arXiv subjects

Maik Gaerner

Publications and source records attributed to Maik Gaerner.

7 recordsLinked to original sources

arXiv2026

Femtosecond all-optical coherent control of spin polarization in altermagnets

Altermagnets constitute an emerging materials platform for spintronic technologies by combining compensated magnetic order with ferromagnet-like spin-split electronic bands. Here, we investigate the proposed d-wave altermagnetic material RuO2 using circularly polarized ultrashort laser pulses. Time-resolved magneto-optical Kerr effect measurements, which are intrinsically sensitive to surface and interface states, reveal the ultrafast spin response of RuO2. In contrast to the demagnetization dynamics characteristic of conventional ferromagnets, we observe a distinct coherent contribution to the complex Kerr rotation that appears during the light-matter interaction and lasts for about 200 fs. Similar signatures have been associated with spin-momentum locking and directional band splitting in spin-split surface states of topological insulators as well as spin-orbit-coupled semiconductors. They are governed by a finite Raman coherence time. We interpret this coherent response as evidence for transient spin-polarized surface states in RuO2, consistent with the emergence of altermagnetic surface states that are directly relevant to spin-polarized transport at surfaces and interfaces.

cond-mat.other↗

arXiv2026

Stable Asymmetric Magnetization Reversal in Epitaxial Co(001)/CoO(001) Bilayer

The exchange bias (EB) in ferromagnetic/antiferromagnetic (FM/AFM) bilayer systems causes a shift of the magnetic hysteresis curve after field cooling through the Néel temperature of the AFM. In some cases, this shift is accompanied by an asymmetry between ascending and descending branches. In the past, this asymmetric magnetization reversal has been studied in different bilayer systems, including polycrystalline Co/CoO thin films. Here we investigate the asymmetric magnetization reversal in an epitaxial fcc-Co(001)/CoO(001) thin film grown on MgO(001) by molecular beam epitaxy at varying temperatures up to room temperature after field cooling along the easy and the hard axes. Room temperature measurements of the longitudinal and transverse magneto-optic Kerr effect show different magnetization reversal processes via stable intermediate states for different angles between external magnetic field and magnetic easy axes. Once the sample is cooled below the blocking temperature, a pronounced asymmetric magnetization reversal can be observed. We show that in contrast to polycrystalline bilayers, the loop asymmetry stays constant after multiple training cycles and that the magnitude of the asymmetry is directly correlated with the magnitude of the EB.

cond-mat.mtrl-sci↗

arXiv2026

Cubic magneto-optic Kerr effect in Co(111) thin films

The magneto-optic Kerr effect (MOKE) is often applied as a tool for the magnetic characterization of thin films. Here, the change in polarization upon reflection from the magnetized sample is mainly regarded as being linearly proportional to the magnetization $\mathbf{M}$ (LinMOKE). MOKE contributions of second order in $\mathbf{M}$, also known as quadratic MOKE (QMOKE), which are proportional to $\mathbf{M}^2$, have also been studied in the past and used in thin film characterization. Recently, we reported on a systematic investigation of third-order MOKE contributions, named cubic MOKE (CMOKE) in Ni(111) thin films. This CMOKE manifests itself as an anisotropic contribution to the MOKE signal (with regard to the crystallographic orientation) measured in longitudinal or transversal configuration in full magnetic saturation. While LinMOKE (odd in $\mathbf{M}$) and QMOKE (even in $\mathbf{M}$) can easily be separated by methods based on magnetization parity, this no longer holds true for LinMOKE and CMOKE (odd in $\mathbf{M}$). It is therefore crucial to be aware of CMOKE contributions in order to correctly interpret MOKE data. Here, we report on the observation of CMOKE in thin film heterostructures with structurally twinned and untwinned Co(111) layers, demonstrating that a large CMOKE is not only present in Ni thin films. Additionally, we show that the observed anisotropic contributions cannot stem from LinMOKE by analyzing their dependence on the angle of incidence (AoI) of light. While the QMOKE is almost vanishing in Co(111) using light with wavelengths of 635\,nm and 406\,nm, the CMOKE contributions reach up to about 30\% of the LinMOKE contribution at an AoI of 45 degrees and become even more dominant towards normal AoI, which emphasizes the importance of higher-order MOKE effects in magneto-optic experiments.

physics.optics↗

arXiv2026

Cubic-in-magnetization contributions to the magneto-optic Kerr effect investigated for Ni(001) and Ni(111) thin films

