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Magdalena Marganska

Publications and source records attributed to Magdalena Marganska.

At least 19 recordsLinked to original sources

Taming quantum interference: a route to high electrical conductance in carbon nanotube assemblies

In nanostructured networks, transport is governed by junctions between neighbouring building blocks. Improving their alignment and removing defects is the intuitive route to better electron transport. At low temperatures, when transport becomes coherent, a junction cannot always be reduced to a single effective resistance, because electron-wave interference can strongly enhance or suppress transmission even in nominally ideal junctions. Using carbon nanotube (CNT) networks as a model system, we explore coherent transport through experimentally relevant junctions, from single and multiple single-walled CNT (SWCNT) contacts to double-walled CNT (DWCNT) and multi-walled CNT (MWCNT) junctions, with atomistic tight-binding non-equilibrium Green's-function calculations, also under a perpendicular magnetic field. We use analytically solvable minimal models to identify transport regimes expected for quasi-1D nanoscale junctions, and an electron-waveguide picture to interpret their CNT-specific manifestations. For single SWCNT--SWCNT junctions, high-transmission windows are set mainly by overlap length, doping and magnetic field. Gateway states can enhance conductance when some CNT subbands are gapped, and in some cases a magnetic field can restore transmission by lifting an interference blockade. In more complex architectures, added paths become selective: multi-junctions generate resonant filtering, while additional walls redistribute transmission instead of acting as independent channels. DWCNT junctions remain outer-wall dominated and SWCNT-like, whereas MWCNT junctions redistribute transmission among coupled walls and show a more complex field response. Our ultrahigh-field measurements likewise show lower, more field-sensitive conductance in MWCNT than SWCNT fibres. This work turns microscopic interference mechanisms into design principles for high-conductance, field-stable CNT conductors.

cond-mat.mes-hall

Generation of an anomalous linearly dispersing spin-polarized band in Bi-based topological insulators

We report the generation of an anomalous linearly dispersing, spin-polarized band in Bi-based topological insulator (TI) thin films, induced by soft Ar-ion bombardment followed by annealing. This extra band -- which we call the anomalous linearly dispersing state (ALS) -- is superimposed on the regular band structure including the topological surface state (TSS), spans an unusually large energetic range of up to ${\sim}\,\SI{650}{\milli\electronvolt}$ at the $Γ$-point, and appears near the Fermi energy. Spin-resolved measurements indicate spin-momentum locking with a helicity \emph{opposite} to that of the regular TSS. The Fermi velocity of the ALS, $v_\mathrm{F} = (5.1\pm 0.4)\times 10^{5}\,\frac m s$, is indistinguishable from that of the regular TSS, $(5.3\pm 0.5)\times 10^{5}\,\frac m s$. The observation is reproducible across samples of varying thickness and was confirmed at two independent synchrotron radiation facilities. We discuss different mechanisms for the physical origin of the observed ALS including sputtering-induced TSS relocation, bi-layer formation by,e.g., chalcogen removal, and high-index surface relocation.

cond-mat.mtrl-sci

Quantum Limits of Electronic Transport in Nanostructured Macroscopic Conductors

Macroscopic assemblies of one- and two-dimensional materials promise to translate nanoscale electronic properties into device-scale performance, yet the microscopic principles governing charge transport in such networks remain unresolved. In these systems, conductivity is often interpreted using phenomenological models that do not explicitly connect electronic structure to macroscopic magnetotransport. Here we develop a unified atomistic framework that links quantum-coherent transport, thermal disorder and magnetic-field effects, and combine it with ultrahigh-field magnetotransport measurements up to 60 T over a broad temperature range on carbon nanotube fibres. We show that positive magnetoresistance is controlled by junction overlap length, whereas negative magnetoresistance arises predominantly from lattice-mismatched heterojunctions rather than weak localisation alone. Statistical analysis of a large-scale numerical dataset reveals that the experimentally observed positive quadratic magnetoresistance originates from junction transport. These results show that macroscopic transport in disordered low-dimensional networks is governed primarily by junction-level quantum interference rather than solely by defects or doping.

cond-mat.mtrl-sci

Transcendental momentum quantization in semiconducting Rashba nanowires and zero energy states in their normal and superconducting phase

We study finite system properties of the canonical low energy model for a semiconducting nanowire with Rashba spin-orbit coupling. The case of an isolated wire as well as of one proximitized by an s-wave superconductor are considered. Already for the normal wire, the presence of spin-orbit coupling leads to eigenstates of the finite system composed of more than two momentum eigenstates. The quantization condition for the wavevectors is not that of a quantum box, but given instead by a transcendental equation linking the involved wavevectors. For the wire with superconducting pairing, the presence of electron and hole channels complicates the composition of the eigenstates. In this case we derive an approximate quantization condition close to the phase boundary, and a condition for the appearance of exact zero energy states. It can be satisfied both in the topological and in the trivial phase. Both the trivial and topological zero energy states contribute to the linear transport through Andreev reflection and direct transmission processes, with their relative importance depending on the degree of the states' localization at the boundary.

