arXiv subjects

Marc Jankowski

Publications and source records attributed to Marc Jankowski.

At least 19 recordsLinked to original sources

arXiv2025

Programmable on-chip nonlinear photonics

Nonlinear photonics uses coherent interactions between optical waves to engineer functionality that is not possible with purely linear optics. Traditionally, the function of a nonlinear-optical device is determined during design and fixed during fabrication. In this paper, we present a photonic device with highly programmable nonlinear functionality: an optical slab waveguide with an arbitrarily reconfigurable two-dimensional distribution of $\chi^{(2)}$ nonlinearity. The nonlinearity is realized using electric-field-induced $\chi^{(2)}$ in a $\chi^{(3)}$ material. The programmability is engineered by massively parallel control of the electric-field distribution within the device using a photoconductive layer and optical programming with a spatial light pattern. To showcase the versatility of our device, we demonstrated spectral, spatial, and spatio-spectral engineering of second-harmonic generation by tailoring arbitrary quasi-phase-matching (QPM) grating structures in two dimensions. Second-harmonic light was generated with programmable spectra, enabled by real-time in situ inverse design of QPM gratings. Flexible spatial control was also achieved, including the generation of complex waveforms such as Airy beams and the simultaneous engineering of spectral and spatial features. This allowed us to create distinct spatial light profiles across multiple wavelengths. The programmability also allowed us to demonstrate in situ, real-time compensation of fluctuations in pump laser wavelength. Our work shows that we can transcend the conventional one-device--one-function paradigm, expanding the potential applications of nonlinear optics in situations where fast device reconfigurability is not merely practically convenient but essential -- such as in programmable optical quantum gates and quantum light sources, all-optical signal processing, optical computation, and structured light for sensing.

physics.optics↗

arXiv2024

Hybrid AM/FM Mode-Locking of Singly-Resonant OPOs

We investigate a new mode-locking regime in the singly-resonant OPO employing simultaneous amplitude- and frequency-modulation of the intracavity field. This OPO exhibits deterministic, "turn-key" formation of a stable, broadband, chirped frequency comb with high conversion efficiency. Comb-forming dynamics follow a simple phase-space dynamical model, governed by cavity dispersion and modulator chirp, which agrees closely with full numerical simulations. The comb exhibits fast, mode-hop-free tuning over the full gain window of the OPA crystal, controlled by the modulator frequency. Conditions for comb stability, and techniques to enhance comb bandwidth through intentional phase-mismatch and chirping, are investigated.

physics.optics↗

arXiv2024

Arbitrary control over multimode wave propagation for machine learning

Controlled multimode wave propagation can enable more space-efficient photonic processors than architectures based on discrete components connected by single-mode waveguides. Instead of defining discrete elements, one can sculpt the continuous substrate of a photonic processor to perform computations through multimode interference in two dimensions. Here we designed and demonstrated a device with a refractive index that can be rapidly reprogrammed across space, allowing arbitrary control of wave propagation. The device, a two-dimensional programmable waveguide, uses parallel electro-optic modulation of the refractive index of a slab waveguide with about $10^4$ programmable spatial degrees of freedom. We implemented neural network inference on benchmark tasks with up to $49$-dimensional vectors in a single pass, without digital pre-processing or post-processing. Theoretical and numerical analyses further indicated that two-dimensional programmable waveguides may offer not only a constant-factor reduction in device area but also a scaling benefit, with the area required growing as $N^{1.5}$ rather than $N^2$.

physics.optics↗

arXiv2024

Ultrafast second-order nonlinear photonics -- from classical physics to non-Gaussian quantum dynamics

