arXiv subjects

Makina Yabashi

Publications and source records attributed to Makina Yabashi.

53 records · Page 3Linked to original sources

arXiv2019

Element-selective tracking ultrafast demagnetization process in Co/Pt multilayer thin films by the resonant magneto-optical Kerr effect

We examined the photo-induced dynamics of ferromagnetic Co/Pt thin films demonstrating perpendicular magnetic anisotropy with element specificity using resonant polar magneto-optical Kerr effect measurements at Pt~N${}_{6,7}$ and Co~M${}_{2,3}$ edges with an x-ray free electron laser. The obtained results showed a clear element dependence of photo-induced demagnetization time scales: $τ_\textrm{demag.}^\textrm{Co}=80\pm60~\textrm{fs}$ and $τ_\textrm{demag.}^\textrm{Pt}=640\pm140~\textrm{fs}$. This dependence is explained by the induced moment of the Pt atom by current flow from the Co layer through the interfaces. The observed magnetization dynamics of Co and Pt can be attributed to the characteristics of photo-induced Co/Pt thin film phenomena including all-optical switching.

cond-mat.mtrl-sci↗

arXiv2019

Scientific Opportunities with an X-ray Free-Electron Laser Oscillator

An X-ray free-electron laser oscillator (XFELO) is a new type of hard X-ray source that would produce fully coherent pulses with meV bandwidth and stable intensity. The XFELO complements existing sources based on self-amplified spontaneous emission (SASE) from high-gain X-ray free-electron lasers (XFEL) that produce ultra-short pulses with broad-band chaotic spectra. This report is based on discussions of scientific opportunities enabled by an XFELO during a workshop held at SLAC on June 29 - July 1, 2016

physics.ins-det↗

arXiv2018

Effect of Anisotropic Hybridization in YbAlB$_4$ Probed by Linear Dichroism in Core-Level Hard X-ray Photoemission Spectroscopy

We have probed the crystalline electric-field ground states of pure $|J = 7/2, J_z = \pm 5/2\rangle$ as well as the anisotropic $c$-$f$ hybridization in both valence fluctuating systems $α$- and $β$-YbAlB$_4$ by linear polarization dependence of angle-resolved core level photoemission spectroscopy. Interestingly, the small but distinct difference between \abyb was found in the polar angle dependence of linear dichroism, indicating the difference in the anisotropy of $c$-$f$ hybridization which may be essential to a heavy Fermi liquid state in $α$-YbAlB$_4$ and a quantum critical state in $β$-YbAlB$_4$.

cond-mat.str-el↗

arXiv2018

A micro channel-cut crystal X-ray monochromator for a self-seeded hard X-ray free-electron laser

A channel-cut Si(111) crystal with a channel width of 90 $μ$m was developed for achieving reflection self-seeding in hard X-ray free-electron lasers (XFELs). With the crystal, a monochromatic seed pulse is produced from a broadband XFEL pulse generated in the first-half undulators with an optical delay of 119 fs at 10 keV. The small optical delay allows a temporal overlap between the seed optical pulse and the electron bunch by using a small magnetic chicane for the electron beam at the middle of the undulator section. A peak reflectivity reached 67%, which is a reasonable value as compared with the theoretical one of 81%. By using this monochromator, a monochromatic seed pulse without broadband background in spectrum was obtained at SACLA with a conversion efficiency from a broadband XFEL pulse of $\sim 2 \times 10^{-2}$, which is $\sim 10$ times higher than that of transmission self-seeding using a thin diamond (400) monochromator.

physics.ins-det↗

arXiv2018

Ultrafast demagnetization of Pt magnetic moment in L1${}_0$-FePt probed by hard x-ray free electron laser

We demonstrate ultrafast magnetization dynamics in a 5d transition metal using circularly-polarized x-ray free electron laser in the hard x-ray region. A decay time of light-induced demagnetization of L1${}_0$-FePt was determined to be $τ_\textrm{Pt} = 0.6\ \textrm{ps}$ using time-resolved x-ray magnetic circular dichroism at the Pt L${}_3$ edge, whereas magneto-optical Kerr measurements indicated the decay time for total magnetization as $τ_\textrm{total} = 0.1\ \textrm{ps}$. A transient magnetic state with the photo-modulated magnetic coupling between the 3d and 5d elements is firstly demonstrated.

cond-mat.mtrl-sci↗

arXiv2018

Linear dichroism in angle-resolved core-level photoemission spectra reflecting 4f ground-state symmetry of strongly correlated cubic Pr compounds

We report experimentally observed linear dichroism in angle-resolved core-level photoemission spectra of PrIr2Zn20 and PrB6 in cubic symmetry. The different anisotropic 4f charge distributions between the compounds due to the crystalline-electric-field splitting are responsible for the difference in the linear dichroism, which has been verified by spectral simulations with the full multiplet theory for a single-site Pr3+ ion in cubic symmetry. The observed linear dichroism and polarization-dependent spectra in two different photoelectron directions for PrIr2Zn20 are reproduced by theoretical analysis for the Gamma_3 ground state, whereas those of the Pr 3d and 4d core levels indicate the Gamma_5 ground state for PrB6.

