arXiv subjects

M. Zahirul Alam

Publications and source records attributed to M. Zahirul Alam.

8 recordsLinked to original sources

arXiv2025

An epsilon-near-zero-based nonlinear platform for ultrafast re-writable holography

We re-examine real-time holography for all-optical structuring of light and optical computation using a contemporary material: a subwavelength-thick, spatially unstructured film of indium tin oxide (ITO). When excited by spatially structured light at epsilon-near-zero frequencies, the film acts as an efficient and reconfigurable diffractive optical platform for all-optical modulation of light such as spatial structuring and optical computations. We demonstrate a few percent of absolute diffraction efficiency over greater than 300 nm bandwidth around telecom wavelengths using a film four orders of magnitude thinner than and up to six orders of magnitude faster than standard holographic materials. Our findings highlight the potential of using epsilon-near-zero-based nanostructures for efficient modulation of spatially structured light and rapid prototyping without complex nanofabrication processes.

physics.optics↗

arXiv2025

Hybrid Deep Reconstruction for Vignetting-Free Upconversion Imaging through Scattering in ENZ Materials

Optical imaging through turbid or heterogeneous environments (collectively referred to as complex media) is fundamentally challenged by scattering, which scrambles structured spatial and phase information. To address this, we propose a hybrid-supervised deep learning framework to reconstruct high-fidelity images from nonlinear scattering measurements acquired with a time-gated epsilon-near-zero (ENZ) imaging system. The system leverages four-wave mixing (FWM) in subwavelength indium tin oxide (ITO) films to temporally isolate ballistic photons, thus rejecting multiply scattered light and enhancing contrast. To recover structured features from these signals, we introduce DeepTimeGate, a U-Net-based supervised model that performs initial reconstruction, followed by a Deep Image Prior (DIP) refinement stage using self-supervised learning. Our approach demonstrates strong performance across different imaging scenarios, including binary resolution patterns and complex vortex-phase masks, under varied scattering conditions. Compared to raw scattering inputs, it boosts average PSNR by 124%, SSIM by 231%, and achieves a 10 times improvement in intersection-over-union (IoU). Beyond enhancing fidelity, our method removes the vignetting effect and expands the effective field-of-view compared to the ENZ-based optical time gate output. These results suggest broad applicability in biomedical imaging, in-solution diagnostics, and other scenarios where conventional optical imaging fails due to scattering.

physics.optics↗

arXiv2025

High-fidelity spatial information transfer through dynamic scattering media by an epsilon-near-zero time-gate

Transparent conducting oxides (TCO) such as indium-tin-oxide (ITO) exhibit strong optical nonlinearity in the frequency range where their permittivities are near zero. We leverage this nonlinear optical response to realize a sub-picosecond time-gate based on upconversion (or sum-) four-wave mixing (FWM) between two ultrashort pulses centered at the epsilon-near-zero (ENZ) wavelength in a sub-micron-thick ITO film. The time-gate removes the effect of both static and dynamic scattering on the signal pulse by retaining only the ballistic photons of the pulse, that is, the photons that are not scattered. Thus, the spatial information encoded in either the intensity or the phase of the signal pulse can be preserved and transmitted with high fidelity through scattering media. Furthermore, in the presence of time-varying scattering, our time-gate can reduce the resulting scintillation by two orders of magnitude. In contrast to traditional bulk nonlinear materials, time gating by sum-FWM in a sub-wavelength-thick ENZ film can produce a scattering-free upconverted signal at a visible wavelength without sacrificing spatial resolution, which is usually limited by the phase-matching condition. Our proof-of-principle experiment can have implications for potential applications such as \textit{in vivo} diagnostic imaging and free-space optical communication.

physics.optics↗

arXiv2021

Relaxed phase-matching constraints in zero-index waveguides

The nonlinear optical response of materials is the foundation upon which applications such as frequency conversion, all-optical signal processing, molecular spectroscopy, and nonlinear microscopy are built. However, the utility of all such parametric nonlinear optical processes is hampered by phase-matching requirements. Quasi-phase-matching, birefringent phase matching, and higher-order-mode phase matching have all been developed to address this constraint, but the methods demonstrated to date suffer from the inconvenience of only being phase-matched for a single, specific arrangement of beams, typically co-propagating, resulting in cumbersome experimental configurations and large footprints for integrated devices. Here, we experimentally demonstrate that these phase-matching requirements may be satisfied in a parametric nonlinear optical process for multiple, if not all, configurations of input and output beams when using low-index media. Our measurement constitutes the first experimental observation of direction-independent phase matching for a medium sufficiently long for phase matching concerns to be relevant. We demonstrate four-wave mixing from spectrally distinct co- and counter-propagating pump and probe beams, the backward-generation of a nonlinear signal, and excitation by an out-of-plane probe beam. These results explicitly show that the unique properties of low-index media relax traditional phase-matching constraints, which can be exploited to facilitate nonlinear interactions and miniaturize nonlinear devices, thus adding to the established exceptional properties of low-index materials.

