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Marco Clementi

Publications and source records attributed to Marco Clementi.

At least 19 recordsLinked to original sources

Harnessing bound states in the continuum for quantum and nonlinear photonics in silicon nitride microresonators

In this work we theoretically and experimentally investigate bound states in the continuum (BICs) in a reconfigurable integrated photonic structure, focusing on spontaneous four-wave mixing. We consider a configuration in which only one mode, the idler, is tuned to the BIC condition, and show that suppressing the radiative loss of this single mode profoundly reshapes the overall nonlinear dynamics. In particularly, we realize electrically tunable Friedrich-Wintgen BICs with Q > 10^6 in an interferometrically coupled silicon-nitride microresonator. Although inaccessible through linear excitation, the BIC is populated by four-wave mixing and read out through its radiative photon partner. In the low-gain regime, we investigate the spectral, correlation, and coherence properties of the generated photon pairs, revealing distinctive signatures in the signal-idler correlations and an extracted signal whose coherence time approaches the intrinsic-loss-limited lifetime of the dark idler. In the high-gain regime, making one mode participating in optical parametric amplification a BIC enhances the parametric gain by 12 dB and lowers the oscillation threshold by 1.6 dB. These results establish BICs as a tool for mode-selective lifetime engineering, enabling control over both biphoton wavepackets and the threshold dynamics of integrated parametric devices.

physics.optics

Thermo-optic dynamics of effective epsilon-near-zero media

Epsilon-near-zero (ENZ) photonic media exhibit extreme optical dispersion that enables unconventional light-matter interactions and enhanced optical nonlinearities. Recent studies suggested that thermo-optic effects, traditionally regarded as slow and secondary, can be strongly modified under the ENZ condition. Here we establish thermo-optic reconfiguration of effective media as a unified physical framework to describe both static and transient thermo-optic phenomena in ENZ systems. Using a CMOS-compatible effective medium operating in the visible spectral range, we experimentally demonstrate that temperature variation, whether under thermal equilibrium or transient excitation, reconfigures the constitutive parameters defining the ENZ condition, giving rise to pronounced linear and nonlinear optical responses. At thermal equilibrium, this reconfiguration manifests itself as static ENZ wavelength shift with an unprecedentedly large thermal-spectral modulation rate and an effective thermo-optic coefficient on the order of $10^{-1}$ K$^{-1}$. Under ultrafast excitation, we observe a picosecond-scale thermo-optic nonlinear response induced by transient heating. This response can be consistently interpreted as a time-dependent reconfiguration of the effective ENZ medium, corresponding to a transient evolution of its optical parameters. By reframing thermo-optic effects as a process of static and dynamic reconfiguration of effective media, this work provides a unified perspective that bridges thermo-optic physics, effective-medium theory, and time-varying photonics.

physics.optics

Gigahertz-rate thin-film lithium niobate receiver for time-bin quantum communication

Time-bin encoded quantum states of light are crucial for quantum technology applications. The integration of manipulation functionalities into chip-scale devices is essential for deploying scalable, high-performance, and cost-effective quantum networks. Here we develop a fully integrated, high-throughput quantum receiver based on the thin-film lithium niobate (TFLN) platform, capable of high-speed electro-optic manipulation of time-bin encoded quantum states. The device's novel architecture enables active switching of time-bin quantum states with an electro-optic bandwidth exceeding 30 Ghz, while supporting real-time arbitrary projective measurements with a bandwidth of over 1 GHz. We showcase its versatility and performance through several applications, including the certification of entanglement with Bell's inequality violation by 38 standard deviations and with >95% visibility. We then apply it to a fiber-based quantum communication scenario, where we experimentally demonstrate an entanglement-based quantum key distribution (QKD) protocol, achieving stable finite-size secure key rates exceeding 25 kbit/s over 12 hours of continuous operation. By leveraging a high-speed active switching scheme, the system overcomes the need for temporal post-selection, eliminating a fundamental loophole that compromises the security of time-bin entanglement-based QKD protocols and relaxes the temporal resolution requirements of single-photon detectors. Moreover, it enables active selection of the projection basis, increasing the flexibility for communication parties. This approach establishes a versatile and scalable architecture for time-bin encoded quantum communication, enabling practical protocols on industry-grade photonic technology.

