SearcharxivSearch

arXiv subjects

Marco Ornigotti

Publications and source records attributed to Marco Ornigotti.

At least 19 recordsLinked to original sources

Quantum many-body effects in the optical response of ideal thin films

We study quantum many-body effects in the long-wavelength optical response of confined electrons at finite temperatures. We simulate homogeneous electron gas confined in one dimension into a slab of nanoscale thickness. We demonstrate how the slab boundaries break down the ideal Drude response of free charge carriers, giving rise to scattering effects due to both the surfaces and quantum many-body interactions. We use a recent path-integral Monte Carlo (PIMC) approach developed in [Tiihonen et al. Phys. Rev. A 113, 053711] to quantify these effects in high accuracy. We perform phenomenological fits to Drude and Drude-Lorentz models parameters, manifesting various trends of the optical response with physical parameters like density and temperature, and numerical effects like finite size and the quantum statistics.

physics.optics

Stability of Orbital Angular Momentum Modes in Conventional and Ring-Core Optical Fibers

Modal dynamics in multimode optical fibers are fundamentally governed by the inter- play between phase matching and intermodal coupling. In this work, we investigate the fundamental coupling mechanisms in ring-core fibers and identify a geometry-induced cou- pling suppression that significantly reduces coupling coefficients between orbital angular momentum modes compared to conventional multimode step-index fibers. This mechanism provides a clear physical explanation for the superior transmission stability of orbital angular momentum modes in ring-core fibers and establishes specific geometric constraints for the design of ring-core fiber-based mode converters.

physics.optics

Quantum Theory of Third-harmonic Generation in Epsilon-Near-Zero Materials

We present a theoretical framework, based on the Green's tensor quantization method, to describe third-harmonic generation in epsilon-near-zero (ENZ) materials and derive analytical, closed-form solutions for the generation efficiency. We validate our model against experimental measurements of wavelength- and angle-resolved third-harmonic generation efficiency from 30 nm-thin ITO nanolayers at low pump intensity, described under the undepleted pump approximation. Our results provide a local and scalar effective model for quantum nonlinear processes in dispersive and lossy ENZ media, and establishes a simple and reliable framework for investigating a variety of nonlinear optical phenomena with applications to quantum sensing, quantum information, and quantum nondemolition measurements.

physics.optics

A Collective Propagation Law of Optical Vortex Constellations and Longitudinal Sensing

Optical vortices are ubiquitous phenomena naturally appearing in wave physics, yet higher-order charges inherently split into constellations of lowest-order singularities at the smallest deviation from an ideal situation. While these constellations are common phenomena in real-world scenarios, characterizing their longitudinal evolution typically relies on exhaustive full-field descriptions or the ambiguous, sequential tracking of individual singularities. Here, we reveal and experimentally demonstrate a simple deterministic law describing the paraxial longitudinal propagation of an arbitrary constellation of optical vortices in standard Gaussian backgrounds. By mapping the constituting singularity coordinates to their elementary symmetric polynomials (ESPs), we capture the holistic evolution of the constellation during propagation, completely bypassing the practical need to sequentially track indistinguishable vortices. We further show that such complex ESPs provide a useful metrological tool for the estimation of longitudinal displacements. Our results reveal a previously unrecognized compact description of collective vortex dynamics, introducing a new route to longitudinal sensing through singularimetry.

physics.optics

Mid-Infrared Single-Photon Detection via Enhanced Cross-Phase Modulation in Topology-Optimized Epsilon-Near-Zero Dual-Wavelength Nanocavities

