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Ma Chunlan

Publications and source records attributed to Ma Chunlan.

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Phase-slip residual-order spin state in FeSe

In unconventional superconductors, the microscopic form of magnetic correlations is crucial for identifying the origin of spin fluctuations and the associated pairing interaction. FeSe superconducts without chemical doping and shows no static long-range magnetic order, yet inelastic neutron scattering reveals a strong stripe response, finite linewidths, and reproducible Neel-side spectral weight. Here we propose a phase-slip residual-order spin state (ROSS). Stripe, Neel, pair-checkerboard, and staggered trimer antiferromagnetic states can be unified as symmetric phase-slip derivatives of a stripe background, while more general asymmetric phase slips form lower-energy configurations and reconstruct the spin structure factor S(q) within a finite coherence length. The ROSS therefore reconciles the absence of static magnetic order with strong spin excitations, provides a microscopic picture for the origin of spin fluctuations in FeSe, and establishes a magnetic basis for understanding pairing in unconventional superconducting systems with similar magnetic fingerprints.

cond-mat.supr-con

Revisiting the configurations of hydrogen impurities in SrTiO3: Insights from first-principles local vibration mode calculations

The specific configurations of hydrogen impurities in SrTiO3 (STO) are still ambiguous. In this study, we systematically investigate the configurations and vibrational properties of hy-drogen impurities in cubic STO using first-principles local vibration mode calculations. Em-ploying the appropriate hybrid exchange correlation functional with the fraction of exact ex-change setting to 0.2, we revisit the interstitial hydrogen (Hi), Hi complexes (2Hi), and various intrinsic cation vacancy complexes with Hi, including VSr-Hi, VSr-2Hi, VTi-Hi, and VTi-2Hi. Comparison of the computed vibrational frequencies with experimental infrared absorption bands reveals that Hi, with a frequency of 3277 cm-1, is unlikely to account for the dominant absorption bands near 3500 cm-1. Instead, strontium vacancy complexes with interstitial hydro-gen (VSr-Hi and VSr-2Hi) exhibit vibrational frequencies that align with the main absorption bands, whereas titanium vacancy complex with two interstitial hydrogen (VTi-2Hi) corresponds to additional absorption bands around 3300 cm-1. These findings provide insights into the im-portance of hydrogen-related complexes in governing the electronic properties of STO, and meanwhile underscore the necessity of employing accurate exchange correlation functionals for reliable theoretical predictions of vibrational properties.

cond-mat.mtrl-sci