quant-ph

Quantum inference on a classically trained quantum extreme learning machine

Quantum extreme learning machines (QELMs) are unconventional computing architectures that bear remarkable promise in both classical and quantum machine-learning tasks, such as the estimation of quantum state properties. However, the probabilistic nature of quantum measurements demands extensive repetitions for training to precisely estimate expectation values, imposing stringent trade-offs among experimental resources, acquisition time, and signal-to-noise ratio, particularly for large datasets. Here, we introduce a paradigm shift by training the QELM exclusively with intense classical fields, namely twin beams generated by stimulated emission, while performing inference directly on previously unseen genuine quantum input states to predict their quantum properties. This strategy dramatically reduces acquisition times while substantially enhancing the signal-to-noise ratio. Using frequency-bin encoded biphoton states, implemented here for the first time in a quantum machine learning architecture, we demonstrate entanglement witnessing of two-qubit states with (93 +- 4)% accuracy, multi-dimensional entanglement detection, and learning of the Hamiltonian governing photon-pair generation with a fidelity of (96 +- 4)%. Our results open a new pathway toward faster and more robust training of photonic quantum extreme learning machines for quantum feature extraction.

quant-ph

Reconfigurable Resonant Multimode Nonlinear Coupling for UV-to-infrared Frequency Generation

On-chip coherent visible and near-infrared (NIR) light generation has broad applications in metrology, bio-sensing, and quantum information. High-Q microresonators are ideal candidates for generating light across such broad wavelength ranges via efficient second- ($\chi^{(2)}$) and third-order ($\chi^{(3)}$) nonlinear optical processes. However, harnessing these diverse nonlinearities simultaneously in a single microresonator remains elusive yet highly attractive both fundamentally and technologically. Here, we demonstrate coherent light generation from the ultraviolet to NIR in a silicon nitride microresonator pumped by a single continuous-wave telecom laser. This broad frequency generation arises from the interplay of $\chi^{(2)}$ and $\chi^{(3)}$ nonlinear processes. A cascade of nonlinear processes, including harmonic generation and optical parametric oscillation (OPO), is initiated by the photoinduced second harmonic generation enabled by all-optical poling. The dynamic reconfigurability of this $\chi^{(2)}$ nonlinearity enables access to different transverse spatial modes at the second harmonic, enabling highly tunable OPO processes triggered by hybrid modal phase matching conditions and yielding milliwatt-level NIR light. This work sheds new insights into the fundamental physics of cooperative nonlinear multimode interactions in resonant systems and provides a versatile approach for reconfigurable OPOs, highlighting their potential to generate light at wavelengths beyond the reach of photonic integrated lasers.

physics.optics

High-purity frequency-degenerate photon pair generation via cascaded SFG/SPDC in thin film lithium niobate

Frequency-degenerate photon pairs generated using nonlinear photonic integrated devices are a crucial resource for scalable quantum information processing and metrology. However, their realization is hindered by unwanted parametric processes occurring within the same phase matching band, which degrade the signal-to-noise ratio and reduce the purity of the associated quantum states. Here, we propose a dual-pump scheme to produce frequency-degenerate photon pairs, based on cascaded sum-frequency generation and spontaneous parametric down-conversion occurring within a single waveguide, while strongly suppressing parasitic photon pair generation from single-pump processes. This approach significantly simplifies the design compared to microresonator-based methods and enables both pumping and collection of photon pairs entirely in the telecom band. We experimentally validate the concept in a layer-poled thin film lithium niobate waveguide, achieving frequency-degenerate photon pair generation with a brightness of \SI{1.0(3)e5}{\hertz \per \nm \per \square \milli \watt } and a 40 dB suppression of unwanted single-pump processes.

quant-ph

Broadband spectral mapping of photo-induced second-harmonic generation in silicon nitride microresonators

