SearcharxivSearch

arXiv subjects

Mara Galli

Publications and source records attributed to Mara Galli.

3 recordsLinked to original sources

Iterative approach for high-quality binary intensity hologram generation in augmented reality applications

Binary amplitude spatial light modulators, such as digital micromirror devices (DMDs), are increasingly relevant for computer generated holography due to their high refresh rates, low cost, and due to the emergence of subwavelength pixel architectures. However, the binary constraint limits the reconstruction quality, as conventional approaches rely on a binarization applied as a final step after hologram computation which leads to reduced efficiency and contrast. We introduce an iterative estimation approach for the generation of off axis binary amplitude holograms, in which the binarization constraint is applied at each iteration. We validate the approach through numerical simulations and experimental reconstruction using a DMD based optical setup. Quantitative and qualitative comparisons with random superposition and Gerchberg Saxton methods demonstrate significant improvements in image contrast, light efficiency, and reconstruction fidelity, with comparable computational cost. The proposed method provides a practical route toward high quality CGH using binary modulators and supports emerging applications requiring high speed and high resolution holographic projection.

physics.optics

Attosecond correlated electron dynamics at C$_{60}$ giant plasmon resonance

Fullerenes have unique physical and chemical properties that are associated with their delocalized conjugated electronic structure. Among them, there is a giant ultra-broadband - and therefore ultrafast - plasmon resonance, which for C$_{60}$ is in the extreme-ultraviolet energy range. While this peculiar resonance has attracted considerable interest for the potential downscaling of nanoplasmonic applications such as sensing, drug delivery and photocatalysis at the atomic level, its electronic character has remained elusive. The ultrafast decay time of this collective excitation demands attosecond techniques for real-time access to the photoinduced dynamics. Here, we uncover the role of electron correlations in the giant plasmon resonance of C$_{60}$ by employing attosecond photoemission chronoscopy. We find a characteristic photoemission delay of up to 200 attoseconds pertaining to the plasmon that is purely induced by coherent large-scale correlations. This result provides novel insight into the quantum nature of plasmonic resonances, and sets a benchmark for advancing nanoplasmonic applications.

physics.atom-ph

Correlation-driven sub-3 fs charge migration in ionised adenine

Sudden ionisation of a relatively large molecule can initiate a correlation-driven process dubbed charge migration, where the electron density distribution is expected to rapidly change. Capturing this few-femtosecond/attosecond charge redistribution represents the real-time observation of the electron correlation in the molecule. So far, there has been no experimental evidence of this process. Here we report on a time-resolved study of the correlation-driven charge migration process occurring in the bio-relevant molecule adenine after ionisation by a 15-35 eV attosecond pulse . We find that, the production of intact doubly charged adenine - via a shortly-delayed laser-induced second ionisation event - represents the signature of a charge inflation mechanism resulting from the many-body excitation. This conclusion is supported by first-principles time-dependent simulations. Our findings opens new important perspectives for the control of the molecular reactivity at the electronic timescale.

physics.chem-ph