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Maciej Lewenstein

Publications and source records attributed to Maciej Lewenstein.

At least 91 records · Page 5Linked to original sources

High Harmonic Tracking of Ultrafast Electron Dynamics across the Mott to Charge Density Wave Phase Transition

Different insulator phases compete with each other in strongly correlated materials with simultaneous local and non-local interactions. It is known that the homogeneous Mott insulator converts into a charge density wave (CDW) phase when the non-local interactions are increased, but there is ongoing debate on whether and in which parameter regimes this transition is of first order, or of second order with an intermediate bond-order wave phase. Here we show that strong-field optics applied to an extended Fermi-Hubbard system can serve as a powerful tool to reveal the nature of the quantum phase transition. Specifically, we show that in the strongly interacting regime characteristic excitations such as excitons, biexcitons, excitonic strings, and charge droplets can be tracked by the non-linear optical response to an ultrafast and intense laser pulse. Subcycle analysis of high harmonic spectra unravels the ultrafast dynamics of these increasingly complex objects, which partially escape the scrutiny of linear optics. Their appearance in the high harmonic spectrum provides striking evidence of a first-order transition into the CDW phase, and makes a strong case for using strong-field optics as a powerful tool to reveal the nature of quasiparticles in strongly correlated matter, and to track the electron dynamics during a first-order quantum phase transition.

cond-mat.str-el↗

Metrological robustness of high photon number optical cat states

In the domain of quantum metrology, cat states have demonstrated their utility despite their inherent fragility with respect to losses. Here, we introduce noise robust optical cat states which exhibit a metrological robustness for phase estimation in the regime of high photon numbers. These cat states are obtained from the intense laser driven process of high harmonic generation (HHG), and show a resilience against photon losses. Focusing on a realistic scenario including experimental imperfections we opt for the case in which we can maximize the lower bound of the quantum Fisher information (QFI) instead of analyzing the best case scenario. We show that the decrease of the QFI in the lossy case is suppressed for the HHG-cat state compared to the even and odd counterparts. In the regime of small losses of just a single photon, the HHG-cat state remains almost pure while the even/odd cat state counterparts rapidly decohere to the maximally mixed state. More importantly, this translates to a significantly enhanced robustness for the HHG-cat against photon loss, demonstrating that high photon number optical cat states can indeed be used for metrological applications even in the presence of losses.

quant-ph↗

Population annealing with topological defect driven nonlocal updates for spin systems with quenched disorder

Population Annealing, one of the currently state-of-the-art algorithms for solving spin-glass systems, sometimes finds hard disorder instances for which its equilibration quality at each temperature step is severely damaged. In such cases one can therefore not be sure about having reached the true ground state without vastly increasing the computational resources. In this work we seek to overcome this problem by proposing a quantum-inspired modification of Population Annealing. Here we focus on three-dimensional random plaquette gauge model which ground state energy problem seems to be much harder to solve than standard spin-glass Edwards-Anderson model. In analogy to the Toric Code, by allowing single bond flips we let the system explore non-physical states, effectively expanding the configurational space by the introduction of topological defects that are then annealed through an additional field parameter. The dynamics of these defects allow for the effective realization of non-local cluster moves, potentially easing the equilibration process. We study the performance of this new method in three-dimensional random plaquette gauge model lattices of various sizes and compare it against Population Annealing. With that we conclude that the newly introduced non-local moves are able to improve the equilibration of the lattices, in some cases being superior to a normal Population Annealing algorithm with a sixteen times higher computational resource investment.

cond-mat.dis-nn↗

Catching thermal avalanches in the disordered XXZ model

We study the XXZ model with a random magnetic field in contact with a weakly disordered spin chain, acting as a finite thermal bath. We revise Fermi's golden rule description of the interaction between the thermal bath and the XXZ spin chain, contrasting it with a nonperturbative quantum avalanche scenario for the thermalization of the system. We employ two-point correlation functions to define the extent $ξ_d$ of the thermalized region next to the bath. Unbounded growth of $ξ_d$ proportional to the logarithm of time or faster is a signature of an avalanche. Such behavior signifies the thermalization of the system, as we confirm numerically for a generic initial state in the ergodic and critical regimes of the XXZ spin chain. In the many-body localized regime, a clear termination of avalanches is observed for specifically prepared initial states and, surprisingly, is not visible for generic initial product states. Additionally, we extract the localization length of the local integrals of motion and show that a bath made out of a weakly disordered XXZ chain has a similar effect on the system as a bath modeled by a Hamiltonian from a Gaussian orthogonal ensemble of random matrices. We also comment on the result of the earlier study (Phys. Rev. B 108, L020201 (2023)), arguing that the observed thermalization is due to external driving of the system and does not occur in the autonomous model. Our work reveals experimentally accessible signatures of quantum avalanches and identifies conditions under which termination of the avalanches may be observed.

