arXiv subjects

Marco Aprili

Publications and source records attributed to Marco Aprili.

At least 19 recordsLinked to original sources

arXiv2025

Fast and Continuous Detection of Single Microwave Photons via Photo-assisted Quasiparticle Tunneling to a Superconducting Island

We demonstrate a single-photon detector operating in the microwave domain, based on photo-assisted quasiparticle tunneling events that poison a superconducting island. The detection relies on continuously monitoring the island's charge parity using microwave reflectometry. This scheme achieves 10\% detection efficiency with sub \SI{50}{\ns} time resolution and short dead time ($\sim \SI{1}{\us}$), for microwave photons at \SI{10}{\GHz}. The detector features three junctions connected to a superconducting island, which together carry out photoelectric conversion and charge readout. The enhanced light--matter coupling, crucial to photon to quasiparticle conversion, is provided by a granular aluminum-based high-impedance microwave resonator. The time resolved detection of itinerant microwave photon opens up new perspectives in quantum sensing, microwave quantum optics and mesoscopic physics.

cond-mat.mes-hall↗

arXiv2023

Efficient Microwave Photon to Electron Conversion in a High Impedance Quantum Circuit

We demonstrate an efficient and continuous microwave photon to electron converter with large quantum efficiency ($83\%$) and low dark current. These unique properties are enabled by the use of a high kinetic inductance disordered superconductor, granular aluminium, to enhance light-matter interaction and the coupling of microwave photons to electron tunneling processes. As a consequence of strong coupling, we observe both linear and non-linear photon-assisted processes where 2, 3 and 4 photons are converted into a single electron at unprecedentedly low light intensities. Theoretical predictions, which require quantization of the photonic field within a quantum master equation framework, reproduce well the experimental data. This experimental advancement brings the foundation for high-efficiency detection of individual microwave photons using charge-based detection techniques.

quant-ph↗

arXiv2023

Imaging the Quantum Capacitance of Strained MoS2 Monolayers by Electrostatic Force Microscopy

We implemented radio frequency-assisted electrostatic force microscopy (RF-EFM) to investigate the electric field response of biaxially strained molybdenum disulfide (MoS2) monolayers (MLs) in the form of mesoscopic bubbles, produced via hydrogen (H)-ion irradiation of the bulk crystal. MoS2 ML, a semiconducting transition metal dichalcogenide, has recently attracted significant attention due to its promising optoelectronic properties, further tunable by strain. Here, we take advantage of the RF excitation to distinguish the intrinsic quantum capacitance of the strained ML from that due to atomic scale defects, presumably sulfur vacancies or H-passivated sulfur vacancies. In fact, at frequencies fRF larger than the inverse defect trapping time, the defect contribution to the total capacitance and to transport is negligible. Using RF-EFM at fRF = 300 MHz, we visualize simultaneously the bubble topography and its quantum capacitance. Our finite-frequency capacitance imaging technique is non-invasive and nanoscale, and can contribute to the investigation of time and spatial-dependent phenomena, such as the electron compressibility in quantum materials, which are difficult to measure by other methods.

cond-mat.mes-hall↗

arXiv2022

Quantum bath engineering of a high impedance microwave mode through quasiparticle tunneling

We demonstrate a new approach to dissipation engineering in microwave quantum optics. For a single mode, dissipation usually corresponds to quantum jumps, where photons are lost one by one. Here, we are able to tune the minimal number of lost photons per jump to be two (or more) with a simple dc voltage. As a consequence, different quantum states experience different dissipation. Causality implies that the states must also experience different energy shifts. Our measurements of these Lamb shifts are in good agreement with the predictions of the Kramers-Kronig relations for single quantum states in a regime of highly non-linear bath coupling. This work opens new possibilities for quantum state manipulation in circuit QED, without relying on the Josephson effect.

quant-ph↗

arXiv2021

Coherent and incoherent tunneling into YSR states revealed by atomic scale shot-noise spectroscopy

