SearcharxivSearch

arXiv subjects

Maarten A. Brems

Publications and source records attributed to Maarten A. Brems.

15 recordsLinked to original sources

Skyrmion Lattice Domain Formation in a Non-Flat Energy Landscape

Magnetic skyrmions are chiral spin structures with non-trivial topology that comprise two-dimensional quasi-particles and are promising information carriers for data storage and processing devices. Skyrmion lattices in magnetic thin films exhibit Kosterlitz-Thouless-Halperin-Nelson-Young (KTHNY) phase transitions and have garnered significant interest for studying emergent 2D phase behavior. In experimental skyrmion lattices, the main factor limiting the quasi-long-range order in thin films has been the non-flat energy landscape - often referred to as pinning effects. We demonstrate direct control of the skyrmion lattice order by effectively tuning the energy landscape employing magnetic field oscillations. By quantifying lattice order and dynamics, we explore how domain boundaries form and evolve due to pinning effects in Kerr microscopy experiments and in Brownian dynamics simulations, offering a pathway to control and study emergent skyrmion lattice properties and 2D phase behavior.

cond-mat.mes-hall

Skyrmion Lattice Order Controlled by Confinement Geometry

Magnetic skyrmions forming two-dimensional (2D) lattices provide a versatile platform for investigating phase transitions predicted by Kosterlitz-Thouless-Halperin-Nelson-Young (KTHNY) theory. While 2D melting in skyrmion systems has been demonstrated, achieving controlled ordering in skyrmion lattices remains challenging due to pinning effects from a non-uniform energy landscape, which often results in polycrystalline structures. Skyrmions in thin films, however, offer thermal diffusion with high tunability and can be directly imaged via Kerr microscopy, enabling real-time observation of their dynamics. To regulate lattice order in such flexible systems, we introduce geometric confinements of varying shapes. Combining Kerr microscopy experiments with Thiele model simulations, we demonstrate that confinement geometry critically influences lattice order. Specifically, hexagonal confinements commensurate with the skyrmion lattice stabilize monodomain hexagonal ordering, while incommensurate geometries induce domain formation and reduce overall order. Understanding these boundary-driven effects is essential for advancing the study of 2D phase behavior and for the design of skyrmion-based spintronic applications, ranging from memory devices to unconventional computing architectures.

cond-mat.mes-hall

Real-Time Modeling of Skyrmion Dynamics in Arbitrary 2D Spatially Dependent Pinning Potential Landscapes

Non-flat energy landscapes leading to localized pinning of skyrmions pose an inherent and unavoidable challenge for studies of fundamental 2D spin structure dynamics as well as applications. Accounting for pinning is a key requirement for predictive modeling of skyrmion systems, as it impacts the systems' dynamics and introduces randomizing effects. In this article, we use magneto-optical Kerr microscopy to image skyrmions in a magnetic thin film system in real time and analyze their hopping dynamics within the non-flat energy landscape. To achieve a fully quantitative model, we utilize skyrmion diffusion and dwell times at pinning sites to extrapolate the pinning energy landscape into regions that cannot be sampled on reasonable experimental time scales. For evaluation with a coarse-grained Thiele model, we perform long-time measurements of skyrmion diffusion and then develop a two-step procedure to determine simulation parameters by comparing them to experimentally accessible behavior. This provides a direct conversion between simulation and experimental units, which is the missing key step that has previously prevented quantitative quasiparticle modeling. We demonstrate the predictive power of our approach by measuring the experimentally unexplored density dependence of skyrmion diffusion and show that it is in excellent agreement with simulation predictions. Our technique thus enables quantitative skyrmion simulations on experimental time and length scales, allowing for predictive in-silico prototyping of skyrmion devices.

cond-mat.stat-mech

Realizing Quantitative Quasiparticle Modeling of Skyrmion Dynamics in Arbitrary Potentials

We demonstrate fully quantitative Thiele model simulations of magnetic skyrmion dynamics on previously unattainable experimentally relevant large length and time scales by ascertaining the key missing parameters needed to calibrate the experimental and simulation time scales and current-induced forces. Our work allows us to determine complete spatial pinning energy landscapes that enable quantification of experimental studies of diffusion in arbitrary potentials within the Lifson-Jackson framework. Our method enables us to ascertain the time scales, and by isolating the effect of ultra-low current density (order $10^6 A/m^2$) generated torques we directly infer the total force acting on the skyrmion for a quantitative modelling.

cond-mat.stat-mech

Imaging Topological Defect Dynamics Mediating 2D Skyrmion Lattice Melting

Topological defects are the key feature mediating 2D phase transitions. However, both resolution and tunability have been lacking to access the dynamics of the transitions. With dynamic Kerr microscopy, we directly capture the melting of a confined 2D magnetic skyrmion lattice with high resolution in real-time and -space. Skyrmions in magnetic thin films are two-dimensional, topologically non-trivial quasi-particles that provide rich dynamics as well as unique tunability as an essential ingredient for controlling phase behavior: We tune the skyrmion size and effective temperature on the fly to drive the two-step melting through an intermediate hexatic regime between the solid lattice and the isotropic liquid. We quantify the characteristic occurrence of topological defects mediating the transitions and reveal the so-far inaccessible dynamics of the lattice dislocations. The full real-time and -space imaging reveals the diffusion coefficient of the dislocations, which we find to be orders of magnitudes higher than that of the skyrmions.