cond-mat.dis-nn↗

Towards the Intuitive Understanding of Quantum World: Sonification of Rabi Oscillations, Wigner functions, and Quantum Simulators

Recently, there has been considerable interest in "sonifying" scientific data; however, sonifying quantum processes using the newest quantum technologies, including Noise Intermediate Scale Quantum devices and quantum random number generators, is still an emerging area of research. Music technologists and composers employ the growing accessibility to diverse data from quantum mechanics as musical tools in the hope of generating new sound expressions. How different is the quantum world from the classical one, and is it possible to express the quantum world using sounds? Quantum phenomena are very different from those that we experience in our everyday lives. Thus, it is challenging to understand them intuitively. In this paper, we propose sonification as a method toward an intuitive understanding of various quantum mechanical phenomena, from Rabi oscillations and resonance fluorescence of a single atom through the generation of Schrödinger cat states in strong laser field physics to insulator-superfluid transition in quantum many-body systems. This paper illustrates various methods we experimented with in sonification and score representations of quantum data depending on the source data and performance settings.

quant-ph↗

Sonification of Wigner functions: case study of intense light-matter interactions

In quantum mechanics, the Wigner function $ρ_W(\textbf{r},\textbf{p})$ serves as a phase-space representation, capturing information about both the position $\textbf{r}$ and momentum $\textbf{p}$ of a quantum system. The Wigner function facilitates the calculation of expectation values of observables, examination of quantum system dynamics, and analysis of coherence and correlations. Therefore, it might serve as a tool to express quantum systems intuitively, for example, by using sonification techniques. This paper summarizes the experimental strategies employed in a previous project and delineates a new approach based on its outcomes. Emphasizing the attribution of specific Wigner functions to their underlying quantum states, dynamics, and sources; our proposed methodology seeks to refine the sonification and scoring process, aiming to enhance intuitive understanding and interpretation of quantum phenomena.

quant-ph↗

Stabilization of Hubbard-Thouless pumps through nonlocal fermionic repulsion

Thouless pumping represents a powerful concept to probe quantized topological invariants in quantum systems. We explore this mechanism in a generalized Rice-Mele Fermi-Hubbard model characterized by the presence of competing onsite and intersite interactions. Contrary to recent experimental and theoretical results, showing a breakdown of quantized pumping induced by the onsite repulsion, we prove that sufficiently large intersite interactions allow for an interaction-induced recovery of Thouless pumps. Our analysis further reveals that the occurrence of stable topological transport at large interactions is connected to the presence of a spontaneous bond-order-wave in the ground-state phase diagram of the model. Finally, we discuss a concrete experimental setup based on ultracold magnetic atoms in an optical lattice to realize the newly introduced Thouless pump. Our results provide a new mechanism to stabilize Thouless pumps in interacting quantum systems.

cond-mat.quant-gas↗

Chirped pulse control over the melting of superconductors

Strong field terahertz pulses are increasingly used to excite and control quantum materials at the ultrafast timescale. They have found widespread application by enabling direct addressing of the superconducting gap or Josephson resonances and are essential in Higgs spectroscopy. Large non-linear optical signals can be induced by the strong coupling of the THz and superconducting degrees of freedom. However, far less attention has been paid to the strong bi-directional coupling between field and material this implies. Here, we use the framework of the time-dependent Ginzburg-Landau equations to study the full field and material evolution of a superconductor driven by strong field terahertz pulses. We find that at high field strengths, the backreaction of the superconductor induces large changes to the driving pulse, which in turn leads to a runaway melting of the superconducting condensate. This results in a surprisingly large sensitivity to the initial driving pulse chirp, enabling these purely dynamical changes to result in order of magnitude different levels of melting. We also find large-scale spectral shifting of the driving pulse to occur in just a few hundred nanometers of propagation through a superconductor. We attribute these effects to an inverse plasma redshift, in which the driving field breaks Cooper pairs and decreases the free-electron mobility, analogous to reducing the density of a plasma.

