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Mansoo Choi

Publications and source records attributed to Mansoo Choi.

20 records · Page 2Linked to original sources

Tunable Large Resonant Absorption in a Mid-IR Graphene Salisbury Screen

Enhancing the interaction strength between graphene and light is an important objective for those seeking to make graphene a relevant material for future optoelectronic applications. Plasmonic modes in graphene offer an additional pathway of directing optical energy into the graphene sheet, while at the same time displaying dramatically small optical confinement factors that make them an interesting means of coupling light to atomic or molecular emitters. Here we show that graphene plasmonic nanoresonators can be placed a quarter wavelength from a reflecting surface and electronically tuned to mimic a surface with an impedance closely matched to freespace (Z0 = 377Ω). This geometry - known in early radar applications as a Salisbury screen - allows for an order of magnitude (from 2.3 to 24.5%) increase of the optical absorption in the graphene and provides an efficient means of coupling to the highly confined graphene plasmonic modes.

cond-mat.mes-hall↗

CO2 laser-driven reactions in pure acetylene flow

We show that multiple-photon absorption of radiation from a 10.56 μm cw CO2 laser by intermediates (ethylene, vinylidene) generated in pure acetylene flow makes them decompose to carbon dimers and excited hydrogen. The latter associates with downstream acetylene to feedback those laser absorbing intermediates thus making the reactions self-sustained in the absence of oxygen. This process is different from acetylene self-decomposition that may occur at higher temperature and pressure. The results of our work may be useful for understanding the generation of various carbon allotropes and interstellar dust from acetylene.

physics.chem-ph↗