By employing a pump-probe technique for enhanced spectral mapping of the dynamics in nonlinear frequency conversion, we demonstrate that photo-induced second-harmonic generation (SHG) in silicon nitride (Si3N4) microresonators can persist when transitioning from the preferred doubly resonant condition--where the resonances of the optical harmonics are required to be matched--to a highly detuned state where the generated second harmonic is significantly shifted away from its corresponding resonance. This results in an unconventionally broad conversion bandwidth. Other intriguing phenomena, such as detuning-dependent all-optical poling and nonlinear multi-mode interaction, are also presented for the first time with direct experimental evidence. Our findings provide new insights into the physics of photo-induced second-order (\chi^{(2)}) nonlinearity, highlighting its potential applications for nonlinear \chi^{(2)} photonics in integrated Si3N4 platform

physics.optics

Time-resolved certification of frequency-bin entanglement over multi-mode channels

Frequency-bin entangled photons can be efficiently produced on-chip which offers a scalable, robust and low-footprint platform for quantum communication, particularly well-suited for resource-constrained settings such as mobile or satellite-based systems. However, analyzing such entangled states typically requires active and lossy components, limiting scalability and multi-mode compatibility. We demonstrate a novel technique for processing frequency-encoded photons using linear interferometry and time-resolved detection. Our approach is fully passive and compatible with spatially multi-mode light, making it suitable for free-space and satellite to ground applications. As a proof-of-concept, we utilize frequency-bin entangled photons generated from a high-brightness multi-resonator source integrated on-chip to show the ability to perform arbitrary projective measurements over both single- and multi-mode channels. We report the first measurement of the joint temporal intensity between frequency-bin entangled photons, which allows us to certify entanglement by violating the Clauser-Horne-Shimony-Holt (CHSH) inequality, with a measured value of $|S|=2.32\pm0.05$ over multi-mode fiber. By combining time-resolved detection with energy-correlation measurements, we perform full quantum state tomography, yielding a state fidelity of up to $91\%$. We further assess our ability to produce non-classical states via a violation of time-energy entropic uncertainty relations and investigate the feasibility of a quantum key distribution protocol. Our work establishes a resource-efficient and scalable approach toward the deployment of robust frequency-bin entanglement over free-space and satellite-based links.

quant-ph

Post-selection free time-bin entanglement on a thin-film lithium niobate photonic chip

Time-bin entanglement is the most commonly used form of entanglement for quantum communication protocols over fiber networks, due to the natural resilience of this encoding scheme to thermal phase fluctuations in optical fibers. Projective measurements on some bases in the time-bin encoding need, however, post-selection of the measured events, introducing a loophole in Bell tests and requiring high temporal resolution. In this work, we demonstrate chip-integrated receivers for time-bin entanglement certification including a high-speed optical switch to remove such post-selection loophole. The receivers are realized using thin-film lithium niobate and operate at a switching frequency of 5 GHz, enabling high secure key rates. We demonstrate a Bell inequality violation by more than 24 standard deviations without the need for time resolution at the time-bin separation level.

quant-ph

Integrated tunable green light source on silicon nitride

Integrated green light sources are essential for telecommunications and quantum applications, while the performance of current on-chip green light generation is still limited in power and tunability. In this work, we demonstrate green light generation in silicon nitride microresonators using photo-induced second-order nonlinearities, achieving up to 3.5 mW green power via second-harmonic generation and densely tunable over a 29 nm range. In addition, we report milliwatt-level all-optical poling (AOP) threshold, allowing for amplifier-free continuous-wave AOP. Furthermore, we demonstrate non-cascaded sum-frequency generation, leveraging the combination of AOP and simultaneous coherent frequency combs generation at 1 $\mu$m. Such comb-assisted AOP enables switching of the green light generation over an 11 nm range while maintaining the pump within a single resonance. The combination of such highly efficient photo-induced nonlinearity and multi-wavelength AOP enables the realization of low-threshold, high-power, widely-tunable on-chip green sources.