cond-mat.mes-hall

A universal route to chiral Ising superconductivity in monolayer TaS$_2$ and NbSe$_2$

We investigate Ising superconductivity in two archetypal intrinsic superconductors, monolayer 1H-TaS$_2$ and 1H-NbSe$_2$, in a bottom-up approach. Using ab initio-based tight-binding parameterizations for the relevant low-energy d-bands, the screened interaction is evaluated microscopically, in a scheme including Bloch overlaps. In direct space, the screened potential displays for both systems long-range Friedel oscillations alternating in sign. Upon scaling, the oscillation pattern becomes universal, with the periodic features locked to the lattice. Solving the momentum-resolved gap equations, a chiral ground state with p-like symmetry is generically found. Due to the larger Ising spin-orbit coupling, the chiral gap is more anisotropic in TaS$_2$ than in NbSe$_2$. This is reflected in tunneling spectra displaying V-shaped features for the former, in quantitative agreement with low-temperature scanning tunneling experiments on TaS$_2$. At the same time, our results reconcile the apparent discordance with hard gap tunneling spectra reported for the sibling NbSe$_2$.

cond-mat.supr-con

Adjudicating Conduction Mechanisms in High Performance Carbon Nanotube Fibers

The performance of carbon nanotube (CNT) cables, a contender for copper-wire replacement, is tied to its metallic and semi-conducting-like conductivity responses with temperature; the origin of the semi-conducting-like response however is an underappreciated incongruity in literature. With controlled aspect-ratio and doping-degree, over 61 unique cryogenic experiments including anisotropy and Hall measurements, CNT cable performance is explored at extreme temperatures (65 mK) and magnetic fields (60 T). A semi-conducting-like conductivity response with temperature becomes temperature-independent approaching absolute-zero, uniquely demonstrating the necessity of heterogeneous fluctuation induced tunneling; complete de-doping leads to localized hopping, contrasting graphite's pure metallic-like response. High-field magneto-resistance (including +22% longitudinal magneto-resistance near room-temperature) is analyzed with hopping and classical two-band models, both similarly yielding a parameter useful for conductor development. Varying field-orientation angle uncovers two-and four-fold symmetries from Aharonov-Bohm-like corrections to curvature-induced bandgap. Tight-binding calculations using Green's Function formalism model large-scale, coherent transport in commensurate CNT bundles in magnetic field, revealing non-uniform transmission across bundle cross-sections with doping restoring uniformity; independent of doping, transport in bundle-junction-bundle systems are predominantly from CNTs adjacent to the other bundle. The final impact is predicting the ultimate conductivity of heterogeneous CNT cables using temperature and field-dependent transport, surpassing conductivity of traditional metals.

cond-mat.mtrl-sci

Friedel oscillations and chiral superconductivity in monolayer NbSe$_2$

In 1965 Kohn and Luttinger proposed a genuine electronic mechanism for superconductivity. Despite the bare electrostatic interaction between two electrons being repulsive, in a metal electron-hole fluctuations can give rise to Friedel oscillations of the screened Coulomb potential. Cooper pairing among the electrons then emerges when taking advantage of the attractive regions. The nature of the leading pairing mechanism in some two-dimensional transition metal dichalcogenides is still debated. Focusing on NbSe$_2$, we show that superconductivity can be induced by the Coulomb interaction when accounting for screening effects on the trigonal lattice with multiple orbitals. Using ab initio-based tight-binding parametrizations for the relevant low-energy d-bands, we evaluate the screened interaction microscopically, in a scheme including Bloch overlaps. In the direct space, we find long-range Friedel oscillations alternating in sign, a key to the Kohn-Luttinger mechanism. The momentum-resolved gap equations predict two degenerate solutions at the critical temperature Tc, signaling the unconventional nature of the pairing. Their complex linear combination, i.e., a chiral gap with p-like symmetry, provides the ground state of the system. Our prediction of a fully gapped chiral phase well below Tc is in excellent agreement with the spectral function extracted from tunneling spectroscopy measurements of single-layer NbSe$_2$.

