arXiv subjects

Manfred Sigrist

Publications and source records attributed to Manfred Sigrist.

At least 37 records · Page 2Linked to original sources

arXiv2021

Spin response and topology of a staggered Rashba superconductor

Inversion symmetry is a key symmetry in unconventional superconductors and even its local breaking can have profound implications. For inversion-symmetric systems, there is a competition on a microscopic level between the spin-orbit coupling associated with the local lack of inversion and hybridizing terms that `restore' inversion. Investigating a layered system with alternating mirror-symmetry breaking, we study this competition considering the spin response of different superconducting order parameters for the case of strong spin-orbit coupling. We find that signatures of the local non-centrosymmetry, such as an increased spin susceptibility in spin-singlet superconductors for $T\rightarrow 0$, persist even into the quasi-three-dimensional regime. This leads to a direction dependent spin response which allows to distinguish different superconducting order parameters. Furthermore, we identify several regimes with possible topological superconducting phases within a symmetry-indicator analysis. Our results may have direct relevance for the recently reported Ce-based superconductor CeRh$_2$As$_2$ and beyond.

cond-mat.supr-con↗

arXiv2021

Unsplit superconducting and time reversal symmetry breaking transitions in Sr$_2$RuO$_4$ under hydrostatic pressure and disorder

There is considerable evidence that the superconducting state of Sr$_2$RuO$_4$ breaks time reversal symmetry. In the experiments showing time reversal symmetry breaking its onset temperature, $T_\text{TRSB}$, is generally found to match the critical temperature, $T_\text{c}$, within resolution. In combination with evidence for even parity, this result has led to consideration of a $d_{xz} \pm id_{yz}$ order parameter. The degeneracy of the two components of this order parameter is protected by symmetry, yielding $T_\text{TRSB} = T_\text{c}$, but it has a hard-to-explain horizontal line node at $k_z=0$. Therefore, $s \pm id$ and $d \pm ig$ order parameters are also under consideration. These avoid the horizontal line node, but require tuning to obtain $T_\text{TRSB} \approx T_\text{c}$. To obtain evidence distinguishing these two possible scenarios (of symmetry-protected versus accidental degeneracy), we employ zero-field muon spin rotation/relaxation to study pure Sr$_2$RuO$_4$ under hydrostatic pressure, and Sr$_{1.98}$La$_{0.02}$RuO$_4$ at zero pressure. Both hydrostatic pressure and La substitution alter $T_\text{c}$ without lifting the tetragonal lattice symmetry, so if the degeneracy is symmetry-protected $T_\text{TRSB}$ should track changes in $T_\text{c}$, while if it is accidental, these transition temperatures should generally separate. We observe $T_\text{TRSB}$ to track $T_\text{c}$, supporting the hypothesis of $d_{xz} \pm id_{yz}$ order.

cond-mat.supr-con↗

arXiv2021

Unusual $H$-$T$ phase diagram of CeRh$_2$As$_2$ -- the role of staggered non-centrosymmetricity

Superconductivity in a crystalline lattice without inversion is subject to complex spin-orbit-coupling effects, which can lead to mixed-parity pairing and an unusual magnetic response. In this study, the properties of a layered superconductor with alternating Rashba spin-orbit coupling in the stacking of layers, hence (globally) possessing a center of inversion, is analyzed in an applied magnetic field, using a generalized Ginzburg-Landau model. The superconducting order parameter consists of an even- and an odd-parity pairing component which exchange their roles as dominant pairing channel upon increasing the magnetic field. This leads to an unusual kink feature in the upper critical field and a first-order phase transition within the mixed phase. We investigate various signatures of this internal phase transition. The physics we discuss here could explain the recently found $H$--$T$ phase diagram of the heavy Fermion superconductor CeRh$_2$As$_2$.

cond-mat.supr-con↗

arXiv2020

Magnetoresistance oscillation study of the half-quantum vortex in doubly connected mesoscopic superconducting cylinders of Sr2RuO4

