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Maciej Lisicki

Publications and source records attributed to Maciej Lisicki.

At least 19 recordsLinked to original sources

Phoretic flow in a three-dimensional wedge geometry

Understanding how chemically induced surface transport generates fluid motion in confined geometries is essential for the rational design of microscale pumping devices and active microfluidic systems. Here we develop a theoretical framework for chemically driven phoretic flows in a three-dimensional wedge geometry in the diffusion-dominated regime. We formulate both the diffusion and hydrodynamic problems using a Fourier-Kontorovich-Lebedev spectral representation, exploiting the translational invariance and radial structure of the wedge. Green's functions for the concentration field are derived for reflecting and mixed reflecting-absorbing boundaries, reducing to finite image-like sums or closed-form expressions for commensurate wedge angles. The resulting slip velocity is then used to construct the three-dimensional Stokes flow through the Papkovich-Neuber representation, yielding explicit spectral solutions for the velocity field. These results establish a Green's-function framework for phoretic pumping in wedge-shaped confinement and provide analytical benchmarks for numerical simulations of chemically driven transport in confined microfluidic systems.

cond-mat.soft↗

Under pressure: poroelastic regulation of flow in espresso brewing

The sensory richness of coffee is widely recognised and arises from the complex chemistry and immersion in cultural practices of coffee preparation. In contrast, the physical complexity of espresso has received less attention. The multiphase reactive flow through a dissolving, elastic porous medium remains challenging to describe. Using a controlled experimental setup based on a café-grade espresso machine, we demonstrate that the interplay between elasticity and porosity governs the long-time flow rate during espresso extraction and, consequently, the concentration of solubles in the final beverage. We introduce a minimal model that captures the resulting non-linear pressure-flow relationship and propose a methodology capable of reproducing the time-dependent behaviour of the espresso brewing process. Finally, we show that dissolution dynamics play a central role in determining the temporal evolution of flow during extraction.

physics.flu-dyn↗

Flow-induced bending response rheometer to measure viscoelastic bending of microrods

Soft, microscale hydrogel fibers and rods play important roles in tissue engineering, flexible electronics, soft robotics, drug delivery, sensors, and other applications. Their viscoelastic mechanical properties, while critical for their function, can be challenging to characterize. We present a flow-induced bending response (FIBR) rheometer that quantifies the bending modulus and viscoelastic properties of small, hydrated fibers and rods using flow through a glass capillary. The fiber is positioned across the capillary entrance, and pressure-driven, controlled inflow of water exerts a quantifiable force on the sample. Fiber deflection is determined by video microscopy obtained simultaneously with measurements of flow rate. We develop an analytical model to resolve the hydrodynamic forces applied to the rod, and use Euler-Bernoulli beam theory to determine its material properties. Using a constant volume flow rate of water enables measurement of steady rod deflection, and thus the bending modulus. Application of viscous forces to the rod in a stepwise, cyclic or oscillatory manner enables measurement of time-dependent responses, creep recovery, viscoelastic moduli, and other properties. We demonstrate the versatility of this technique on natural and synthetic materials spanning diameters from 5 to 300 microns and elastic moduli ranging from 100 Pa to >100 MPa. Because the technique uses water to exert forces on the fiber, it works particularly well for hydrated materials, such as hydrogels and biological fibers, providing a versatile platform to characterize microscale mechanical properties of elongated structures.

cond-mat.soft↗

Biomedical active matter: Emergence and breakdown of collective functionalities

Living systems are made of active materials with microscopic components that work together to perform macroscopic biological tasks. The breakdown of these collective functionalities leads to diseases, which, conversely, could be treated by exploiting self-organization in healthcare technologies. Here, we review recent advances in this rapidly growing field of biomedical active matter. The main themes are (1) collective self-assembly and spatiotemporal coordination; (2) collective motion, transport, and navigation; (3) collective sensing, signaling, and communication; and (4) collective adaptation, evolution, and learning. We discuss these emerging processes in a wide range of systems, including protein folding, biomolecular condensates, cytoskeleton dynamics, intracellular flows, bacterial biofilms, quorum sensing, cilia synchronization, wound healing, biolocomotion, neurons, endocrine signalling, and cardiovascular flow networks. For each, we highlight medical conditions associated with reduced collective functionality and how they may be treated using microrobotic swarms, bioinspired metamaterials, diagnostics, lab-on-chip devices, organoids, and other active and adaptive matter innovations.

