the high temperature regime, the crossover time becomes large as a result of the decreased spin diffusion coefficient. The analytic results capture all the quantitative features of the experimental results, while the full numerical calculations agree quantitatively well with the experimental data obtained from the Doppler velocimetry of spin propagation [Yang {\it et al.}, Nat. Phys. {\bf 8}, 153 (2012)]. We further predict that the coherent spin precession, originally thought to be broken down at high temperature, is robust up to the room temperature for narrow quantum wells. We point out that one has to carry out the experiments longer to see the effect of the coherent spin precession at higher temperature due to the larger crossover time.

cond-mat.mes-hall↗

Finite-size effect of antiferromagnetic transition and electronic structure in LiFePO4

The finite-size effect on the antiferromagnetic (AF) transition and electronic configuration of iron has been observed in LiFePO4. Determination of the scaling behavior of the AF transition temperature (TN) versus the particle-size dimension (L) in the critical regime 1-TN(L)/TN(XTL)\simL^-1 reveals that the activation nature of the AF ordering strongly depends on the surface energy. In addition, the effective magnetic moment that reflects the electronic configuration of iron in LiFePO4 is found to be sensitive to the particle size. An alternative structural view based on the polyatomic ion groups of (PO4)3- is proposed.

cond-mat.mtrl-sci↗

Some comments on the note "Comment on 'Single-parameter quantum charge and spin pumping in armchair graphene nanoribbons' by Zhu and Berakdar (arXiv:1207.3457)"

In response to the comment by Zhu and Berakdar (arXiv:1207.3457) that the physical system considered by them in their previous work [Ding et al., PRB 84, 115433 (2011)] is conceptually different from ours in the appendix of our latest paper [Zhou and Wu, arXiv:1206.3435], we show why they are relevant and further point out conceptually the problems in their work. We also point out that the main supporting arguments in their comment are incorrect.

cond-mat.mes-hall↗

Single-parameter quantum charge and spin pumping in armchair graphene nanoribbons

We investigate quantum charge and spin pumping in armchair graphene nanoribbons under a single ac gate voltage connected with nonmagnetic/ferromagnetic leads via the nonequilibrium Green's function method. In the case of nonmagnetic leads, where only part of the nanoribbon is subject to an ac gate voltage to break the left-right spatial symmetry, we discover that peaks of the charge pumping current appear at the Fermi energies around the subband edges in the ac-field-free region of the nanoribbon. In the case of ferromagnetic leads with the lead magnetizations being antiparallel to break the left-right symmetry, similar peaks appear in the spin pumping current when the Fermi energies are around the edges of the the majority-spin subbands in the ferromagnetic leads. All these peaks originate from the pronounced symmetry breaking in the transmissions with energies being around the corresponding subband edges. Moreover, we predict a {\em pure} spin current in the case of ferromagnetic leads with the whole graphene nanoribbon under an ac gate voltage. The ac-field-strength and -frequency dependences of the pumping current are also investigated with the underlying physics revealed.

cond-mat.mes-hall↗

Electron spin relaxation in GaAs$_{1-x}$Bi$_x$: Effects of spin-orbit tuning by Bi incorporation

The electron spin relaxation in $n$-type and intrinsic GaAs$_{1-x}$Bi$_x$ with Bi composition $0\le x \le 0.1$ is investigated from the microscopic kinetic spin Bloch equation approach. The incorporation of Bi is shown to markedly decrease the spin relaxation time as a consequence of the modification of the spin-orbit interaction. We demonstrate that the density and temperature dependences of spin relaxation time in GaAs$_{1-x}$Bi$_x$ resemble the ones in GaAs. Meanwhile, the Bir-Aronov-Pikus mechanism is found to be negligible compared to the D'yakonov-Perel' mechanism in intrinsic sample. Due to the absence of direct measurement of the electron effective mass in the whole compositional range under investigation, we further explore the effect of a possible variation of electron effective mass on the electron spin relaxation.

cond-mat.mtrl-sci↗

Strongly modulated transmissions in gapped armchair graphene nanoribbons with sidearm or on-site gate voltage

We propose two schemes of field-effect transistor based on gapped armchair graphene nanoribbons connected to metal leads, by introducing sidearms or on-site gate voltages. We make use of the band gap to reach excellent switch-off character. By introducing one sidearm or on-site gate to the graphene nanoribbon, conduction peaks appear inside the gap regime. By further applying two sidearms or on-site gates, these peaks are broadened to conduction plateaus with a wide energy window, thanks to the resonance from the dual structure. The position of the conduction windows inside the gap can be fully controlled by the length of the sidearms or the on-site gate voltages, which allows "on" and "off" operations for a specific energy window inside the gap regime. The high robustness of both the switch-off character and the conduction windows is demonstrated and shows the feasibility of the proposed dual structures for real applications.