Photonic integrated circuits with second-order ($\chi^{(2)}$) nonlinearities are rapidly scaling to remarkably low powers. At this time, state-of-the-art devices achieve saturated nonlinear interactions with thousands of photons when driven by continuous-wave lasers, and further reductions in these energy requirements enabled by the use of ultrafast pulses may soon push nonlinear optics into the realm of single-photon nonlinearities. This tutorial reviews these recent developments in ultrafast nonlinear photonics, discusses design strategies for realizing few-photon nonlinear interactions, and presents a unified treatment of ultrafast quantum nonlinear optics using a framework that smoothly interpolates from classical behaviors to the few-photon scale. These emerging platforms for quantum optics fundamentally differ from typical realizations in cavity quantum electrodynamics due to the large number of coupled optical modes. Classically, multimode behaviors have been well studied in nonlinear optics, with famous examples including soliton formation and supercontinuum generation. In contrast, multimode quantum systems exhibit a far greater variety of behaviors, and yet closed-form solutions are even sparser than their classical counterparts. In developing a framework for ultrafast quantum optics, we will identify what behaviors carry over from classical to quantum devices, what intuition must be abandoned, and what new opportunities exist at the intersection of ultrafast and quantum nonlinear optics. While this article focuses on establishing connections between the classical and quantum behaviors of devices with $\chi^{(2)}$ nonlinearities, the frameworks developed here are general and are readily extended to the description of dynamical processes based on third-order ($\chi^{(3)}$) nonlinearities.

physics.optics↗

arXiv2023

Mesoscopic ultrafast nonlinear optics -- The emergence of multimode quantum non-Gaussian physics

Over the last few decades, nonlinear optics has become significantly more nonlinear, traversing nearly a billionfold improvement in energy efficiency, with ultrafast nonlinear nanophotonics in particular emerging as a frontier for combining both spatial and temporal engineering. At present, cutting-edge experiments in nonlinear nanophotonics place us just above the mesoscopic regime, where a few hundred photons suffice to trigger nonlinear saturation. In contrast to classical or deep-quantum optics, the mesoscale is characterized by dynamical interactions between mean-field, Gaussian, and non-Gaussian quantum features, all within a close hierarchy of scales. When combined with the inherent multimode complexity of optical fields, such hybrid quantum-classical dynamics present theoretical, experimental, and engineering challenges to the contemporary framework of quantum optics. In this review, we highlight the unique physics that emerges in multimode nonlinear optics at the mesoscale and outline key principles for exploiting both classical and quantum features to engineer novel functionalities. We briefly survey the experimental landscape and draw attention to outstanding technical challenges in materials, dispersion engineering, and device design for accessing mesoscopic operation. Finally, we speculate on how these capabilities might usher in some new paradigms in quantum photonics, from quantum-augmented information processing to nonclassical-light-driven dynamics and phenomena to all-optical non-Gaussian measurement and sensing. The physics unlocked at the mesoscale present significant challenges and opportunities in theory and experiment alike, and this review is intended to serve as a guidepost as we begin to navigate this new frontier in ultrafast quantum nonlinear optics.

quant-ph↗

arXiv2023

Quantum noise dynamics in nonlinear pulse propagation

The propagation of ultrafast pulses in dispersion-engineered waveguides, exhibiting strong field confinement in both space and time, is a promising avenue towards single-photon nonlinearities in an all-optical platform. However, quantum engineering in such systems requires new numerical tools and physical insights to harness their complicated multimode and nonlinear quantum dynamics. In this work, we use a self-consistent, multimode Gaussian-state model to capture the nonlinear dynamics of broadband quantum fluctuations and correlations, including entanglement. Notably, despite its parametrization by Gaussian states, our model exhibits nonlinear dynamics in both the mean field and the quantum correlations, giving it a marked advantage over conventional linearized treatments of quantum noise, especially for systems exhibiting gain saturation and strong nonlinearities. Numerically, our approach takes the form of a Gaussian split-step Fourier (GSSF) method, naturally generalizing highly efficient SSF methods used in classical ultrafast nonlinear optics; the equations for GSSF evaluate in $O(M^2\log M)$ time for an $M$-mode system with $O(M^2)$ quantum correlations. To demonstrate the broad applicability of GSSF, we numerically study quantum noise dynamics and multimode entanglement in several ultrafast systems, from canonical soliton propagation in third-order ($\chi^{(3)}$) waveguides to saturated $\chi^{(2)}$ broadband parametric generation and supercontinuum generation, e.g., as recently demonstrated in thin-film lithium niobate nanophotonics.

quant-ph↗

arXiv2023

Mid-infrared spectroscopy with a broadly tunable thin-film lithium niobate optical parametric oscillator