cond-mat.str-el↗

arXiv2018

Dynamics of the photoinduced insulator-to-metal transition in a nickelate film

The control of materials properties with light is a promising approach towards the realization of faster and smaller electronic devices. With phases that can be controlled via strain, pressure, chemical composition or dimensionality, nickelates are good candidates for the development of a new generation of high performance and low consumption devices. Here we analyze the photoinduced dynamics in a single crystalline NdNiO$_3$ film upon excitation across the electronic gap. Using time-resolved reflectivity and resonant x-ray diffraction, we show that the pump pulse induces an insulator-to-metal transition, accompanied by the melting of the charge order. Finally we compare our results to similar studies in manganites and show that the same model can be used to describe the dynamics in nickelates, hinting towards a unified description of these photoinduced phase transitions.

cond-mat.str-el↗

arXiv2018

Superfluorescence, free-induction decay, and four-wave mixing: propagation of free-electron laser pulses through a dense sample of helium ions

We report an experimental and numerical study of the propagation of free-electron laser pulses (wavelength 24.3 nm) through helium gas. Ionisation and excitation populates the He$^{+}$ 4$p$ state. Strong, directional emission was observed at wavelengths of 469 nm, 164 nm, 30.4 nm, and 24.5 nm. We interpret the emissions at 469 nm and 164 nm as 4$p$-3$s$-2$p$ cascade superfluorescence, that at 30.4 nm as yoked superfluorescence on the 2$p$-1$s$ transition, and that at 25.6 nm as free-induction decay of the 3$p$ state.

physics.atom-ph↗

arXiv2017

Sub-nanometre resolution of atomic motion during electronic excitation in phase-change materials

Phase-change materials based on Ge-Sb-Te alloys are widely used in industrial applications such as nonvolatile memories, but reaction pathways for crystalline-to-amorphous phase-change on picosecond timescales remain unknown. Femtosecond laser excitation and an ultrashort x-ray probe is used to show the temporal separation of electronic and thermal effects in a long-lived ($>$100 ps) transient metastable state of Ge$_{2}$Sb$_{2}$Te$_{5}$ with muted interatomic interaction induced by a weakening of resonant bonding. Due to a specific electronic state, the lattice undergoes a reversible nondestructive modification over a nanoscale region, remaining cold for 4 ps. An independent time-resolved x-ray absorption fine structure experiment confirms the existence of an intermediate state with disordered bonds. This newly unveiled effect allows the utilization of non-thermal ultra-fast pathways enabling artificial manipulation of the switching process, ultimately leading to a redefined speed limit, and improved energy efficiency and reliability of phase-change memory technologies.

cond-mat.mtrl-sci↗

arXiv2017

Single-Shot 3D Diffractive Imaging of Core-Shell Nanoparticles with Elemental Specificity

We report 3D coherent diffractive imaging of Au/Pd core-shell nanoparticles with 6 nm resolution on 5-6 femtosecond timescales. We measured single-shot diffraction patterns of core-shell nanoparticles using very intense and short x-ray free electron laser pulses. By taking advantage of the curvature of the Ewald sphere and the symmetry of the nanoparticle, we reconstructed the 3D electron density of 34 core-shell structures from single-shot diffraction patterns. We determined the size of the Au core and the thickness of the Pd shell to be 65.0 +/- 1.0 nm and 4.0 +/- 0.5 nm, respectively, and identified the 3D elemental distribution inside the nanoparticles with an accuracy better than 2%. We anticipate this method can be used for quantitative 3D imaging of symmetrical nanostructures and virus particles.

physics.ins-det↗

arXiv2015

Evidence for Gamma_8 Ground-State Symmetry of Cubic YbB12 Probed by Linear Dichroism in Core-Level Photoemission

We have successfully observed linear dichroism in angle-resolved Yb3+ 3d5/2 core-level photoemission spectra for YbB12 in cubic symmetry. Its anisotropic 4f charge distribution due to the crystal-field splitting is responsible for the linear dichroism, which has been verified by spectral simulations using ionic calculations with the full multiplet theory for a single-site Yb3+ ion in cubic symmetry. The observed linear dichroism as well as the polarization-dependent spectra in two different photoelectron directions for YbB12 are quantitatively reproduced by theoretical analysis for the Gamma_8 ground state, indicating the Gamma_8 ground-state symmetry for the Yb3+ ions mixed with the Yb2+ state.

cond-mat.str-el↗

arXiv2014

Simultaneous measurements of super-radiance at multiple wavelengths from helium excited states: (I) Experiment