The observation of the highly unusual half-quantum vortex (HQV) in a single crystalline superconductor excludes unequivocally the spin-singlet symmetry of the superconducting order parameter. HQVs were observed previously in mesoscopic samples of Sr2RuO4 in cantilever torque magnetometry measurements, thus providing direct evidence for spin-triplet pairing in the material. In addition, it raised important questions on HQV, including its stability and dynamics. These issues have remained largely unexplored, in particular, experimentally. We report in this paper the detection of HQVs in mesoscopic, doubly connected cylinders of single-crystalline Sr2RuO4 of a mesoscopic size and the examination of the effect of the in-plane magnetic field needed for the observation of the HQV by magnetoresistance (MR) oscillations measurements. Several distinct features found in our data, especially a dip and secondary peaks in the MR oscillations seen only in the presence of a sufficiently large in-plane magnetic field as well as a large measurement current, are linked to the formation of the HQV fluxoid state in and crossing of an Abrikosov HQV through the sample. The conclusion is drawn from the analysis of our data using a model of thermally activated vortex crossing overcoming a free-energy barrier which is modulated by the applied magnetic flux enclosed in the cylinder as well as the measurement current. Evidence for the trapping of an HQV fluxoid state in the sample was also found. Our observation of the HQV in mesoscopic Sr2RuO4 provided not only additional evidence for spin-triplet superconductivity in Sr2RuO4 but also insights into the physics of HQV, including its spontaneous spin polarization, stability, and dynamics. Our study also revealed a possible effect of the measurement current on the magnitude of the spontaneous spin polarization associated with the HQV.

cond-mat.supr-con↗

arXiv2020

Impurity induced double transitions for accidentally degenerate unconventional pairing states

Non-magnetic impurities can lift the accidental degeneracy of unconventional pairing states, such as the $(d + i g)$-wave state recently proposed for Sr$_2$RuO$_4$. This type of effect would lead to a superconducting double transition upon impurity doping. In a model calculation it is shown how this behavior depends on material parameters and how it could be detected.

cond-mat.supr-con↗

arXiv2020

Braiding Majorana corner modes in a second-order topological superconductor

We propose the concept of a device based on a square-shaped sample of a two-dimensional second-order topological helical superconductor which hosts two zero-dimensional Majorana quasiparticles at the corners. The two zero-energy modes rely on particle-hole symmetry (PHS) and their spacial position can be shifted by rotating an in-plane magnetic field and tuning proximity-induced spin-singlet pairing. We consider an adiabatic cycle performed on the degenerate ground-state manifold and show that it realizes the braiding of the two modes whereby they accumulate a non-trivial statistical phase $π$ within one cycle. Alongside with the PHS-ensured operator algebra, the fractional statistics confirms the Majorana nature of the zero-energy excitations. A schematic design for a possible experimental implementation of such a device is presented, which could be a step towards realizing non-Abelian braiding.

cond-mat.mes-hall↗

arXiv2020

Half-quantum vortices on c-axis domain walls in chiral p-wave superconductors

Chiral superconductors are two-fold degenerate and domains of opposite chirality can form, separated by domain walls. There are indications of such domain formation in the quasi two-dimensional putative chiral $p$-wave superconductor Sr$_2$RuO$_4$, yet no experiment has explicitly resolved individual domains in this material. In this work, $c$-axis domain walls lying parallel to the layers in chiral $p$-wave superconductors are explored from a theoretical point of view. First, using both a phenomenological Ginzburg-Landau and a quasiclassical Bogoliubov-deGennes approach, a consistent qualitative description of the domain wall structure is obtained. While these domains are decoupled in the isotropic limit, there is a finite coupling in anisotropic systems and the domain wall can be treated as an effective Josephson junction. In the second part, the formation and structure of half-quantum vortices (HQV) on such $c$-axis domain walls are discussed.

cond-mat.supr-con↗

arXiv2020

Phenomenology of the chiral $d$-wave state in the hexagonal pnictide superconductor SrPtAs

The pairing symmetry of the hexagonal pnictide superconductor SrPtAs is discussed with taking into account its multiband structure. The topological chiral $d$-wave state with time-reversal-symmetry breaking has been anticipated from the spontaneous magnetization observed by the muon-spin-relaxation experiment. We point out in this paper that the recent experimental reports on the nuclear-spin-lattice relaxation rate $T_1^{-1}$ and superfluid density $n_s(T)$, which seemingly support the conventional $s$-wave pairing, are also consistent with the chiral $d$-wave state. The compatibility of the gap and multiband structures is crucial in this argument. We propose that the measurement of the bulk quasiparticle density of states would be useful for the distinction between two pairing states.

cond-mat.supr-con↗

arXiv2019

Microscopic evidence for a chiral superconducting order parameter in the heavy fermion superconductor UTe2

Spin-triplet superconductivity is a condensate of electron pairs with spin-1 and an odd-parity wavefunction. A particularly interesting manifestation of triplet pairing is a chiral p-wave state which is topologically non-trivial and a natural platform for realizing Majorana edge modes. Triplet pairing is however rare in solid state systems and so far, no unambiguous identification has been made in any bulk compound. Since pairing is most naturally mediated by ferromagnetic spin fluctuations, uranium based heavy fermion systems containing f electron elements that can harbor both strong correlations and magnetism are considered ideal candidate spin-triplet superconductors. In this work we present scanning tunneling microscopy (STM) studies of the newly discovered heavy fermion superconductor, UTe2 with a T$_{SC}$ of 1.6 K. We find signatures of coexisting Kondo effect and superconductivity which show competing spatial modulations within one unit-cell. STM spectroscopy at step edges show signatures of chiral in-gap states, predicted to exist at the boundaries of a topological superconductor. Combined with existing data indicating triplet pairing, the presence of chiral edge states suggests that UTe2 is a strong candidate material for chiral-triplet topological superconductivity.

