arXiv subjects

M. Weidemüller

Publications and source records attributed to M. Weidemüller.

35 records · Page 2Linked to original sources

arXiv2011

Population redistribution in optically trapped polar molecules

We investigate the rovibrational population redistribution of polar molecules in the electronic ground state induced by spontaneous emission and blackbody radiation. As a model system we use optically trapped LiCs molecules formed by photoassociation in an ultracold two-species gas. The population dynamics of vibrational and rotational states is modeled using an ab-initio electric dipole moment function and experimental potential energy curves. Comparison with the evolution of the v"=3 electronic ground state yields good qualitative agreement. The analysis provides important input to assess applications of ultracold LiCs molecules in quantum simulation and ultracold chemistry.

physics.atom-ph↗

arXiv2011

Interaction enhanced imaging of individual atoms embedded in dense atomic gases

We propose a new all-optical method to image individual atoms within dense atomic gases. The scheme exploits interaction induced shifts on highly polarizable excited states, which can be spatially resolved via an electromagnetically induced transparency resonance. We focus in particular on imaging strongly interacting many-body states of Rydberg atoms embedded in an ultracold gas of ground state atoms. Using a realistic model we show that it is possible to image individual impurity atoms with enhanced sensitivity and high resolution despite photon shot noise and atomic density fluctuations. This new imaging scheme is ideally suited to equilibrium and dynamical studies of complex many-body phenomena involving strongly interacting atoms. As an example we study blockade effects and correlations in the distribution of Rydberg atoms optically excited from a dense gas.

physics.atom-ph↗

arXiv2010

Doorway states and the Bose-Hubbard model

We introduce an efficient method to solve the Mott-Hubbard model. The Schrödinger equation is solved by the successive construction of doorway states. The ground state wavefunction derived by this method contains all relevant many-body correlations introduced by the hamiltonian, but the dimensionality of the Hilbert space is greatly reduced. We apply the doorway method to obtain the chemical potential, the on-site fluctuations and the visibility of the interference pattern arising from atoms in a one-dimensional periodic lattice. Excellent agreement with exact numerical calculations as well as recent experimental observations is found.

cond-mat.other↗

arXiv2010

Influence of a Feshbach resonance on the photoassociation of LiCs

We analyse the formation of ultracold 7Li133Cs molecules in the rovibrational ground state through photoassociation into the B1Pi state, which has recently been reported [J. Deiglmayr et al., Phys. Rev. Lett. 101, 133004 (2008)]. Absolute rate constants for photoassociation at large detunings from the atomic asymptote are determined and are found to be surprisingly large. The photoassociation process is modeled using a full coupled-channel calculation for the continuum state, taking all relevant hyperfine states into account. The enhancement of the photoassociation rate is found to be caused by an `echo' of the triplet component in the singlet component of the scattering wave function at the inner turning point of the lowest triplet a3Sigma+ potential. This perturbation can be ascribed to the existence of a broad Feshbach resonance at low scattering energies. Our results elucidate the important role of couplings in the scattering wave function for the formation of deeply bound ground state molecules via photoassociation.

physics.atom-ph↗

arXiv2010

The permanent dipole moment of LiCs in the ground state

Recently we demonstrated the formation of ultracold polar LiCs molecules in deeply bound levels of the X1S+ ground state, including the rovibrational ground state [J. Deiglmayr et al., Phys. Rev. Lett. 101, 133004 (2008)]. Here we report on the first experimental determination of the permanent electric dipole moment of deeply bound LiCs molecules. For X1S+,v"=2 and v"=3 we measure values of mu=5.5(2) Debye and 5.3(2) Debye respectively.

physics.atom-ph↗

arXiv2010

Real-time phase-shift detection of the surface plasmon resonance

We investigate a method to directly measure the phase of a laser beam reflected from a metallic film after excitation of surface plasmon polaritons. This method permits real time access to the phase information, it increases the possible speed of data acquisition, and it may thus prove useful for increasing the sensitivity of surface plasmon based sensors.

