arXiv subjects

Marc. J. J. Vrakking

Publications and source records attributed to Marc. J. J. Vrakking.

3 recordsLinked to original sources

arXiv2021

Characterization of laser-induced ionization dynamics in solid dielectrics

The formation of an electron-hole plasma during the interaction of intense femtosecond laser pulses with transparent solids lies at the heart of femtosecond laser processing. Advanced micro- and nanomachining applications require improved control over the excitation characteristics. Here, we relate the emission of low-order harmonics to the strong laser-field-induced plasma formation. Together with a measurement of the total plasma density we identify the contribution of two competing ionization mechanisms - strong-field and electron-impact ionization.

physics.optics↗

arXiv2019

Molecular movie of ultrafast coherent rotational dynamics

Recording molecular movies on ultrafast timescales has been a longstanding goal for unravelling detailed information about molecular dynamics. We present the direct experimental recording of very-high-resolution and -fidelity molecular movies over more than one-and-a-half periods of the laser-induced rotational dynamics of carbonylsulfide (OCS) molecules. Utilising the combination of single-quantum-state selection and an optimised two-pulse sequence to create a tailored rotational wavepacket, an unprecedented degree of field-free alignment, $\langle \cos^{2}{θ_{2D}}\rangle=0.96$ ($\langle \cos^{2}θ\rangle=0.94$) was achieved, exceeding the theoretical limit for single-pulse alignment. The very rich experimentally observed quantum dynamics is fully recovered by the angular probability distribution obtained from solutions of the time-dependent Schrödinger equation with parameters refined against the experiment. The populations and phases of rotational states in the retrieved time-dependent three-dimensional wavepacket rationalised the observed very high degree of alignment.

physics.chem-ph↗

arXiv2018

43 W, 1.55 μm and 12.5 W, 3.1 μm dual-beam, sub-10 cycle, 100 kHz optical parametric chirped pulse amplifier

We present a 100 kHz optical parametric chirped pulse amplifier (OPCPA) developed for strong-field attosecond physics and soft-X-ray transient absorption experiments. The system relies on noncollinear potassium titanyl arsenate (KTA) booster OPCPAs and is pumped by a 240 W, 1.1 ps Yb:YAG Innoslab chirped pulse laser amplifier. Two optically synchronized infrared output beams are simultaneously available: a 430 μJ, 51 fs, carrier-envelope phase (CEP) stable beam at 1.55 μm and an angular-dispersion-compensated, 125 μJ, 73 fs beam at 3.1 μm.

physics.ins-det↗