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Marco Barbieri

Publications and source records attributed to Marco Barbieri.

At least 127 records · Page 7Linked to original sources

Direct observation of sub-binomial light

Nonclassical states of light are necessary resources for quantum technologies such as cryptography, computation and the definition of metrological standards. Observing signatures of nonclassicality generally requires inferring either the photon number distribution or a quasi-probability distribution indirectly from a set of measurements. Here, we report an experiment in which the nonclassical character of families of quantum states is assessed by direct inspection of the outcomes from a multiplexed photon counter. This scheme does not register the actual photon number distribution; the statistics of the detector clicks alone serve as a witness of nonclassicality, as proposed by Sperling et al. in Phys. Rev. Lett. 109, 093601 (2012). Our work paves a way for the practical characterisation of increasingly sophisticated states and detectors.

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On-chip low loss heralded source of pure single photons

A key obstacle to the experimental realization of many photonic quantum-enhanced technologies is the lack of low-loss sources of single photons in pure quantum states. We demonstrate a promising solution: generation of heralded single photons in a silica photonic chip by spontaneous four-wave mixing. A heralding efficiency of 40%, corresponding to a preparation efficiency of 80% accounting for detector performance, is achieved due to efficient coupling of the low-loss source to optical fibers. A single photon purity of 0.86 is measured from the source number statistics without filtering, and confirmed by direct measurement of the joint spectral intensity. We calculate that similar high-heralded-purity output can be obtained from visible to telecom spectral regions using this approach. On-chip silica sources can have immediate application in a wide range of single-photon quantum optics applications which employ silica photonics.

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Requirements for two-source entanglement concentration

Entanglement enhancement is a key task for quantum technologies. This operation performed on states produced by parametric down-conversion sources has been the object of several recent experimental investigations. In particular, conditional preparation by photon-subtraction has been shown to improve the entanglement of these states. Here we analyse the role played by non-Gaussian and Gaussian measurements in more general entanglement concentration operations performed on a pair of two-mode squeezed vacua. We find stringent requirements for achieving an improved entanglement enhancement by measuring jointly these two resource states.

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Efficient optical pumping and high optical depth in a hollow-core photonic-crystal fibre for a broadband quantum memory

The generation of large multiphoton quantum states - for applications in computing, metrology, and simulation - requires a network of high-efficiency quantum memories capable of storing broadband pulses. Integrating these memories into a fibre offers a number of advantages towards realising this goal: strong light-matter coupling at low powers, simplified alignment, and compatibility with existing photonic architectures. Here, we introduce a large-core kagome-structured hollow-core fibre as a suitable platform for an integrated fibre-based quantum memory with a warm atomic vapour. We demonstrate, for the first time, efficient optical pumping in a hollow-core photonic-crystal fibre with a warm atomic vapour, where (90 $\pm$ 1)% of atoms are prepared in the ground state. We measure high optical depths (3$\times 10^{4}$) and, also, narrow homogeneous linewidths that do not exhibit significant transit-time broadening. Our results establish that kagome fibres are suitable for implementing a broadband, room-temperature quantum memory.

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Homodyne estimation of Gaussian quantum discord

We address the experimental estimation of Gaussian quantum discord for two-mode squeezed thermal state, and demonstrate a measurement scheme based on a pair of homodyne detectors assisted by Bayesian analysis which provides nearly optimal estimation for small value of discord. Besides, though homodyne detection is not optimal for Gaussian discord, the noise ratio to the ultimate quantum limit, as dictacted by the quantum Cramer-Rao bound, is limited to about 10 dB.

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Multi-photon state engineering by heralded interference between single photons and coherent states

We develop a technique for generating multi-photon nonclassical states via interference between coherent and Fock states using quantum catalysis. By modulating the coherent field strength, the number of catalyst photons and the ratio of the beam splitter upon which they interfere, a wide range of nonclassical phenomena can be created, including squeezing of up to 1.25 dB, anti- and super-bunched photon statistics and states exhibiting over 90% fidelity to displaced coherent superposition states. We perform quantum catalysis experimentally, showing tunability into the nonclassical regime. Our protocol is not limited by weak nonlinearities that underlie most known strategies of preparing multi-photon nonclassical states. Successive iterations of this protocol can lead to direct control over the weights of higher-order terms in the Fock basis, paving the way towards conditional preparation of "designer" multi-photon states for applications in quantum computation, communication and metrology.