cond-mat.supr-con↗

Analog simulation of high harmonic generation in atoms

The demanding experimental access to the ultrafast dynamics of materials challenges our understanding of their electronic response to applied strong laser fields. For this purpose, trapped ultracold atoms with highly controllable potentials have become an enabling tool to describe phenomena in a scenario where some effects are more easily accessible and twelve orders of magnitude slower. In this work, we introduce a mapping between the parameters of attoscience platform and atomic cloud simulators, and propose an experimental protocol to access the emission spectrum of high harmonic generation, a regime that has so far been elusive to cold atom simulation. As we illustrate, the benchmark offered by these simulators can provide new insights on the conversion efficiency of extended and short nuclear potentials, as well as the response to applied elliptical polarized fields or ultrashort few-cycle pulses.

physics.atom-ph↗

Decoupled few-femtosecond phase transitions in vanadium dioxide

The nature of the insulator-to-metal phase transition in vanadium dioxide (VO2) is one of the longest-standing problems in condensed-matter physics. Ultrafast spectroscopy has long promised to determine whether the transition is primarily driven by the electronic or structural degree of freedom, but measurements to date have been stymied by their sensitivity to only one of these components and/or their limited temporal resolution. Here we use ultra-broadband few-femtosecond pump-probe spectroscopy to resolve the electronic and structural phase transitions in VO2 at their fundamental time scales. We find that the system transforms into a bad-metallic phase within 10 fs after photoexcitation, but requires another 100 fs to complete the transition, during which we observe electronic oscillations and a partial re-opening of the bandgap, signalling a transient semi-metallic state. Comparisons with tensor-network simulations and density-functional theory calculations show these features originate from oscillations around the equilibrium high-symmetry atomic positions during an unprecedentedly fast structural transition, in which the vanadium dimers separate and untwist with two different timescales. Our results resolve the complete structural and electronic nature of the light-induced phase transition in VO2 and establish ultra-broadband few-femtosecond spectroscopy as a powerful new tool for studying quantum materials out of equilibrium.

cond-mat.str-el↗

Light-induced phase transitions in vanadium dioxide: a tensor network study

Nonequilibrium phase transitions driven by light pulses represent a rapidly developing field in condensed matter physics. As one of the archetypal strongly correlated materials, vanadium dioxide (VO2) undergoes a structural phase transition (SPT) from a monoclinic (M1) to rutile (R) structure and an insulator-to-metal transition (IMT) either when heated above 340 K or when excited by an ultrafast laser pulse. Here, we present a tensor network study of the light-induced phase transitions in VO2 based on a quasi-one-dimensional model with all the important ingredients -- multi-orbital character, electron-lattice coupling, and electron-electron correlations -- being included. We show that this model qualitatively captures the equilibrium properties of VO2 by calculating the ground state phase diagram and finite-temperature phase transitions. A hybrid quantum-classical tensor-network method is used to simulate the dynamics following photoexcitation. We find that the structure can transform faster than the harmonic phonon modes of M1 phase, suggesting lattice nonlinearity is key in the SPT. We also find separate timescales for the evolution of dimerization and tilt distortions in the lattice dynamics, as well as the loss and subsequent partial restoration behavior of the displacements, which can provide an explanation for the complex dynamics observed in recent experiments [C. Brahms et al., arXiv:XXXX.XXXXX]. Moreover, decoupled SPT and IMT dynamics are observed in the numerical simulations: while the initial M1 structure transforms to the R one in tens of femtoseconds, the IMT occurs quasi-instantaneously, consistent with recent experimental findings. Our theoretical studies provide insight into the light-induced phase transitions of VO2, revealing unexpected non-monotonic transformation pathways and paving the way for future studies of non-thermal phase transformations.

cond-mat.str-el↗

Nonclassical states of light after high-harmonic generation in semiconductors: a Bloch-based perspective

High-harmonic generation has emerged as a pivotal process in strong-field physics, yielding extreme ultraviolet radiation and attosecond pulses with a wide range of applications. Furthermore, its emergent connection with the field of quantum optics has revealed its potential for generating non-classical states of light. Here, we investigate the process of high-harmonic generation in semiconductors under a quantum optical perspective while using a Bloch-based solid-state description. Through the implementation of quantum operations based on the measurement of high-order harmonics, we demonstrate the generation of non-classical light states similar to those found when driving atomic systems. These states are characterized using diverse quantum optical observables and quantum information measures, showing the influence of electron dynamics on their properties. Additionally, we analyze the dependence of their features on solid characteristics such as the dephasing time and crystal orientation, while also assessing their sensitivity to changes in driving field strength. This study provides insights into HHG in semiconductors and its potential for generating non-classical light sources.