cond-mat.supr-con

Tracing Dirac points of topological surface states by ferromagnetic resonance

Ferromagnetic resonance is used to reveal features of the buried electronic band structure at interfaces between ferromagnetic metals and topological insulators. By monitoring the evolution of magnetic damping, the application of this method to a hybrid structure consisting of a ferromagnetic layer and a 3D topological insulator reveals a clear fingerprint of the Dirac point and exhibits additional features of the interfacial band structure not otherwise observable. The underlying spin-pumping mechanism is discussed in the framework of dissipation of angular momentum by topological surface states (TSSs). Tuning of the Fermi level within the TSS was verified both by varying the stoichiometry of the topological insulator layer and by electrostatic backgating and the damping values obtained in both cases show a remarkable agreement. The high energy resolution of this method additionally allows us to resolve the energetic shift of the local Dirac points generated by local variations of the electrostatic potential. Calculations based on the chiral tunneling process naturally occurring in TSS agree well with the experimental results.

cond-mat.mes-hall

Two bands Ising superconductivity from Coulomb interactions in monolayer NbSe$_2$

The nature of superconductivity in monolayer transition metal dichalcogenides is still an object of debate. It has already been argued that repulsive Coulomb interactions, combined with the disjoint Fermi surfaces around the $K$, $K'$ valleys and at the $Γ$ point, can lead to superconducting instabilities in monolayer NbSe$_2$. Here, we demonstrate the two bands nature of superconductivity in NbSe$_2$. It arises from the competition of repulsive long range intravalley and short range intervalley interactions together with Ising spin-orbit coupling. The two distinct superconducting gaps, one for each spin-orbit split band, consist of a mixture of s-wave and f-wave components. Their different amplitudes are due to different normal densities of states of the two bands at the Fermi level. Using a microscopic multiband BCS approach, we derive and self-consistently solve the gap equation, demonstrating the stability of nontrivial solutions in a realistic parameter range. We find a universal behavior of the temperature dependence of the gaps and of the critical in-plane field which is consistent with various sets of existing experimental data.

cond-mat.supr-con

Supercurrent and phase slips in a ballistic carbon nanotube embedded into a van der Waals heterostructure

We demonstrate long-range superconducting correlations in a several micrometer-long carbon nanotube encapsulated in a van der Waals stack between hBN and NbSe$_2$. We show that a substantial supercurrent flows through the nanotube section beneath the NbSe$_2$ crystal as well as through the 2 $μ$m-long section not in contact with it. As expected for superconductors of nanoscopic cross section, the current-induced breakdown of superconductivity is characterized by resistance steps due to the nucleation of phase slip centers. All elements of our hybrid device are active building blocks of several recently proposed setups for realization of Majorana fermions in carbon nanotubes.

cond-mat.supr-con

Linear and non-linear transport across a finite Kitaev chain: an exact analytical study

We present exact analytical results for the differential conductance of a finite Kitaev chain in an N-S-N configuration, where the topological superconductor is contacted on both sides with normal leads. Our results are obtained with the Keldysh non-equilibrium Green's functions technique, using the full spectrum of the Kitaev chain without resorting to minimal models. A closed formula for the linear conductance is given, and the analytical procedure to obtain the differential conductance for the transport mediated by higher excitations is described. The linear conductance attains the maximum value of $e^2/h$ only for the exact zero energy states. Also the differential conductance exhibits a complex pattern created by numerous crossings and anticrossings in the excitation spectrum. We reveal the crossings to be protected by the inversion symmetry, while the anticrossings result from a pairing-induced hybridization of particle-like and hole-like solutions with the same inversion character. Our comprehensive treatment of the Kitaev chain allows us also to identify the contributions of both local and non-local transmission processes to transport at arbitrary bias voltage. Local Andreev reflection processes dominate the transport within the bulk gap and diminish for higher excited states, but reemerge when the bias voltage probes the avoided crossings. The non-local direct transmission is enhanced above the bulk gap, but contributes also to the transport mediated by the topological states.

cond-mat.mes-hall

Exact eigenvectors and eigenvalues of the finite Kitaev chain and its topological properties

We present a comprehensive, analytical treatment of the finite Kitaev chain for arbitrary chemical potential. We derive the momentum quantization conditions and present exact analytical formulae for the resulting energy spectrum and eigenstate wave functions, encompassing boundary and bulk states. In accordance with an analysis based on the winding number topological invariant, and as expected from the bulk-edge correspondence, the boundary states are topological in nature. They can have zero, exponentially small or even finite energy. A numerical analysis confirms their robustness against disorder.

cond-mat.mes-hall

Unhiding a concealed resonance by multiple Kondo transitions in a quantum dot

Kondo correlations are responsible for the emergence of a zero-bias peak in the low temperature differential conductance of Coulomb blockaded quantum dots. In the presence of a global SU(2)$\otimes$SU(2) symmetry, which can be realized in carbon nanotubes, they also inhibit inelastic transitions which preserve the Kramers pseudospins associated to the symmetry. We report on magnetotransport experiments on a Kondo correlated carbon nanotube where resonant features at the bias corresponding to the pseudospin-preserving transitions are observed. We attribute this effect to a simultaneous enhancement of pseudospin-non-preserving transitions occurring at that bias. This process is boosted by asymmetric tunneling couplings of the two Kramers doublets to the leads and by asymmetries in the potential drops at the leads. Hence, the present work discloses a fundamental microscopic mechanisms ruling transport in Kondo systems far from equilibrium.