physics.optics

Ultrabroadband Milliwatt-Level Resonant Frequency Doubling on a Chip

Microresonators are powerful tools to enhance the efficiency of second-order nonlinear optical processes, such as second-harmonic generation, which can coherently bridge octave-spaced spectral bands. However, dispersion constraints such as phase-matching and doubly resonant conditions have so far limited demonstrations to narrowband operation. In this work, we overcome these limitations showing ultrabroadband resonant frequency doubling in a novel integrated device, wherein the resonant enhancement of pump and second harmonic are individually addressed in two distinct and linearly uncoupled microring resonators, each adjusted to target the respective spectral band. The two microresonators are designed and tuned independently, yet share a common interaction region that grants nonlinear coupling over a quasi-phase-matching bandwidth exceeding 200 nm, enabled by the inscription of a photoinduced $\chi^{(2)}$ grating. The system allows to not only conveniently disentangle the design parameters of the two microresonators but also to reconfigure the doubly resonant condition electrically, and the phase-matching condition optically. We demonstrate milliwatt-level addressable second-harmonic generation over the entire telecom band and then configure the device to internally generate and upconvert a Kerr frequency comb with bandwidth exceeding 100 nm and upconverted power up to 10 mW.

physics.optics

Self-organized spatiotemporal quasi-phase-matching in microresonators

Quasi-phase-matching (QPM) is a widely adopted technique for mitigating stringent momentum conservation in nonlinear optical processes such as second-harmonic generation (SHG). It effectively compensates for the phase velocity mismatch between optical harmonics by introducing a periodic spatial modulation to the nonlinear optical medium. Such a mechanism has been further generalized to the spatiotemporal domain, where a non-stationary spatial QPM can induce a frequency shift of the generated light. Here we demonstrate how a spatiotemporal QPM grating, consisting in a concurrent spatial and temporal modulation of the nonlinear response, naturally emerges through all-optical poling in silicon nitride microresonators. Mediated by the coherent photogalvanic effect, a traveling space-charge grating is self-organized, affecting momentum and energy conservation, resulting in a quasi-phase-matched and Doppler-shifted second harmonic. Our observation of the photoinduced spatiotemporal QPM expands the scope of phase matching conditions in nonlinear photonics.

physics.optics

A chip-scale second-harmonic source via injection-locked all-optical poling

Second-harmonic generation allows for coherently bridging distant regions of the optical spectrum, with applications ranging from laser technology to self-referencing of frequency combs. However, accessing the nonlinear response of a medium typically requires high-power bulk sources, specific nonlinear crystals, and complex optical setups, hindering the path toward large-scale integration. Here we address all of these issues by engineering a chip-scale second-harmonic (SH) source based on the frequency doubling of a semiconductor laser self-injection-locked to a silicon nitride microresonator. The injection-locking mechanism, combined with a high-Q microresonator, results in an ultra-narrow intrinsic linewidth at the fundamental harmonic frequency as small as 57 Hz. Owing to the extreme resonant field enhancement, quasi-phase-matched second-order nonlinearity is photoinduced through the coherent photogalvanic effect and the high coherence is mapped on the generated SH field. We show how such optical poling technique can be engineered to provide efficient SH generation across the whole C and L telecom bands, in a reconfigurable fashion, overcoming the need for poling electrodes. Our device operates with milliwatt-level pumping and outputs SH power exceeding 2 mW, for an efficiency as high as 280%/W under electrical driving. Our findings suggest that standalone, highly-coherent, and efficient SH sources can be integrated in current silicon nitride photonics, unlocking the potential of $χ^{(2)}$ processes in the next generation of integrated photonic devices.

physics.optics

Programmable frequency-bin quantum states in a nano-engineered silicon device

Photonic qubits should be controllable on-chip and noise-tolerant when transmitted over optical networks for practical applications. Furthermore, qubit sources should be programmable and have high brightness to be useful for quantum algorithms and grant resilience to losses. However, widespread encoding schemes only combine at most two of these properties. Here, we overcome this hurdle by demonstrating a programmable silicon nano-photonic chip generating frequency-bin entangled photons, an encoding scheme compatible with long-range transmission over optical links. The emitted quantum states can be manipulated using existing telecommunication components, including active devices that can be integrated in silicon photonics. As a demonstration, we show our chip can be programmed to generate the four computational basis states, and the four maximally-entangled Bell states, of a two-qubits system. Our device combines all the key-properties of on-chip state reconfigurability and dense integration, while ensuring high brightness, fidelity, and purity.

