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M. Weigand

Publications and source records attributed to M. Weigand.

At least 19 recordsLinked to original sources

Quasi-1D Spin Textures: From Chiral Soliton Lattice to Fan State

In most helimagnets, an applied magnetic field aligns the propagation direction of a helical spin texture with the field, resulting in a conical state and obscuring the unwinding process. Here, we access a complementary regime in the anisotropic chiral magnet Mn$_{1.4}$PtSn, where crystal symmetry constrains the propagation direction of the spin modulation. Using resonant elastic X-ray scattering in a vector magnet, we track the evolution of quasi-one-dimensional spin textures that propagate along a chiral crystallographic axis while the magnetic field is applied perpendicular to this direction. Together with micromagnetic simulations, our measurements reveal a transformation from the zero-field $\pi$-chiral soliton lattice into a fan-like state. In this state, the propagation direction remains transverse to the applied field, while the spins oscillate about the field direction. During magnetization, the modulation length decreases continuously with the field and approaches the field-polarized state. Simulations indicate that magnetostatic interactions in finite samples play a key role in stabilizing this behavior. Our results provide evidence for a fan-like regime in a chiral magnet and highlight how field orientation can be used to control one-dimensional spin textures.

cond-mat.mtrl-sci

Linear dichroic soft X-ray microscopy of ferroelectric stripe domains in epitaxial K$_\mathbf{0.6}$Na$_\mathbf{0.4}$NbO$_\mathbf{3}$

Functional properties of ferroelectric thin films are governed by domains that can be engineered by epitaxial strain. Soft X-ray microscopy can image domain structures with elemental and electronic sensitivity, but hitherto its application to strain-stabilized domains has been hindered by the absorption of soft X-rays in epitaxial substrates. Here, it is demonstrated how this limitation can be overcome by locally back-thinning the (110) TbScO$_3$ substrate of epitaxial K$_{0.6}$Na$_{0.4}$NbO$_3$ ferroelectric thin films to achieve soft X-ray transparency at the O K-edge around 530 eV. Strain-induced ferroelectric stripe domains with periods down to 44 nm were resolved by scanning transmission X-ray microscopy and coherent diffractive imaging by exploiting the X-ray linear dichroism of hybridized O 2p-Nb 4d states, providing sensitivity to in-plane polarization components under normal incidence. The results establish soft X-ray microscopy for nanoscale imaging of epitaxial ferroelectric domains structures and open perspectives for time-resolved studies thereof.

cond-mat.mtrl-sci

Nanoscale imaging of spin textures with locally varying altermagnetic response in $\alpha$-Fe$_2$O$_3$

Altermagnetism is a recently identified magnetic state in which time-reversal symmetry is broken despite a collinear compensated spin structure. The response of altermagnets is determined not only by their $d$-, $g$-, or $i$-wave spin order, but also the orientation of their N\'eel vector $\mathbf{L}$. Therefore, accessing a response that fundamentally depends on the orientation of $\mathbf{L}$, such as the anomalous Hall effect, remains experimentally challenging in particular at the nanoscale. Here, we harness nano-spectroscopic X-ray magnetic circular dichroism (XMCD) to investigate nanoscale modulated altermagnetic responses in $\alpha$-Fe$_2$O$_3$ (Hematite). By performing spectroscopy across the temperature-induced $\mathbf{L}$-reorientation Morin transition, we observe the on-and-off switching of XMCD, in agreement with our theoretical calculations. Although the bulk XMCD vanishes below the Morin temperature, we confirm the reorientation of $\mathbf{L}$ by harnessing polarization-independent X-ray absorption spectroscopy. Moreover, we observe a finite XMCD signal in nanoscale domain walls with locally modulated N\'eel vectors, while the surrounding domains exhibit no XMCD. At room temperature, we instead identify altermagnetic meron spin textures that exhibit XMCD in their planar regions but no XMCD in their nanoscopic cores. Our results establish a pathway to harness complex spin textures with nanoscale functionalities in a broader class of altermagnets with various $\mathbf{L}$-orientations and using light, earth-abundant elements.

cond-mat.mtrl-sci

First Proton-Induced Cross Sections on a Stored Rare Ion Beam: Measurement of 118Te(p,{\gamma}) for Explosive Nucleosynthesis