We use the Green's tensor quantization theory for open resonant nanostructures with absorption losses to study cross-phase modulation (XPM) at the single-photon level in nanoscale Kerr-type epsilon-near-zero (ENZ) materials with an effective nonlinear susceptibility integrated inside dual-wavelength nanocavities. We obtain analytical formulas for the XPM frequency shifts in hybrid nanocavities that simultaneously trap a classical probe beam at 1.5 $\mu$m and single-photon pump at 3 $\mu$m wavelengths. We present a comprehensive analysis of the fundamental limits for mid-infrared single-photon detection in the quantum nondemolition modality for nanostructured cadmium oxide (CdO) regions with ENZ-enhanced nonlinearity embedded in a silicon (Si) environment inversely designed by free-form topology optimization. We numerically implement our theoretical results using finite element simulations within the rigorous framework of quasi-normal modes, demonstrating a single-photon XPM frequency shift $\Delta f_s \approx 55.6 \text{ GHz}$ with fractional shift (i.e., frequency pulling) $\Delta f_s / f_s \approx 2.78 \times 10^{-4}$ and addressing the feasibility of detection in the hybrid Si-CdO dual-wavelength nanocavity, either with a classical probe beam or a squeezed probe state, including the contributions of traditional limitations from self-phase modulation noise, thermorefractive noise, shot noise, and free-carrier absorption effects. Finally, we present a comparative size scaling analysis of the XPM phase shift and phase noise contributions for dual-wavelength nanocavities based on CdO and indium tin oxide (ITO) nonlinear ENZ materials. This work establishes a robust benchmark for the engineering of mid-infrared single-photon nonlinear devices such as nondemolition quantum detectors, sensors, and all-optical gates on a solid state photonic platform.

physics.optics

Path integral quantization of the electromagnetic field in nonlinear dielectric materials

We construct a quantum theory of light in nonlinear dielectric media with dispersion and absorption. We employ a mesoscopic model for the light-matter interaction that include a fourth-order nonlinearity in the material response. Quantization is performed by constructing an effective action in a path-integral formalism by integrating out matter and bath degrees of freedom. We show how a nonlinear response function associated with Kerr nonlinearity is obtained through the model and, after full field quantization, we derive the Feynman rules from this theory.

quant-ph

High-purity amplification of circularly polarized orbital angular momentum modes in an active spun ring-core tapered fiber

Structured light, optical fields engineered in their spatial, polarization, or phase degrees of freedom, has become a key resource across advanced communication, sensing, imaging, and quantum technologies. Optical fibers nowadays play an essential role in this landscape, providing stable and scalable platforms for guiding, and amplifying complex modes such as vector and orbital angular momentum (OAM) beams. In this work, we demonstrate an active spun ring-shaped tapered fiber as a gain medium for efficient amplification of OAM modes preserving their modal purity and polarization topology. OAM beams with topological charges l = 1 and l = 2 carrying 60 ps pulses at 15 MHz repetition rate at 1030 nm wavelength are amplified over 1.2 W average power with modal purity over 95%. The spatially resolved measurement of the OAM beam polarization topology revealed small distortion due to the coupling in to neighbour modes. These results demonstrate the high potential of active spun ring-shaped tapered fibers for power scaling of complex beams, preserving their phase and polarization structure simultaneously.

physics.optics

The Geometry of Paraxial Vector Beams

This work unveils a novel and fundamental connection between structured light and topological field theory by showing how the natural geometrical setting for paraxial vector beams is that of a $SU(2)$ principal bundle over $\mathbb{R}^{2+1}$. Going beyond the usual high-order Poincaré sphere approach, we show how the nonseparable structure of polarisation and spatial modes in vector beams is naturally described by a non-Abelian Chern-Simons gauge theory. In this framework, we link the Chern-Simons charge to spin-orbit coupling, and we propose a simple way to experimentally detect the presence of non-Abelian phases through Wilson lines. This new insight on vector beams opens new possibilities for realising and probing topological quantum field theories using classical optics, as well as it lays the foundation for implementing topologically protected classical and quantum information protocols with structured light.

physics.optics

Path-integral Monte Carlo estimator for the dipole polarizability of quantum plasma

We present a path-integral Monte Carlo estimator for calculating the dipole polarizability of interacting Coulomb plasma in the long-wavelength limit, i.e., the optical region. We present comprehensive details and method validation studies for our approach based on both collective and one-particle dipole autocorrelation functions in the imaginary time. The simulation of thermal equilibrium in imaginary time has exact Coulomb interactions and Boltzmann quantum statistics. For reference, we use analytically continued Drude model as the long-wavelength limit of the Lindhard response. Our collective response shows perfect match to the analytical reference. The one-particle response is used in systematic studies of physical and numerical parameters, and to discuss the phenomenological Drude scattering model.