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Estimation of a quantum interaction parameter using weak measurements: Theory and experiment

We investigate the estimation of a small interaction parameter from the outcomes of weak quantum measurements implemented by the interaction. The relation of weak values and sensitivity is explained and the different contributions of postselected results are identified using experimental data. The results show how weak values can be used to control the distribution of input state sensitivity between different postselected outcomes.

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Multi-photon quantum interference in a multi-port integrated photonic device

Increasing the complexity of quantum photonic devices is essential for many optical information processing applications to reach a regime beyond what can be classically simulated, and integrated photonics has emerged as a leading platform for achieving this. Here, we demonstrate three-photon quantum operation of an integrated device containing three coupled interferometers, eight spatial modes and many classical and nonclassical interferences. This represents a critical advance over previous complexities and the first on-chip nonclassical interference with more than two photonic inputs. We introduce a new scheme to verify quantum behaviour, using classically characterised device elements and hierarchies of photon correlation functions. We accurately predict the device's quantum behaviour and show operation inconsistent with both classical and bi-separable quantum models. Such methods for verifying multiphoton quantum behaviour are vital for achieving increased circuit complexity. Our experiment paves the way for the next generation of integrated photonic quantum simulation and computing devices.

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Heralded processes on continuous-variable spaces as quantum maps

Conditional evolution is crucial for generating non-Gaussian resources for quantum information tasks in the continuous variable scenario. However, tools are lacking for a convenient representation of heralded process in terms of quantum maps for continuous variable states, in the same way as Wigner functions are able to give a compact description of the quantum state. Here we propose and study such a representation, based on the introduction of a suitable transfer function to describe the action of a quantum operation on the Wigner function. We also reconstruct the maps of two relevant examples of conditional process, that is, noiseless amplification and photon addition, by combining experimental data and a detailed physical model. This analysis allows to fully characterize the effect of experimental imperfections in their implementations.

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Improving the maximum transmission distance of continuous-variable quantum key distribution using a noiseless amplifier

We show that the maximum transmission distance of continuous-variable quantum key distribution in presence of a Gaussian noisy lossy channel can be arbitrarily increased using a linear noiseless amplifier. We explicitly consider a protocol using amplitude and phase modulated coherent states with reverse reconciliation. We find that a noiseless amplifier with amplitude gain g can increase the maximum admissible losses by a factor 1/g^2.

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Multipartite optomechanical entanglement from competing nonlinearities

We investigate the nature of the three-mode interaction inside an optomechanically-active microtoroid with a sizeable chi^(2) coefficient. Experimental techniques are quickly advancing to the point where structures with the necessary properties can be made, and we argue that these provide a natural setting in which to observe rich dynamics leading, for instance, to genuine tripartite steady-state entanglement. We also show that this approach lends itself to a full characterisation of the three-mode state of the system.

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Hardy's paradox and violation of a state-independent Bell inequality in time

Tests such as Bell's inequality and Hardy's paradox show that joint probabilities and correlations between distant particles in quantum mechanics are inconsistent with local realistic theories. Here we experimentally demonstrate these concepts in the time domain, using a photonic entangling gate to perform nondestructive measurements on a single photon at different times. We show that Hardy's paradox is much stronger in time and demonstrate the violation of a temporal Bell inequality independent of the quantum state, including for fully mixed states.

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A method for characterizing coherent-state quantum gates

We discuss and implement experimentally a method for characterizing quantum gates operating on superpositions of coherent states. The peculiarity of this encoding of qubits is to work with a non-orthogonal basis, and therefore some technical limitations prevent us from using standard methods, such as process tomography. We adopt a different technique, that relies on some a-priori knowledge about the physics underlying the functioning of the device. A parameter characterizing the global quality of the quantum gate is obtained by \virtually" processing an entangled state.