We present the first nuclear cross-section measurements of (p,{\gamma}) and (p,n) reactions on 118Te at energies relevant for the {\gamma}-process nucleosynthesis. Absolute cross-section values for center-of-mass energies of 6, 7 and 10 MeV are provided, together with a theoretical extrapolation to the Gamow window. This experiment marks the first time that direct proton-induced reactions have been measured on a radioactive ion beam at the Experimental Storage Ring (ESR) at GSI, Darmstadt. This paves the way for a large variety of measurements, delivering new constraints for explosive nucleosynthesis and for physics beyond nuclear stability.

nucl-ex

Storage, Accumulation and Deceleration of Secondary Beams for Nuclear Astrophysics

Low-energy investigations on rare ion beams are often limited by the available intensity and purity of the ion species in focus. Here, we present the first application of a technique that combines in-flight production at relativistic energies with subsequent secondary beam storage, accumulation and finally deceleration to the energy of interest. Using the FRS and ESR facilities at GSI, this scheme was pioneered to provide a secondary beam of $^{118}$Te$^{52+}$ for the measurement of nuclear proton-capture at energies of 6 and 7 MeV/u. The technique provided stored beam intensities of about $10^6$ ions at high purity and brilliance, representing a major step towards low-energy nuclear physics studies using rare ion beams.

physics.ins-det

$^{179}$Ta(n,$γ$) cross-section measurement and the astrophysical origin of $^{180}$Ta isotope

Tantalum-180m is nature's rarest (quasi) stable isotope and its astrophysical origin is an open question. A possible production site of this isotope is the slow neutron capture process in Asymptotic Giant Branch stars, where it can be produced via neutron capture reactions on unstable $^{179}$Ta. We report a new measurement of the $^{179}$Ta($n,γ$)$^{180}$Ta cross section at thermal neutron energies via the activation technique. Our results for the thermal and resonance-integral cross-sections are 952 $\pm$ 57 b and 2013 $\pm$ 148 b, respectively. The thermal cross section is in good agreement with the only previous measurement (Phys. Rev C {\bf 60} 025802, 1999), while the resonance integral is different by a factor of $\approx$1.7. While neutron energies in this work are smaller than the energies in a stellar environment, our results may lead to improvements in theoretical predictions of the stellar cross section.

nucl-ex

Mode purity and structural analysis of x-ray vortices generated by spiral zone plates

In the visible spectrum vortex beams have found various applications, ranging from optical tweezers to super-resolution imaging. Recently, these beams have been demonstrated using X-rays and electron beams. However, so far, no in-depth discussion has been carried out on the vortex quality, which could become essential for a variety of vortex applications. Here, we investigate the mode conversion efficiency (MCE), vortex structure and stability (in terms of vortex splitting) of the vortex fields generated by spiral zone plates (SZP). We have designed and fabricated SZPs with varying topological charge of both binary and kinoform profile. Kinoforms are known for their 100 % diffraction efficiency in the ideal case. In this work, both types are contrasted with regard to the vortex quality. Utilizing ptychographic coherent diffraction imaging and by comparing to simulations the wavefront of the generated fields is characterized. It was found, that the MCE and vortex structure exhibit the same dependencies on material and ZP properties as the diffraction efficiency (DE) and that the kinoform profile in this sense also improves the vortex quality. With growing SZP charge the MCE decreases. The results link the parameters of optics to the properties of the vortices and help to maximize the performance of ZP based vortex generators for future applications.

physics.optics

Deterministic Generation and Guided Motion of Magnetic Skyrmions by Focused He$^+$-Ion Irradiation

Magnetic skyrmions are quasiparticles with non-trivial topology, envisioned to play a key role in next-generation data technology while simultaneously attracting fundamental research interest due to their emerging topological charge. In chiral magnetic multilayers, current-generated spin-orbit torques or ultrafast laser excitation can be used to nucleate isolated skyrmions on a picosecond timescale. Both methods, however, produce randomly arranged skyrmions, which inherently limits the precision on the location at which the skyrmions are nucleated. Here, we show that nanopatterning of the anisotropy landscape with a He$^+$-ion beam creates well-defined skyrmion nucleation sites, thereby transforming the skyrmion localization into a deterministic process. This approach allows to realize control of individual skyrmion nucleation as well as guided skyrmion motion with nanometer-scale precision, which is pivotal for both future fundamental studies of skyrmion dynamics and applications.

cond-mat.mtrl-sci

X-Ray Imaging of Mixed States of Skyrmions and Helices in FeGe

We report scanning transmission X-ray microscopy of mixed helical and skyrmion magnetic states in thin FeGe lamellae. This imaging of the out-of-plane magnetism allows clear identification of the different magnetic states, and reveals details about the coexistence of helical and skyrmion states. In particular, our data show that finite length helices are continuously deformable down to the size of individual skyrmions and are hence topologically equivalent to skyrmions. Furthermore, we observe transition states between helical and skyrmion states across the thickness of the lamella that are evidence for frozen Bloch points in the sample after field cooling.