cond-mat.stat-mech

Skyrmion flow in periodically modulated channels

Magnetic skyrmions, topologically stabilized chiral magnetic textures with particle-like properties have so far primarily been studied statically. Here, we experimentally investigate the dynamics of skyrmion ensembles in metallic thin film conduits where they behave as quasi-particle fluids. By exploiting our access to the full trajectories of all fluid particles by means of time-resolved magneto-optical Kerr microscopy, we demonstrate that boundary conditions of skyrmion fluids can be tuned by modulation of the channel geometry. We observe as a function of channel width deviations from classical flow profiles even into the no- or partial-slip regime. Unlike conventional colloids, the skyrmion Hall effect can also introduce transversal flow-asymmetries and even local motion of single skyrmions against the driving force which we explore with particle-based simulations, demonstrating the unique properties of skyrmion liquid flow that uniquely deviates from previously known behavior of other quasi-particles.

cond-mat.mes-hall

Gesture recognition with Brownian reservoir computing using geometrically confined skyrmion dynamics

Physical reservoir computing (RC) is a beyond von-Neumann computing paradigm that harnesses the dynamical properties of a complex physical system (reservoir) to process information efficiently in tasks such as pattern recognition. This hardware-centered approach drastically reduces training efforts and holds potential for significantly reduced energy consumption operation. Magnetic skyrmions, topological, particle-like spin textures, are considered highly promising candidates for reservoir computing systems due to their non-linear interactions and established mechanisms for low power manipulation combined with thermally excited dynamics. So far spin-based reservoir computing has been used for static detection or has been based on intrinsic magnetization dynamics timescales, that require cumbersome rescaling of typically slower real-world data. Here we harness the power of time-multiplexed skyrmion RC by adjusting the intrinsic timescales of the reservoir to the timescales of real-world temporal patterns: we recognize hand gestures recorded with range-doppler radar on a millisecond timescale and feed the data as a time-dependent voltage excitation directly into our device. We observe the temporal evolution of the skyrmion trajectory using read-out at just one position of the reservoir, which allows for scaling onto the nanometer scale. We find that our hardware solution exhibits competitive performance compared with a state-of-the-art energy-intensive software-based neural network. The key advantage of our hardware approach lies in its capacity to seamlessly integrate data from sensors without the need for temporal conversion, thanks to the time-dependent input and tunable intrinsic timescales of the skyrmion dynamics in the reservoir. This feature enables real-time feeding of the reservoir, opening a multitude of applications.

cond-mat.mtrl-sci

Perspective on unconventional computing using magnetic skyrmions

Learning and pattern recognition inevitably requires memory of previous events, a feature that conventional CMOS hardware needs to artificially simulate. Dynamical systems naturally provide the memory, complexity, and nonlinearity needed for a plethora of different unconventional computing approaches. In this perspective article, we focus on the unconventional computing concept of reservoir computing and provide an overview of key physical reservoir works reported. We focus on the promising platform of magnetic structures and, in particular, skyrmions, which potentially allow for low-power applications. Moreover, we discuss skyrmion-based implementations of Brownian computing, which has recently been combined with reservoir computing. This computing paradigm leverages the thermal fluctuations present in many skyrmion systems. Finally, we provide an outlook on the most important challenges in this field.

cs.ET

Coarse-graining collective skyrmion dynamics in confined geometries

Magnetic skyrmions are magnetic quasi-particles with enhanced stability and different manipulation mechanisms using external fields and currents making them promising candidates for future applications for instance in neuromorphic computing. Recently, several measurements and simulations have shown that thermally activated skyrmions in confined geometries, as they are necessary for device applications, arrange themselves predominantly based on commensurability effects. In this simulational study, based on the Thiele model, we investigate the enhanced dynamics and degenerate non-equilibrium steady state of a system in which the intrinsic skyrmion-skyrmion and skyrmion-boundary interaction compete with thermal fluctuations as well as current-induced spin-orbit torques. The investigated system is a triangular-shaped confinement geometry hosting four skyrmions, where we inject spin-polarized currents between two corners of the structure. We coarse-grain the skyrmion states in the system to analyze the intricacies of skyrmion arrangements of the skyrmion ensemble. In the context of neuromorphic computing, such methods address the key challenge of optimizing read-out positions in confined geometries and form the basis to understand collective skyrmion dynamics in systems with competing interactions on different scales.

cond-mat.mtrl-sci

AlphaFold predicts the most complex protein knot and composite protein knots

The computer artificial intelligence system AlphaFold has recently predicted previously unknown three-dimensional structures of thousands of proteins. Focusing on the subset with high-confidence scores, we algorithmically analyze these predictions for cases where the protein backbone exhibits rare topological complexity, i.e. knotting. Amongst others, we discovered a $7_1$-knot, the most topologically complex knot ever found in a protein, as well several 6-crossing composite knots comprised of two methyltransferase or carbonic anhydrase domains, each containing a simple trefoil knot. These deeply embedded composite knots occur evidently by gene duplication and interconnection of knotted dimers. Finally, we report two new five-crossing knots including the first $5_1$-knot. Our list of analyzed structures forms the basis for future experimental studies to confirm these novel knotted topologies and to explore their complex folding mechanisms.