The pair breaking potential of individual magnetic impurities in s-wave superconductors generates localized states inside the superconducting gap commonly referred to as Yu- Shiba-Rusinov (YSR) states whose isolated nature makes them ideal building blocks for artificial structures that may host Majorana fermions. One of the challenges in this endeavor is to understand their intrinsic lifetime, $\hbar/\Lambda$, which is expected to be limited by the inelastic coupling with the continuum thus leading to decoherence. Here we use shot-noise scanning tunneling microscopy to reveal that electron tunnelling into superconducting 2H-NbSe$_2$ mediated by YSR states is ordered as function of time, as evidenced by a reduction of the noise. Moreover, our data show the concomitant transfer of charges e and 2e, indicating that incoherent single particle and coherent Andreev processes operate simultaneously. From the quantitative agreement between experiment and theory we obtain $\Lambda$ = 1 $\mu$eV $\ll$ $k_BT$ demonstrating that shot-noise can probe energy- and time scales inaccessible by conventional spectroscopy whose resolution is thermally limited.

cond-mat.supr-con↗

arXiv2021

Gate-Assisted Phase Fluctuations in All-Metallic Josephson Junctions

The discovery that a gate electrode suppresses the supercurrent in purely metallic systems is missing a complete physical understanding of the mechanisms at play. We here study the origin of this reduction in a Superconductor-Normal metal-Superconductor Josephson junction by performing, on the same device, a detailed investigation of the gate-dependent switching probability together with the local tunnelling spectroscopy of the normal metal. We demonstrate that high energy electrons leaking from the gate trigger the reduction of the critical current which is accompanied by an important broadening of the switching histograms. The switching rates are well described by an activation formula including an additional term accounting for the injection of rare high energy electrons from the gate. The rate of electrons obtained from the fit remarkably coincides with the independently measured leakage current. Concomitantly, a negligible elevation of the local temperature is found by tunnelling spectroscopy which excludes overheating scenarios.

cond-mat.supr-con↗

arXiv2021

Tunable high speed atomic rotor in Bi$_{2}$Se$_{3}$ revealed by current noise

The ability to manipulate individual atoms and molecules using a scanning tunnelling microscope (STM) has been crucial for the development of a vast array of atomic scale devices and structures ranging from nanoscale motors and switches to quantum corrals. Molecular motors in particular have attracted considerable attention in view of their potential for assembly into complex nanoscale machines. Whereas the manipulated atoms or molecules are usually on top of a substrate, motors embedded in a lattice can be very beneficial for bottom-up construction, and may additionally be used to probe the in uence of the lattice on the electronic properties of the host material. Here, we present the discovery of controlled manipulation of a rotor in Fe doped Bi$_{2}$Se$_{3}$. We find that the current into the rotor, which can be finely tuned with the voltage, drives omni-directional switching between three equivalent orientations, each of which can be frozen in at small bias voltage. Using current fluctuation measurements at 1MHz and model simulations, we estimate that switching rates of hundreds of kHz for sub-nA currents are achieved.

cond-mat.str-el↗

arXiv2020

Dynamical I-V Characteristics of SNS Junctions

We have probed the switching dynamics of the Josephson critical current of a superconducting weak link by measuring its voltage/current characteristics while applying an ac current bias in the range 1-200 MHz. The weak link between two Nb reservoirs is formed by an mesoscopic Al wire above its critical temperature. We observe a dynamical phase transition as a function of the frequency and amplitude of the ac current. While at low frequency the transition driven by increasing the current bias is well described by the standard Kramers theory, at high frequency the switching histograms become hysteretic and much narrower than expected by thermal fluctuations. The crossover frequency between the two regimes is set by the electron-phonon interaction rate in the normal metal.

cond-mat.mes-hall↗

arXiv2019

Nonadiabatic Dynamics of Strongly Driven Diffusive Josephson Junctions

By measuring the Josephson emission of a diffusive Superconductor-Normal metal-Superconductor (SNS) junction at a finite temperature we reveal a non-trivial sensitivity of the supercurrent to microwave irradiation. We demonstrate that the harmonic content of the current-phase relation is modified due to the energy redistribution of quasiparticles in the normal wire induced by the electromagnetic field. The distortion originates from the phase-dependent out-of-equilibrium distribution function which is strongly affected by the ac-response of the spectral supercurrent. For phases close to $π$, transitions accross the Andreev gap are dynamically favored leading to a supercurrent reduction. This finding is supported by a comparison with the quasiclassical Green's function theory of superconductivity in diffusive SNS junctions under microwave irradiation.