cond-mat.str-el

Determination of the $^{209}$Bi(n,$γ$)$^{210g}$Bi cross section using the NICE-Detector

The capture cross section of $^{209}$Bi(n,$γ$)$^{210g}$Bi was measured at different astrophysically energies including thermal capture cross section (25 meV), resonance integral, and the Maxwellian averaged cross section at a thermal energy of $kT$ = 30 keV. The partial capture cross section ($σ_g$) was determined using the activation technique and by measuring the $^{210}$Po activity. The newly developed and tested NICE detector setup was used to measure the $α$-activity of the $^{210}$Po. Using this setup the thermal and resonance integral cross sections were determined to be $16.2\;\pm\;0.97$~mb and $89.81\;\pm\;8.0$~mb, respectively. And the Maxwellian average cross section was measured to be $2.01\;\pm\;0.38$~mb.

nucl-ex

Determination of luminosity for in-ring reactions: A new approach for the low-energy domain

Luminosity is a measure of the colliding frequency between beam and target and it is a crucial parameter for the measurement of absolute values, such as reaction cross sections. In this paper, we make use of experimental data from the ESR storage ring to demonstrate that the luminosity can be precisely determined by modelling the measured Rutherford scattering distribution. The obtained results are in good agreement with an independent measurement based on the x-ray normalization method. Our new method provides an alternative way to precisely measure the luminosity in low-energy stored-beam configurations. This can be of great value in particular in dedicated low-energy storage rings where established methods are difficult or impossible to apply.

nucl-ex

Observation of compact ferrimagnetic skyrmions in DyCo$_3$ film

Owing to the experimental discovery of magnetic skyrmions stabilized by the Dzyaloshinskii-Moriya and/or dipolar interactions in thin films, there is a recent upsurge of interest in magnetic skyrmions with antiferromagnetic spins in order to overcome the fundamental limitations inherent with skyrmions in ferromagnetic materials. Here, we report on the observation of compact ferrimagnetic skyrmions for the class of amorphous alloys consisting of 4f rare-earth and 3d transition-metal elements with perpendicular magnetic anisotropy, using a DyCo$_3$ film, that are identified by combining x-ray magnetic scattering, scanning transmission x-ray microscopy, and Hall transport technique. These skyrmions, with antiparallel aligned Dy and Co magnetic moments and a characteristic core radius of about 40~nm, are formed during the nucleation and annihilation of the magnetic maze-like domain pattern exhibiting a topological Hall effect contribution. Our findings provide a promising route for fundamental research in the field of ferrimagnetic/antiferromagnetic spintronics towards practical applications.

cond-mat.mtrl-sci

Electron capture of Xe$^{54+}$ in collisions with H${_2}$ molecules in the energy range between 5.5 MeV/u and 30.9 MeV/u

The electron capture process was studied for Xe$^{54+}$ colliding with H$_2$ molecules at the internal gas target of the ESR storage ring at GSI, Darmstadt. Cross section values for electron capture into excited projectile states were deduced from the observed emission cross section of Lyman radiation, being emitted by the hydrogen-like ions subsequent to the capture of a target electron. The ion beam energy range was varied between 5.5 MeV/u and 30.9 MeV/u by applying the deceleration mode of the ESR. Thus, electron capture data was recorded at the intermediate and in particular the low collision energy regime, well below the beam energy necessary to produce bare xenon ions. The obtained data is found to be in reasonable qualitative agreement with theoretical approaches, while a commonly applied empirical formula significantly overestimates the experimental findings.

physics.atom-ph

Real-space imaging of confined magnetic skyrmion tubes

Magnetic skyrmions are topologically nontrivial particles with a potential application as information elements in future spintronic device architectures. While they are commonly portrayed as two dimensional objects, in reality magnetic skyrmions are thought to exist as elongated, tube-like objects extending through the thickness of the sample. Study of this skyrmion tube (SkT) state is highly relevant for investigating skyrmion metastability and for implementation in recently proposed magnonic computing. However, direct experimental imaging of skyrmion tubes has yet to be reported. Here, we demonstrate the first real-space observation of skyrmion tubes in a lamella of FeGe using resonant magnetic x-ray imaging and comparative micromagnetic simulations, confirming their extended structure. The formation of these structures at the edge of the sample highlights the importance of confinement and edge effects in the stabilisation of the SkT state, opening the door to further investigations into this unexplored dimension of the skyrmion spin texture.

