arXiv subjects

Maarten R. Wegewijs

Publications and source records attributed to Maarten R. Wegewijs.

At least 19 recordsLinked to original sources

arXiv2024

RealTimeTransport: An open-source C++ library for quantum transport simulations in the strong coupling regime

The description of quantum transport in the strong system-reservoir coupling regime poses a significant theoretical and computational challenge that demands specialized tools for accurate analysis. RealTimeTransport is a new open-source C++ library that enables the computation of both stationary and transient transport observables for generic quantum systems connected to metallic reservoirs. It computes the Nakajima-Zwanzig memory kernels for both dynamics and transport in real-time going beyond traditional expansions in the bare system-reservoir couplings. Currently, several methods are available: (i) A renormalized perturbation theory in leading and next-to-leading order which avoids the low-temperature breakdown that limits the traditional theory. (ii) Starting from this well-behaved reference solution a 2- and 3-loop self-consistent renormalization-group transformation of the memory kernels is implemented. This allows refined quantitative predictions even in the presence of many body resonances, such as the Kondo enhancement of cotunneling. This paper provides an overview of the theory, the architecture of RealTimeTransport and practical demonstrations of the currently implemented methods. In particular, we analyze the stationary transport through a serial double quantum dot and showcase for the $T=0$ interacting Anderson model the complete time-development of single-electron tunneling (SET), cotunneling-assisted SET (CO-SET) and inelastic cotunneling resonances throughout the entire gate-bias stability diagram. We discuss the range of applicability of the implemented methods and benchmark them against other advanced approaches.

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arXiv2023

Transient transport spectroscopy of an interacting quantum dot proximized by a superconductor: Charge- and heat-currents after a switch

We analyze the time-evolution of a quantum dot which is proximized by a large-gap superconductor and weakly probed using the charge and heat currents into a wide-band metal electrode. We map out the full time dependence of these currents after initializing the system by a switch. We find that due to the proximity effect there are two simple yet distinct switching procedures which initialize a non-stationary mixture of the gate-voltage dependent eigenstates of the proximized quantum dot. We find in particular that the ensuing time-dependent heat current is a sensitive two-particle probe of the interplay of strong Coulomb interaction and induced superconducting pairing. The pairing can lead to a suppression of charge and heat current decay which we analyze in detail. The analysis of the results makes crucial use of analytic formulas obtained using fermionic duality, a ``dissipative symmetry'' of the master equation describing this class of open systems.

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arXiv2022

Solution of master equations by fermionic-duality: Time-dependent charge and heat currents through an interacting quantum dot proximized by a superconductor

We analyze the time-dependent solution of master equations by exploiting fermionic duality, a dissipative symmetry applicable to a large class of open systems describing quantum transport. Whereas previous studies mostly exploited duality relations after partially solving the evolution equations, we here systematically exploit the invariance under the fermionic duality mapping from the very beginning when setting up these equations. Moreover, we extend the resulting simplifications -- so far applied to the local state evolution- to non-local observables such as transport currents. We showcase the exploitation of fermionic duality for a quantum dot with strong interaction -- covering both the repulsive and attractive case -- proximized by contact with a large-gap superconductor which is weakly probed by charge and heat currents into a wide-band normal-metal electrode. We derive the complete time-dependent analytical solution of this problem involving non-equilibrium Cooper pair transport, Andreev bound states and strong interaction. Additionally exploiting detailed balance we show that even for this relatively complex problem the evolution towards the stationary state can be understood analytically in terms of the stationary state of the system itself via its relation to the stationary state of a dual system with inverted Coulomb interaction, superconducting pairing and applied voltages.

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arXiv2020

Thermovoltage in quantum dots with attractive interaction

We study the linear and nonlinear thermovoltage of a quantum dot with effective attractive electron-electron interaction and weak, energy-dependent tunnel-coupling to electronic contacts. Remarkably, we find that the thermovoltage shows signatures of repulsive interaction which can be rationalized. These thermovoltage characteristics are robust against large potential and temperature differences well into the nonlinear regime, which we expect can be demonstrated in current state-of-the-art experiments. Furthermore, under nonlinear operation, we find extended regions of large power production at efficiencies on the order of the Curzon-Ahlborn bound interrupted only by a characteristic sharp dip.