cond-mat.mes-hall

Optical Vortex Dynamics in non-uniform twisted Ring-Core Fibers

In this work, we present a thorough analysis of the propagation of fiber modes carrying orbital angular momentum in twisted, tapered, ring-core optical fibers. In particular, by generalizing the usual coupled-mode approach to include the effect of twisting and tapering, we discuss how it is possible to achieve efficient power transfer between modes carrying different amounts of orbital angular momentum. Our simulation allows us to get a clear insight into the dynamics of vortex modes propagating through twisted ring core fibers.

physics.optics

Nonlinear Quantum Electrodynamics of Epsilon-Near-Zero Nanocavities

We investigate single-photon nonlinear refractive index change and frequency shift of Epsilon-Near-Zero (ENZ) sub-wavelength nanocavities. We apply the rigorous quantum Langevin-noise approach in the framework of Green's tensor quantization method to realistic ENZ materials with causal dispersion and derive closed-form analytical solutions for cavities with spherical geometry. This is achieved by employing a fully nonperturbative methodology for the analysis of open quantum systems with single-photon Kerr-type nonlinearity. The analytical results are validated numerically using the established quasi-normal mode expansion method and extended to nonspherical nanocavity geometries that can be experimentally fabricated using state-of-the-art electron lithography. Our findings establish a rigorous benchmark for understanding single-photon nonlinear optical effects in Kerr-type ENZ nanostructures with losses and are of importance to emerging quantum technology applications, including on-chip single-photon nondemolition detection, quantum sensing, and controlled quantum gates driven by enhanced photon blockade effects at the nanoscale.

physics.optics

Nonlinear Optical Microscopy of Semiconductor Metal-Nanocavities

We use second and third harmonic generation microscopy to investigate the nonlinear optical response of GaAs nanocavities embedded in a gold film and compare them to bare GaAs nanocavities. Our results reveal that the surrounding metallic environment significantly modifies both the intensity and spatial distribution of the nonlinear signals. When the harmonic wavelength is spectrally detuned from the nanocavity resonance, the effects due to the metallic environment start suppressing the SHG contrast. Numerical simulations confirm that at a 1060 nm pump wavelength, the SHG produced at 530 nm is suppressed due to the dominant plasmonic response of gold. Meanwhile, the THG produced at 353 nm, which coincides with the nanocavity resonance, enables high contrast imaging. Furthermore, by shifting the pump to 710 nm, aligning SHG at 356 nm with the nanocavity resonance, we recover strong SHG contrast, demonstrating a pathway to enhanced imaging of metal-semiconductor heterostructures.

physics.optics

Structured Light-Matter Interaction: Twisted Photons in Graphene

In this work we present a numerical framework for studying the interaction of structured electromagnetic fields, i.e., light pulses carrying orbital angular momentum (OAM), interacting with a single layer of graphene. Our approach is based on a two-step process, where first the interaction of structured light with matter, modelled by a suitable Dirac equation is solved and then coupled with Maxwell's equations, for studying the properties in both space and frequency domain of the generated nonlinear electromagnetic field. As an example of application of our method we investigate third harmonic generation by an OAM pulse. We check that OAM conservation through harmonic generation is conserved, and we report on both the spatial and frequency features of the third harmonic signal, comparing it with the traditional frequency response for spatially uniform field.

physics.optics

Higher-order Poincaré Spheres and Spatio-Spectral Poincaré Beams

The study of fundamental optics effects has been stimulated through the increasing ability to structure light in all its degrees of freedom (DOFs) in sophisticated but simple experimental settings. However, with such an increase in experimental capabilities, it has also become important to study theoretical descriptions for a more intuitive understanding of the underlying concepts. Here, we introduce a visual representation of light that is structured in its transverse space, frequency, and polarization in the form of a higher-order Poincaré sphere and discuss interesting links to its fundamental counterpart. We further leverage this connection to discuss and experimentally generate light possessing all possible polarization states across its spatio-spectral shape, which we term spatio-spectral Poincaré beams. By invoking all DOFs of light in the powerful description of higher-order Poincaré spheres, our work can pave the way for a deeper understanding and beneficial application of structured light as a powerful tool in optics.