Mid-infrared spectroscopy, an important and widespread technique for sensing molecules, has encountered barriers stemming from sources either limited in tuning range or excessively bulky for practical field use. We present a compact, efficient, and broadly tunable optical parametric oscillator (OPO) device surmounting these challenges. Leveraging a dispersion-engineered singly-resonant OPO implemented in thin-film lithium niobate-on-sapphire, we achieve broad and controlled tuning over an octave, from 1.5 to 3.3 microns by combining laser and temperature tuning. The device generates > 25 mW of mid-infrared light at 3.2 microns, offering a power conversion efficiency of 15% (45% quantum efficiency). We demonstrate the tuning and performance of the device by successfully measuring the spectra of methane and ammonia, verifying our approach's relevance for gas sensing. Our device signifies an important advance in nonlinear photonics miniaturization and brings practical field applications of high-speed and broadband mid-infrared spectroscopy closer to reality.

physics.optics↗

arXiv2023

Integrated frequency-modulated optical parametric oscillator

Optical frequency combs have revolutionized precision measurement, time-keeping, and molecular spectroscopy. A substantial effort has developed around "microcombs": integrating comb-generating technologies into compact, reliable photonic platforms. Current approaches for generating these microcombs involve either the electro-optic (EO) or Kerr mechanisms. Despite rapid progress, maintaining high efficiency and wide bandwidth remains challenging. Here, we introduce a new class of microcomb -- an integrated optical frequency comb generator that combines electro-optics and parametric amplification to yield a frequency-modulated optical parametric oscillator (FM-OPO). In stark contrast to EO and Kerr combs, the FM-OPO microcomb does not form pulses but maintains operational simplicity and highly efficient pump power utilization with an output resembling a frequency-modulated laser. We outline the working principles of FM-OPO and demonstrate them by fabricating the complete optical system in thin-film lithium niobate (LNOI). We measure pump to comb internal conversion efficiency exceeding 93% (34% out-coupled) over a nearly flat-top spectral distribution spanning approximately 1,000 modes (approximately 6 THz). Compared to an EO comb, the cavity dispersion rather than loss determines the FM-OPO bandwidth, enabling broadband combs with a smaller RF modulation power. The FM-OPO microcomb, with its robust operational dynamics, high efficiency, and large bandwidth, contributes a new approach to the field of microcombs and promises to herald an era of miniaturized precision measurement, and spectroscopy tools to accelerate advancements in metrology, spectroscopy, telecommunications, sensing, and computing.

physics.optics↗

arXiv2023

Surface Modification and Coherence in Lithium Niobate SAW Resonators

Lithium niobate is a promising material for developing quantum acoustic technologies due to its strong piezoelectric effect and availability in the form of crystalline thin films of high quality. However, at radio frequencies and cryogenic temperatures, these resonators are limited by the presence of decoherence and dephasing due to two-level systems. To mitigate these losses and increase device performance, a more detailed picture of the microscopic nature of these loss channels is needed. In this study, we fabricate several lithium niobate acoustic wave resonators and apply different processing steps that modify their surfaces. These treatments include argon ion sputtering, annealing, and acid cleans. We characterize the effects of these treatments using three surface-sensitive measurements: cryogenic microwave spectroscopy measuring density and coupling of TLS to mechanics, x-ray photoelectron spectroscopy and atomic force microscopy. We learn from these studies that, surprisingly, increases of TLS density may accompany apparent improvements in the surface quality as probed by the latter two approaches. Our work outlines the importance that surfaces and fabrication techniques play in altering acoustic resonator coherence, and suggests gaps in our understanding as well as approaches to address them.

quant-ph↗

arXiv2022

Degenerate optical parametric amplification in CMOS silicon

Silicon is a common material for photonics due to its favorable optical properties in the telecom and mid-wave IR bands, as well as compatibility with a wide range of complementary metal-oxide semiconductor (CMOS) foundry processes. Crystalline inversion symmetry precludes silicon from natively exhibiting second-order nonlinear optical processes. In this work, we build on recent work in silicon photonics that break this material symmetry using large bias fields, thereby enabling $\chi^{(2)}$ interactions. Using this approach, we demonstrate both second-harmonic generation (with a normalized efficiency of $0.2\,\%\,\mathrm{W^{-1} cm^{-2}}$) and, to our knowledge, the first degenerate $\chi^{(2)}$ optical parametric amplifier (with relative gain of $0.02\,\mathrm{dB}$ using $3\,\mathrm{mW}$ of pump power on-chip at a pump wavelength of $1196\,\mathrm{nm}$) using silicon-on-insulator waveguides fabricated in a CMOS-compatible commercial foundry. We expect this technology to enable the integration of novel nonlinear optical devices such as optical parametric amplifiers, oscillators, and frequency converters into large-scale, hybrid photonic-electronic systems by leveraging the extensive ecosystem of CMOS fabrication.