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arXiv2017

Thermoelectrics of Interacting Nanosystems -- Exploiting Superselection instead of Time-Reversal Symmetry

Thermoelectric transport is traditionally analyzed using relations imposed by time-reversal symmetry, ranging from Onsager's results to fluctuation relations in counting statistics. In this paper, we show that a recently discovered duality relation for fermionic systems -- deriving from the fundamental fermion-parity superselection principle of quantum many-particle systems -- provides new insights into thermoelectric transport. Using a master equation, we analyze the stationary charge and heat currents through a weakly coupled, but strongly interacting single-level quantum dot subject to electrical and thermal bias. In linear transport, the fermion-parity duality shows that features of thermoelectric response coefficients are actually dominated by the average and fluctuations of the charge in a dual quantum dot system, governed by attractive instead of repulsive electron-electron interaction. In the nonlinear regime, the duality furthermore relates most transport coefficients to much better understood equilibrium quantities. Finally, we naturally identify the fermion-parity as the part of the Coulomb interaction relevant for both the linear and nonlinear Fourier heat. Altogether, our findings hence reveal that next to time-reversal, the duality imposes equally important symmetry restrictions on thermoelectric transport. As such, it is also expected to simplify computations and clarify the physical understanding for more complex systems than the simplest relevant interacting nanostructure model studied here.

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arXiv2016

Transport mirages in single-molecule devices

Molecular systems can exhibit a complex, chemically tailorable inner structure which allows for targeting of specific mechanical, electronic and optical properties. At the single-molecule level, two major complementary ways to explore these properties are molecular quantum-dot structures and scanning probes. This article outlines comprehensive principles of electron-transport spectroscopy relevant to both these approaches and presents a new, high-resolution experiment on a high-spin single-molecule junction exemplifying these principles. Such spectroscopy plays a key role in further advancing our understanding of molecular and atomic systems, in particular the relaxation of their spin. In this joint experimental and theoretical analysis, particular focus is put on the crossover between resonant regime [single-electron tunneling (SET)] and the off-resonant regime [inelastic electron (co)tunneling (IETS)]. We show that the interplay of these two processes leads to unexpected mirages of resonances not captured by either of the two pictures alone. Although this turns out to be important in a large fraction of the possible regimes of level positions and bias voltages, it has been given little attention in molecular transport studies. Combined with nonequilibrium IETS -- four-electron pump-probe excitations -- these mirages provide crucial information on the relaxation of spin excitations. Our encompassing physical picture is supported by a master-equation approach that goes beyond weak coupling. The present work encourages the development of a broader connection between the fields of molecular quantum-dot and scanning probe spectroscopy.

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arXiv2016

Relaxation of quantum dots in a magnetic field at finite bias -- charge, spin and heat currents

We perform a detailed study of the effect of finite bias and magnetic field on the tunneling-induced decay of the state of a quantum dot by applying a recently discovered general duality [PRB 93, 81411 (2016)]. This duality provides deep physical insight into the decay dynamics of electronic open quantum systems with strong Coulomb interaction. It associates the amplitudes of decay eigenmodes of the actual system to the eigenmodes of a so-called dual system with attractive interaction. Thereby, it predicts many surprising features in the transient transport and its dependence on experimental control parameters: the attractive interaction of the dual model shows up as sharp features in the amplitudes of measurable time-dependent currents through the actual repulsive system. In particular, for interacting quantum dots, the time-dependent heat current exhibits a decay mode that dissipates the interaction energy and that is tied to the fermion parity of the system. We show that its decay amplitude has an unexpected gate-voltage dependence that is robust up to sizable bias voltages and then bifurcates, reflecting that the Coulomb blockade is lifted in the dual system. Furthermore, combining our duality relation with the known Iche-duality, we derive new symmetry properties of the decay rates as a function of magnetic field and gate voltage. Finally, we quantify charge- and spin-mode mixing due to the magnetic field using a single mixing parameter.