cond-mat.mes-hall↗

arXiv2019

Zeeman tunability of Andreev bound states in van-der-Waals tunnel barriers

Quantum dots proximity-coupled to superconductors are attractive research platforms due to the intricate interplay between the single-electron nature of the dot and the many body nature of the superconducting state. These have been studied mostly using nanowires and carbon nanotubes, which allow a combination of tunability and proximity. Here we report a new type of quantum dot which allows proximity to a broad range superconducting systems. The dots are realized as embedded defects within semiconducting tunnel barriers in van-der-Waals layers. By placing such layers on top of thin NbSe$_2$, we can probe the Andreev bound state spectra of such dots up to high in-plane magnetic fields without observing effects of a diminishing superconducting gap. As tunnel junctions defined on NbSe$_2$ have a hard gap, we can map the sub-gap spectra without background related to the rest of the junction. We find that the proximitized defect states invariably have a singlet ground state, manifest in the Zeeman splitting of the sub-gap excitation. We also find, in some cases, bound states which converge to zero energy and remain there. We discuss the role of the spin-orbit term, present both in the barrier and the superconductor, in the realization of such topologically trivial zero-energy states.

cond-mat.supr-con↗

arXiv2019

High Kinetic Inductance Microwave Resonators Made by He-Beam Assisted Deposition of Tungsten Nanowires

We evaluate the performance of hybrid microwave resonators made by combining sputtered Nb thin films with Tungsten nanowires grown with a He-beam induced deposition technique. Depending on growth conditions the nanowires have a typical width $w\in[35-75]$~nm and thickness $t\in[5-40]$~nm. We observe a high normal state resistance $R_{sq}\in [65-150]$ $Ω/sq$ which together with a critical temperature $T_c\in[4-6]~K$ ensure a high kinetic inductance making the resonator strongly nonlinear. Both lumped and coplanar waveguide resonators were fabricated and measured at low temperature exhibiting internal quality factors up to $3990$ at $4.5$~GHz in the few photon regime. Analyzing the wire length, temperature and microwave power dependence we extracted a kinetic inductance for the W nanowire of $L_K\approx15$ pH/sq, which is 250 times higher than the geometrical inductance, and a Kerr non-linearity as high as $K_{W,He}/2π=200 \pm 120$~Hz/photon at $4.5$~GHz. The nanowires made with the helium focused ion beam are thus versatile objects to engineer compact, high impedance, superconducting environments with a mask and resist free direct write process.

cond-mat.mes-hall↗

arXiv2019

Spin-Orbit induced phase-shift in Bi$_{2}$Se$_{3}$ Josephson junctions

The transmission of Cooper pairs between two weakly coupled superconductors produces a superfluid current and a phase difference; the celebrated Josephson effect. Because of time-reversal and parity symmetries, there is no Josephson current without a phase difference between two superconductors. Reciprocally, when those two symmetries are broken, an anomalous supercurrent can exist in the absence of phase bias or, equivalently, an anomalous phase shift $φ_0$ can exist in the absence of a superfluid current. We report on the observation of an anomalous phase shift $φ_0$ in hybrid Josephson junctions fabricated with the topological insulator Bi$_2$Se$_3$ submitted to an in-plane magnetic field. This anomalous phase shift $φ_0$ is observed directly through measurements of the current-phase relationship in a Josephson interferometer. This result provides a direct measurement of the spin-orbit coupling strength and open new possibilities for phase-controlled Josephson devices made from materials with strong spin-orbit coupling.

cond-mat.supr-con↗

arXiv2018

Observation of the Unconventional Photon Blockade in the Microwave Domain

We have observed the unconventional photon blockade effect for microwave photons using two coupled superconducting resonators. As opposed to the conventional blockade, only weakly nonlinear resonators are required. The blockade is revealed through measurements of the second order correlation function $g^{(2)}(t)$ of the microwave field inside one of the two resonators. The lowest measured value of $g^{(2)}(0)$ is 0.4 for a resonator population of approximately $10^{-2}$ photons. The time evolution of $g^{(2)}(t)$ exhibits an oscillatory behavior, which is characteristic of the unconventional photon blockade.