physics.bio-ph↗

Surfing on metachronal waves: ciliary transport by inertial coasting

Motile cilia drive biological fluid transport through whip-like beating motions that synchronize into metachronal waves. The lengths of these cilia span three orders of magnitude, from microns in human airways to millimeters in ctenophores. While recent studies have considered ciliary flows at intermediate Reynolds numbers, the effect of inertia on coordinated particle transport remains unexplored. Here, we address this gap using "Pufflets," the inertial counterparts of Stokeslets. These Pufflets describe rapidly accelerating flows generated by short-lived impulses, encoded by spatiotemporally singular momentum injections. To produce such rapid impulses experimentally, we designed an Atwood machine that generates long-lived Pufflet flows, which we capture with high-speed PIV measurements that agree well with analytical theory and simulations. Moreover, we find that pairs of equal and opposite Pufflets can drive net particle displacements and mixing due to time reversal symmetry breaking, which would be impossible in Stokes flow. Finally, we consider metachronal waves of Pufflets. Remarkably, we discover that particles can surf on these waves by coasting inertially from one cilium to the next, leading to highly efficient particle transport. This work paves the way toward understanding rapidly accelerating flows and collective transport driven by biological and artificial cilia.

physics.bio-ph↗

Diffusioosmotic corner flows

We study flows generated within a two-dimensional corner by the chemical activity of the confining boundaries. Catalytic reactions at the surfaces induce diffusioosmotic motion of the viscous fluid throughout the domain. The presence of chemically active sectors can give rise to steady eddies reminiscent of classical Moffatt vortices, which are mechanically induced in similar confined geometries. In our approach, an exact analytical solution of the diffusion problem in a wedge geometry is derived and coupled to the diffusioosmotic slip-velocity formulation, yielding the stream function of associated Stokes flow. In selected limiting cases, simple closed-form expressions provide clear physical insight into the underlying mechanisms. Our results open new perspectives for the design of microscale mixing strategies in dead-end pores and cornered microfluidic channels, and offer benchmarks for numerical simulations of confined (diffusio)osmotic systems.

physics.flu-dyn↗

The trimer paradox: the effect of stiff constraints on equilibrium distributions in overdamped dynamics

We reconsider the classical problem of a freely joined chain of Brownian particles connected by elastic springs and study its conformational probability distribution function in the overdamped regime in the limit of infinite stiffness of constraints. We show that the well-known solution by Fixman [Proc. Natl. Acad. Sci. USA 71, 3050 (1974)] is missing a shape-related term, later alluded to but not computed by Helfand [J. Chem. Phys 71, 5000 (1979)]. In our approach, the shape term, also termed zero-point energy, arises explicitly from a careful treatment of the distributional limit. We present a computationally feasible method for the calculation of the shape term and demonstrate its validity in a couple of examples.

cond-mat.stat-mech↗

Bridging advection and diffusion in the encounter dynamics of sedimenting marine snow

Sinking marine snow particles, composed primarily of organic matter, control the global export of photosynthetically fixed carbon from the ocean surface to depth. The fate of sedimenting marine snow particles is in part regulated by their encounters with suspended, micron-sized objects, which leads to mass accretion by the particles and potentially alters their buoyancy, and with bacteria that can colonize the particles and degrade them. Their collision rates are typically calculated using two types of models focusing either on direct (ballistic) interception with a finite interaction range, or advective-diffusive capture with a zero interaction range. Since the range of applicability of the two models is unknown, and many relevant marine encounter scenarios span across both regimes, quantifying such encounters remains challenging, because the two models yield asymptotically different predictions at high Péclet numbers. Here, we reconcile the two limiting approaches by quantifying the encounters in the general case using a combination of theoretical analysis and numerical simulations. Solving the advection-diffusion equation in Stokes flow around a sphere to model mass transfer to a large sinking particle by small yet finite-sized objects, we determine a new formula for the Sherwood number as a function of two dimensionless parameters: the Péclet number and the ratio of small to large particle sizes. We find that diffusion can play a significant role in generating encounters even at high Pe. At Pe as high as $10^6$, the direct interception model underestimates the encounter rate by up to two orders of magnitude. This overlooked contribution of diffusion to encounters suggests that important processes affecting the fate of marine snow, such as colonization by bacteria and plankton or accretion of neutrally buoyant gels, may proceed at a rate much faster than previously thought.