*The abstract of this article is too long to be included in the arXiv metadata; please see the paper for the full abstract.* ...In this paper, we introduce the detailed theory of cubic-in-magnetization magneto-optic Kerr effect (CMOKE) by deriving the magneto-optic tensor of third order in magnetization, denoted as $\bm{H}$, and comparing the strength of CMOKE for different crystal orientations theoretically and experimentally. In crystals with cubic symmetry, the tensor $\bm{H}$ is described by two independent parameters $H_{123}$ and $H_{125}$. Together with the linear magneto-optic tensor $\bm{K}$ and quadratic magento-optic tensor $\bm{G}$, the permittivity tensor is described up to third order in magnetization. We analytically describe equations of the MOKE including the contribution of QMOKE and CMOKE itself for (001)- and (111)-oriented cubic crystal structures. Those are compared to experimental measurements of two samples with an (001)- and (111)-oriented fcc Ni layer, respectively. Further, we use Yeh's 4$\times$4 transfer matrix calculus to simulate and describe the experimental measurements phenomenologically from the permittivity tensor up to third order in $\bm{M}$. We find that the MOKE anisotropy that stems from the magneto-optic tensor $\bm{H}$ described as $\Delta H = H_{123}-3H_{125}$, is much more pronounced for the (111)-oriented cubic crystal structure, for which it manifests as three-fold in-plane angular dependencies of MOKE with longitudinal and also with transversal magnetization direction, respectively.

physics.optics↗

arXiv2026

Surface-Localized Magnetic Order in RuO2 Thin Films Revealed by Low-Energy Muon Probes

Ruthenium dioxide (RuO2) has recently emerged as a candidate altermagnet, yet its intrinsic magnetic ground state, particularly in thin films, remains debated. This study aims to clarify the nature and spatial extent of the magnetic order in RuO2 thin films grown under different conditions. Thin films of RuO2 with thicknesses of 30 nm and 33 nm are fabricated by pulsed laser deposition and sputtering onto TiO2(110) and Al2O3(1-102) substrates, respectively. Low-energy muon spin rotation/relaxation (LE-muSR) with depth-resolved sensitivity measurements is performed in transverse magnetic fields (TF) from 4 K to 290 K. The muSR data collected with a muon implantation energy of 1 keV reveal that magnetic signals originate from the near-surface region of the film (<10 nm), and the affected volume fraction is at most about 8.5%. The localized magnetic response is consistent across different substrates, growth techniques, and parameter sets, suggesting a common origin related to surface defects and dimensionality effects. The combined use of TF-muSR and the study of depth-dependent implantation with low-energy muons provides direct evidence for surface-confined, inhomogeneous static magnetic order in RuO2 thin films, helping reconcile discrepancies. These findings underscore the importance of considering reduced-dimensional contributions and motivate further investigation into the role of defects, strain, and stoichiometry on the magnetic properties of RuO2, especially at the surface.

cond-mat.mes-hall↗

arXiv2025

Fostering Innovation: Streamlining Magnetocaloric Materials Research by Digitalization

Refrigeration based on the magnetocaloric effect (MCE) can contribute to energysaving, environmentally friendly cooling in private households, or industrial application. The cooling is based on the reversible heat release or uptake during a phase-transformation of the materials that can be controlled by a magnetic field. This process could replace conventional compression-based refrigeration, which often relies on environmentally harmful refrigerants. Here we show, how to digitalize the process chain for the synthesis, theoretical and experimental characterization, and prototypical application of magnetocaloric alloy. Different Heusler alloys are examined experimentally as model systems for potential application in magnetic cooling. OTTR templates are used for the acquisition and semantic representation of knowledge in the development of an ontology. The ontology, when combined with unstructured data, can be exploited to train a model that can then be used to predict missing facts, which can help to gain new insights and to generate new hypotheses. Furthermore, tools are developed that automate data acquisition into ontological structures and workflows are implemented that provide an easy-to-use theoretical and experimental evaluation of the MCE from first principles and raw data.

cond-mat.mtrl-sci↗

arXiv2024

Cubic magneto-optic Kerr effect in Ni(111) thin films with and without twinning

In most studies utilizing the magneto-optic Kerr effect (MOKE), the detected change of polarized light upon reflection from a magnetized sample is supposed to be proportional to the magnetization $\boldsymbol{M}$. However, MOKE signatures quadratic in $\boldsymbol{M}$ have also been identified and utilized, e.g., to sense the structural order in Heusler compounds, to detect spin-orbit torques or to image antiferromagnetic domains. In our study, we observe a strong anisotropic MOKE contribution of third order in $\boldsymbol{M}$ in Ni(111) thin films, attributed to a cubic magneto-optic tensor $\propto $ $\boldsymbol{M}^3$. We further show that the angular dependence of cubic MOKE (CMOKE) is affected by the amount of structural domain twinning in the sample. Our detailed study on CMOKE for two selected photon energies will open up new opportunities for CMOKE applications with sensitivity to twinning properties of thin films, e.g. CMOKE spectroscopy and microscopy or time-resolved CMOKE.

physics.optics↗