physics.optics↗

arXiv2021

Enhanced Nonlinear Optical Responses of Layered Epsilon-Near-Zero Metamaterials at Visible Frequencies

Optical materials with vanishing dielectric permittivity, known as epsilon-near-zero (ENZ) materials, have been shown to possess enhanced nonlinear optical responses in their ENZ region. These strong nonlinear optical properties have been firmly established in homogeneous materials; however, it is as of yet unclear whether metamaterials with effective optical parameters can exhibit a similar enhancement. Here, we probe an optical ENZ metamaterial composed of a subwavelength periodic stack of alternating Ag and SiO$_2$ layers and measure a nonlinear refractive index $n_2 = (1.2 \pm 0.1) \times 10^{-12}$ m$^2$/W and nonlinear absorption coefficient $β= (-1.5 \pm 0.2) \times 10^{-5}$ m/W at its effective zero-permittivity wavelength. The measured $n_2$ is $10^7$ times larger than $n_2$ of fused silica and four times larger than that the $n_2$ of silver. We observe that the nonlinear enhancement in $n_2$ scales as $1/(n_0 \mathrm{Re}[n_0])$, where $n_0$ is the linear effective refractive index. As opposed to homogeneous ENZ materials, whose optical properties are dictated by their intrinsic material properties and hence are not widely tunable, the zero-permittivity wavelength of the demonstrated metamaterials may be chosen to lie anywhere within the visible spectrum by selecting the right thicknesses of the sub-wavelength layers. Consequently, our results offer the promise of a means to design metamaterials with large nonlinearities for applications in nanophotonics at any specified optical wavelength.

physics.optics↗

arXiv2021

Ultra-high-Q resonances in plasmonic metasurfaces

Plasmonic nanostructures hold promise for the realization of ultra-thin sub-wavelength devices, reducing power operating thresholds and enabling nonlinear optical functionality in metasurfaces. However, this promise is substantially undercut by absorption introduced by resistive losses, causing the metasurface community to turn away from plasmonics in favour of alternative material platforms (e.g., dielectrics) that provide weaker field enhancement, but more tolerable losses. Here, we report a plasmonic metasurface with a quality-factor (Q-factor) of 2340 in the telecommunication C band by exploiting surface lattice resonances (SLRs), exceeding the record by an order of magnitude. Additionally, we show that SLRs retain many of the same benefits as localized plasmonic resonances, such as field enhancement and strong confinement of light along the metal surface. Our results demonstrate that SLRs provide an exciting and unexplored method to tailor incident light fields, and could pave the way to flexible wavelength-scale devices for any optical resonating application.

physics.optics↗

arXiv2020

On modifications of fundamental radiative processes in near-zero-index media of various dimensions

Spontaneous emission, stimulated emission and absorption are the three fundamental radiative processes describing light-matter interactions. Here, we theoretically study the behaviour of these fundamental processes inside an unbounded medium exhibiting a vanishingly small refractive index, i.e., a near-zero-index (NZI) host medium. We present a generalized framework to study these processes and find that the spatial dimension of the NZI medium has profound effects on the nature of the fundamental radiative processes. Our formalism highlights the role of the number of available optical modes as well as the ability of an emitter to couple to these modes as a function of the dimension and the class of NZI media. We demonstrate that the fundamental radiative processes are inhibited in 3D homogeneous lossless zero index materials but may be strongly enhanced in a zero index medium of reduced dimensionality. Our findings have implications in thermal, nonlinear and quantum optics as well as in designing quantum metamaterials at optical or microwave frequencies.

physics.optics↗

arXiv2017

Beyond the perturbative description of the nonlinear optical response of low-index materials

We show that standard approximations in nonlinear optics are violated for situations involving a small value of the linear refractive index. Consequently, the conventional equation for the intensity-dependent refractive index, $n(I) = n_0 + n_2 I$, becomes inapplicable in epsilon-near-zero and low-index media, even in the presence of only third-order effects. For the particular case of indium tin oxide, we find that the $χ^{(3)}$, $χ^{(5)}$ and $χ^{(7)}$ contributions to refraction eclipse the linear term; thus, the nonlinear response can no longer be interpreted as a perturbation in these materials. Although the response is non-perturbative, we find no evidence that the power series expansion of the material polarization diverges.

physics.optics↗