physics.flu-dyn↗

Coiling instability in the kitchen

Manipulation of viscous liquids is an essential kitchen activity - from pouring golden syrup onto a pancake to decorating a cake with whipped cream frosting, from streaming ketchup on top of French fries to dispensing molten chocolate onto a strawberry. Typical viscosities in these and many other kitchen flows, and the heights from which the streams are dispensed, make such jets susceptible to the coiling instability. Indeed, the coiling of a thin thread of poured maple syrup is a source of fascination for children and adults alike, whereas the folding of the stream of ketchup squeezed out from a plastic bottle is a phenomenon familiar to all. In this paper, we review the fluid dynamics of such kitchen flows and discuss separately the case when the substrate is stationary (honey on a toast), and when it translates (cookies on a conveyor belt) or rotates (a pancake on a spinning hot plate). It is hoped that this may encourage experimentation and enjoyment of physics in the kitchen, and perhaps even lead to more elegant if not more tasty culinary results.

physics.flu-dyn↗

Twist and turn. Elastohydrodynamics of microscale active fibres

Cellular locomotion often involves the motion of thin, elastic filaments, such as cilia and flagella, in viscous environments. The manuscript serves as a general introduction to the topic of modelling microscale elastohydrodynamics. We briefly characterise the specific features of biological filaments that affect their propulsion modes, and discuss the theoretical framework for their description, along with selected biological and artificial examples of active systems.

cond-mat.soft↗

Tuning upstream swimming of micro-robots by shape and cargo size

The navigation of micro-robots in complex flow environments is controlled by rheotaxis, the reorientation with respect to flow gradients. Here we demonstrate how payloads can be exploited to enhance the motion against flows. Using fully resolved hydrodynamic simulations, the mechanisms are described that allow micro-robots of different shapes to reorient upstream. We find that cargo pullers are the fastest at most flow strengths, but pushers feature a non-trivial optimum as a function of the counter flow strength. Moreover, the rheotactic performance can be maximised by tuning the micro-robot shape or cargo size. These results may be used to control micro-swimmer navigation, but they also apply to rheotaxis in microbial ecology and the prevention of bacterial contamination dynamics.

cond-mat.soft↗

Goldilocks fluctuations: dynamic constraints on loop formation in scale-free transport networks

Adaptive transport networks are known to contain loops when subject to hydrodynamic fluctuations. However, fluctuations are no guarantee that a loop will form, as shown by loop-free networks driven by oscillating flows. We provide a complete stability analysis of the dynamical behaviour of any loop formed by fluctuating flows. We find a threshold for loop stability that involves an interplay of geometric constraints and hydrodynamic forcing mapped to constant and fluctuating components. Loops require fluctuation in the relative size of the flux between nodes, not just a temporal variation in the flux at a given node. Hence, there is both a minimum and a maximum amount of fluctuation relative to the constant-flux component where loops are supported.

cond-mat.dis-nn↗

Eukaryotic swimming cells are shaped by hydrodynamic constraints

Eukaryotic swimming cells such as spermatozoa, algae or protozoa use flagella or cilia to move in viscous fluids. The motion of their flexible appendages in the surrounding fluid induces propulsive forces that balance with the viscous drag on the cells and lead to a directed swimming motion. Here, we use our recently built database of cell motility (BOSO-Micro) to investigate the extent to which the shapes of eukaryotic swimming cells may be optimal from a hydrodynamic standpoint. We first examine the morphology of flexible flagella undergoing waving deformation and show that their amplitude-to-wavelength ratio is near the one predicted theoretically to optimise the propulsive efficiency of active filaments. Next, we consider ciliates, for which locomotion is induced by the collective beating of short cilia covering their surface. We show that the aspect ratio of ciliates are close to the one predicted to minimise the viscous drag of the cell body. Both results strongly suggest a key role played by hydrodynamic constraints, in particular viscous drag, in shaping eukaryotic swimming cells.

cond-mat.soft↗

The slow viscous flow around doubly-periodic arrays of infinite slender cylinders

The slow viscous flow through a doubly-periodic array of cylinders does not have an analytical solution. However, as a reduced model for the flow within fibrous porous media, this solution is important for many real-world systems. We asymptotically determine the flow around a doubly-periodic array of infinite slender cylinders, by placing doubly-periodic two-dimensional singularity solutions within the cylinder and expanding the no-slip condition on the cylinder's surface in powers of the cylinder radius. The asymptotic solution provides a closed-form estimate for the flow and forces as a function of the radius and the dimensions of the cell. The force is compared to results from lattice-Boltzmann simulations of low-Reynolds-number flows in the same geometry, and the accuracy of the no-slip condition on the surface of the cylinder, predicted by the asymptotic theory, is checked. Finally, the behaviour of the flow, flux, force and effective permeability of the cell is investigated as a function of the geometric parameters. The structure of the asymptotic permeability is consistent with other models for the flow parallel to an array of rods. These models could be used to help understand the flows within porous systems composed of fibres and systems involving periodic arrays such as deterministic lateral displacement.