physics.optics↗

arXiv2022

Ultra-broadband mid-infrared generation in dispersion-engineered thin-film lithium niobate

Thin-film lithium niobate (TFLN) is an emerging platform for compact, low-power nonlinear-optical devices, and has been used extensively for near-infrared frequency conversion. Recent work has extended these devices to mid-infrared wavelengths, where broadly tunable sources may be used for chemical sensing. To this end, we demonstrate efficient and broadband difference frequency generation between a fixed 1-micron pump and a tunable telecom source in uniformly-poled TFLN-on-sapphire by harnessing the dispersion-engineering available in tightly-confining waveguides. We show a simultaneous 1-2 order-of-magnitude improvement in conversion efficiency and ~5-fold enhancement of operating bandwidth for mid-infrared generation when compared to conventional lithium niobate waveguides. We also examine the effects of mid-infrared loss from surface-adsorbed water on the performance of these devices.

physics.optics↗

arXiv2022

Reduced Material Loss in Thin-film Lithium Niobate Waveguides

Thin-film lithium niobate has shown promise for scalable applications ranging from single-photon sources to high-bandwidth data communication systems. Realization of the next generation high-performance classical and quantum devices, however, requires much lower optical losses than the current state of the art ($\sim$10 million). Unfortunately, material limitations of ion-sliced thin-film lithium niobate have not been explored, and therefore it is unclear how high-quality factor can be achieved in this platform. Here we evaluate the material limited quality factor of thin-film lithium niobate photonic platform can be as high as $Q\approx 1.8\times10^{8}$ at telecommunication wavelengths, corresponding to a propagation loss of 0.2 dB/m.

physics.optics↗

arXiv2022

Temporal trapping: a route to strong coupling and deterministic optical quantum computation

The realization of deterministic photon-photon gates is a central goal in optical quantum computation and engineering. A longstanding challenge is that optical nonlinearities in scalable, room-temperature material platforms are too weak to achieve the required strong coupling, due to the critical loss-confinement tradeoff in existing photonic structures. In this work, we introduce a novel confinement method, dispersion-engineered temporal trapping, to circumvent the tradeoff, paving a route to all-optical strong coupling. Temporal confinement is imposed by an auxiliary trap pulse via cross-phase modulation, which, combined with the spatial confinement of a waveguide, creates a "flying cavity" that enhances the nonlinear interaction strength by at least an order of magnitude. Numerical simulations confirm that temporal trapping confines the multimode nonlinear dynamics to a single-mode subspace, enabling high-fidelity deterministic quantum gate operations. With realistic dispersion engineering and loss figures, we show that temporally trapped ultrashort pulses could achieve strong coupling on near-term nonlinear nanophotonic platforms. Our results highlight the potential of ultrafast nonlinear optics to become the first scalable, high-bandwidth, and room-temperature platform that achieves a strong coupling, opening a new path to quantum computing, simulation, and light sources.

quant-ph↗

arXiv2021

Onset of non-Gaussian quantum physics in pulsed squeezing with mesoscopic fields

We study the emergence of non-Gaussian quantum features in pulsed squeezed light generation with a mesoscopic number (i.e., dozens to hundreds) of pump photons. Due to the strong optical nonlinearities necessarily involved in this regime, squeezing occurs alongside significant pump depletion, compromising the predictions made by conventional semiclassical models for squeezing. Furthermore, nonlinear interactions among multiple frequency modes render the system dynamics exponentially intractable in na\"ive quantum models, requiring a more sophisticated modeling framework. To this end, we construct a nonlinear Gaussian approximation to the squeezing dynamics, defining a "Gaussian interaction frame" (GIF) in which non-Gaussian quantum dynamics can be isolated and concisely described using a few dominant (i.e., principal) supermodes. Numerical simulations of our model reveal non-Gaussian distortions of squeezing in the mesoscopic regime, largely associated with signal-pump entanglement. We argue that the state of the art in nonlinear nanophotonics is quickly approaching this regime, providing an all-optical platform for experimental studies of the semiclassical-to-quantum transition in a rich paradigm of coherent, multimode nonlinear dynamics. Mesoscopic pulsed squeezing thus provides an intriguing case study of the rapid rise in dynamic complexity associated with semiclassical-to-quantum crossover, which we view as a correlate of the emergence of new information-processing capacities in the quantum regime.

