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Marco Grioni

Publications and source records attributed to Marco Grioni.

24 records · Page 2Linked to original sources

Ag-coverage-dependent symmetry of the electronic states of the Pt(111)-Ag-Bi interface: The ARPES view of a structural transition

We studied by angle-resolved photoelectron spectroscopy the strain-related structural transition from a pseudomorphic monolayer (ML) to a striped incommensurate phase in an Ag thin film grown on Pt(111). We exploited the surfactant properties of Bi to grow ordered Pt(111)-xMLAg-Bi trilayers with 0 < x < 5 ML, and monitored the dispersion of the Bi-derived interface states to probe the structure of the underlying Ag film. We find that their symmetry changes from threefold to sixfold and back to threefold in the Ag coverage range studied. Together with previous scanning tunneling microscopy and photoelectron diffraction data, these results provide a consistent microscopic description of the coverage-dependent structural transition.

cond-mat.mtrl-sci↗

Anisotropy effects on Rashba and topological insulator spin polarized surface states: a unified phenomenological description

Spin polarized two-dimensional electronic states have been previously observed on metallic surface alloys with giant Rashba splitting and on the surface of topological insulators. We study the surface band structure of these systems, in a unified manner, by exploiting recent results of k.p theory. The model suggests a different way to address the effect of anisotropy in Rashba systems. Changes in the surface band structure of various Rashba compounds can be captured by a single effective parameter which quantifies the competition between the Rashba effect and the hexagonal warping of the constant energy contours. The same model provides a unified phenomenological description of the surface states belonging to materials with topologically trivial and non-trivial band structures.

cond-mat.mtrl-sci↗

A band structure scenario for the giant spin-orbit splitting observed at the Bi/Si(111) interface

The Bi/Si(111) (sqrt{3} x sqrt{3})R30 trimer phase offers a prime example of a giant spin-orbit splitting of the electronic states at the interface with a semiconducting substrate. We have performed a detailed angle-resolved photoemission (ARPES) study to clarify the complex topology of the hybrid interface bands. The analysis of the ARPES data, guided by a model tight-binding calculation, reveals a previously unexplored mechanism at the origin of the giant spin-orbit splitting, which relies primarily on the underlying band structure. We anticipate that other similar interfaces characterized by trimer structures could also exhibit a large effect.

cond-mat.mtrl-sci↗

Tunable spin-gaps in a quantum-confined geometry

We have studied the interplay of a giant spin-orbit splitting and of quantum confinement in artificial Bi-Ag-Si trilayer structures. Angle-resolved photoelectron spectroscopy (ARPES) reveals the formation of a complex spin-dependent gap structure, which can be tuned by varying the thickness of the Ag buffer layer. This provides a means to tailor the electronic structure at the Fermi energy, with potential applications for silicon-compatible spintronic devices.

cond-mat.mtrl-sci↗

Giant Spin-splitting in the Bi/Ag(111) Surface Alloy

Surface alloying is shown to produce electronic states with a very large spin-splitting. We discuss the long range ordered bismuth/silver(111) surface alloy where an energy bands separation of up to one eV is achieved. Such strong spin-splitting enables angular resolved photoemission spectroscopy to directly observe the region close to the band edge, where the density of states shows quasi-one dimensional behavior. The associated singularity in the local density of states has been measured by low temperature scanning tunneling spectroscopy. The implications of this new class of materials for potential spintronics applications as well as fundamental issues are discussed.

cond-mat.mtrl-sci↗

Bounded Luttinger liquids as a universality class of quantum critical behavior

We show that one-dimensional quantum systems with gapless degrees of freedom and open boundary conditions form a new universality class of quantum critical behavior, which we propose to call ``bounded Luttinger liquids''. They share the following properties with ordinary (periodic) Luttinger liquids: absence of fermionic quasi-particle excitations, charge-spin separation, anomalous power-law correlations with exponents whose scaling relations are parametrized by a single coupling constant per degree of freedom, $K_ν$. The values of $K_ν$ are independent of boundary conditions, but the representation of the critical exponents in terms of these $K_ν$ depends on boundary conditions. We illustrate these scaling relations by exploring general rules for boundary critical exponents derived earlier using the Bethe Ansatz solution of the 1D Hubbard model together with boundary conformal field theory, and the theory of Luttinger liquids in finite-size systems. We apply this theory to the photoemission properties of the organic conductors $(TMTSF)_2X$, and discuss to what extent the assumption of finite strands with open boundaries at the sample surface can reconcile the experimental results with independent information on the Luttinger liquid state in these materials.

cond-mat.str-el↗