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arXiv2015

Charge fluctuations in nonlinear heat transport

We show that charge fluctuation processes are crucial for the nonlinear heat conductance through an interacting nanostructure, even far from a resonance. We illustrate this for an Anderson quantum dot accounting for the first two leading orders of the tunneling in a master equation. The often made assumption that off-resonant transport proceeds entirely by virtual occupation of charge states, underlying exchange-scattering models, can fail dramatically for heat transport. The identified energy-transport resonances in the Coulomb blockade regime provide new qualitative information about relaxation processes, for instance by strong negative differential heat conductance relative to the heat current. These can go unnoticed in the charge current, making nonlinear heat-transport spectroscopy with energy-level control a promising experimental tool.

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arXiv2014

Spintronic magnetic anisotropy

An attractive feature of magnetic adatoms and molecules for nanoscale applications is their superparamagnetism, the preferred alignment of their spin along an easy axis preventing undesired spin reversal. The underlying magnetic anisotropy barrier --a quadrupolar energy splitting-- is internally generated by spin-orbit interaction and can nowadays be probed by electronic transport. Here we predict that in a much broader class of quantum-dot systems with spin larger than one-half, superparamagnetism may arise without spin-orbit interaction: by attaching ferromagnets a spintronic exchange field of quadrupolar nature is generated locally. It can be observed in conductance measurements and surprisingly leads to enhanced spin filtering even in a state with zero average spin. Analogously to the spintronic dipolar exchange field, responsible for a local spin torque, the effect is susceptible to electric control and increases with tunnel coupling as well as with spin polarization.

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arXiv2012

Interaction-induced charge and spin pumping through a quantum dot at finite bias

We investigate charge and spin transport through an adiabatically driven, strongly interacting quantum dot weakly coupled to two metallic contacts with finite bias voltage. Within a kinetic equation approach, we identify coefficients of response to the time-dependent external driving and relate these to the concepts of charge and spin emissivities previously discussed within the time-dependent scattering matrix approach. Expressed in terms of auxiliary vector fields, the response coefficients allow for a straightforward analysis of recently predicted interaction-induced pumping under periodic modulation of the gate and bias voltage [Phys. Rev. Lett. 104, 226803 (2010)]. We perform a detailed study of this effect and the related adiabatic Coulomb blockade spectroscopy, and, in particular, extend it to spin pumping. Analytic formulas for the pumped charge and spin in the regimes of small and large driving amplitude are provided for arbitrary bias. In the absence of a magnetic field, we obtain a striking, simple relation between the pumped charge at zero bias and at bias equal to the Coulomb charging energy. At finite magnetic field, there is a possibility to have interaction-induced pure spin pumping at this finite bias value, and generally, additional features appear in the pumped charge. For large-amplitude adiabatic driving, the magnitude of both the pumped charge and spin at the various resonances saturate at values which are independent of the specific shape of the pumping cycle. Each of these values provide an independent, quantitative measurement of the junction asymmetry.

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arXiv2012

Parallel carbon nanotube quantum dots and their interactions

We present quantum transport measurements of interacting parallel quantum dots formed in the strands of a carbon nanotube rope. In this molecular quantum dot system, transport is dominated by one quantum dot, while additional resonances from parallel side dots appear, which exhibit a weak gate coupling. This differential gating effect provides a tunability of the quantum dot system with only one gate electrode and provides control over the carbon nanotube strand that carries the current. By tuning the system to different states we use quantum transport as a spectroscopic tool to investigate the inter-dot coupling and show a route to distinguish between various side dots. By comparing the experimental data with master equation calculations, we identify conditions for the tunneling rates that are required in order to observe different manifestations of the inter-dot coupling in the transport spectra.

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arXiv2012

Density-operator approaches to transport through interacting quantum dots: Simplifications in fourth-order perturbation theory