quant-ph↗

arXiv2021

Quasi-static Optical Parametric Amplification

High-gain optical parametric amplification is an important nonlinear process used both as a source of coherent infrared light and as a source of nonclassical light. In this work, we experimentally demonstrate an approach to optical parametric amplification that enables extremely large parametric gains with low energy requirements. In conventional nonlinear media driven by femtosecond pulses, multiple dispersion orders limit the effective interaction length available for parametric amplification. Here, we use the dispersion engineering available in periodically poled thin-film lithium niobate nanowaveguides to eliminate several dispersion orders at once. The result is a quasi-static process; the large peak intensity associated with a short pump pulse can provide gain to signal photons without undergoing pulse distortion or temporal walk-off. We characterize the parametric gain available in these waveguides using optical parametric generation, where vacuum fluctuations are amplified to macroscopic intensities. When driven with pulse energies in excess of 10 pJ, we observe saturated parametric gains as large as 88 dB (146 dB/cm). The devices shown here achieve saturated optical parametric generation with orders of magnitude less pulse energy than previous techniques.

physics.optics↗

arXiv2021

Mid-infrared nonlinear optics in thin-film lithium niobate on sapphire

Periodically poled thin-film lithium niobate (TFLN) waveguides have emerged as a leading platform for highly efficient frequency conversion in the near-infrared. However, the commonly used silica bottom-cladding results in high absorption loss at wavelengths beyond 2.5 $\mu$m. In this work, we demonstrate efficient frequency conversion in a TFLN-on-sapphire platform, which features high transparency up to 4.5 $\mu$m. In particular, we report generating mid-infrared light up to 3.66 $\mu$m via difference-frequency generation of a fixed 1-$\mu$m source and a tunable telecom source, with normalized efficiencies up to 200%/W-cm$^2$. These results show TFLN-on-sapphire to be a promising platform for integrated nonlinear nanophotonics in the mid-infrared.

physics.optics↗

arXiv2021

Dispersion-engineered $\chi^{(2)}$ nanophotonics: a flexible tool for nonclassical light

This article reviews recent progress in quasi-phasematched $\chi^{(2)}$ nonlinear nanophotonics, with a particular focus on dispersion-engineered nonlinear interactions. Throughout this article, we establish design rules for the bandwidth and interaction lengths of various nonlinear processes, and provide examples for how these processes can be engineered in nanophotonic devices. In particular, we apply these rules towards the design of sources of non-classical light and show that dispersion-engineered devices can outperform their conventional counterparts. Examples include ultra-broadband optical parametric amplification as a resource for measurement-based quantum computation, dispersion-engineered spontaneous parametric downconversion as a source of separable biphotons, and synchronously pumped nonlinear resonators as a potential route towards single-photon nonlinearities.

physics.optics↗

arXiv2021

Supercontinuum Generation by Saturated Second-Order Nonlinear Interactions

We propose a new approach to supercontinuum generation and carrier-envelope-offset detection based on saturated second-order nonlinear interactions in dispersion-engineered nanowaveguides. The technique developed here broadens the interacting harmonics by forming stable bifurcations of the pulse envelopes due to an interplay between phase-mismatch and pump depletion. We first present an intuitive heuristic model for spectral broadening by second-harmonic generation of femtosecond pulses, and show that this model agrees well with experiments. Then, having established strong agreement between theory and experiment, we develop scaling laws that determine the energy required to generate an octave of bandwidth as a function of input pulse duration, device length, and input pulse chirp. These scaling laws suggest that future realization based on this approach could enable supercontinuum generation with orders of magnitude less energy than current state-of-the-art devices.

physics.optics↗