cond-mat.mes-hall↗

Electron spin rephasing in $n$-type (001) GaAs quantum wells

We investigate the electron spin dephasing in the presence of spin phase recovering by a serried $π$-pulse sequence in $n$-type (001) GaAs quantum wells in a wide range of temperature and density regimes. Our numerical calculation is based on the kinetic spin Bloch equation approach with all the relevant scatterings explicitly included. We find that the rephasing pulse sequence with a long inter-pulse spacing only has a marginal influence on the spin lifetime in both the strong and weak scattering limits. We show that the spin lifetime can be significantly increased by reducing the inter-pulse spacing. More interestingly, we show that the temperature and density dependences of the spin lifetime in the case of short inter-pulse spacing coincide with those of the momentum scattering time in the low temperature regime, where nonmonotonic behaviors can appear. The origin of this feature is that the scattering under the quick rephasing manipulation mainly performs as the source of the dephasing channel instead of the key to suppress the inhomogeneous broadening. The contributions of the relevant scattering mechanisms are also discussed.

cond-mat.mes-hall↗

Hole spin relaxation in $p$-type (111) GaAs quantum wells

Hole spin relaxation in $p$-type (111) GaAs quantum wells is investigated in the case with only the lowest hole subband, which is heavy-hole like in (111) GaAs/AlAs and light-hole like in (111) GaAs/InP quantum wells, being relevant. The subband Löwdin perturbation method is applied to obtain the effective Hamiltonian including the Dresselhaus and Rashba spin-orbit couplings. Under a proper gate voltage, the total in-plane effective magnetic field in (111) GaAs/AlAs quantum wells can be strongly suppressed in the whole momentum space, while the one in (111) GaAs/InP quantum wells can be suppressed only on a special momentum circle. The hole spin relaxation due to the D'yakonov-Perel' and Elliott-Yafet mechanisms is calculated by means of the fully microscopic kinetic spin Bloch equation approach with all the relevant scatterings explicitly included. For (111) GaAs/AlAs quantum wells, extremely long heavy-hole spin relaxation time (upto hundreds of nanoseconds) is predicted. In addition, we predict a pronounced peak in the gate-voltage dependence of the heavy-hole spin relaxation time due to the D'yakonov-Perel' mechanism. This peak origins from the suppression of the unique inhomogeneous broadening in (111) GaAs/AlAs quantum wells. Moreover, the Elliott-Yafet mechanism influences the spin relaxation only around the peak area due to the small spin mixing between the heavy and light holes in quantum wells with small well width. We also show the anisotropy of the spin relaxation. In (111) GaAs/InP quantum wells, a mild peak, similar to the case for electrons in (111) GaAs quantum wells, is also predicted in the gate-voltage dependence of the light-hole spin relaxation time. The contribution of the Elliott-Yafet mechanism is always negligible in this case.

cond-mat.mes-hall↗

Electron spin relaxation in graphene with random Rashba field: Comparison of D'yakonov-Perel' and Elliott-Yafet--like mechanisms

Aiming to understand the main spin relaxation mechanism in graphene, we investigate the spin relaxation with random Rashba field induced by both adatoms and substrate, by means of the kinetic spin Bloch equation approach. The charged adatoms on one hand enhance the Rashba spin-orbit coupling locally and on the other hand serve as Coulomb potential scatterers. Both effects contribute to spin relaxation limited by the D'yakonov-Perel' mechanism. In addition, the random Rashba field also causes spin relaxation by spin-flip scattering, manifesting itself as an Elliott-Yafet--like mechanism. Both mechanisms are sensitive to the correlation length of the random Rashba field, which may be affected by the environmental parameters such as electron density and temperature. By fitting and comparing the experiments from the Groningen group [Józsa {\it et al.}, Phys. Rev. B {\bf 80}, 241403(R) (2009)] and Riverside group [Pi {\it et al.}, Phys. Rev. Lett. {\bf 104}, 187201 (2010); Han and Kawakami, {\it ibid.} {\bf 107}, 047207 (2011)] which show either D'yakonov-Perel'-- (with the spin relaxation rate being inversely proportional to the momentum scattering rate) or Elliott-Yafet--like (with the spin relaxation rate being proportional to the momentum scattering rate) properties, we suggest that the D'yakonov-Perel' mechanism dominates the spin relaxation in graphene. The latest experimental finding of a nonmonotonic dependence of spin relaxation time on diffusion coefficient by Jo {\it et al.} [Phys. Rev. B {\bf 84}, 075453 (2011)] is also well reproduced by our model.

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