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Single-photon device requirements for operating linear optics quantum computing outside the post-selection basis

Photonics is a promising architecture for the realisation of quantum information processing, since the two-photon interaction, or non-linearity, necessary to build logical gates can efficiently be realised by the use of interference with ancillary photons and detection. Although single-photon sources and detectors are pivotal in realisations of such systems, clear guidelines for the required performance of realistic systems are yet to be defined. We present our detailed numerical simulation of several quantum optics circuits including sources and detectors all represented in multi-dimensional Fockspaces, which allows to obtain experimentally realistic performance bounds for for these devices. In addition, the single-photon source based on switched parametric down-conversion is studied, which in principle could reach the required performance. Three approaches for implementing the switching hierarchy of the photons are simulated, and their anticipated performance is obtained. Our results define the bar for the optical devices needed to achieve the first level of linear-optics quantum computing outside the coincidence basis.

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Non-Gaussianity of quantum states: an experimental test on single-photon added coherent states

Non Gaussian states and processes are useful resources in quantum information with continuous variables. An experimentally accessible criterion has been proposed to measure the degree of non Gaussianity of quantum states, based on the conditional entropy of the state with a Gaussian reference. Here we adopt such criterion to characterise an important class of non classical states, single-photon added coherent states. Our studies demonstrate the reliability and sensitivity of this measure, and use it to quantify how detrimental is the role of experimental imperfections in our realisation.

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Implementation of a non-deterministic optical noiseless amplifier

Quantum mechanics imposes that any amplifier that works independently on the phase of the input signal has to introduce some excess noise. The impossibility of such a noiseless amplifier is rooted into unitarity and linearity of quantum evolution. A possible way to circumvent this limitation is to interrupt such evolution via a measurement, providing a random outcome able to herald a successful - and noiseless - amplification event. Here we show a successful realisation of such an approach; we perform a full characterization of an amplified coherent state using quantum homodyne tomography, and observe a strong heralded amplification, with about 6dB gain and a noise level significantly smaller than the minimal allowed for any ordinary phase-independent device.

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Anti-symmetrization reveals hidden entanglement

Two-photon anti-bunching at a beamsplitter is only possible if the photons are entangled in a specific state, anti-symmetric in the spatial modes. Thus, observation of anti-bunching is an indication of entanglement in a degree of freedom which might not be easily accessible in an experiment. We experimentally demonstrate this concept in the case of the interference of two frequency entangled photons with continuous frequency detunings. The principle of anti-symmetrisation of the spatial part of a wavefunction and subsequent detection of hidden entanglement via anti-bunching at a beamsplitter may facilitate the observation of entanglement in other systems, like atomic ensembles or Bose-Einstein condensates. The analogue for fermionic systems would be to observe bunching.

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Towards Quantum Chemistry on a Quantum Computer

The fundamental problem faced in quantum chemistry is the calculation of molecular properties, which are of practical importance in fields ranging from materials science to biochemistry. Within chemical precision, the total energy of a molecule as well as most other properties, can be calculated by solving the Schrodinger equation. However, the computational resources required to obtain exact solutions on a conventional computer generally increase exponentially with the number of atoms involved. This renders such calculations intractable for all but the smallest of systems. Recently, an efficient algorithm has been proposed enabling a quantum computer to overcome this problem by achieving only a polynomial resource scaling with system size. Such a tool would therefore provide an extremely powerful tool for new science and technology. Here we present a photonic implementation for the smallest problem: obtaining the energies of H2, the hydrogen molecule in a minimal basis. We perform a key algorithmic step - the iterative phase estimation algorithm - in full, achieving a high level of precision and robustness to error. We implement other algorithmic steps with assistance from a classical computer and explain how this non-scalable approach could be avoided. Finally, we provide new theoretical results which lay the foundations for the next generation of simulation experiments using quantum computers. We have made early experimental progress towards the long-term goal of exploiting quantum information to speed up quantum chemistry calculations.

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