quant-ph

Observation of SQUID-like behavior in fiber laser with intra-cavity epsilon-near-zero effect

Establishing relations between fundamental effects in far-flung areas of physics is a subject of great interest in the current research. We here report realization of a novel photonic system akin to the radio-frequency superconducting quantum interference device (RF-SQUID), in a fiber laser cavity with epsilon-near-zero (ENZ) nanolayers as intra-cavity components. Emulating the RF-SQUID scheme, the photonic counterpart of the supercurrent, represented by the optical wave, circulates in the cavity, passing through effective optical potential barriers. Different ENZ wavelengths translate into distinct spectral outputs through the variation of cavity resonances, emulating the situation with a frequency-varying tank circuit in the RF-SQUID. Due to the presence of the ENZ element, the optical potential barrier is far lower for selected frequency components, granting them advantage in the gain-resource competition. The findings reported in this work provide a deeper insight into the ultrafast ENZ photonics, revealing a new path towards the design of nanophotonic on-chip devices with various operational functions, and offer a new approach to study superconducting and quantum-mechanical systems.

physics.optics

Single-photon nonlinearities and blockade from a strongly driven photonic molecule

Achieving the regime of single-photon nonlinearities in photonic devices just exploiting the intrinsic high-order susceptibilities of conventional materials would open the door to practical semiconductor-based quantum photonic technologies. Here we show that this regime can be achieved in a triply resonant integrated photonic device made of two coupled ring resonators, without necessarily requiring low volume confinement, in a material platform displaying an intrinsic third-order nonlinearity. By strongly driving one of the three resonances of the system, a weak coherent probe at one of the others results in a strongly suppressed two-photon probability at the output, evidenced by antibunched second-order correlation function at zero-time delay under continuous wave driving.

quant-ph

Single SiGe Quantum Dot Emission Deterministically Enhanced in a High-Q Photonic Crystal Resonator

We report the resonantly enhanced radiative emission from a single SiGe quantum dot (QD), which is deterministically embedded into a bichromatic photonic crystal resonator (PhCR) at the position of its largest modal electric field by a scalable method. By optimizing our molecular beam epitaxy (MBE) growth technique, we were able to reduce the amount of Ge within the whole resonator to obtain an absolute minimum of exactly one QD, accurately positioned by lithographic methods relative to the PhCR, and an otherwise flat, a few monolayer thin, Ge wetting layer (WL). With this method, record quality (Q) factors for QD-loaded PhCRs up to $Q\sim 10^5$ are achieved. A comparison with control PhCRs on samples containing a WL but no QDs is presented, as well as a detailed analysis of the dependence of the resonator-coupled emission on temperature, excitation intensity, and emission decay after pulsed excitation. Our findings undoubtedly confirm a single QD in the center of the resonator as a potentially novel photon source in the telecom spectral range.

physics.optics

Thermo-Optically Induced Transparency on a photonic chip

Controlling the optical response of a medium through suitably tuned coherent electromagnetic fields is highly relevant in a number of potential applications, from all-optical modulators to optical storage devices. In particular, electromagnetically induced transparency (EIT) is an established phenomenon in which destructive quantum interference creates a transparency window over a narrow spectral range around an absorption line, which, in turn, allows to slow and ultimately stop light due to the anomalous refractive index dispersion. Here we report on the observation of a new form of either induced transparency or amplification of a weak probe beam in a strongly driven silicon photonic crystal resonator at room temperature. The effect is based on the oscillating temperature field induced in a nonlinear optical cavity, and it reproduces many of the key features of EIT while being independent of either atomic or mechanical resonances. Such thermo-optically induced transparency (TOIT) will allow a versatile implementation of EIT-analogues in an integrated photonic platform, at almost arbitrary wavelength of interest, room temperature and in a practical, low cost and scalable system.

physics.optics