quant-ph↗

Spectral properties of critical 1+1D Abelian-Higgs model

The presence of gauge symmetry in 1+1D is known to be redundant, since it does not imply the existence of dynamical gauge bosons. As a consequence, in the continuum, the Abelian-Higgs model, the theory of bosonic matter interacting with photons, just possesses a single phase, as the higher dimensional Higgs and Coulomb phases are connected via non-perturbative effects. However, recent research published in [Phys. Rev. Lett. 128, 090601 (2022)] has revealed an unexpected phase transition when the system is discretized on the lattice. This transition is described by a conformal field theory with a central charge of $c=3/2$. In this paper, we aim to characterize the two components of this $c=3/2$ theory -- namely the free Majorana fermionic and bosonic parts -- through equilibrium and out-of-equilibrium spectral analyses.

hep-th↗

Universal representation by Boltzmann machines with Regularised Axons

It is widely known that Boltzmann machines are capable of representing arbitrary probability distributions over the values of their visible neurons, given enough hidden ones. However, sampling -- and thus training -- these models can be numerically hard. Recently we proposed a regularisation of the connections of Boltzmann machines, in order to control the energy landscape of the model, paving a way for efficient sampling and training. Here we formally prove that such regularised Boltzmann machines preserve the ability to represent arbitrary distributions. This is in conjunction with controlling the number of energy local minima, thus enabling easy \emph{guided} sampling and training. Furthermore, we explicitly show that regularised Boltzmann machines can store exponentially many arbitrarily correlated visible patterns with perfect retrieval, and we connect them to the Dense Associative Memory networks.

cond-mat.stat-mech↗

Generation of scalable many-body Bell correlations in spin chains with short-range two-body interactions

Dynamical generation of strong and scalable quantum resources, like many-body entanglement and Bell correlations, in spin-$1/2$ chains, is possible with all-to-all interactions, either for constant interaction strength realizing one-axis twisting protocol or for power-law decaying potentials. We show, however, that such quantum resources can also be dynamically generated with a finite range of interactions. We identify a necessary critical range and indicate a critical time when scalable quantum correlations appear. Finally, we show that the certification of generated states is accessible in the modern quantum simulator platforms.

quant-ph↗

Frustrated magnets without geometrical frustration in bosonic flux ladders

We propose a scheme to realize a frustrated Bose-Hubbard model with ultracold atoms in an optical lattice that comprises the frustrated spin-1/2 quantum XX model. Our approach is based on a square ladder of magnetic flux close to $π$ with one real and one synthetic spin dimension. Although this system does not have geometrical frustration, we show that at low energies it maps into an effective triangular ladder with staggered fluxes for specific values of the synthetic tunneling. We numerically investigate its rich phase diagram and show that it contains bond-ordered-wave and chiral superfluid phases. Our scheme gives access to minimal instances of frustrated magnets without the need for real geometrical frustration, in a setup of minimal experimental complexity.

cond-mat.quant-gas↗

Synthetic dimensions for topological and quantum phases: Perspective

In this Perspective article we report on recent progress on studies of synthetic dimensions, mostly, but not only, based on the research realized around the Barcelona groups (ICFO, UAB), Donostia (DIPC), Poznań (UAM), Kraków (UJ), and Allahabad (HRI). The concept of synthetic dimensions works particularly well in atomic physics, quantum optics, and photonics, where the internal degrees of freedom (Zeeman sublevels of the ground state, metastable excited states, or motional states for atoms, and angular momentum states or transverse modes for photons) provide the synthetic space. We describe our attempts to design quantum simulators with synthetic dimensions, to mimic curved spaces, artificial gauge fields, lattice gauge theories, twistronics, quantum random walks, and more.

quant-ph↗

Entanglement and squeezing of the optical field modes in high harmonic generation

Squeezing of optical fields, used as a powerful resource for many applications, and the radiation properties in the process of high harmonic generation have thus far been considered separately. In this Letter, we want to clarify that the joint quantum state of all the optical field modes in the process of high harmonic generation is in general entangled and squeezed. We show that this is already the case in the simplest scenario of driving uncorrelated atoms by a classical laser light field. The previous observation of product coherent states after the high harmonic generation process is a consequence of the assumption that the ground state depletion can be neglected, which is related to vanishing dipole moment correlations. Furthermore, we analyze how the resulting quadrature squeezing in the fundamental laser mode after the interaction can be controlled and explicitly show that all field modes are entangled.

quant-ph↗