cond-mat.str-el

Extracting the Dynamic Magnetic Contrast in Time-Resolved X-ray Transmission Microscopy

Using a time-resolved detection scheme in scanning transmission X-ray microscopy (STXM) we measured element resolved ferromagnetic resonance (FMR) at microwave frequencies up to 10\,GHz and a spatial resolution down to 20\,nm at two different synchrotrons. We present different methods to separate the contribution of the background from the dynamic magnetic contrast based on the X-ray magnetic circular dichroism (XMCD) effect. The relative phase between the GHz microwave excitation and the X-ray pulses generated by the synchrotron, as well as the opening angle of the precession at FMR can be quantified. A detailed analysis for homogeneous and inhomogeneous magnetic excitations demonstrates that the dynamic contrast indeed behaves as the usual XMCD effect. The dynamic magnetic contrast in time-resolved STXM has the potential be a powerful tool to study the linear and non-linear magnetic excitations in magnetic micro- and nano-structures with unique spatial-temporal resolution in combination with element selectivity.

cond-mat.mes-hall

Nanoscale X-Ray Imaging of Spin Dynamics in Yttrium Iron Garnet

Time-resolved scanning transmission x-ray microscopy (TR-STXM) has been used for the direct imaging of spin wave dynamics in thin film yttrium iron garnet (YIG) with spatial resolution in the sub 100 nm range. Application of this x-ray transmission technique to single crystalline garnet films was achieved by extracting a lamella (13x5x0.185 $\mathrm{μm^3}$) of liquid phase epitaxy grown YIG thin film out of a gadolinium gallium garnet substrate. Spin waves in the sample were measured along the Damon-Eshbach and backward volume directions of propagation at gigahertz frequencies and with wavelengths in a range between 100~nm and 10~$\mathrmμ$m. The results were compared to theoretical models. Here, the widely used approximate dispersion equation for dipole-exchange spin waves proved to be insufficient for describing the observed Damon-Eshbach type modes. For achieving an accurate description, we made use of the full analytical theory taking mode-hybridization effects into account.

cond-mat.mes-hall

Approaching the Gamow window with stored ions: Direct measurement of $^{124}$Xe(p,$γ$) in the ESR storage ring

We report the first measurement of low-energy proton-capture cross sections of $^{124}$Xe in a heavy ion storage ring. $^{124}$Xe$^{54+}$ ions of five different beam energies between 5.5 AMeV and 8 AMeV were stored to collide with a windowless hydrogen target. The $^{125}$Cs reaction products were directly detected. The interaction energies are located on the high energy tail of the Gamow window for hot, explosive scenarios such as supernovae and X-ray binaries. The results serve as an important test of predicted astrophysical reaction rates in this mass range. Good agreement in the prediction of the astrophysically important proton width at low energy is found, with only a 30% difference between measurement and theory. Larger deviations are found above the neutron emission threshold, where also neutron- and $γ$-widths significantly impact the cross sections. The newly established experimental method is a very powerful tool to investigate nuclear reactions on rare ion beams at low center-of-mass energies.

nucl-ex

Coherent excitation of heterosymmetric spin waves with ultrashort wavelengths

In the emerging field of magnonics, spin waves are foreseen as signal carriers for future spintronic information processing and communication devices, owing to both the very low power losses and a high device miniaturisation potential predicted for short-wavelength spin waves. Yet, the efficient excitation and controlled propagation of nanoscale spin waves remains a severe challenge. Here, we report the observation of high-amplitude, ultrashort dipole-exchange spin waves (down to 80 nm wavelength at 10 GHz frequency) in a ferromagnetic single layer system, coherently excited by the driven dynamics of a spin vortex core. We used time-resolved x-ray microscopy to directly image such propagating spin waves and their excitation over a wide range of frequencies. By further analysis, we found that these waves exhibit a heterosymmetric mode profile, involving regions with anti-Larmor precession sense and purely linear magnetic oscillation. In particular, this mode profile consists of dynamic vortices with laterally alternating helicity, leading to a partial magnetic flux closure over the film thickness, which is explained by a strong and unexpected mode hybridisation. This spin-wave phenomenon observed is a general effect inherent to the dynamics of sufficiently thick ferromagnetic single layer films, independent of the specific excitation method employed.

cond-mat.mes-hall