cond-mat.mtrl-sci↗

arXiv2019

Superconducting order parameter of Sr$_2$RuO$_4$: a microscopic perspective

The character of the superconducting phase of Sr$_2$RuO$_4$, is topic of a longstanding discussion. The classification of the symmetry allowed order parameters has relied on the tetragonal symmetry of the lattice and on cylindrical Fermi surfaces, usually taken to be featureless, not including the non-trivial symmetry aspects related to their orbital content. Here we show how the careful account of the orbital degree of freedom in Sr$_2$RuO$_4$, leads to a much richer classification of order parameters. We analyse the stability and degeneracy of these new order parameters from the perspective of the concept of superconducting fitness and propose a new best order parameter candidate.

cond-mat.supr-con↗

arXiv2019

Superconducting gap anisotropy and topological singularities due to lattice translational symmetry and their thermodynamic signatures

Symmetry arguments based on the point group of a system and thermodynamic measurements are often combined to identify the order parameter in unconventional superconductors. However, lattice translations, which can induce additional momenta with vanishing order parameter in the Brillouin zone, are neglected, especially in gap functions otherwise expected to be constant, such as in chiral superconductors. After a general analysis of the symmetry conditions for vanishing gap functions, we study the case of chiral $p$- and chiral $f$-wave pairing on a square lattice, a situation relevant for Sr$_2$RuO$_4$. Specifically, we calculate the impurity-induced density of states, specific heat, superfluid density and thermal conductivity employing a self-consistent T-matrix calculation and compare our results to the case of a nodal ($d$-wave) order parameter. While there is a clear distinction between a fully gapped chiral state and a nodal state, the strongly anisotropic case is almost indistinguishable from the nodal case. Our findings illustrate the difficulty of interpreting thermodynamic measurements. In particular, we find that the available measurements are consistent with a chiral ($f$-wave) order parameter. Our results help to reconcile the thermodynamic measurements with the overall picture of chiral spin-triplet superconductivity in Sr$_2$RuO$_4$.

cond-mat.supr-con↗

arXiv2019

Deviation from the Fermi-Liquid Transport Behavior in the Vicinity of a Van Hove Singularity

Recent experiments revealed non-Fermi-liquid resistivity in the unconventional superconductor Sr$_{2}$RuO$_{4}$ when strain pushes one of the Fermi surfaces close to a van Hove singularity. The origin of this behavior and whether it can be understood from a picture of well defined quasiparticles is unclear. We employ a Boltzmann transport analysis beyond the single relaxation-time approximation based on a single band which undergoes a Lifshitz transition, where the Fermi surface crosses a van Hove singularity, either due to uni-axial or epitaxial strain. First analytically investigating impurity scattering, we clarify the role of the diverging density of states together with the locally flat band at the point of the Lifshitz transition. Additionally including electron-electron scattering numerically, we find good qualitative agreement with resistivity measurements on uni-axially strained Sr$_{2}$RuO$_{4}$, including the temperature scaling and the temperature dependence of the resistivity peak. Our results imply that even close to the Lifshitz transition, a description starting from well-defined quasiparticles holds. To test the validity of Boltzmann transport theory near a van Hove singularity, we provide further experimentally accessible parameters, such as thermal transport, the Seebeck coefficient, and Hall resistivity and compare different strain scenarios.

cond-mat.str-el↗

arXiv2018

Spin and Valley States in Gate-defined Bilayer Graphene Quantum Dots

In bilayer graphene, electrostatic confinement can be realized by a suitable design of top and back gate electrodes. We measure electronic transport through a bilayer graphene quantum dot, which is laterally confined by gapped regions and connected to the leads via p-n junctions. Single electron and hole occupancy is realized and charge carriers $n = 1, 2,\dots 50$ can be filled successively into the quantum system with charging energies exceeding $10 \ \mathrm{meV}$. For the lowest quantum states, we can clearly observe valley and Zeeman splittings with a spin g-factor of $g_{s}\approx 2$. In the low field-limit, the valley splitting depends linearly on the perpendicular magnetic field and is in qualitative agreement with calculations.

cond-mat.mes-hall↗

arXiv2018

Identifying the dominant pairing interaction in high-$T_c$ FeSe superconductors through Leggett modes