q-bio.BM

Constructing coarse-grained skyrmion potentials from experimental data with Iterative Boltzmann Inversion

In an effort to understand skyrmion behavior on a coarse-grained level, skyrmions are often described as 2D quasi particles evolving according to the Thiele equation. Interaction potentials are the key missing parameters for predictive modeling of experiments. We apply the Iterative Boltzmann Inversion technique commonly used in soft matter simulations to construct potentials for skyrmion-skyrmion and skyrmion-magnetic material boundary interactions from a single experimental measurement without any prior assumptions of the potential form. We find that the two interactions are purely repulsive and can be described by an exponential function for experimentally relevant skyrmions. This captures the physics on experimental time and length scales that are of interest for most skyrmion applications and typically inaccessible to atomistic or micromagnetic simulations.

cond-mat.mtrl-sci

Brownian reservoir computing realized using geometrically confined skyrmions

Reservoir computing (RC) has been considered as one of the key computational principles beyond von-Neumann computing. Magnetic skyrmions, topological particle-like spin textures in magnetic films are particularly promising for implementing RC, since they respond strongly nonlinear to external stimuli and feature inherent multiscale dynamics. However, despite several theoretical proposals that exist for skyrmion reservoir computing, experimental realizations have been elusive until now. Here, we propose and experimentally demonstrate a conceptually new approach to skyrmion RC that leverages the thermally activated diffusive motion of skyrmions. By confining the electrically gated and thermal skyrmion motion, we find that already a single skyrmion in a confined geometry suffices to realize non-linearly separable functions, which we demonstrate for the XOR gate along with all other Boolean logic gate operations. Besides this universality, the reservoir computing concept ensures low training costs and ultra-low power operation with current densities orders of magnitude smaller than those used in existing spintronic reservoir computing demonstrations. Our proposed concept can be readily extended by linking multiple confined geometries and/or by including more skyrmions in the reservoir, suggesting high potential for scalable and low-energy reservoir computing.

cond-mat.mtrl-sci

Skyrmion pinning energetics in thin film systems

A key issue for skyrmion dynamics and devices are pinning effects present in real systems. While posing a challenge for the realization of conventional skyrmionics devices, exploiting pinning effects can enable non-conventional computing approaches if the details of the pinning in real samples are quantified and understood. We demonstrate that using thermal skyrmion dynamics, we can characterize the pinning of a sample and we ascertain the spatially resolved energy landscape. To understand the mechanism of the pinning, we probe the strong skyrmion size and shape dependence of the pinning. Magnetic microscopy imaging demonstrates that in contrast to findings in previous investigations, for large skyrmions the pinning originates at the skyrmion boundary and not at its core. The boundary pinning is strongly influenced by the very complex pinning energy landscape that goes beyond the conventional rigid quasi-particle description. This gives rise to complex skyrmion shape distortions and allows for dynamic switching of pinning sites and flexible tuning of the pinning.

cond-mat.mtrl-sci

Circuits and excitations to enable Brownian token-based computing with skyrmions

Brownian computing exploits thermal motion of discrete signal carriers (tokens) for computations. In this paper we address two major challenges that hinder competitive realizations of circuits and application of Brownian token-based computing in actual devices for instance based on magnetic skyrmions. To overcome the problem that crossings generate for the fabrication of circuits, we design a crossing-free layout for a composite half-adder module. This layout greatly simplifies experimental implementations as wire crossings are effectively avoided. Additionally, our design is shorter to speed up computations compared to conventional designs. To address the key issue of slow computation based on thermal excitations, we propose to overlay artificial diffusion induced by an external excitation mechanism. For instance, if magnetic skyrmions are used as tokens, artificially induced diffusion by spin-orbit torques or other mechanisms increases the speed of computations by several orders of magnitude. Combined with conventional Brownian computing the latter could greatly enhance the application scenarios of token-based computing for instance for low power devices such as autonomous sensors with limited power that is harvested from the environment.

cond-mat.mes-hall

Commensurability between element symmetry and the number of skyrmions governing skyrmion diffusion in confined geometries

Magnetic skyrmions are topological magnetic structures, which exhibit quasi-particle properties and can show enhanced stability against perturbation from thermal noise. Recently, thermal Brownian diffusion of these quasi-particles has been found in continuous films and applications in unconventional computing have received significant attention, which however require structured elements. Thus, as the next necessary step, we here study skyrmion diffusion in confined geometries and find it to be qualitatively different: The diffusion is governed by the interplay between the total number of skyrmions and the structure geometry. In particular, we ascertain the effect of circular and triangular geometrical confinement and find that for triangular geometries the behavior is drastically different for the cases when the number of skyrmions in the element is either commensurate or incommensurate with a symmetric filling of the element. This influence of commensurability is corroborated by simulations of a quasi-particle model.

cond-mat.mtrl-sci