physics.optics↗

arXiv2010

Coherent Population Trapping with Controlled Interparticle Interactions

We investigate Coherent Population Trapping in a strongly interacting ultracold Rydberg gas. Despite the strong van der Waals interactions and interparticle correlations, we observe the persistence of a resonance with subnatural linewidth at the single-particle resonance frequency as we tune the interaction strength. This narrow resonance cannot be understood within a meanfield description of the strong Rydberg--Rydberg interactions. Instead, a many-body density matrix approach, accounting for the dynamics of interparticle correlations, is shown to reproduce the observed spectral features.

physics.atom-ph↗

arXiv2009

Autoionization of an ultracold Rydberg gas through resonant dipole coupling

We investigate a possible mechanism for the autoionization of ultracold Rydberg gases, based on the resonant coupling of Rydberg pair states to the ionization continuum. Unlike an atomic collision where the wave functions begin to overlap, the mechanism considered here involves only the long-range dipole interaction and is in principle possible in a static system. It is related to the process of intermolecular Coulombic decay (ICD). In addition, we include the interaction-induced motion of the atoms and the effect of multi-particle systems in this work. We find that the probability for this ionization mechanism can be increased in many-particle systems featuring attractive or repulsive van der Waals interactions. However, the rates for ionization through resonant dipole coupling are very low. It is thus unlikely that this process contributes to the autoionization of Rydberg gases in the form presented here, but it may still act as a trigger for secondary ionization processes. As our picture involves only binary interactions, it remains to be investigated if collective effects of an ensemble of atoms can significantly influence the ionization probability. Nevertheless our calculations may serve as a starting point for the investigation of more complex systems, such as the coupling of many pair states proposed in [Tanner et al., PRL 100, 043002 (2008)].

physics.atom-ph↗

arXiv2008

Formation of ultracold dipolar molecules in the lowest vibrational levels by photoassociation

We recently reported the formation of ultracold LiCs molecules in the rovibrational ground state X1Sigma+,v''=0,J''=0 [J. Deiglmayr et al., PRL 101, 133004 (2008)]. Here we discuss details of the experimental setup and present a thorough analysis of the photoassociation step including the photoassociation line shape. We predict the distribution of produced ground state molecules using accurate potential nergy curves combined with an ab-initio dipole transition moment and compare this prediction with experimental ionization spectra. Additionally we improve the value of the dissociation energy for the X1Sigma+ state by high resolution spectroscopy of the vibrational ground state.

physics.atom-ph↗

arXiv2008

Formation of ultracold polar molecules in the rovibrational ground state

Ultracold LiCs molecules in the absolute ground state X$^1Σ^+$, v"=0, J"=0 are formed via a single photo-association step starting from laser-cooled atoms. The selective production of v"=0, J"=2 molecules with a 50-fold higher rate is also demonstrated. The rotational and vibrational state of the ground state molecules is determined in a setup combining depletion spectroscopy with resonant-enhanced multi-photon ionization time-of-flight spectroscopy. Using the determined production rate of up to 5x10^3 molecules/s, we describe a simple scheme which can provide large samples of externally and internally cold dipolar molecules.

quant-ph↗

arXiv2007

A planar multipole ion trap

We report on the realisation of a chip-based multipole ion trap manufactured using micro-electromechanical systems (MEMS) technology. It provides ion confinement in an almost field-free volume between two planes of radiofrequency electrodes, deposited on glass substrates, which allows for optical access to the trap. An analytical model of the effective trapping potential is presented and compared with numerical calculations. Stable trapping of argon ions is achieved and a lifetime of 16s is measured. Electrostatic charging of the chip surfaces is studied and found to agree with a numerical estimate.