physics.optics

Field theory description of the non-perturbative optical nonlinearity of epsilon-near-zero media

In this paper we introduce a fully non-perturbative approach for the description of the optical nonlinearity of epsilon-near-zero (ENZ) media. In particular, based on the rigorous Feynman path integral method, we develop a dressed Lagrangian field theory for light-matter interactions and discuss its application to dispersive Kerr-like media with order-of-unity light-induced refractive index variations. Specifically, considering the relevant case of Indium Tin Oxide (ITO) nonlinearities, we address the novel regime of non-perturbative refractive index variations in ENZ media and establish that it follows naturally from a scalar field theory with a Born-Infeld (BI) Lagrangian. Moreover, we developed a predctive model that includes the intrinsic saturation effects originating from the light-induced modification of the Drude terms in the linear dispersion of ITO materials. Our results extend the Huttner-Barnett-Bechler electrodynamics model to the case of non-perturbative optical Kerr-like media providing an intrinsically nonlinear, field-theoretic framework for understanding the exceptional nonlinearity of ITO materials beyond traditional perturbation theory.

physics.optics

High-order aberrations of vortex constellations

When reflected from an interface, a laser beam generally drifts and tilts away from the path predicted by ray optics, an intriguing consequence of its finite transverse extent. Such beam shifts manifest more dramatically for structured light fields, and in particular for optical vortices. Upon reflection, a field containing a high-order optical vortex is expected to experience not only geometrical shifts, but an additional splitting of its high-order vortex into a constellation of unit-charge vortices, a phenomenon known as topological aberration. In this article, we report on the first direct observation of the topological aberration effect, measured through the transformation of a vortex constellation upon reflection. We develop a general theoretical framework to study topological aberrations in terms of the elementary symmetric polynomials of the coordinates of a vortex constellation, a mathematical abstraction which we prove to be the physical quantity of interest. Using this approach, we are able to verify experimentally the aberration of constellations of up to three vortices reflected from a thin metallic film. Our work not only deepens the understanding of the reflection of naturally occurring structured light fields such as vortex constellations but also sets forth a potential method for studying the interaction of twisted light fields with matter.

physics.optics

Time-varying media, relativity, and the arrow of time

We study the implications of time-varying wave mechanics, and show how the standard wave equation is modified if the speed of a wave is not constant in time. In particular, waves which experience longitudinal acceleration are shown to have clear relativistic properties when a constant reference speed exists. Moreover, the accelerating wave equation admits only solutions propagating forward in time, which are continuous across material interfaces. We then consider the special case of electromagnetic waves, finding that the Abraham-Minkowski controversy is caused by relativistic effects, and the momentum of light is in fact conserved between different media. Furthermore, we show that the accelerating waves conserve energy when the wave is moving along a geodesic and demonstrate two example solutions. We conclude with some remarks on the role of the accelerating wave equation in the context of the arrow of time.

physics.optics

2D Weyl Materials in the Presence of Constant Magnetic Fields

In this work we investigate the effect of a constant external, or artificial, magnetic field on the nonlinear response of 2D Weyl materials. We calculate the Landau Levels for tilted cones in 2D Weyl materials by treating the tilting in a perturbative manner, and employ perturbation theory to calculate the tilting-induced correction to the magnetic field induced Landau spectrum. We then calculate the induced current as a function of the tilting coefficients and extract the correspondent nonlinear signal. Then, we analyze how changing tilting parameter affects nonlinear signal. Our findings show the possibility of achieving a significant tunability of the nonlinear response, by suitably engineering the orientation and degree of tilt of Dirac cones in 2D Weyl materials.

cond-mat.mes-hall