Heavily electron-doped and single-layer FeSe superconduct at much higher temperatures than bulk FeSe. There have been a number of proposals attempting to explain the origin of the enhanced transition temperature, including the proximity to magnetic, nematic and antiferro-orbital critical points, as well as possible strong interfacial phonon coupling in the case of single-layer FeSe. In this paper, we examine the effect of the various mechanisms in an effective two-band model. Within our model, the fluctuations associated with these instabilities contribute to different parts of the effective multiband interactions. We propose to use the collective phase fluctuation between the bands--the Leggett mode--as a tool to identify the dominant effective pairing interaction in these systems. The Leggett mode can be resolved by means of optical probes such as electronic Raman scattering. We point out that the Leggett mode in these systems, if present, shall manifest in the Raman $B_{1g}$ channel.

cond-mat.supr-con↗

arXiv2018

Spontaneous thermal Hall effect in three-dimensional chiral superconductors with gap nodes

Generic chiral superconductors with three-dimensional electronic structure have nodal gaps and are not strictly topological. Nevertheless, they exhibit a spontaneous thermal Hall effect (THE), i.e. a transverse temperature gradient in response to a heat current even in the absence of an external magnetic field. While in some cases this THE can be quantized analogous to the Quantum Hall effect, this is not the case for nodal superconductors in general. In this study we determine the spontaneous THE for tight binding models with tetragonal and hexagonal crystal symmetry with chiral $p$- and d-wave superconducting phase. At the zero-temperature limit, the thermal Hall conductivity $ κ_{xy} $ provides information on the structure of the gap function on the Fermi surface and the Andreev bound states on the surface. The temperature dependence at very low temperatures is determined by the types of gap nodes, point or line nodes, leading to characteristic power law behaviors in the temperature, as known for other quantities such as specific heat or London penetration depth. The generic behavior is discussed on simple models analytically, while the analysis of the tight-binding models is given numerically.

cond-mat.supr-con↗

arXiv2018

Spontaneous surface flux pattern in chiral p-wave superconductors - revisited

In chiral $p$-wave superconductors, magnetic flux patterns may appear spontaneously when translational symmetry is broken such as at surfaces, domain walls, or impurities. However, in the candidate material Sr$_2$RuO$_4$ no direct signs of such magnetic fields have been detected experimentally. In this paper, the flux pattern at the edge of a disk-shaped sample is examined using the phenomenological Ginzburg Landau approach. The detailed shape of the flux pattern, including self-screening, is computed numerically for different surface types by systematically scanning a range of boundary conditions. Moreover, specific features of the electronic structure are included qualitatively through the coefficients in the Ginzburg Landau functional. Both the shape and the magnitude of the flux pattern are found to be highly sensitive to all considered parameters. In conclusion, such spontaneous magnetic flux patterns are not a universal feature of chiral $p$-wave superconductors.

cond-mat.supr-con↗

arXiv2018

Superconductivity without inversion and time-reversal symmetries

The traditional symmetries that protect superconductivity are time-reversal and inversion. Here, we examine the minimal symmetries protecting superconductivity in two dimensions and find that time-reversal symmetry and inversion symmetry are not required, and having a combination of either symmetry with a mirror operation on the basal plane is sufficient. We classify superconducting states stabilized by these two symmetries, when time-reversal and inversion symmetries are not present, and provide realistic minimal models as examples. Interestingly, several experimentally realized systems, such as transition metal dichalcogenides and the two-dimensional Rashba system belong to this category, when subject to an applied magnetic field.

cond-mat.supr-con↗

arXiv2018

Orbitally limited pair-density wave phase of multilayer superconductors

We investigate the magnetic field dependence of an ideal superconducting vortex lattice in the parity-mixed pair-density wave phase of multilayer superconductors within a circular cell Ginzburg-Landau approach. In multilayer systems, due to local inversion symmetry breaking, a Rashba spin-orbit coupling is induced at the outer layers. This combined with a perpendicular paramagnetic (Pauli) limiting magnetic field stabilizes a staggered layer dependent pair-density wave phase in the superconducting singlet channel. The high-field pair-density wave phase is separated from the low-field BCS phase by a first-order phase transition. The motivating guiding question in this paper is: what is the minimal necessary Maki parameter $α_M$ for the appearance of the pair-density wave phase of a superconducting trilayer system? To address this problem we generalize the circular cell method for the regular flux-line lattice of a type-II superconductor to include paramagnetic depairing effects. Then, we apply the model to the trilayer system, where each of the layers are characterized by Ginzburg-Landau parameter $κ_0$, and a Maki parameter $α_M$. We find that when the spin-orbit Rashba interaction compares to the superconducting condensation energy, the orbitally limited pair-density wave phase stabilizes for Maki parameters $α_M> 10$.

cond-mat.supr-con↗