In this paper, we report the results of measurements of the intensities and delays of super-radiance decays from excited helium atoms at multiple wavelengths. The experiment was performed using extreme ultraviolet radiation produced by the free electron laser at the SPring-8 Compact SASE Source test accelerator facility as an excitation source. We observed super-radiant transitions on the $1s3p \to 1s2s$ ($λ=$502 nm), $1s3d \to 1s2p$ ($λ=$668 nm), and $1s3s \to 1s2p$ ($λ=$728 nm) transitions. The pulse energy of each transition and its delay time were measured as a function of the target helium gas density. Several interesting features of the data, some of which appear to contradict with the predictions of the simple two-level super-radiance theory, are pointed out.

physics.atom-ph↗

arXiv2014

Probing Strongly Correlated 4f-Orbital Symmetry of the Ground State in Yb Compounds by Linear Dichroism in Core-Level Photoemission

We show that the strongly correlated 4f-orbital symmetry of the ground state is revealed by linear dichroism in core-level photoemission spectra as we have discovered for YbRh2Si2 and YbCu2Si2. Theoretical analysis tells us that the linear dichroism reflects the anisotropic charge distributions resulting from crystalline electric field. We have successfully determined the ground-state 4f symmetry for both compounds from the polarization-dependent angle-resolved core-level spectra at a low temperature well below the first excitation energy. The excited-state symmetry is also probed by temperature dependence of the linear dichroism where the high measuring temperatures are of the order of the crystal-field-splitting energies.

cond-mat.str-el↗

arXiv2013

Single-shot 3D structure determination of nanocrystals with femtosecond X-ray free electron laser pulses

Coherent diffraction imaging (CDI) using synchrotron radiation, X-ray free electron lasers (X-FELs), high harmonic generation, soft X-ray lasers, and optical lasers has found broad applications across several disciplines. An active research direction in CDI is to determine the structure of single particles with intense, femtosecond X-FEL pulses based on diffraction-before-destruction scheme. However, single-shot 3D structure determination has not been experimentally realized yet. Here we report the first experimental demonstration of single-shot 3D structure determination of individual nanocrystals using ~10 femtosecond X-FEL pulses. Coherent diffraction patterns are collected from high-index-faceted nanocrystals, each struck by a single X-FEL pulse. Taking advantage of the symmetry of the nanocrystal, we reconstruct the 3D structure of each nanocrystal from a single-shot diffraction pattern at ~5.5 nm resolution. As symmetry exists in many nanocrystals and virus particles, this method can be applied to 3D structure studies of such particles at nanometer resolution on femtosecond time scales.

physics.optics↗

arXiv2010

Polaronic behavior of photoelectron spectra of Fe3O4 revealed by both hard X-ray and extremely low energy photons

Hard X-ray and extremely low energy bulk-sensitive photoelectron spectroscopy has been performed in the temperature range of 100-330 K for Fe3O4. In the high temperature phase just above the Verwey transition, the intensity at the Fermi level (EF) is still negligible, but it increases gradually with further increasing the temperature (250 K, 330 K) in consistence with the temperature dependence of the conductivity. The spectral behaviors near EF with temperature are well explained by the model, which takes the polaron effect into account.

cond-mat.str-el↗

arXiv2007

Recoil effects of photoelectrons in a solid

High energy resolution C 1$s$ photoelectron spectra of graphite were measured at the excitation energy of 340, 870, 5950 and 7940eV using synchrotron radiation. On increasing the excitation energy, i.e., increasing kinetic energy of the photoelectron, the bulk origin C 1$s$ peak position shifts to higher binding energies. This systematic shift is due to the kinetic energy loss of the high-energy photoelectron by kicking the atom, and is clear evidence of the recoil effect in photoelectron emission. It is also observed that the asymmetric broadening increases for the higher energy photoelectrons. All these recoil effects can be quantified in the same manner as the Mössbauer effect for $γ$-ray emission from nuclei embedded in crystals.

cond-mat.other↗

arXiv2003

Resonant Inelastic X-Ray Scattering (RIXS) in SrCuO$_{2}$

The resonant inelastic x-ray scattering (RIXS) was measured in an insulating SrCuO$_{2}$ with changing the incident photon energy ($hν$) near the Cu $1s$ absorption edge (K-edge). Complex structures and their dependences on the momentum transfer($Δk$) and $hν$ were observed. The $hν$ dependence of the RIXS spectra measured for a constant $Δk$=2.4$π$ has shown a remarkable enhancement near the absorption maximum and a shift of the spectral weight toward larger loss-energy with increasing $hν$. Also, the energy of the inelastic loss peak in the RIXS spectra for the fixed excitation at 8.993 keV, 10 eV below the absorption maximum, has shown a clear dependence on $Δk$. These results are in a qualitative agreement with a theoretical prediction. Full utilization of the potential of the high brilliance X ray light source at BL19LXU of SPring-8 with 27 m long insertion device will open up a breakthrough in RIXS for heavy transition metal compounds in accordance with the improvement in focussing and analyzing elements.

cond-mat.str-el↗