quant-ph↗

arXiv2018

Tunneling into the vortex state of NbSe$_2$ with van der Waals junctions

We have performed device-based tunnelling spectroscopy of NbSe$_2$ in the vortex state with a magnetic field applied both parallel and perpendicular to the $a-b$ plane. Our devices consist of layered semiconductors placed on top of exfoliated NbSe$_2$ using the van der Waals transfer technique. At zero field, the spectrum exhibits a hard gap, and the quasiparticle peak is split into low and high energy features. The two features, associated with the effective two-band nature of superconductivity in NbSe$_2$, exhibit markedly distinct responses to the application of magnetic field, suggesting an order-of-magnitude difference in the spatial extent of the vortex cores of the two bands. At energies below the superconducting gap, the hard gap gives way to vortex-bound Caroli-de Gennes-Matricon states, allowing the detection of individual vortices as they enter and exit the junction. Analysis of the sub-gap spectra upon application of parallel magnetic field allows us to track the process of vortex surface formation and spatial rearrangement in the bulk.

cond-mat.supr-con↗

arXiv2018

Quantum dynamics of a microwave resonator strongly coupled to a tunnel junction

We consider the coupling of a single mode microwave resonator to a tunnel junction whose contacts are at thermal equilibrium. We derive the quantum master equation describing the evolution of the resonator field in the strong coupling regime, where the characteristic impedance of the resonator is larger than the quantum of resistance. We first study the case of a normal-insulator-normal junction and show that a dc driven single photon source can be obtained. We then consider the case of a superconductor-insulator-normal and superconductor-insulator-superconductor junction. There, we show that the Lamb shift induced by the junction gives rise to a nonlinear spectrum of the resonator even when the junction induced losses are negligible. We discuss the resulting dynamics and consider possible applications including quantum Zeno dynamics and the realization of a qubit.

cond-mat.mes-hall↗

arXiv2018

Atomic scale shot-noise using broadband scanning tunnelling microscopy

We have developed a broadband scanning tunnelling microscope capable of conventional, low frequency (<10 kHz), microscopy as well spectroscopy and shot-noise detection at 1 MHz. After calibrating our AC circuit on a gold surface, we illustrate our capability to detect shot-noise at the atomic scale and at low currents (<1 nA) by simultaneously measuring the atomically resolved differential conductance and shot-noise on the high temperature superconductor Bi$_{2}$Sr$_{2}$CaCu$_{2}$O$_{8+x}$. We further show our direct sensitivity to the temperature of the tunnelling electrons at low voltages. Our broadband probe opens up the possibility to study charge and correlation effects at the atomic scale in all materials accessible to STM.

cond-mat.mes-hall↗

arXiv2017

Spectroscopy of bulk and few-layer superconducting NbSe$_2$ with van der Waals tunnel junctions

Tunnel junctions, a well-established platform for high-resolution spectroscopy of superconductors, require defect-free insulating barriers with clean engagement to metals on both sides. Extending the range of materials accessible to tunnel junction fabrication, beyond the limited selection which allows high-quality oxide formation, requires the development of alternative fabrication techniques. Here we show that van-der-Waals (vdW) tunnel barriers, fabricated by stacking layered semiconductors on top of the transition metal dichalcogenide (TMD) superconductor NbSe$_2$, sustain a stable, low noise tunneling current, and exhibit strong suppression of sub-gap tunneling. We utilize the technique to measure the spectra of bulk (20 nm) and ultrathin (3- and 4-layer) devices at 70 mK. The spectra exhibit two distinct energy gaps, the larger of which decreases monotonously with thickness and $T_C$, in agreement with BCS theory. The spectra are analyzed using a two-band model modified to account for depairing. We show that in the bulk, the smaller gap exhibits strong depairing in an in-plane magnetic field, consistent with a high Fermi velocity. In the few-layer devices, depairing of the large gap is negligible, consistent with out-of-plane spin-locking due to Ising spin-orbit coupling. Our results demonstrate the utility of vdW tunnel junctions in mapping the intricate spectral evolution of TMD superconductors over a range of magnetic fields.

cond-mat.supr-con↗

arXiv2017

Shiba Bound States across the mobility edge in doped InAs nanowires

We present a study of Andreev Quantum Dots (QDots) fabricated with small-diameter (30 nm) Si-doped InAs nanowires where the Fermi level can be tuned across a mobility edge separating localized states from delocalized states. The transition to the insulating phase is identified by a drop in the amplitude and width of the excited levels and is found to have remarkable consequences on the spectrum of superconducting SubGap Resonances (SGRs). While at deeply localized levels, only quasiparticles co-tunneling is observed, for slightly delocalized levels, Shiba bound states form and a parity changing quantum phase transition is identified by a crossing of the bound states at zero energy. Finally, in the metallic regime, single Andreev resonances are observed.

cond-mat.supr-con↗