cond-mat.str-el

Transverse profile and 3D spin canting of a Majorana state in carbon nanotubes

The full spatial 3D profile of Majorana bound states (MBS) in a nanowire-like setup featuring a semiconducting carbon nanotube (CNT) as the central element is discussed. By accurate tight-binding calculations we show that the chiral nature of the CNT lattice is imprinted in the MBS wave function which has a helical structure, anisotropic in the transverse direction. The local spin canting angle displays a similar spiral pattern, varying around the CNT circumference. We reconstruct the intricate 3D profile of the MBS wave function analytically, using an effective low energy Hamiltonian accounting both for the electronic spin and valley degrees of freedom of the CNT. We find that the four components of the Majorana spinor are related by the three symmetries of our Bogoliubov-de Gennes (BdG) Hamiltonian, reducing the number of independent components to one. A Fourier transform analysis uncovers the presence of three contributions to the MBS, one from the $Γ$-point and one from each of the Fermi points, with further complexity added by the presence of two valley states in each contribution.

cond-mat.mes-hall

Majorana quasiparticles in semiconducting carbon nanotubes

Engineering effective p-wave superconductors hosting Majorana quasiparticles (MQPs) is nowadays of particular interest, also in view of the possible utilization of MQPs in fault-tolerant topological quantum computation. In quasi one-dimensional systems, the parameter space for topological superconductivity is significantly reduced by the coupling between transverse modes. Together with the requirement of achieving the topological phase under experimentally feasible conditions, this strongly restricts in practice the choice of systems which can host MQPs. Here we demonstrate that semiconducting carbon nanotubes (CNTs) in proximity with ultrathin s-wave superconductors, e.g. exfoliated NbSe$_2$, satisfy these needs. By precise numerical tight-binding calculations in the real space we show the emergence of localized zero-energy states at the CNT ends above a critical value of the applied magnetic field. Knowing the microscopic wave functions, we unequivocally demonstrate the Majorana nature of the localized states. An accurate analytical model Hamiltonian is used to calculate the topological phase diagram.

cond-mat.mes-hall

The two classes of low energy spectra in finite carbon nanotubes

Electrons in carbon nanotubes (CNTs) possess spin and orbital degrees of freedom. The latter is inherited from the bipartite graphene lattice with two inequivalent Dirac points. The electronic spectra obtained in several transport experiments on CNT quantum dots in parallel magnetic field often show an anticrossing of spectral lines assigned to the opposite Dirac valleys. So far this valley mixing has been attributed to the disorder, with impurity induced scattering. We show that this effect can arise also in ultraclean CNTs of the armchair class and it can be caused solely by the presence of the boundaries. In contrast, in CNTs of the zigzag class it does not occur. These two fundamentally different classes of spectra arise because of different symmetries of the low energy eigenstates of the two types of CNTs. The magnitude of the level splitting depends in a nonmonotonous way on the distance of the involved energy levels from the charge neutrality point.

cond-mat.mes-hall

Signatures of spin-orbit interaction in transport properties of finite carbon nanotubes in a parallel magnetic field

The transport properties of finite nanotubes placed in a magnetic field parallel to their axes are investigated. Upon including spin-orbit coupling and curvature effects, two main phenomena are analyzed which crucially depend on the tube's chirality: i) Finite carbon nanotubes in a parallel magnetic field may present a suppression of current due to the localization at the edges of otherwise conducting states. This phenomenon occurs due to the magnetic-field dependent open boundary conditions obeyed by the carbon nanotube's wave functions. The transport is fully suppressed above threshold values of the magnetic field which depend on the nanotube chirality, length and on the spin-orbit coupling. ii) Reversible spin polarized currents can be obtained upon tuning the magnetic field, exploiting the curvature-induced spin-orbit splitting.

cond-mat.mes-hall

Magnetic field induced localization in carbon nanotubes

The electronic spectra of long carbon nanotubes (CNTs) can, to a very good approximation, be obtained using the dispersion relation of graphene with both angular and axial periodic boundary conditions. In short CNTs one must account for the presence of open ends, which may give rise to states localized at the edges. We show that when a magnetic field is applied parallel to the tube axis, it modifies both momentum quantization conditions, causing hitherto extended states to localize near the ends. This localization is gradual and initially the involved states are still conducting. Beyond a threshold value of the magnetic field, which depends on the nanotube chirality and length, the localization is complete and the transport is suppressed.

cond-mat.mes-hall