arXiv subjects

Marc Guetg

Publications and source records attributed to Marc Guetg.

6 recordsLinked to original sources

arXiv2026

Generation of high-fluence and high-intensity hard x-ray attosecond pulses at European XFEL

By combining hard x-ray attosecond pulses from the European XFEL with total-reflection focusing x-ray optics, we generated nanofocused hard x-ray attosecond pulses with intensities and fluences comparable to the highest values attained in the hard x-ray regime. A peak intensity on the order of 10$^{20}$ W/cm$^2$ is confirmed through the observation of saturation in amplified spontaneous emission from copper atoms. These x-ray pulses enable new scientific opportunities, including the exploration of higher-order nonlinear light--matter interactions, damage-free structure determination, and coherent control of atoms and molecules.

physics.optics↗

arXiv2026

High-power attosecond X-ray free-electron lasers: physics and design strategy

Attosecond pulses from X-ray free-electron laser (XFEL) have opened new opportunities for probing ultrafast electronic dynamics on the Angstrom--attosecond spatiotemporal scale. Most attosecond XFEL concepts rely on generating an ultrashort high-current spike through either external laser modulation or accelerator-based beam manipulation. Despite their different implementations, these approaches share the same essential physics, namely that the XFEL amplification is confined to a short effective lasing window within the electron beam. However, existing studies are often scheme-specific and do not yet provide a unified quantitative picture of how fundamental electron-beam properties constrain high-power attosecond performance. In this work, we investigate the general physics and scheme-independent requirements for generating high-power attosecond X-ray pulses from a short current spike. From the perspective of post-saturation superradiant evolution, we show that the effective lasing length of the electron beam governs both the attainable peak power and the pulse duration. We further examine the distinct roles of slice energy spread, slice emittance, energy chirp, undulator tapering, and transverse beam tilt. Our results reveal the trade-off between peak power, pulse shortening, and single-spike probability, and provide facility-independent guidelines for optimizing electron-beam phase-space manipulation toward terawatt-class attosecond XFEL operation.

physics.acc-ph↗

arXiv2025

Single-shot sorting of M\"ossbauer time-domain data at X-ray free-electron lasers

M\"ossbauer spectroscopy is widely used to study structure and dynamics of matter with remarkably high energy resolution, provided by the narrow nuclear resonance line widths. However, the narrow width implies low count rates, such that experiments commonly average over extended measurement times or many x-ray pulses (``shots''). This averaging impedes the study of non-equilibrium phenomena. It has been suggested that X-ray free-electron lasers (XFELs) could enable M\"ossbauer single-shot measurements without averaging, and a proof-of-principle demonstration has been reported. However, so far, only a tiny fraction of all shots resulted in signal-photon numbers which are sufficiently high for a single-shot analysis. Here, we demonstrate coherent nuclear-forward-scattering of self-seeded XFEL radiation, with up to 900 signal-photons per shot. We develop a sorting approach which allows us to include all data on a single-shot level, independent of the signal content of the individual shots. It utilizes the presence of different dynamics classes, i.e. different nuclear evolutions after each excitation. Each shot is assigned to one of the classes, which can then be analyzed separately. Our approach determines the classes from the data without requiring theory modeling nor prior knowledge on the dynamics, making it also applicable to unknown phenomena. We envision that our approach opens up new grounds for M\"ossbauer science, enabling the study of out-of-equilibrium transient dynamics of the nuclei or their environment.

quant-ph↗

arXiv2024

Attosecond soft X-ray pulses generated by chirp-dispersed manipulation in an XFEL reveal nonlinear core-electron dynamics in neon

Free-electron lasers have demonstrated their capability of generating intense attosecond X-ray pulses, which are the key to studying electron dynamics at their natural time scale and in specifically targeted electronic states, but come at the expanse of complicated generation schemes and stochastic pulse shapes. Here, we demonstrate a novel and simple operation concept based on the manipulation of the electron-bunch chirp-dispersion and working with the full 4.5 MHz repetition rate at the European XFEL in Germany. With a high-fidelity single-shot temporal characterisation, we detect X-ray pulses with durations of down to 200 attoseconds and peak powers reaching into the terawatt regime at ~1 keV photon energy. As a direct application, we present simultaneous measurements of nonlinear X-ray-matter interaction via time-resolved electron spectroscopy. Using the derived temporal pulse information and restricting the durations to a regime where individual X-ray pulses are shorter than the single-core-hole life time in neon atoms, we reveal an otherwise hidden peak-intensity dependence in the nonlinear dynamics of double-core-hole formation. Our results open the field of attosecond science to the investigation of electronic processes not only in the ground state but also in systems driven far off their equilibrium. They shed light on highly transient intermediate steps in complex electronic dynamics and thus promise to help build the conceptual bridge between fundamental physical processes and chemical photo-reactions.

physics.optics↗

arXiv2018

Wake Measurements of a Dechirper Jaw with Non-Zero Tilt Angle

The RadiaBeam/SLAC dechirper at the Linac Coherent Light Source (LCLS) is being used as a fast kicker, by inducing transverse wakefields, to e.g. facilitate Fresh-slice, two-color laser operation. The dechirper jaws are independently adjustable at both ends, and it is difficult to avoid leaving residual (longitudinal) tilt in them during set-up. In this report we develop a model independent method of removing unknown tilt in a jaw. In addition, for a short uniform bunch passing by a single dechirper plate, we derive an explicit analytical formula for the transverse wake kick as function of average plate offset and tilt angle. We perform wake kick measurements for the different dechirper jaws of the RadiaBeam/SLAC dechirper, and find that the agreement between measurement and theory is excellent.

physics.acc-ph↗

arXiv2017

Measurements of wake-induced electron beam deflection in a dechirper at the Linac Coherent Light Source

The RadiaBeam/SLAC dechirper, a structure consisting of pairs of flat, metallic, corrugated plates, %a corrugated structure in flat geometry, has been installed just upstream of the undulators in the Linac Coherent Light Source (LCLS). As a dechirper, with the beam passing between the plates on axis, longitudinal wakefields are induced that can remove unwanted energy chirp in the beam. However, with the beam passing off axis, strong transverse wakes are also induced. This mode of operation has already been used for the production of intense, multi-color photon beams using the Fresh-Slice technique, and is being used to develop a diagnostic for attosecond bunch length measurements. Here we measure, as function of offset, the strength of the transverse wakefields that are excited between the two plates, and also for the case of the beam passing near to a single plate. We compare with analytical formulas from the literature, and find good agreement. This report presents the first systematic measurements of the transverse wake strength in a dechirper, one that has been excited by a bunch with the short pulse duration and high energy found in an X-ray free electron laser.

physics.acc-ph↗