physics.atom-ph↗

arXiv2007

Evaporation of buffer gas-thermalized anions out of a multipole rf ion trap

We identify plain evaporation of ions as the fundamental loss mechanism out of a multipole ion trap. Using thermalized negative Cl- ions we find that the evaporative loss rate is proportional to a Boltzmann factor. This thermodynamic description sheds new light on the dynamics of particles in time-varying confining potentials. It specifically allows us to extract the effective depth of the ion trap as the activation energy for evaporation. As a function of the rf amplitude we find two distinct regimes related to the stability of motion of the trapped ions. For low amplitudes the entire trap allows for stable motion and the trap depth increases with the rf field. For larger rf amplitudes, however, rapid energy transfer from the field to the ion motion can occur at large trap radii, which leads to a reduction of the effective trapping volume. In this regime the trap depth decreases again with increasing rf amplitude. We give an analytical parameterization of the trap depth for various multipole traps that allows predictions of the most favorable trapping conditions.

physics.atom-ph↗

arXiv2006

Photodetachment of cold OH- in a multipole ion trap

The absolute photodetachment cross section of OH- anions at a rotational and translational temperature of 170K is determined by measuring the detachment-induced decay rate of the anions in a multipole radio-frequency ion trap. In comparison with previous results, the obtained cross section shows the importance of the initial rotational state distribution. Using a tomography scan of the photodetachment laser through the trapped ion cloud, the derived cross section is model-independent and thus features a small systematic uncertainty. The tomography also yields the column density of the OH- anions in the 22-pole ion trap in good agreement with the expected trapping potential of a large field free region bound by steep potential walls.

physics.atom-ph↗

arXiv2006

Mechanical effect of van der Waals interactions observed in real time in an ultracold Rydberg gas

We present time-resolved spectroscopic measurements of Rydberg-Rydberg interactions in an ultracold gas, revealing the pair dynamics induced by long-range van der Waals interactions between the atoms. By detuning the excitation laser, a specific pair distribution is prepared. Penning ionization on a microsecond timescale serves as a probe for the pair dynamics under the influence of the attractive long-range forces. Comparison with a Monte Carlo model not only explains all spectroscopic features but also gives quantitative information about the interaction potentials. The results imply that the interaction-induced ionization rate can be influenced by the excitation laser. Surprisingly, interaction-induced ionization is also observed for Rydberg states with purely repulsive interactions.

physics.atom-ph↗

arXiv2002

Magnetic field control of elastic scattering in a cold gas of fermionic lithium atoms

We study elastic collisions in an optically trapped spin mixture of fermionic lithium atoms in the presence of magnetic fields up to 1.5kG by measuring evaporative loss. Our experiments confirm the expected magnetic tunability of the scattering length by showing the main features of elastic scattering according to recent calculations. We measure the zero crossing of the scattering length that is associated with a predicted Feshbach resonance at 530(3)G. Beyond the resonance we observe the expected large cross section in the triplet scattering regime.

physics.atom-ph↗

arXiv1999

Cold inelastic collisions between lithium and cesium in a two-species magneto-optical trap

We investigate collisional properties of lithium and cesium which are simultaneously confined in a combined magneto-optical trap. Trap-loss collisions between the two species are comprehensively studied. Different inelastic collision channels are identified, and inter-species rate coefficients as well as cross sections are determined. It is found that loss rates are independent of the optical excitation of Li, as a consequence of the repulsive Li$^*$-Cs interaction. Li and Cs loss by inelastic inter-species collisions can completely be attributed to processes involving optically excited cesium (fine-structure changing collisions and radiative escape). By lowering the trap depth for Li, an additional loss channel of Li is observed which results from ground-state Li-Cs collisions changing the hyperfine state of cesium.

physics.atom-ph↗

arXiv1996

Adiabatically changing the phase-space density of a trapped Bose gas

We show that the degeneracy parameter of a trapped Bose gas can be changed adiabatically in a reversible way, both in the Boltzmann regime and in the degenerate Bose regime. We have performed measurements on spin-polarized atomic hydrogen in the Boltzmann regime demonstrating reversible changes of the degeneracy parameter (phase-space density) by more than a factor of two. This result is in perfect agreement with theory. By extending our theoretical analysis to the quantum degenerate regime we predict that, starting close enough to the Bose-Einstein phase transition, one can cross the transition by an adiabatic change of the trap shape.

physics.atom-ph↗