physics.flu-dyn↗

Pychastic: Precise Brownian Dynamics using Taylor-Itō integrators in Python

In the last decade, Python-powered physics simulations ecosystem has been growing steadily, allowing greater interoperability, and becoming an important tool in numerical exploration of physical phenomena, particularly in soft matter systems. Driven by the need for fast and precise numerical integration in colloidal dynamics, here we formulate the problem of Brownian Dynamics (BD) in a mathematically consistent formalism of the Itō calculus, and develop a Python package to assist numerical computations. We show that, thanks to the automatic differentiation packages, the classical truncated Taylor-Itō integrators can be implemented without the burden of computing the derivatives of the coefficient functions beforehand. Furthermore, we show how to circumvent the difficulties of BD simulations such as calculations of the divergence of the mobility tensor in the diffusion equation and discontinuous trajectories encountered when working with dynamics on $S^2$ and $SO(3)$. The resulting Python package, Pychastic, is capable of performing BD simulations including hydrodynamic interactions at speeds comparable to dedicated implementations in lower-level programming languages, but with a much simpler end-user interface.

cond-mat.soft↗

Culinary fluid mechanics and other currents in food science

Innovations in fluid mechanics are leading to better food since ancient history, while creativity in cooking inspires applied and fundamental science. Here, we review how recent advances in hydrodynamics are changing food science, and we highlight how the surprising phenomena that arise in the kitchen lead to discoveries and technologies across the disciplines, including rheology, soft matter, biophysics and molecular gastronomy. This review is structured like a menu, where each course highlights different aspects of culinary fluid mechanics. Our main themes include multiphase flows, complex fluids, thermal convection, hydrodynamic instabilities, viscous flows, granular matter, porous media, percolation, chaotic advection, interfacial phenomena, and turbulence. For every topic, we first provide an introduction accessible to food professionals and scientists in neighbouring fields. We then assess the state-of-the-art knowledge, the open problems, and likely directions for future research. New gastronomic ideas grow rapidly as the scientific recipes keep improving too.

physics.pop-ph↗

Rechargeable self-assembled droplet microswimmers driven by surface phase transitions

The design of artificial microswimmers is often inspired by the strategies of natural microorganisms. Many of these creatures exploit the fact that elasticity breaks the time-reversal symmetry of motion at low Reynolds numbers, but this principle has been notably absent from model systems of active, self-propelled microswimmers. Here we introduce a class of microswimmer that spontaneously self-assembles and swims without using external forces, driven instead by surface phase transitions induced by temperature variations. The swimmers are made from alkane droplets dispersed in aqueous surfactant solution, which start to self-propel upon cooling, pushed by rapidly growing thin elastic tails. When heated, the same droplets recharge by retracting their tails, swimming for up to tens of minutes in each cycle. Thermal oscillations of approximately 5 degrees Celsius induce the swimmers to harness heat from the environment and recharge multiple times. We develop a detailed elastohydrodynamic model of these processes and highlight the molecular mechanisms involved. The system offers a convenient platform for examining symmetry breaking in the motion of swimmers exploiting flagellar elasticity. The mild conditions and biocompatible media render these microswimmers potential probes for studying biological propulsion and interactions between artificial and biological swimmers.

cond-mat.soft↗

The Bank Of Swimming Organisms at the Micron Scale (BOSO-Micro)

Unicellular microscopic organisms living in aqueous environments outnumber all other creatures on Earth. A large proportion of them are able to self-propel in fluids with a vast diversity of swimming gaits and motility patterns. In this paper we present a biophysical survey of the available experimental data produced to date on the characteristics of motile behaviour in unicellular microswimmers. We assemble from the available literature empirical data on the motility of four broad categories of organisms: bacteria (and archaea), flagellated eukaryotes, spermatozoa and ciliates. Whenever possible, we gather the following biological, morphological, kinematic and dynamical parameters: species, geometry and size of the organisms, swimming speeds, actuation frequencies, actuation amplitudes, number of flagella and properties of the surrounding fluid. We then organise the data using the established fluid mechanics principles for propulsion at low Reynolds number. Specifically, we use theoretical biophysical models for the locomotion of cells within the same taxonomic groups of organisms as a means of rationalising the raw material we have assembled, while demonstrating the variability for organisms of different species within the same group. The material gathered in our work is an attempt to summarise the available experimental data in the field, providing a convenient and practical reference point for future studies.

physics.bio-ph↗