Various theoretical methods address transport effects in quantum dots beyond single-electron tunneling while accounting for the strong interactions in such systems. In this paper we report a detailed comparison between three prominent approaches to quantum transport: the fourth-order Bloch-Redfield quantum master equation (BR), the real-time diagrammatic technique (RT), and the scattering rate approach based on the T-matrix (TM). Central to the BR and RT is the generalized master equation for the reduced density matrix. We demonstrate the exact equivalence of these two techniques. By accounting for coherences (nondiagonal elements of the density matrix) between nonsecular states, we show how contributions to the transport kernels can be grouped in a physically meaningful way. This not only significantly reduces the numerical cost of evaluating the kernels but also yields expressions similar to those obtained in the TM approach, allowing for a detailed comparison. However, in the TM approach an ad hoc regularization procedure is required to cure spurious divergences in the expressions for the transition rates in the stationary (zero-frequency) limit. We show that these problems derive from incomplete cancellation of reducible contributions and do not occur in the BR and RT techniques, resulting in well-behaved expressions in the latter two cases. Additionally, we show that a standard regularization procedure of the TM rates employed in the literature does not correctly reproduce the BR and RT expressions. All the results apply to general quantum dot models and we present explicit rules for the simplified calculation of the zero-frequency kernels. Although we focus on fourth-order perturbation theory only, the results and implications generalize to higher orders. We illustrate our findings for the single impurity Anderson model with finite Coulomb interaction in a magnetic field.

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arXiv2011

Readout of carbon nanotube vibrations based on spin-phonon coupling

We propose a scheme for spin-based detection of the bending motion in suspended carbon-nanotubes, using the curvature-induced spin-orbit interaction. We show that the resulting effective spin-phonon coupling can be used to down-convert the high-frequency vibration-modulated spin-orbit field to spin-flip processes at a much lower frequency. This vibration-induced spin-resonance can be controlled with an axial magnetic field. We propose a Pauli spin blockade readout scheme and predict that the leakage current shows pronounced peaks as a function of the external magnetic field. Whereas the resonant peaks allow for frequency readout, the slightly off-resonant current is sensitive to the vibration amplitude.

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arXiv2011

Spin-dependent electronic hybridization in a rope of carbon nanotubes

We demonstrate single electron addition to different strands of a carbon nanotube rope. Anticrossings of anomalous conductance peaks occur in quantum transport measurements through the parallel quantum dots forming on the individual strands. We determine the magnitude and the sign of the hybridization as well as the Coulomb interaction between the carbon nanotube quantum dots, finding that the bonding states dominate the transport. In a magnetic field the hybridization is shown to be selectively suppressed due to spin effects.

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arXiv2010

Spin quadrupoletronics: moving spin anisotropy around

We show that spin anisotropy can be transferred to an isotropic system by transport of spin quadrupole moment. We derive the quadrupole moment current and continuity equation and study a high-spin valve structure consisting of two ferromagnets coupled to a quantum dot probing an impurity spin. The quadrupole back-action on their coupled spin results in spin torques and anisotropic spin relaxation which do not follow from standard spin current considerations. We demonstrate the detection of the impurity spin by charge transport and its manipulation by electric fields.

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arXiv2010

Electric Field Controlled Magnetic Anisotropy in a Single Molecule

We have measured quantum transport through an individual Fe$_4$ single-molecule magnet embedded in a three-terminal device geometry. The characteristic zero-field splittings of adjacent charge states and their magnetic field evolution are observed in inelastic tunneling spectroscopy. We demonstrate that the molecule retains its magnetic properties, and moreover, that the magnetic anisotropy is significantly enhanced by reversible electron addition / subtraction controlled with the gate voltage. Single-molecule magnetism can thus be electrically controlled.

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arXiv2010

Interaction-induced adiabatic non-linear transport

We calculate the time-dependent non-linear transport current through an interacting quantum dot in the single-electron tunneling regime (SET). We show that an additional dc current is generated by the electron-electron interaction by adiabatic out-of-phase modulation of the gate and bias voltage. This current can arise only when two SET resonance conditions are simultaneously satisfied. We propose an adiabatic transport spectroscopy where lock-in measurement of a "time-averaged stability diagram" probes interactions, tunnel asymmetries and changes in the ground state spin-degeneracy.

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arXiv2010

Transport via coupled states in a C60 peapod quantum dot

We have measured systematic repetitions of avoided crossings in low temperature three-terminal transport through a carbon nanotube with encapsulated C60 molecules. We show that this is a general effect of the hybridization of a host quantum dot with an impurity. The well-defined nanotube allows identification of the properties of the impurity, which we suggest to be a chain of C60 molecules inside the nanotube. This electronic coupling between the two subsystems opens the interesting and potentially useful possibility of contacting the encapsulated molecules via the tube.

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